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Depleted uranium oxide supported nickel catalyst for autothermal CO_(2)methanation in non-adiabatic reactor under induction heating

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Journal of Energy Chemistry 2023年第10期85卷 310-323,I0010页

作者： lai truong-phuoc Jean-Mario Nhut Loïc Vidal Cuong Duong-Viet Sécou Sall Corinne Petit Christophe Sutter Mehdi Arab Alex Jourdan Cuong Pham-Huu Institute of Chemistry and Processes for Energy Environment and Health(ICPEES)ECPMUMR 7515 CNRS-University of Strasbourg25 rue Becquerel67087 Strasbourg Cedex 02France BlackLeaf SAS 210 rue Geiler de Kaysersberg67400 IllkirchFrance Institute of Materials Science of Mulhouse IS2MUMR 7361Universitéde Haute-AlsaceCNRS15rue Jean Starcky-BP 248868057 MulhouseFrance ORANO Tricastin Direction de La Recherche&DéveloppementSite du TRICASTIN BP 1626701 Pierrelatte CedexFrance

Undoped nickel-based catalysts supported on depleted uranium oxide allow one to carry out CO_(2)methanation process under extremely low reaction temperature under atmospheric pressure and powered by a contactless induction heating.By adjusting the reaction conditions,the catalyst is able to perform CO_(2)methanation reaction under autothermal process operated inside a non-adiabatic reactor,without any external energy supply.Such autothermal process is possible thanks to the high apparent density of the UO_x which allows one to confine the reaction heat in a small catalyst volume in order to confine the exothermicity of the reaction inside the catalyst and to operate the reaction at equilibrium heat in-heat out.Such autothermal operation mode allows one to significantly reduce the complexity of the process compared to that operated using adiabatic reactor,where complete insulation is required to prevent heat disequilibrium,in order to reduce as much as possible,the heat exchange with the external medium.The catalyst displays an extremely high stability as a function of time on stream as no apparent deactivation.It is expected that such new catalyst with unprecedented catalytic performance could open new era in the field of heterogeneous catalysis where traditional supports show their limitations to operate catalytic processes under severe reaction conditions.

关键词： CO_(2)methanation Auto-methanation Induction heating Depleted uranium oxide Electrification process Operando DRIFTS

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氮掺杂碳纳米管包覆碳化硅作为不含金属的催化剂(英文)

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催化学报 2014年第6期35卷 906-913页

作者： Cuong Duong-Viet Housseinou Ba Yuefeng Liu lai truong-phuoc Jean-Mario Nhut Cuong Pham-Huu Institute of Chemistry and Processes for Energy Environment and Health (ICPEES) ECPM UMR 7515 du CNRS-University of Strasbourg 25 rue Becquerel 67087 Strasbourg Cedex 02 France Hanoi University of Mining and Geology Dong Ngac Tu Liem Hanoi Viet Nam

A hierarchical metal-free catalyst consisting of nitrogen-doped carbon nanotubes decorated onto a silicon carbide (N-CNTs/SiC) macroscopic host structure was prepared. The influence of N-CNTs incorporation on the physical properties of the support was evaluated using different characterization techniques. The catalyst was tested as a metal-free catalyst in the selective oxidation of H2S and steam-free dehydrogenation of ethylbenzene. The N-CNTs/SiC catalyst exhibited extremely good desulfurization performance compared to a Fe2O3/SiC catalyst under less conducive reaction conditions such as low temperature, high space velocity, and a low O2-to-H2S molar ratio. For the dehy-drogenation of ethylbenzene, a higher dehydrogenation activity was obtained with the N-CNTs/SiC catalyst compared to a commercial K-Fe/Al2O3 catalyst. The N-CNTs/SiC catalyst also displayed good stability as a function of time on stream for both reactions, which was attributed to the strong anchoring of the nitrogen dopant in the carbon matrix. The extrudate shape of the SiC support allowed the direct macroscopic shaping of the catalyst for use in a conventional fixed-bed reactor without the problems of catalyst handling, transportation, and pressure drop across the catalyst bed that are encountered with nanoscopic carbon-based catalysts.

关键词：催化剂组成碳纳米管碳化硅含金属氮掺杂固定床反应器复合材料氧化铝催化剂

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Push forward LC-MS-based therapeutic drug monitoring and pharmacometabolomics for anti-tuberculosis precision dosing and comprehensive clinical management

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Journal of Pharmaceutical Analysis 2024年第1期14卷 16-38页

作者： Nguyen Quang Thu Nguyen Tran Nam Tien Nguyen Thi Hai Yen Thuc-Huy Duong Nguyen phuoc Long Huy truong Nguyen Department of Pharmacology and PharmacoGenomics Research Center Inje University College of MedicineBusan47392Republic of Korea Department of Chemistry University of EducationHo Chi Minh City700000Viet Nam Faculty of Pharmacy Ton Duc Thang UniversityHo Chi Minh City700000Viet Nam

The spread of tuberculosis(TB),especially multidrug-resistant TB and extensively drug-resistant TB,has strongly motivated the research and development of new anti-TB drugs.New strategies to facilitate drug combinations,including pharmacokinetics-guided dose optimization and toxicology studies of first-and second-line anti-TB drugs have also been introduced and recommended.Liquid chromatography-mass spectrometry(LC-MS)has arguably become the gold standard in the analysis of both endo-and exo-genous compounds.This technique has been applied successfully not only for therapeutic drug monitoring(TDM)but also for pharmacometabolomics analysis.TDM improves the effectiveness of treatment,reduces adverse drug reactions,and the likelihood of drug resistance development in TB patients by determining dosage regimens that produce concentrations within the therapeutic target window.Based on TDM,the dose would be optimized individually to achieve favorable outcomes.Pharmacometabolomics is essential in generating and validating hypotheses regarding the metabolism of anti-TB drugs,aiding in the discovery of potential biomarkers for TB diagnostics,treatment monitoring,and outcome evaluation.This article highlighted the current progresses in TDM of anti-TB drugs based on LC-MS bioassay in the last two decades.Besides,we discussed the advantages and disadvantages of this technique in practical use.The pressing need for non-invasive sampling approaches and stability studies of anti-TB drugs was highlighted.Lastly,we provided perspectives on the prospects of combining LC-MS-based TDM and pharmacometabolomics with other advanced strategies(pharmacometrics,drug and vaccine developments,machine learning/artificial intelligence,among others)to encapsulate in an all-inclusive approach to improve treatment outcomes of TB patients.

关键词： Tuberculosis Therapeutic drug monitoring LC-MS MIPD Pharmacometabolomics Precision medicine

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Use of the knowledge,attitude,and practice(KAP)model to examine sustainable agriculture in Thailand

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Regional Sustainability 2022年第1期3卷 41-52页

作者： LIAO Xuewei Thi phuoc lai NGUYEN Nophea SASAKI Development Planning Management and Innovation(DPMI) Department of Development and SustainabilitySchool of EnvironmentResources and DevelopmentAsian Institute of Technology(AIT)Pathumthani12120Thailand Natural Resource Management(NRM) Department of Development and SustainabilitySchool of EnvironmentResources and DevelopmentAsian Institute of Technology(AIT)Pathumthani12120Thailand

Sustainable agriculture plays an important role in achieving sustainable development goals with regard to food security and environmental conservation.Sustainable agriculture relies on sustainable farming practices that reduce greenhouse gas production,the wise use of local natural resources,and reductions in negative impacts on the environment and human health.Sustainable farming practices can be driven by various factors,such as the socio-environmental setting,socio-cognitive factors,agricultural institutions,and policy.This study used the knowledge,attitude,and practice(KAP)model to examine farmers’knowledge,attitudes,and practices in the area of sustainable agriculture.It also considered the factors affecting farmers’knowledge,attitudes,and practices.Two different socio-environmental contextual settings in Surin Province(a Thai-Cambodian border province)of Thailand are considered.The results show that there are differences between the two different socio-environmental contextual settings with regard to farmers’sustainable agricultural practice perceptions,knowledge,and attitudes.Farmers’perceptions of environmental degradation,the number of years of agricultural experience,and agricultural policy drive farmers’attitudes and individual sustainable practices.Another major result of the study is that individual farmers’attitudes and practices promote collective sustainable agricultural behaviors.The implication of these findings is that it is necessary to improve the learning ability of individual farmers on the environment and sustainable agricultural practices through social learning and scientific knowledge dissemination,so as to produce sustainable collective development behaviors.

关键词： Socio-environmental context Individual and collective practices Sustainable agriculture KAP model Thailand

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The effectiveness of light emitting diode(LED)lamps in the offshore purse seine fishery in Vietnam

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Aquaculture and Fisheries 2023年第5期8卷 551-557页

作者： Nguyen Dang Nhat Do Thanh Tien truong Van Dan Nguyen Duy Quynh Tram Nguyen Quang Lich Ho Dang Phuc Nguyen Ngoc phuoc School of Engineering and Technology Hue University01 Dien Bien PhuHue City52000Viet Nam Faculty of Engineering and Food Technology University of Agriculture and ForestryHue University102 Phung HungHue City52000Viet Nam Faculty of Fisheries University of Agriculture and ForestryHue University102 Phung HungHue City52000Viet Nam Institute of Mathematics Vietnam Academy of Science and Technology18 Hoang Quoc VietCau Giay DistrictHanoi11300Viet Nam

Fishing with artificial light has become one of the most advanced,efficient,and common methods for the night-time purse seining in Vietnam.This study evaluated the radiation spectrum,CIE chromaticity coordinates,correlated color temperature(CCT),catch rate,fuel consumption,and CO_(2)emissions when using Light emitting diode(LED)lamps(0.196 kW)in comparison with the use of metal halide(MH)lights(1 kW)in the offshore purse seine fishery in Quang Tri province,Vietnam.The fishing efficiency of the purse seine fishing boats using LED lamps has increased 1.58 times in catch rate than MH lights,although the energy consumption of LED lamp is 4 times smaller.Fuel consumption of boats per trip using LED lamps was one third of that using MH lights.The use of LED reduced the radiation spectrum,especially the intense UV radiation which negatively affects the health of fishermen.This study also showed the potential of CO_(2)emission reduction up to 1.09 tons of CO_(2)per trip per boat from the use of LED lamps in the offshore purse seine fishing boats.

关键词： Light emitting diode(LED)lamp Metal halide(MH)light Offshore purse seine fishery Quang tri province Vietnam

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Hydrogen roles approaching ideal electrical and optical properties for undoped and Al doped ZnO thin films

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Journal of Materiomics 2022年第1期8卷 123-135页

作者： Dung Van Hoang Nam Hoang Vu Nga Thi Do Anh Tuan Thanh Pham truong Huu Nguyen Jer-lai Kuo Thang Bach Phan Vinh Cao Tran Laboratory of Advanced Materials University of ScienceHoChiMinh City700000Viet Nam Vietnam National University HoChiMinh City700000Viet Nam HoChiMinh City Institute of Physics HoChiMinh City700000Viet Nam Institute of Atomic and Molecular Sciences Academia SinicaTaipei10617Taiwan Center for Innovative Materials and Architectures(INOMAR) HoChiMinh City700000Viet Nam Faculty of Materials Science&Technology University of ScienceHoChiMinh City700000Viet Nam

This paper distinguished hydrogen roles to improve electron mobility and carrier concentration in ZnO and Al doped ZnO sputtered films.By combining experimental evidences and theoretical results,we find out that hydrogen located at oxygen vacancy sites(H_(O))is the main factor gives rise to increase simultaneously mobility and carrier concentration which has not been mentioned before.Introducing appropriate hydrogen content during sputtering not only results in crystalline relaxation but also supports doping Al into ZnO,increasing carrier concentration and electron mobility in the film.First principles calculations confirmed hydrogen substitutional stability for oxygen vacancy,significantly reducing electron conductivity effective mass and hence increasing electron mobility.In particular,0.8%hydrogen partial pressure ratio achieved 61 cm^(2)V^(-1)s^(-1)maximum electron mobility,optical transmittance above 82%in visible and near-infrared regions,and 2×10^(20) cm^(-3)carrier concentrations for H-Al co-doped ZnO film.These values approach ideal electrical and optical properties for transparent conducting oxide films.The presence of one maximum electron mobility was attributed to competition between increasing mobility due to restoring effective electron mass and hydrogen passivation of native defects,and decreased electron mobility due to electron-phonon scattering.

关键词： High electron mobility Hydrogen roles Passivation effects Effective electron mass DFT calculations Doped ZnO thin Film

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软木塞基碳量子点的水热合成及其生物相融荧光成像应用

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新型炭材料 2022年第3期37卷 595-602页

作者： Quang Ngo Khoa Hieu Nguyen Ngoc Bao Vo Van Quoc phuoc Vo Thi Ngoc Le Xuan Diem Doc Luong Quang Tri Nguyen Minh Son Le Vu truong Son Le Van Thanh Ha Che Thi Cam University of Sciences Hue University77 Nguyen HueHueVietnam Faculty of Environmental and Natural Sciences Duy Tan UniversityDa Nang550000Vietnam Institute for Research and Training in Medicine Biology and PharmacyDuy Tan UniversityDa Nang550000Vietnam University of Agriculture and Forestry Hue University102 Phung HungHueVietnam University of Science and Education The University of Da Nang459 Ton Duc ThangLien ChieuDa NangVietnam

以废弃酒瓶软木塞为原料,采用低成本、简单的水热方法合成碳量子点。通过TEM、FTIR、Raman、UV-Vis、PL光谱对碳量子点的结构和光学性能进行分析表征。结果表明,碳量子点的平均直径为6.2±2.7 nm,PL激发谱和碳量子点表面的官能团有关。... 详细信息

以废弃酒瓶软木塞为原料,采用低成本、简单的水热方法合成碳量子点。通过TEM、FTIR、Raman、UV-Vis、PL光谱对碳量子点的结构和光学性能进行分析表征。结果表明,碳量子点的平均直径为6.2±2.7 nm,PL激发谱和碳量子点表面的官能团有关。用硫酸奎宁作为参考,碳量子点的量子效率为1.54%。将获得的碳量子点应用在骨髓间充质干细胞的细胞生物成像上,发现用碳量子点处理后,骨髓间充质干细胞分别在320~380 nm、450~490 nm和450~490 nm范围显示绿色、黄色和红色荧光,表明了碳量子点在荧光成像领域具有潜在的应用价值。

关键词：碳点水热合成荧光荧光图像废酒瓶塞

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Detecting Chlorophyll a Concentration and Bloom Patterns at Upwelling Area in South Central Vietnam by High Resolution Multi-satellite Data

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Journal of Environmental Science and Engineering(A) 2015年第5期4卷 215-224页

作者： Tong phuoc Hoang Son truong Minh Chuan Hoang Cong Tin Institute of Oceanography Vietnam Academy Sciences and Technology Nha Trang 8458 Vietnam Department of Education and Administration Kien Giang University Kien Giang 8477 Vietnam Department of Environment and Agriculture Curtin University WA 6102 Australia

Study on Chlorophyll a (Chl. a) distribution and bloom patterns is essential in the upwelling areas that constitute the main fishery grounds of Vietnam. Based on high resolution satellite imagery and monthly in-situ data in period from 2007 to 2008, the spatial and temporal variations of Chl. a in the upwelling region including algal blooms have been detected. Anomalies of higher Chl. a concentration and bloom patterns occurred at different periods, locations, and bloom shapes in coastal waters of Southern Center of Vietnam. The appearances of these bloom are related to four difference reasons, such as: (i) Their locations coincided to main center of upwelling phenomena that usually occur during southwest monsoon (SWM); (ii) Effect of northeast monsoon (NEM) that brings and attaches the nutrient into the coast and created "floating" algae bloom patches in coastal zones; (iii) The algae blooms can be potentially associated with Harmful Algae Bloom (HAB) during the SWM or local eddies during NEM and (iv) Their appearances are also as a result of distinctive nutrient inflow from Mekong delta and pumping of nutrients by internal waves in coastal shallow waters.

关键词：高分辨率卫星影像叶绿素含量上升流区数据检测越南有害藻类水华中南部沿海水域

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Compensation of Zn substitution and secondary phase controls effective mass and weighted mobility in In and Ga co-doped ZnO material

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Journal of Materiomics 2021年第4期7卷 742-755页

作者： Oanh Kieu truong Le Anh Tuan Thanh Pham Ngoc Kim Pham Trang Huyen Cao Pham truong Huu Nguyen Dung Van Hoang Hanh Kieu Thi Ta Dai Cao truong Hoa Thi lai Thuy Dieu Thi Ung Vinh Cao Tran Thang Bach Phan aboratory of Advanced Materials University of ScienceHoChiMinh City700000Viet Nam Vietnam National University HoChiMinh City700000Viet Nam Faculty of Physics and Engineering Physics University of ScienceHoChiMinh City700000Viet Nam Faculty of Materials Science and Technology University of ScienceHoChiMinh City700000Viet Nam Center for Innovative Materials and Architectures(INOMAR) HoChiMinh CityViet Nam Institute of Materials Science Vietnam Academy of Science and TechnologyHanoi100000Viet Nam

Conductivity s and thermal conductivity k are directly related to carrier concentration while Seebeck coefficient S is inversely proportional to carrier concentration.Therefore,improving thermoelectric(TE)performance is challenging.Here,the first-time analysis of secondary phase-controlled TE performance in terms of density-of-state effective mass m*d,weighted mobility mw and quality factor B is discussed in ZnO system.The results show that the secondary spinel phase Ga2O_(3)(ZnO)9 not only impacts on k but also on s and S at high temperature,while the effect of carrier concentration seem to be dominant at low temperature.For the high-spinel-segregation sample,a compensation of dopant atoms from the spinel to substitutional sites in the ZnO matrix at high temperature leads to a low decreased rate of temperaturedependent m*d.The compensation process also induces a band sharpening,a small mw reduction,and a large B enhancement.As a result,In and Ga co-doped ZnO bulk with the highest spinel segregation achieves the greatest PF improvement by 112.8%,owing to enhanced Seebeck coefficient by 110%as compared to the good Zn-substitution sample.

关键词： Thermoelectrics In and Ga co-Doped ZnO Secondary phase Zn substitution DOS effective Mass Weighted mobility

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Influence of magnetic iron oxide nanoparticles on red blood cells and Caco-2 cells

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Advances in Bioscience and Biotechnology 2010年第5期1卷 439-443页

作者： Daniel Moersdorf Pierre Hugounenq lai Truonc phuoc Hind Mamlouk-Chaouachi Delphine Felder-Flesch Sylvie Begin-Colin Geneviève Pourroy Ingolf Bernhardt 不详

The interactions of two types of cells (red blood cells, Caco-2 cells) with magnetic iron oxide nanoparticles (non-grafted, citrate-grafted, dendrimer-grafted) of 11 nm in size have been investigated. We focused on two important physiological parameters of the cells, the intracellular pH and the intracellular Ca2+ content. The results show that the nanoparticles do not have a significant influence on the pH and Ca2+ content of Caco-2 cells. The Ca2+ content of red blood cells is also not affected but the intracellular pH is slightly reduced.

关键词： Red Blood Cells Caco-2 Cells Ca2+ Content Intracellular PH Magnetic Iron Oxide Nanoparticles

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