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Chinese Science Bulletin 2009年第2期54卷 304-310页

作者： XIE Min li shu jiang Fei WANG TiJian Department of Atmospheric Sciences Nanjing University Nanjing 210093 China

Methane (CH4) is the most important greenhouse gas and reactive trace gas in the atmosphere. Recently, it has been reported that terrestrial plants can emit CH4 under aerobic conditions, which may call for reevaluation of the inventory of CH4 emissions in China. In this paper, those emissions over China and their effects on CH4 concentrations in lower troposphere were investigated. Firstly, based on the work of Keppler et al., the aerobic plant CH4 emission model (PLANTCH4) for China was established. And by using the database of normalized difference vegetation index (NDVI) derived from NOAA/ AVHRR, the distribution of net primary productivity (NPP) over China was simulated, and thereby, for the first time, the amount and distribution of the newly identified source in China were estimated. Secondly, with the aid of the three-dimensional atmospheric chemistry model system (MM5-CALGRID), the effects of the emissions were studied. The results show that the annual aerobic plant CH4 emissions over China amount to 11.83 Tg, i.e. nearly 24% of Chinese total CH4 emissions. And the major fraction (about 43%) comes from forests. When those emissions are considered in modeling, computed countrywide mean surface concentration of CH4 is 29.9% higher than without them, with a maximum increase of 69.61 μg·m-3 in the south of Yunnan Province. In conclusion, to study CH4 emissions from terrestrial plants over China may have important implications for correctly estimating the contribution of China to global CH4 budget, and may call for a reconsideration of the role of CH4 in global and regional environment and climate change.

关键词：环境污染大气污染甲烷治理技术

Model Software Package Development for Laminar Cooling Process in Hot Mill

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Journal of Iron and Steel Research International 2010年第5期17卷 23-27页

作者： TAN Ming-hao li shu-jiang CHAI Tian-you School of Information Science and Engineering Shenyang University of Technology Shenyang 110178 Liaoning China Key Laboratory of Process Industry Automation Ministry of Education Shenyang 110004 Liaoning China Research Center of Automation Northeastern University Shenyang 110004 Liaoning China

The use of computer simulation techniques in the control system design of the laminar cooling process in a hot mill can significantly reduce the development cost while ensuring maximum production safety. The case-based modelling strategy was proposed and implemented in a software package. The functional structure of the software package was discussed in detail. The interfaces and functions of the software package were introduced. The results of industrial experiments can be directly visualized in the software package, allowing accurate and instant comparison of the model predictions with real measurements. The software package provides the simulation platform for research into advanced modelling and control strategies of the laminar cooling process in a hot rolling mill.

关键词： laminar cooling hot rolling model

Synthesis of a new aromatic diacid containing pyridine ring and related polybenzimidazole

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Chinese Chemical Letters 2010年第8期21卷 976-978页

作者： Tao Ma Yan Feng li shu jiang Zhang Feng Chun Yang Chen liang Gong Jiu jiang Zhao College of Chemistry and Chemical Engineering State Key Laboratory of Applied Organic Chemistry Institute of Biochemical Engineering & Environmental TechnologyLanzhou UniversityLanzhou 730000China

A new aromatic diacid monomer containing pyridine unit,4-phenyl-2,6-bis[4-（4-carboxyphenoxy） phenyl]pyridine 3,was successfully synthesized in three steps,starting from *** corresponding pyridine-containing polybenzimidazole was prepared via polycondensation of 3 with tetraaminodiphenyl ether（TADE） in poly（phosphoric acid）（PPA）.The resulting polybenzimidazole exhibits excellent solubility,good thermal stabilities and high thermal resistance.

关键词： Polybenzimidazoles Pyridine-containing diacid monomer Synthesis Thermal stabilities

Synthesis and characterization of novel polyimides based on thiazole-containing diamine

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Chinese Chemical Letters 2007年第10期18卷 1203-1204页

作者： Xin Zhao Yan Feng li shu jiang Zhang Xiao Long-Wang Yu Shao State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringInstitute of Biochemical Engineering ＆ Environmental Technology Lanzhou University Lanzhou 730000 China

A new kind of aromatic diamine monomer containing thiazole unit, 2-amino-5-（4-aminophenyl）-thiazole （AAPT）, was synthesized in three steps, starting from 4-nitroacetophenone. A novel thiazole-containing polyimide was prepared via the polycondensation of AAPT with 6FDA by one-step method. The resulting polyimide exhibits excellent solubility, film-forming capability and high thermal resistance.

关键词： Thiazole Thiazole-containing monomer Synthesis Aromatic diamine

OSMR is a potential driver of inflammation in amyotrophic lateral sclerosis

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Neural Regeneration Research 2024年第11期19卷 2513-2521页

作者： Wenzhi Chen Shishi jiang shu li Cheng li Renshi Xu Department of Neurology Jiangxi Provincial People’s HospitalXiangya Hospital Jiangxi Hospital of Central South UniversityThe Clinical College of Nanchang Medical CollegeThe First Affiliated Hospital of Nanchang Medical CollegeNanchangJiangxi ProvinceChina

Amyotrophic lateral sclerosis is a neurodegenerative disease,and the molecular mechanism underlying its pathology remains poorly ***,inflammation is known to play an important role in the development of this *** identify driver genes that affect the inflammatory response in amyotrophic lateral sclerosis,as well as potential treatment targets,it is crucial to analyze brain tissue samples from patients with both sporadic amyotrophic lateral sclerosis and C9orf72-related amyotrophic lateral ***,in this study we used a network-driven gene analysis tool,NetBID2.0,which is based on SJARACNe,a scalable algorithm for the reconstruction of accurate cellular networks,to experimentally analyze sequencing data from patients with sporadic amyotrophic lateral *** results showed that the OSMR gene is pathogenic in amyotrophic lateral sclerosis and participates in the progression of amyotrophic lateral sclerosis by mediating the neuroinflammatory ***,there were differences in OSMR activity and expression between patients with sporadic amyotrophic lateral sclerosis and those with C9orf72-related amyotrophic lateral *** findings suggest that OSMR may be a diagnostic and prognostic marker for amyotrophic lateral sclerosis.

关键词： amyotrophic lateral sclerosis driver neuroinflammation OSMR C9ORF72 neurodegenerative disease pathogenesis oxidative stress protein misfolding mitochondrial dysfunction

Critical Content of MgO in Spheroidisers

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Journal of Iron and Steel Research International 2006年第1期13卷 1-4页

作者： SHENG Da li shu-jiang LU Yue-mei liN Xiao-ying CHEN Shao-chun Department of Mechanical Engineering Tsinghua University Beijing 100084 China Mechanical Engineering and Automation Institute Fuzhou University Fuzhou 350002 Fuiian China

Magnesium oxide in spheroidiser is harmful to the production of ductile iron for decreasing active magnesium content. To obtain quality ductile iron, the effects of magnesium oxide content in spheroidisers on spheroidising treatment, microstrucure and properties of ductile iron were researched, and the critical magnesium oxide in spheroidisers was determined.

关键词： magnesium oxide critical content spheroidiser ductile iron

Pathways of intraseasonal Kelvin waves in the Indonesian Throughflow regions derived from satellite altimeter observation

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Atmospheric and Oceanic Science Letters 2016年第5期9卷 375-380页

作者： XU Teng-Fei WEI Ze-Xun CAO Guo-Jiao li shu-jiang First Institute of Oceanography State Oceanic AdministrationQingdaoChina Laboratory for Regional Oceanography and Numerica Modeling Qingdao National Laboratory for Marine Science and TechnologyQingdaoChina Key Laboratory of Marine Science and Numerica Modeling State Oceanic AdministrationQingdaoChina

The gridded sea level anomaly（SLA） data-set provided by AVISO is used to track the propagation of intraseasonal Kelvin waves in the Indonesian Throughflow（ITF） region. The large root mean square of intraseasonal SLA along the Sumatra and Java coast is closely related to the propagation of intraseasonal Kelvin waves that derive from the equatorial Indian Ocean. These Kelvin waves are further found to propagate following different pathways at the Lombok Strait. Pathway A propagates eastward throughout the Sumba Strait and Savu Sea to reach the Ombai Strait. Pathway B penetrates into Lombok and propagates northward to reach the Makassar Strait. Pathway C propagates southeastward along the southwest coast of the Sumba Island. The equatorial Kelvin waves take around 15 days to travel from the equatorial Indian Ocean to Lombok Strait, and around 5 days to penetrate into the Makassar and Ombai straits. The Kelvin wave-induced SLA persists in the ITF region for an additional 5 days and then diminishes subsequently. The phase speeds of these intraseasonal Kelvin waves along Pathways A, B, and C are 1.91–2.86, 1.69, and 1.96 m s^-1,respectively—in agreement with the first two baroclinic modes of Kelvin waves.

关键词： Indonesian Throughflow Kelvin waves intraseasonal variability pathway waveguide

Unconventional Fluorescent and Multi-responsive Polysiloxane:Synthesis,Characterization and Biological Applications

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Chinese Journal of Polymer Science 2024年第5期42卷 579-590,I0006页

作者： Xiao-Di li shu-Sheng li Xu-Bao jiang Xiao-li Zhu Xiang Zheng Kong College of Chemistry and Chemical Engineering University of JinanJinan250022China College of Chemical Engineering Tianjin UniversityTianjin300072China Foshan(Southern China)Institute for New Materials Foshan528200China

Owing to their high significance in fundamental study and diverse applications,stimuli-responsive and fluorescent polymers,particularly those with cluster-triggered emission(CTE)featured by non-conjugated chromophores,have drawn tremendous attention in recent *** this work,fluorescent and multi-responsive polysiloxane(FRPS)was synthesized by hydrolytic condensation polymerization of 3-aminopropyl methyl diethoxysilane(APMS)with 3-(N-isopropyl propionamide)iminopropyl methyl diethoxysilane(APMS-NIP),which was formed in situ through aza-Michael addition between APMS and N-isopropyl *** was not only highly sensitive to temperature,pH and CO_(2) in water,but also showed an enhanced and stimuli-adjustable fluorescence *** effects of monomer feeding,pH and CO_(2) on its lower critical solution temperature and fluorescent property were *** fluorescence emission was ascribed to CTE *** addition,FRPS was shown to be highly potential as physiological indicator for cell imaging,and for controlled release and trace detection of *** study provides therefore a type of stimuli-responsive and fluorescent material for potential applications in biomedical fields,and it is also of great significance for understanding of the fluorescence mechanism of polysiloxane-based stimuli-responsive polymers.

关键词： Polysiloxane Multi-responsiveness Cluster-triggered emission Cell imaging Controlled drug release

A high li-ion diffusion kinetics in multidimensional and compact-structured electrodes via vacuum filtration casting

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Journal of Energy Chemistry 2024年第6期93卷 368-376,I0010页

作者： Jieqiong li Ting Ouyang Lu liu shu jiang Yongchao Huang M.-Sadeeq Balogun College of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean EnergyHunan UniversityChangsha 410082HunanChina Institute of Environmental Research at Greater Bay Key Laboratory for Water Quality and Conservation of the Pearl River DeltaMinistry of EducationGuangzhou UniversityGuangzhou 510006GuangdongChina

Manufacturing process,diffusion co-efficient and areal capacity are the three main criteria for regulating thick electrodes for lithium-ion batteries(liBs).However,simultaneously regulating these criteria for liBs is desirable but remains a significant *** this work,niobium pentoxide(Nb_(2)O_(5))anode and lithium iron phosphate(liFePO_(4))cathode materials were chosen as the model materials and demonstrate that these three parameters can be simultaneously modulated by incorporation of micro-carbon fibers(MCF)and carbon nanotubes(CNT)with both Nb_(2)O_(5) and LFP via vacuum filtration *** as-prepared MNC-20 anode and MLC-20 cathode achieves high reversible areal capacity of≈5.4 m A h cm^(-2)@0.1 C and outstanding li-ion diffusion coefficients of≈10~(-8)cm~2 s~(-1)in the half-cell *** assembled MNC-20‖MLC-20 full cell liB delivers maximum energy and power densities of244.04 W h kg^(-1)and 108.86 W kg^(-1),*** excellent electrochemical properties of the asprepared thick electrodes can be attributed to the highly conductive,mechanical compactness and multidimensional mutual effects of the MCF,CNT and active materials that facilitates rapid li-ion diffusion ***,electrochemical impedance spectroscopy(EIS),symmetric cells analysis,and insitu Raman techniques clearly validates the enhanced li-ion diffusion kinetics in the present architecture.

关键词： Thick electrodes Carbon nanotubes li-ion diffusion co-efficient Vacuum filtration technique High areal capacity lithium-ion batteries

Unconventional Fluorescent and Multi-responsive Polyethyleneimine with LCST and UCST Behavior:Synthesis,Characterization and Biological Applications

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Chinese Journal of Polymer Science 2024年第6期42卷 826-837页

作者： Feng-Ming Yin li-li Wu shu-Sheng li Xiao-Na Pan Xiao-li Zhu Xu-Bao jiang Xiang Zheng Kong College of Chemistry and Chemical Engineering University of JinanJinan250022China Shandong Institute for Product Quality Inspection Jinan250102China College of Chemical Engineering Tianjin UniversityTianjin300072China

Non-aromatic fluorescent and multi-responsive materials,exhibiting inherent fluorescence emission and controlled phase change,have garnered significant attention in recent ***,the underlying interaction between their fluorescent properties and phase transition remains *** this study,we synthesized a series of catalyst-free aza-Michael addition-based polyethyleneimine(RFPEI)materials by reacting polyethyleneimine(PEI)with N-isopropyl acrylamide(NIPAM).The resulting RFPEI was comprehensively characterized,and demonstrated dual-phase transition behavior(LCST and UCST)in water,which could be finely tuned by adjusting its composition or external factors such as ***,upon UV irradiation(365 nm),RFPEI exhibited strong fluorescence *** further investigated the effects of NIPAM grafting percentage to PEI,polymer concentration,and pH on the LCST/UCST and fluorescent properties of RFPEI aqueous ***,we showcased the great potential of RFPEI as a versatile tool for physiological cell imaging,trace detection,and controlled release of *** study presents a novel class of stimuli-responsive fluorescent materials with promising applications in the field of biomedicine.

关键词： Polyethyleneimine Multi-responsiveness Intrinsic fluorescence emission Cell imaging Controlled drug release