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Tungsten pnictides for water electrolysis:advances and perspectives

Tungsten 2024年第4期6卷 675-695页

作者： Xue kang Xi-Han Tan Ning Han Jian-Feng Hou Chen-Min yao Zhi-Jie Chen Bing-Jie Ni Department of Chemistry and Chemical Engineering Lyuliang University Department of Materials Engineering State Key Laboratory of Oral & Maxillofacial Reconstruction and Regeneration Key Laboratory of Oral Biomedicine Ministry of Education Hubei Key Laboratory of Stomatology School & Hospital of Stomatology Wuhan University School of Civil and Environmental Engineering The University of New South Wales

Hydrogen fuel is recognized as a promising energy carrier for the sustainable development of global energy system and the green hydrogen production via water electrolysis attracts great *** development of cost-effective electrocatalysts for water electrolysis is important for enhancing green hydrogen production ***,tungsten pnictides(phosphides and nitrides) have emerged as promising catalysts for water electrolysis,and efficient tungsten pnictide-based catalysts with different nanostructures,compositions,and surface chemical properties have been *** this review,recent progress in the design of tungsten pnictide-based electrocatalysts for water electrolysis is comprehensively *** synthesis of tungsten pnictide-based electrocatalysts are discussed ***,current achievements in developing efficient tungsten pnictide electrocatalysts for water electrolysis are detailed,and four key catalyst design strategies(i.e.,nanostructure control,heteroatom doping,defect engineering,and heterostructure design) are *** physicochemical properties-catalytic performance relationship of tungsten pnictide-based electrocatalysts is also *** last,perspectives in this field are put forward for guiding further research on the design and application of high-performance tungsten pnictide-based electrocatalysts.

关键词： Electrocatalysts Hydrogen evolution reaction Oxygen evolution reaction Tungsten nitrides Tungsten phosphides

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Interfacial DMI in Fe/Pt thin films grown on different buffer layers

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Chinese Physics B 2024年第4期33卷 712-718页

作者：张文君魏菲刘冰周阳康仕寿孙兵 School of Physics and Electronic Information Weifang UniversityWeifang 261061China School of Physics and State Key Laboratory of Crystal Materials Shandong UniversityJinan 250100China

We study the interfacial Dzyaloshinskii-Moriya interactions(i-DMI)of Fe/Pt bilayers grown on Si substrates with MgO,SiO_(2),or Ta each as a buffer layer on the basis of wave-vector-resolved Brillouin light scattering(BLS)*** obtained i-DMI energy values for Fe/Pt on MgO,Ta,and SiO_(2) buffer layers are 0.359,0.321,and 0.274 mJ/m~2,*** large i-DMI value observed in Fe/Pt system on the MgO buffer layer can be attributed to the good interfacial quality and the Rshaba effect at the MgO/Fe ***,the MgO/Fe/Pt system,benefiting from better sample quality,exhibits a lower damping ***,layer-resolved first-principles calculations are carried out to gain a more in-depth understanding of the origin of the i-DMI in the Fe/Pt *** results indicate that in the Fe(110)/Pt(111)system,the substantial DMI energy between Fe spins at the interface is related to a significant change in spin-orbit coupling(SOC)energy in the neighboring Pt *** contrast,for the MgO(002)/Fe(002)system,both the DMI and its related SOC energy are concentrated at the interfacial Fe *** investigation will provide a valuable insight into the spintronic community in exploring novel devices with chirality dependence.

关键词： Fe/Pt i-DMI BLS ferromagnetic resonance magnetic relaxation

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Gga-miRNA-181-5p family facilitates chicken myogenesis via targeting TGFBR1 to block TGF-βsignaling

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Journal of Integrative Agriculture 2024年第8期23卷 2764-2777页

作者： Xiaoxu Shen Yongtong Tian Wentao He Can He Shunshun Han yao Han Lu Xia Bo Tan Menggen Ma Houyang kang Jie Yu Qing Zhu Huadong Yin Key Laboratory of Livestock and Poultry Multi-omics Ministry of Agriculture and Rural AffairsCollege of Animal Science and TechnologySichuan Agricultural UniversityChengdu 611130China Farm Animal Genetic Resources Exploration and Innovation Key Laboratory of Sichuan Province Sichuan Agricultural UniversityChengdu 611130China College of Forestry Sichuan Agricultural UniversityChengdu 611130China College of Resources Sichuan Agricultural UniversityChengdu 611130China Triticeae Research Institute Sichuan Agricultural UniversityChengdu 611130China Key Laboratory for Animal Disease Resistance Nutrition of China Institute of Animal NutritionMinistry of Education/Sichuan Agricultural UniversityChengdu 611130China

MicroRNAs(miRNAs)have been demonstrated to control chicken skeletal muscle growth,however,the potential function of the miR-181-5p family in chicken myogenesis remains largely ***,our study identified the two chicken(Gallus gallus;Gga)miR-181-5p family members widely expressed in various tissues,specifically miR-181a-5p and ***,the breast muscles of fast-growing broilers expressed higher levels of miR-181a-5p and miR-181b-5p than those of slow-growing ***,miR-181a-5p and miR-181b-5p both promote the expression level of myogenic factors including myogenin(MyoG),myogenic differentiation 1(MyoD1),and myosin heavy chain(MyHC),meanwhile accelerating the myotube formation of skeletal muscle satellite cells(SMSCs).Mechanistically,miR-181a-5p and miR-181b-5p directly bind to the 3′untranslated region(UTR)of the transforming growth factor beta receptor 1(TGFBR1)mRNA,further reducing the expression of ***1 is a key Transforming growth factor beta(TGF-β)signaling transduction receptor and had a negative function in muscle cell ***,knockdown of TGFBR1 facilitated the expression of chicken myogenic factors,boosted myotube formation,and decreased the SMAD family member 2/3(SMAD2/3)phosphorylation in chicken ***2/3 are downstream of TGF-βsignaling,and miR-181a-5p and miR-181b-5p could reduce the expression of TGFBR1 to further diminish the SMAD2/3 *** findings revealed that the miR-181-5p family targets TGFBR1 to break the TGF-βsignaling transduction,which resulted in promoting chicken skeletal muscle development.

关键词： miRNA-181-5p family SMSCs differentiation TGFBR1 TGF-βsignaling

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Enhanced identification and localization of metabolites in Scutellariae Radix using ion mobility enabled MALDI-Q-TOF/MS imaging

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Journal of Pharmaceutical Analysis 2024年第2期14卷 284-286页

作者： Lixing Nie Lieyan Huang Xiaofei Jia Shuai kang Lingwen yao Yanpei Wu Hao Yuan Yongli Liu Feng Wei Hongyu Jin Xiang Li Shuangcheng Ma National Institutes for Food and Drug Control Beijing102629China Chinese Academy of Medical Science and Peking Union Medical College Beijing100006China Waters Corporation Beijing102600China Hebei Institute for Drug and Medical Device Control Shijiazhuang050227China Department of Pharmacy Medical Supplies Center of the PLA General HospitalBeijing100853China

Unraveling the distribution of metabolites in traditional Chinese medicine(TCM)provides direct indications for understanding their regulatory and functional basis,which is of paramount significance for better utilization and quality control of medicinal plants[1].Recently,imaging techniques such as near-infrared spectroscopy,Raman spectroscopy,and mass spectrometry(MS)were explored to reveal the spatial context of component accumulation and localization[2,3].

关键词： medicine(TCM) Radix Scutellaria

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Tumour response following preoperative chemotherapy is affected by body mass index in patients with colorectal liver metastases

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World Journal of Gastrointestinal Oncology 2024年第2期16卷 331-342页

作者： Hua-Chuan Song Hang-Cheng Zhou Ping Gu Bing Bao Quan Sun Tian-Ming Mei Wei Cui kang yao Huan-Zhang yao Shen-Yu Zhang Yong-Shuai Wang Rui-Peng Song Ji-Zhou Wang Department of General Surgery Provincial Hospital Affiliated to Anhui Medical UniversityHefei 230001Anhui ProvinceChina Department of Hepatobiliary Surgery The First Affiliated Hospital of University of Science and Technology of ChinaDivision of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefei 230001Anhui ProvinceChina Department of Pathology The First Affiliated Hospital of University of Science and Technology of ChinaDivision of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefei 230001Anhui ProvinceChina Department of Gastrointestinal Surgery Tongcheng People’s HospitalTongcheng 231400Anhui ProvinceChina Department of Gastrointestinal Surgery Suzhou Hospital Affiliated to Anhui Medical UniversitySuzhou 234000Anhui ProvinceChina Department of General Surgery Xuancheng People’s HospitalXuancheng 242000Anhui ProvinceChina

BACKGROUND Colorectal cancer is the third most prevalent malignancy globally and ranks second in cancer-related mortality,with the liver being the primary organ of *** chemotherapy is widely recommended for initially or potentially resectable colorectal liver metastases(CRLMs).Tumour pathological response serves as the most important and intuitive indicator for assessing the efficacy of ***,the postoperative pathological results reveal that a considerable number of patients exhibit a poor response to preoperative *** mass index(BMI)is one of the factors affecting the tumori-genesis and progression of colorectal cancer as well as prognosis after various antitumour *** studies have indicated that overweight and obese patients with metastatic colorectal cancer experience worse prognoses than those with normal weight,particularly when receiving first-line chemotherapy regimens in combination with *** To explore the predictive value of BMI regarding the pathologic response following preoperative chemotherapy for *** A retrospective analysis was performed in 126 consecutive patients with CRLM who underwent hepatectomy following preoperative chemotherapy at four different hospitals from October 2019 to July *** and multivariate logistic regression models were applied to analyse potential predictors of tumour pathological *** Kaplan-Meier method with log rank test was used to compare progression-free survival(PFS)between patients with high and low ***<24.0 kg/m^(2) was defined as low BMI,and tumour regression grade 1-2 was defined as complete tumour *** Low BMI was observed in 74(58.7%)patients and complete tumour response was found in 27(21.4%)*** rate of complete tumour response was significantly higher in patients with low BMI(29.7%vs 9.6%,P=0.007).Multivariate analysis revealed that low BMI[odds ratio(OR)=4.56,95%confidence interval(CI):1

关键词： Colorectal liver metastases Body mass index Tumour regression grade Preoperative chemotherapy Hepatectomy

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Optimization of Extraction Process for Total Flavonoids from Penthorum chinense Pursh and Comparison of Their Contents from Different Parts

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Medicinal Plant 2024年第2期15卷 10-14页

作者： Hongsheng LIU Jiqiang yao Xue BAI Jianying kang Yefei YUAN Department of Pharmacy Luzhou Hospital of Traditional Chinese MedicineLuzhou 646000China Luzhou Feixiang Pharmaceutical Technology Co. LtdLuzhou 646000China Department of Pharmacy Southwest Medical UniversityLuzhou 646000China

[Objectives]This study was conducted to optimize the extraction process of total flavonoids from Penthorum chinense Pursh and compare their contents from different parts.[Methods]Single factor and orthogonal experiments were designed to optimize the extraction process of total flavonoids from *** Pursh with the volume fraction of ethanol,the ratio of material to liquid,heating reflux extraction time and extraction times as factors,and the content of total flavonoids as the index.A verification test was carried *** optimized extraction process was adopted to compare the contents of total flavonoids from different parts of *** Pursh.[Results]The best extraction process was extracting the powder of *** Pursh for 2.0 h with 20 times of 55%ethanol by reflux *** this condition,the contents of total flavonoids were 3.63%,8.90%,11.28%,and 4.36%from stems,leaves,flowers and whole grass of *** Pursh,respectively.[Conclusions]The process is reasonable,feasible and stable,and can effectively extract total flavonoids from *** *** contents of total flavonoids from different parts of *** Pursh were quite different,and the value was higher in the leaves and flowers,so the proportions of leaves and flowers should be paid attention to in the industrial processing of *** Pursh.

关键词： Penthorum chinense Pursh Total flavonoids Orthogonal experiments Extraction process Content determination

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A MOF built on 8-connected Ynodes demonstrates simultaneous reverse adsorptive separation: ethane over ethylene and propane over propylene

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Science China Chemistry 2024年

作者： Lu-Lu Ma Jiaqi Liu kang Zhou Zixuan Cao Jiafeng Miao Guo-Ping Yang yao-Yu Wang Jing Li Hao Wang Key Laboratory of Synthetic and Natural Functional Molecule Chemistry of the Ministry of Education Shaanxi Key Laboratory of PhysicoInorganic Chemistry College of Chemistry & Materials Science Northwest University Hoffmann Institute of Advanced Materials Shenzhen Polytechnic University Shenzhen Senior High School Department of Chemistry and Chemical Biology Rutgers UniversityPiscataway

Selective adsorption of paraffins over olefins（mostly C2 and C3） by porous solids could offer tremendous advantages for the purification of olefins, which is, however, challenging as it has stringent requirements on the pore dimensions and pore surface chemistry of the adsorbent. We report here a metal-organic framework（MOF） with novel topology, Y3（μ3-OH）(TCMPB)2(denoted as HIAM-316, TCMPB4-= 1,2,4,5-tetra（4-carboxy-3-methylphenyl）benzene), which shows reversed separation of C2H6/C2H4and C3H8/C3H6simultaneously. The ideal adsorbed solution theory（IAST） selectivities for equimolar binary mixtures of C2H6/C2H4and C3H8/C3H6were calculated to be 1.67 and 1.23 at 1 bar and 298 K for HIAM-316. Its capability of removing paraffines from paraffin/olefin mixtures is validated by breakthrough measurements. Molecular simulations reveal that the preferential adsorption of paraffins over olefins by HIAM-316 may be attributed to the abundant carboxylate oxygen atoms along its channel.

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利用互子带滤波器和稀疏特性的多通道线性预测语音去混响方法

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数据采集与处理 2024年第5期39卷 1135-1146页

作者：康瑶康坊杨飞然国家开放大学数字化部北京100039 奥卢大学机器视觉与信号分析中心奥卢90570 中国科学院噪声与振动重点实验室(声学研究所) 北京100190

多通道线性预测是最为流行的语音去混响方法之一,现有相关研究大多利用子带谱减模型在每一个频带独立地获取期望信号,但这忽略了不同子带之间的相互影响。本文提出一种利用互子带谱减模型的多通道线性预测语音去混响方法。相比于大多数... 详细信息

多通道线性预测是最为流行的语音去混响方法之一,现有相关研究大多利用子带谱减模型在每一个频带独立地获取期望信号,但这忽略了不同子带之间的相互影响。本文提出一种利用互子带谱减模型的多通道线性预测语音去混响方法。相比于大多数方法采用的子带谱减模型,本文方法采用的互子带谱减模型能够利用互子带滤波器来对不同子带之间的相互影响进行建模。本文方法利用复广义高斯分布建模期望信号,相比于常用的高斯分布,复广义高斯分布能够通过调整形状参数来描述语音信号的稀疏特性。在最大似然估计框架下,将语音去混响转化为关于互子带滤波器和子带滤波器的优化问题;并且基于替代最小化方法推导了保证收敛的优化算法。在不同混响时间、不同通道、不同声源和传声器距离情况下的一系列语音去混响实验验证了本文方法的性能显著优于传统去混响算法。

关键词：语音去混响多通道线性预测互子带滤波器复广义高斯分布替代最小化

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GNSS和非实测气象参数的PWV反演方法及其精度评估

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武汉大学学报（信息科学版） 2024年第3期49卷 453-464页

作者：赵庆志刘康李祖锋姚顽强姚宜斌西安科技大学测绘科学与技术学院陕西西安710054 中国电建集团西北勘测设计研究院有限公司陕西西安710065 武汉大学测绘学院湖北武汉430079

水汽是大气的重要组成成分之一,其时空变化受气温、气压等多种气象因素的影响。因此,研究水汽反演影响因素对获取高精度水汽信息具有重要意义。以中国区域为例,研究利用全球导航卫星系统(global navigation satellite sys‐tem,GNSS)和... 详细信息

水汽是大气的重要组成成分之一,其时空变化受气温、气压等多种气象因素的影响。因此,研究水汽反演影响因素对获取高精度水汽信息具有重要意义。以中国区域为例,研究利用全球导航卫星系统(global navigation satellite sys‐tem,GNSS)和非实测气象数据(气温和气压)探测大气可降水量(precipitable water vapor,PWV)的方法。首先,对欧洲中期天气预报中心(European Centre for Medium-Range Weather Forecasting,ECMWF)第5代气候再分析数据集(ECMWF reanalysis v5,ERA5)提供的气温、气压和GNSS反演的天顶对流层延迟进行评估;其次,大气加权平均温度T_(m)是PWV反演的关键参数,对不同的T_(m)计算模型进行分析,确定中国区域最优T_(m)计算模型;最后,根据误差传播理论推导PWV的理论误差,利用非实测数据计算小时分辨率的PWV并进行精度评估。结果表明,利用GNSS获取的中国区域PWV与无线电探空/ERA5 PWV均有较好的时空一致性,降雨期间PWV的误差较非降雨期间稍大。所提方法获取的PWV理论误差为2.0 mm,实际误差为2.1 mm。因此,基于GNSS和非实测气象参数反演的PWV具有较高精度,对于研究中国区域水汽时空变化与分布具有重要意义。

关键词：全球导航卫星系统 ECMWF第5代再分析数据大气加权平均温度大气可降水量

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考虑变井阻的多元复合地基固结理论研究

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工程力学 2024年第6期41卷 44-54页

作者：白垚卢萌盟杨康赵明中国矿业大学力学与土木工程学院江苏徐州221116 中国矿业大学深部岩土力学与地下工程国家重点实验室江苏徐州221116 浙江木石建设项目管理咨询有限公司浙江杭州311199

该文以塑料排水板联合水泥搅拌桩多元复合地基为研究对象,通过假定排水板的渗透系数随时间呈指数型衰减,考虑了排水板在固结过程中的淤堵效应对地基固结性状的影响。同时,该文还考虑排水板的涂抹效应、水泥搅拌桩的扰动效应以及土体的径... 详细信息

该文以塑料排水板联合水泥搅拌桩多元复合地基为研究对象,通过假定排水板的渗透系数随时间呈指数型衰减,考虑了排水板在固结过程中的淤堵效应对地基固结性状的影响。同时,该文还考虑排水板的涂抹效应、水泥搅拌桩的扰动效应以及土体的径-竖向耦合渗流,推导得出多元复合地基的固结控制方程及其解答。通过与已有解答和现场试验的对比分析,验证该文解答的正确性。最后,采用参数敏感性分析法对多元复合地基固结性状进行研究。研究结果表明:复合地基井阻因子θ对固结后期影响较大,当θ值较大时,径向渗流由于排水板的淤堵效应将提前终止,最终仅由竖向渗流使得地基达到完全固结;初始渗透系数k_0越大,井阻因子θ越小,涂抹作用越弱,板和桩的置换率越高,复合地基固结速率就越快。

关键词：多元复合地基排水板变井阻效应固结淤堵效应

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