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Organic X-Ray Image Sensors Using a Medium Bandgap Polymer Donor with Low Dark Current

ENERGY & ENVIRONMENTAL MATERIALS 2024年第6期7卷 230-237页

作者： ha, jong-Woon Eom, Seung hun Cha, Bo Kyung Song, Seyeong Eun, hyeong ju kim, jong h. Park, jong Mok kim, Bongsoo Park, Byoungwook Ko, Seo-jin Yoon, Sung Cheol Lee, Changjin jung, In hwan hwang, Do-hoon Pusan Natl Univ Chem Inst Funct Mat Dept Chem Busan 46241 South Korea Korea Res Inst Chem Technol KRICT Div Adv Energy Mat Res Ctr Daejeon 34114 South Korea Korea Electrotechnol Res Inst KERI Electromed Device Res Ctr Ansan 15588 South Korea Ulsan Natl Inst Sci & Technol UNIST Grad Sch Carbon Neutral Sch Energy & Chem Engn Ulsan 44919 South Korea Ajou Univ Dept Mol Sci & Technol Suwon 16449 South Korea Korea Res Inst Chem Technol Res Ctr Adv Specialty Chem Ulsan 44412 South Korea Ulsan Natl Inst Sci & Technol UNIST Dept Chem Ulsan 44919 South Korea hanyang Univ Dept Organ & Nano Engn Human Tech Convergence Program 222 Wangsimni Ro Seoul 04763 South Korea

The development of portable X-ray detectors is necessary for diagnosing fractures in unconscious patients in emergency situations. however, this is quite challenging because of the heavy weight of the scintillator and silicon photodetectors. The weight and thickness of X-ray detectors can be reduced by replacing the silicon layer with an organic photodetectors. This study presents a novel bithienopyrroledione-based polymer donor that exhibits excellent photodetection properties even in a thick photoactive layer (similar to 700 nm), owing to the symmetric backbone and highly soluble molecular structure of bithienopyrroledione. The ability of bithienopyrroledione-based polymer donor to strongly suppress the dark current density (j(d) similar to 10(-10) A cm(-2)) at a negative bias (-2.0 V) while maintaining high responsivity (R = 0.29 A W-1) even at a thickness of 700 nm results in a maximum shot-noise-limited specific detectivity of D-sh* = 2.18 x 10(13) jones in the organic photodetectors. Printed organic photodetectors are developed by slot-die coating for use in X-ray detectors, which exhibit D-sh* = 2.73 x 10(12) jones with clear rising (0.26 s) and falling (0.29 s) response times upon X-ray irradiation. Detection reliability is also proven by linear response of the X-ray detector, and the X-ray detection limit is 3 mA.

关键词： low dark current low detection limit organic photodetector printable X-ray DETECTORS PhOTOCONDUCTORS SENSITIVITY

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Photo-induced crosslinked and anti-PD-L1 peptide incorporated liposomes to promote PD-L1 multivalent binding for effective immune checkpoint blockade therapy

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Acta Pharmaceutica Sinica B 2024年第3期14卷 1428-1440页

作者： Youngjoo Lee Sukyung Song Suah Yang jinseong kim Yujeong Moon Nayeon Shim hong Yeol Yoon Sehoon kim Man Kyu Shim Kwangmeyung kim KU-KIST Graduate School of Converging Science and Technology Korea UniversitySeoul 02841Republic of Korea Medicinal Materials Research Center Biomedical Research DivisionKorea Institute of Science and Technology(KIST)Seoul 02792Republic of Korea College of Pharmacy Graduate School of Pharmaceutical SciencesEwha Womans UniversitySeoul 03760Republic of Korea Department of Bioengineering Korea UniversitySeoul 02841Republic of Korea

Immune checkpoint blockade(ICB)therapy targeting PD-L1 via monoclonal antibody(m Ab)has shown extensive clinical benefits in the diverse types of advanced ***,most patients are completely refractory to ICB therapy owing to the PD-L1 recycling ***,we propose photo-induced crosslinked and anti-PD-L1 peptide incorporated liposomes(immune checkpoint blockade liposomes;ICB-LPs)to promote PD-L1 multivalent binding for inducing lysosomal degradation of PD-L1 in tumor *** ICB-LPs are prepared by formulation of DC_(8,9)PC with photo-polymerized diacetylenic moiety,1,2-dipalmitoylphosphatidylcholine(DPPC)and anti-PD-L1peptide(D-form NYSKPTDRQYhF)-conjugated DSPE-PEG_(2k)(anti-PD-L1-DSPE-PEG_(2k))in a molar ratio of 45:45:10,followed by cross-linking of liposomal bilayer upon UV *** 10 mol% antiPD-L1-DSPE-PEG_(2k)incorporated ICB-LPs have a nano-sized lipid bilayer structure with an average diameter of 137.7±1.04 nm,showing a high stability in serum ***,the ICB-LPs efficiently promote the multivalent binding with PD-L1 on the tumor cell membrane,which are endocytosed with aim to deliver PD-L1 to the lysosomes,wherein the durable PD-L1 degradation is observed for72 h,in contrast to anti PD-L1 m Abs showing the rapid PD-L1 recycling within 9 *** in vitro coculture experiments with CD8^(+)T cells show that ICB-LPs effectively enhance the T cell-mediated antitumor immune responses against tumor cells by blocking the PD-L1/PD-1 *** ICB-LPs are intravenously injected into colon tumor-bearing mice,they efficiently accumulate within the targeted tumor tissues via both passive and active tumor targeting,inducing a potent T cell-mediated antitumor immune response by effective and durable PD-L1 ***,this study demonstrates the superior antitumor efficacy of crosslinked and anti-PD-L1 peptide incorporated liposome formulation that promotes PD-L1 multivalent binding for trafficking of PD-L1 toward

关键词： Cancer immunotherapy Immune checkpoint blockade PEGylated liposome Crosslinked lipid nanoparticles Anti-PD-L1 peptide Tumor-targeting PD-L1 multivalent binding Lysosomal PD-L1 degradation

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Rapid monitoring of indoor airborne influenza and coronavirus with high air flowrate electrostatic sampling and PCR analysis

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 73-85页

作者： Sanggwon An Sangsoo Choi hyeong Rae kim jungho hwang School of Mechanical Engineering Yonsei UniversitySeoul 02876Republic of Korea Gas Metrology Group Korea Research Institute of Standards and Science(KRISS)Daejeon 34113Republic of Korea

The World health Organization has raised concerns about the possibility of airborne transmission in enclosed and poorly ventilated ***,rapid monitoring of airborne viruses is necessary in multi-use facilities with dense ***,an electrostatic air sampler(250 L/min)was developed in this work to obtain indoor viral aerosol samples for analysis via the Polymerase Chain Reaction(PCR).Aerosol tests with h1N1 and hCoV-229E were performed to evaluate the sample collection *** analysis,along with another aerosol test,was conducted to evaluate the recovery of the virus particles collected by the *** laboratory tests,our electrostatic sampler obtained viral samples that were detectable by PCR under the simulated viral pandemic scenario(3000 RNA copies per cubic meter of air)within 40 *** resulting cycle threshold(C)values were 35.07 and 37.1 for h1N1 and hCoV-229E,*** the performance evaluation in the laboratory,field tests were conducted in a university classroom from October 28 to December 2,*** A and hCoV-229E were detected in two air samples,and the corresponding C,values were 35.3 and *** PCR results are similar to those obtained from laboratory tests,considering the simulatedviralpandemic scenario.

关键词： Airborne virus Electrostatic sampler Rapid monitoring Indoor environment Field test

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Mechanism of reduction-diffusion reaction in Sm-Fe binary system at low temperature using molten salts

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journal of Rare Earths 2024年第10期42卷 1889-1894页

作者： jungryang kim Shusuke Okada Kenta Takagi kimihiro Ozaki Innovative Functional Materials Research Institute National Institute of Advanced Industrial Science and Technology (AIST)

In this study,the mechanism of the reduction-diffusion reaction in a Sm-Fe binary system at low temperature was studied to investigate the possibility of synthesis of a Fe-rich TbCu7-type SmFex（x>9）by the low-temperature diffusion-reduction（LTRD） process using LiCl-KCl eutectic molten ***,the Sm-Fe phase transformation depending on the Sm-Fe composition,the LTRD temperature,and time was investigated,and it is found that the obtained metastable phase is only TbCu7-type SmFe～8.5,which is not a Fe-rich *** Fe content does not change even after an expended LTRD process,and the metastable TbCu7-type SmFe～8.5tends to transform to the stable *** addition,it is found that the Sm-Fe phase starts to synthesize from the Sm-rich phase in the order of SmFe2,SmFe3,and SmFe8.5as the LTRD temperature increases（when the time was 10 h） or the LTRD time increases（when the temperature was 550℃）.Core-shell-like particles are observed in the case of a short LTRD time,and the core and the shell are Fe and the Sm-rich Sm-Fe phase,respectively,indicating that the Sm-rich phase begins to produce on the surface of the Fe *** is difficult to synthesize a Fe-rich TbCu7-type SmFex（x>9） phase with the Sm-Fe binary system,suggesting that a different approach,such as addition of other elements,will be necessary.

关键词： Low-temperature synthesis Molten salts Rare earths Reduction-diffusion process Sm–Fe compounds Synthesis mechanism

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Integration of earth-abundant cocatalysts for high-performance photoelectrochemical energy conversion

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journal of Energy Chemistry 2024年第1期88卷 336-355,I0008页

作者： joonhee Ma Sang hyun Ahn Soo Young kim Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea School of Chemical Engineering and Materials Science Chung-Ang University84 Heukseok-roDongjak-guSeoul 06974Republic of Korea

Photoelectrochemical(PEC)energy conversion has emerged as a promising and efficient approach to sustainable energy harvesting and *** utilizing semiconductor photoelectrodes,PEC devices can harness solar energy and drive electrochemical reactions such as water splitting or carbon dioxide(CO_(2))reduction to generate clean fuels and value-added ***,PEC energy conversion faces several challenges such as high overpotential,sluggish reaction kinetics,charge carrier recombination,and stability issues,which limit its practical ***,significant research has been conducted to improve the overall conversion efficiency of PEC *** particularly promising approach is the use of cocatalysts,which involves introducing specific cocatalysts onto the photoelectrode surface to promote charge separation,improve reaction kinetics,and reduce the overpotential,thereby enhancing the overall performance of PEC energy *** review provides a comprehensive overview of the recent developments in the earth-abundant cocatalysts for PEC water splitting and CO_(2) *** main earth-abundant catalysts for the PEC water splitting include transition-metal dichalcogenide(TMD)-based materials,metal phosphides/carbides,and metal oxides/***,PEC-CO_(2)RR was divided into C_(1) and C_(2+)based on the final product since various products could be produced,focusing on diverse earth-abundant materials-based *** addition,we provide and highlight key advancements achieved in the very recent reports on novel PEC system design engineering with ***,the current problems associated with PEC systems are discussed along with a suggested direction to overcome these obstacles.

关键词： Solar energy Photo-electrochemical Water splitting CO_(2)reduction Cocatalysts

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On breakthroughs and limits: Resolving structural fine-tuning of photosynthetic supercomplexes

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Molecular Plant 2024年第2期17卷 224-226页

作者： Eunchul kim Marcel Dann Division of Environmental Photobiology National Institute for Basic BiologySOKENDAlOkazaki 444-8585Japan Department of Basic Biology The Graduate University for Advanced StudiesSOKENDAlOkazaki 444-8585Japan Bio-Inspired Energy Conversion Technical University of DarmstadtSchnittspahnstraBe 1064287 DarmstadtGermany

Dynamic regulation of photosynthetic supercomplexes is a key strategy allowing plants to adjust their light-harvesting system in response to varying environmental light conditions(Bassi and Dall'Osto,2021).State transition(i.e.,acclimative re-distribution of peripheral antennae between photosystems[PSs]I and II)is one such regulation mechanism that maintains excitation balance between PSl and PSll.

关键词： complexes breakthrough maintain

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A vectorial model for the nonlinear gradient force exerted on metallic Rayleigh nanoparticles

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Chinese Optics Letters 2024年第2期22卷 207-213页

作者：朱政张聿全闵长俊 Aurèle j.LAdam h.Paul Urbach 袁小聪 Research Center for humanoid Sensing Research Institute of Intelligent SensingZhejiang LabHangzhou 311100China Nanophotonics Research Center Institute of Microscale Optoelectronics&State Key Laboratory of Radio Frequency Heterogeneous IntegrationShenzhen UniversityShenzhen 518060China Optics Research Group ImPhys DepartmentFaculty of Applied SciencesDelft University of TechnologyDelft 2628 CJThe Netherlands

Optical tweezers have proved to be a powerful tool with a wide range of *** gradient force plays a vital role in the stable optical trapping of *** scalar method is convenient and effective for analyzing the gradient force in traditional optical ***,when the third-order nonlinear effect of the nano-object is stimulated,the scalar method cannot adequately present the optical response of the metal nanoparticle to the external optical ***,we propose a theoretical model to interpret the nonlinear gradient force using the vector *** combining the optical Kerr effect,the polarizability vector of the metallic nanoparticle is derived.A quantitative analysis is obtained for the gradient force as well as for the optical potential *** vector method yields better agreement with reported experimental *** suggest that this method could lead to a deeper understanding of the physics relevant to nonlinear optical trapping and binding phenomena.

关键词： gradient forces nonlinear effect metallic nanoparticles

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Vastly Synergistic Fe2CuNiS4-Nanoarchitectures Anchored 2D-Nano-Sandwich Derived from Flower-Like-CuFeS2/N-Graphene and Cube-Like-NiFeS2/N-CNTs for Water Oxidation and Nitrophenol Reduction

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ENERGY & ENVIRONMENTAL MATERIALS 2024年第6期7卷 274-289页

作者： Mayakrishnan, Gopiraman Vanaraj, Ramkumar Xiong, junpeng Farooq, Muhammad Ullah, Azeem Zhang, Keqin kim, Seong Cheol kim, Ick Soo Shinshu Univ Inst Fiber Engn IFES Interdisciplinary Cluster Cutting Edge Res ICCER Nano Fus Technol Res GrpDiv Mol & Polymers Tokida 3-15-1 Ueda Nagano 3868567 Japan Yeungnam Univ Sch Chem Engn Gyongsan 38541 South Korea Shinshu Univ Grad Sch Med Sci & Technol Tokida 3-15-1 Ueda Nagano 3868567 Japan Soochow Univ Coll Text & Clothing Engn Natl Engn Lab Modern Silk Suzhou 215123 Peoples R China

Surface area, pore properties, synergistic behavior, homogenous dispersion, and interactions between carbon matrix and metal-nanostructures are the key factors for achieving the better performance of carbon-metal based (electro)catalysts. however, the traditional hydro- or solvothermal preparation of (electro)catalysts, particularly, bi- or tri-metallic nanostructures anchored graphene (G) or carbon nanotubes (CNTs), often pose to poor metal-support interaction, low synergism, and patchy dispersion. At first, bimetallic flower-like-CuFeS2/NG and cube-like-NiFeS2/NCNTs nanocomposites were prepared by solvothermal method. The resultant bimetallic nanocomposites were employed to derive the 2D-nano-sandwiched Fe2CuNiS4/NGCNTs-SW (electro)catalyst by a very simple and green urea-mediated "mix-heat" method. The desired physicochemical properties of Fe2CuNiS4/NGCNTs-SW such as multiple active sites, strong metal-support interaction, homogenous dispersion and enhanced surface area were confirmed by various microscopic and spectroscopic techniques. To the best of our knowledge, this is the first urea-mediated "mix-heat" method for preparing 2D-nano-sandwiched carbon-metal-based (electro)catalysts. The Fe2CuNiS4/NGCNTs-SW was found to be highly effective for alkaline-mediated oxygen evolution reaction at low onset potential of 284.24 mV, and the stable current density of 10 mA cm(-2) in 1.0 m KOh for 10 h. Further, the Fe2CuNiS4/NGCNTs-SW demonstrated excellent catalytic activity in the reduction of 4-nitrophenol with good kapp value of 87.71 x 10(-2) s(-1) and excellent reusability over five cycles. Overall, the developed urea-mediated "mix-heat" method is highly efficient for the preparation of metal-nanoarchitectures anchored 2D-nano-sandwiched (electro)catalysts with high synergism, uniform dispersion and excellent metal-support interaction.

关键词： (electro)catalyst metal-sulfide nanoarchitectures mix-heat N-graphene/N-CNTs synergistic effect urea CELLULOSE NANOFIBER COMPOSITES OXYGEN EVOLUTION TRANSFER hYDROGENATION GRAPhENE CATALYST FACILE ELECTROCATALYST NANOTEChNOLOGY NANOPARTICLES EFFICIENT

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Surface-functionalized hole-selective monolayer for high efficiency single-junction wide-bandgap and monolithic tandem perovskite solar cells

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journal of Energy Chemistry 2024年第1期88卷 317-326,I0008页

作者： Devthade Vidyasagar Yeonghun Yun jae Yu Cho hyemin Lee Kyung Won kim Yong Tae kim Sung Woong Yang jina jung Won Chang Choi Seonu kim Rajendra Kumar Gunasekaran Seok Beom Kang Kwang heo Dong hoe kim jaeyeong heo Sangwook Lee School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Department of Materials Science and Engineering and Optoelectronics Convergence Research CenterChonnam National UniversityGwangju 61186Republic of Korea Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea Department of Nanotechnology and Advanced Materials Engineering Sejong UniversitySeoul 05006Republic of Korea

Carbazole moiety-based 2PACz([2-(9h-carbazol-9-yl)ethyl]phosphonic acid)self-assembled monolayers(SAMs)are excellent hole-selective contact(hSC)materials with abilities to excel the charge-transferdynamics of perovskite solar cells(PSCs).herein,we report a facile but powerful method to functionalize the surface of 2PACz-SAM,by which reproducible,highly stable,high-efficiency wide-bandgap PSCs can be *** 2PACz surface treatment with various donor number solvents improves assembly of 2PACz-SAM and leave residual surface-bound solvent molecules on 2PACz-SAM,which increases perovskite grain size,retards halide segregation,and accelerates hole *** surface functionalization achieves a high power conversion efficiency(PCE)of 17.62%for a single-junction wide-bandgap(~1.77 e V)*** also demonstrate a monolithic all-perovskite tandem solar cell using surfaceengineered hSC,showing high PCE of 24.66%with large open-circuit voltage of 2.008 V and high fillfactor of 81.45%.Our results suggest this simple approach can further improve the tandem device,when coupled with a high-performance narrow-bandgap sub-cell.

关键词： Perovskite solar cells 2PACz Monolithic tandem solar cells Wide bandgap

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Upcycling plastic wastes into value-added products via electrocatalysis and photoelectrocatalysis

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journal of Energy Chemistry 2024年第4期91卷 522-541页

作者： Sungsoon kim Dongjae Kong Xiaolin Zheng jong hyeok Park Department of Chemical&Biomolecular Engineering Yonsei UniversitySeoul 03722Republic of Korea Department of Mechanical Engineering Stanford UniversityStanfordCA 94305USA

Plastic,renowned for its versatility,durability,and cost-effectiveness,is indispensable in modern ***,the annual production of nearly 400 million tons of plastic,coupled with a recycling rate of only 9%,has led to a monumental environmental *** recycling has emerged as a vital response to this crisis,offering sustainable solutions to mitigate its environmental *** these recycling efforts,plastic upcycling has garnered attention,which elevates discarded plastics into higher-value ***,electrocatalytic and photoelectrocatalytic treatments stand at the forefront of advanced plastic *** or photoelectrocatalytic treatments involve chemical reactions that facilitate electron transfer through the electrode/electrolyte interface,driven by electrical or solar energy,*** methods enable precise control of chemical reactions,harnessing potential,current density,or light to yield valuable chemical *** review explores recent progress in plastic upcycling through electrocatalytic and photoelectrocatalytic pathways,offering promising solutions to the plastic waste crisis and advancing sustainability in the plastics industry.

关键词： Plastic upcycling Electrocatalytic reaction Photoelectrocatalytic reaction Value-added product

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