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Plasma spray coating on interconnector toward promoted solid oxide fuel cells and solid oxide electrolysis cells

Frontiers in Energy 2024年第3期18卷 390-398页

作者： junwen CAO Yun ZHEnG Wenqiang ZHAnG Bo YU Institute of nuclear and new Energy Technology(InET) Collaborative Innovation Center of Advanced Nuclear Energy TechnologyTsinghua UniversityBeijing 100084China Department of Chemical Engineering University of WaterlooWaterlooOntario N2L 3G1Canada Institute of new Energy Materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China

Interconnector is a critical component to construct solid oxide cells (SOCs) stack. Oxidation of metallic interconnectors and Cr poisoning caused by oxidation are important factors that lead to long-term performance degradation of SOCs. Coating on the interconnector surface is an important approach to inhibit the oxidation and Cr migration of the interconnector. Herein, (La0.75Sr0.25)0.95MnO3–δ (LSM) and Mn1.5Co1.5O4 (MCO) are used to fabricate the coatings of interconnector. Two advanced thermal spray technology, atmospheric plasma spraying (APS) and low-pressure plasma spray (LPPS), are adopted for the coating preparation. The electrochemical performance, rising and cooling cycle stability, and Cr diffusion inhibition performance of the coatings are tested and evaluated. The result indicates that MCO can generate more uniform and denser coatings than LSM. In addition, MCO coatings prepared by LPPS shows the best electrochemical performance, rising and cooling cycle stability, and Cr diffusion inhibition. The initial area specific resistance (ASR) is 0.0027 Ω·cm2 at 800 °C. After 4 cooling cycle tests, the ASR increases to 0.0032 Ω·cm2 but lower than other samples. Meanwhile, the relative intense of Cr at the interface of SUS430 with MCO coatings fabricated by LPPS is lower than that of MCO fabricated by APS after 4 rising and cooling cycle operations, showing more favorable Cr diffusion inhibition performance.

关键词： interconnector coating plasma spray electrochemical performance Cr diffusion inhibition solid oxide cells(SOCs)

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Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

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Frontiers in Energy 2024年第2期18卷 128-140页

作者： junwen CAO Yikun HU Yun ZHEnG Wenqiang ZHAnG Bo YU Institute of nuclear and new Energy Technology(InET) Collaborative Innovation Center of Advanced Nuclear Energy TechnologyTsinghua UniversityBeijing 100084China Department of Chemical Engineering University of WaterlooWaterlooOntario N2L 3G1Canada Institute of new Energy Materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China

The Haber-Bosch process is the most widely used synthetic ammonia technology at *** its invention,it has provided an important guarantee for global food ***,the traditional Haber-Bosch ammonia synthesis process consumes a lot of energy and causes serious environmental *** the serious pressure of energy and environment,a green,clean,and sustainable ammonia synthesis route is urgently *** synthesis of ammonia is a green and mild new method for preparing ammonia,which can directly convert nitrogen or nitrate into ammonia using electricity driven by solar,wind,or water energy,without greenhouse gas and toxic gas ***,the basic mechanism of the nitrogen reduction reaction(nRR)to ammonia and nitrate reduction reaction(nO_(3)^(-))to ammonia were *** representative approaches and major technologies,such as lithium mediated electrolysis and solid oxide electrolysis cell(SOEC)electrolysis for nRR,high activity catalyst and advanced electrochemical device fabrication for(nO_(3)^(-))RR and electrochemical ammonia synthesis were *** on the above discussion and analysis,the main challenges and development directions for electrochemical ammonia synthesis were further proposed.

关键词： electrochemical ammonia synthesis nitrogen nitrate nitrogen reduction reaction(nRR)to ammonia nitrate reduction reaction(nO_(3)^(-))RR

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Effects of drought on non-structural carbohydrates and C,n,and P stoichiometric characteristics of Pinus yunnanensis seedlings

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Journal of Forestry Research 2024年第1期35卷 90-102页

作者： Zhijuan Zhao Lina Wang Yuanxi Liu Jianli Sun Jiandong Xiao Qiong Dong Lianfang Li Wanjie Zhang Chao Wang junwen Wu College of Forestry Southwest Forestry UniversityKunming 650224YunnanPeople’s Republic of China

To study non-structural carbohydrate character-istics and nutrient utilization strategies of Pinus yunnanen-sis under continuous drought conditions,2-year-old seed-lings were planted in pots with appropriate water,light and moderate and severe drought treatments[(80±5),(65±5),(50±5),and(35±5)%of field water-holding capacity].non-structural carbohydrates,carbon(C),nitrogen(n),and phosphorus(P)concentrations were measured in each plant *** results show that:(1)With increasing drought,non-structural carbohydrates gradually increased in leaves,stems,and coarse roots,while gradually decreased in fine roots;(2)C concentrations of all were relatively stable under different stress *** utilization of each component increased under light and moderate drought conditions,while n and P utilization efficiency of each plant component decreased under severe *** was mainly restricted by n,first decreasing and then increasing with increased drought;(3)There was a correlation between the levels of non-structural carbohydrates and C,n,and P in each *** in n concentration affected the interconversion between soluble sugar and starch,which play a regulatory role in the fluctuation of the concentration of non-structural carbohydrates;and,(4)Plasticity analysis showed that *** seedlings responded to drought mainly by altering starch concentration,the ratio of soluble sugar to starch in leaves and stems,and further by alter-ing n and P utilization ***,these results suggest that the physiological activities of all organs of *** seedlings are restricted under drought and that trade-offs exist between different physiological indicators and *** findings are helpful in understanding non-structural carbohydrate and nutrient adaptation mechanisms under drought in *** seedlings.

关键词： Pinus yunnanensis seedlings Drought non-structural carbohydrates C,n,P stoichiometric characteristics

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Cobalt single-atom catalyst tailored ceramic membrane for selective removal of emerging organic contaminants

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Environmental Science and Ecotechnology 2024年第5期21卷 219-229页

作者： Jiaxuan Yang Jing Zhao Hesong Wang Yatao Liu junwen Ding Tianyi Wang Jinlong Wang Han Zhang Langming Bai Heng Liang State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090PR China Beijing Key Laboratory for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing100083PR China

Water reuse is an effective way to solve the issues of current wastewater increments and water resource ***,a promising method for water reuse,has the characteristics of low energy consumption,easy operation,and high adaptability to coupling with other water treatment ***,emerging organic contaminants(EOCs)in municipal wastewater cannot be effectively intercepted by ultrafiltration,which poses significant challenges to the effluent quality and sustainability of ultrafiltration ***,we develop a cobalt single-atom catalyst-tailored ceramic membrane(Co1-nCnT-CM)in conjunction with an activated peroxymonosulfate(PMS)system,achieving excellent EOCs degradation and anti-fouling *** interfacial reaction mechanism effectively mitigates membrane fouling through a repulsive interaction with natural organic *** generation of singlet oxygen at the Co-n3-C active sites through a catalytic pathway(PMS/PMS*/OH*/O*/OO*/1 O_(2))exhibits selective oxidation of phenols and sulfonamides,achieving>90%removal *** findings elucidate a multi-layered functional architecture within the Co1-nCnT-CM/PMS system,responsible for its superior performance in organic decontamination and membrane maintenance during secondary effluent *** highlights the power of integrating Co1-nCnT-CM/PMS systems in advanced wastewater treatment frameworks,specifically for targeted EOCs removal,heralding a new direction for sustainable water management.

关键词： Single-atom catalytic ceramic membrane Peroxymonosulfate activation Selective oxidation Interfacial response Multi-layer functional zones

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中国特色社会主义政治经济学基本方法论的传承与创新

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经济学动态 2024年第4期 3-11页

作者：黄少安山东大学经济研究院 250100

研究对象统一和规范了所有政治经济学的一般性特征,中国特色社会主义政治经济学也必须符合这个一般性。研究方法、内容、范式和目的决定或赋予不同经济学流派的特色。中国特色社会主义政治经济学的特色有三个维度,在基本方法论维度可能... 详细信息

研究对象统一和规范了所有政治经济学的一般性特征,中国特色社会主义政治经济学也必须符合这个一般性。研究方法、内容、范式和目的决定或赋予不同经济学流派的特色。中国特色社会主义政治经济学的特色有三个维度,在基本方法论维度可能有两个方面的创新或特色:一是发展和完善了的、本质主义与历史主义结合的历史唯物主义;二是有意识地从中华传统的、优秀的文化中寻找相关的、既符合人类合作性又切合中国作为公有制为主体的实际情况的文化元素,提炼成为经济学基本方法论的“主义”。在创建和完善中国特色社会主义政治经济学的过程中,需要处理好几个重要关系:一是处理好“一般”与“特色”的关系;二是处理好积累和传承与创新的关系;三是处理好通用学术语言与学术话语权的关系;四是处理好学理支撑与联系实际和服务现实的关系。

关键词：中国特色社会主义政治经济学一般性与特色基本方法论的传承与创新

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ALS-linked C9orf72 dipeptide repeats inhibit starvation-induced autophagy through modulating BCL2–BECn1 interaction

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Acta Pharmaceutica Sinica B 2024年第5期14卷 2026-2038页

作者： shiqiang Xu Qilian Ma junwen sh.n ningning Li sh.n Sun nana Wang Yang Chen Chunsh.ng Dong Kin Yip Tam Jochen H.M.Prehn Hongfeng Wang Zheng Ying Jiangsu Key Laboratory of neuropsychiatric Diseases and College of Pharmaceutical Sciences Soochow UniversitySuzhou 215123China MOE Key Laboratory of Geriatric Diseases and Immunology College of Pharmaceutical SciencesSuzhou Medical College of Soochow UniversitySuzhou 215123China Jiangsu Province Engineering Research Center of Precision Diagnostics and Therapeutics Development Soochow UniversitySuzhou 215123China Dept.of Physiology&Medical Physics and FUTURE-nEURO Research Centre Royal College of Surgeons in IrelandDublin D02 YN77Ireland Faculty of Health Sciences University of MacaoTaipaMacao 999078China Insititutes of Biology and Medical Science Soochow UniversitySuzhou 215123China

Growing evidences indicate that dysfunction of autophagy contributes to the disease pathogenesis of amyotrophic lateral sclerosis(ALS)and frontotemporal dementia(FTD),two neurodegenerative *** GGGGCC·GGCCCC repeat RnA expansion in chromosome 9 open reading frame 72(C9orf72)is the most genetic cause of both ALS and *** to the previous studies,GGGGCC·GGCCCC repeat undergoes the unconventional repeat-associated non-ATG translation,which produces dipeptide repeat(DPR)*** there is a growing understanding that C9orf72 DPRs have a strong ability to harm neurons and induce C9orf72-linked ALS/FTD,whether these DPRs can affect autophagy remains *** the present study,we find that poly-GR and poly-PR,two arginine-containing DPRs which display the most cytotoxic properties according to the previous studies,strongly inhibit starvation-induced ***,our data indicate that arginine-rich DPRs enhance the interaction between BCL2 and BECn1/Beclin 1 by inhibiting BCL2 phosphorylation,therefore they can impair autophagic clearance of neurodegenerative disease-associated protein aggregates under starvation condition in ***,our study not only highlights the role of C9orf72 DPR in autophagy dysfunction,but also provides novel insight that pharmacological intervention of autophagy using SW063058,a small molecule compound that can disrupt the interaction between BECn1 and BCL2,may reduce C9orf72 DPR-induced neurotoxicity.

关键词： Amyotrophic lateral sclerosis Frontotemporal dementia C9orf72 Autophagy BCL2 BECn1/Beclin 1 Dipeptide repeat neurodegeneration

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High-speed Gan-based laser diode with modulation bandwidth exceeding 5 GHz for 20 Gbps visible light communication

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Photonics Research 2024年第6期12卷 1186-1193页

作者： JUnFEI WAnG JUnHUI HU CHAOWEn GUAn YUQI HOU ZEnGYI XU LEIHAO SUn YUE WAnG YUnInG ZHOU BOOn S.OOI JIAnYAnG shI ZIWEI LI junwen ZHAnG nAn CHI shAOHUA YU CHAO sh.n School of Information Science and Technology Fudan UniversityShanghai 200433China Peng Cheng Laboratory Shenzhen 518000China ZGC Institute of Ubiquitous-X Innovation and Applications Beijing 100876China Photonics Laboratory King Abdullah University of Science and Technology(KAUST)Thuwal 23955-6900Saudi Arabia

Visible light communication(VLC)based on laser diodes demonstrates great potential for high data rate maritime,terrestrial,and aerial wireless data ***,we design and fabricate high-speed blue laser diodes(LDs)grown on c-plane gallium nitride(Gan)*** was achieved through active region design and miniaturization toward a narrow ridge waveguide,short cavity length,and single longitudinal mode Fabry–Perot laser *** fabricated mini-LD has a low threshold current of 31 mA and slope efficiency of 1.02 W/A.A record modulation bandwidth of 5.9 GHz(−3dB)was measured from the *** the developed mini-LD as a transmitter,the VLC link exhibits a high data transmission rate of 20.06 Gbps adopting the bit and power loading discrete multitone(DMT)modulation *** corresponding bit error rate is 0.003,satisfying the forward error correction *** demonstrated Gan-based mini-LD has significantly enhanced data transmission rates,paving the path for energy-efficient VLC systems and integrated photonics in the visible regime.

关键词： communication diode waveguide

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SIZ1-mediated SUMOylation of CPSF100 promotes plant thermomorphogenesis by controlling alternative polyadenylation

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Molecular Plant 2024年第9期17卷 1392-1406页

作者： Zhibo Yu Jun Wang Cheng Zhang Qiuna Zhan Leqian shi Bing Song Danlu Han Jieming Jiang junwen Huang Xiaolin Ou Zhonghui Zhang Jianbin Lai Qingsh.n Quinn Li Chengwei Yang Guangdong Provincial Key Laboratory of Biotechnology for Plant Development School of Life ScienceSouth China Normal UniversityGuangzhou 510631China Key Laboratory of the Ministry of Education for Coastal and Wetland Ecosystems Cllege of the Environment and EcologyXiamen UniversityXiamenFujan 361102China Biomedical Science Division College of Dental MedicineWestern University of Health SciencesPomonaCA 91766USA

Under warm temperatures,plants adjust their morphologies for environmental adaption via precise gene expression ***,the function and regulation of alternative polyadenylation(APA),an important fine-tuning of gene expression,remains unknown in plant *** this study,we found that SUMOylation,a critical post-translational modification,is induced by a long-term treat-ment at warm temperatures via a SUMO ligase SIZ1 in *** of SIZ1 altered the global usage of polyadenylation signals and affected the APA dynamic of thermomorphogenesis-related ***100,a key subunit of the CPSF complex for polyadenylation regulation,is SUMOylated by ***,we demonstrated that SUMOylation is essential for the function of CPSF1oo in genome-wide polyadenylation site choice during *** analyses revealed that the SUMO conjugation on CPSF100 attenuates its interaction with two isoforms of its partner CPSF30,increasing the nuclear accumulation of CPsF1oo for polyadenylation *** summary,our study uncovers a regulatory mechanism of APA via SiZ1-mediated SUMOylation in plant thermomorpho-genesis.

关键词： alternative polyadenylation CPSF100 SiZ1 SUMOylation thermomorphogenesis

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Dynamics of 7Li breakup and its influence on elastic scattering: a study of 7Li + 144Sm system

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Chinese Physics C 2024年第2期48卷 124-134页

作者： A.Morzabayev n.Amangeldi Awad A.Ibraheem D.Soldatkhan G.Yergaliuly B.Mauyey Anuar.A.Orazalievna sh.Hamada L.n.Gumilyov eurasian national university astanakazakhstan Institute of nuclear physics almatykazakhstan Physics department king khalid universityabhasaudi arabia Faculty of science tanta universitytantaegypt

The angular distributions of 7Li+144Sm elastic scattering over the energy range of 21.6–52 MeV are reanalyzed utilizing various interaction *** analysis aims to study the consistency of the implemented potentials in representing the considered data and investigate the cluster nature of the weakly bound 7Li *** will aid in the better understanding the impacts of 7Li breakup on the elastic scattering *** coupling to the breakup channel has a substantial impact on the elastic data and reproduces a repulsive dynamical polarization potential,which drastically diminishes the real potential *** reported impact was simulated by introducing a semi-microscopic repulsive DPP and by implementing the method of continuum discretized coupled *** analysis was also extended to understand the impact of triton transfer on the elastic scattering data.

关键词： phenomenological and semi-microscopic potentials cluster folding dynamic polarization

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Magnetic resonance imaging-guided focused ultrasound thalamotomy launch with remote telemedicine international proctorship

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Chronic Diseases and Translational Medicine 2024年第1期10卷 40-50页

作者： Igor V.Buzaev Rezida M.Galimova Dinara I.nabiullina Sergey n.Illarioshkin naufal sh.Zagidullin shamil M.Safin Department of Surgery Bashkir State Medical UniversityUfaRussia Intelligent neurosurgery Clinic Ltd.International Medical Center V.S.Buzaev memorialUfaRussia Directorate Research Center of NeurologyVolokolamskoye ShosseMoscowRussia

Background: COVID-19 limitations have hindered the implementation of new technologies by preventing proctors from coming to the *** share our first experience of magnetic resonance imaging(MRI)-guided focused ultrasound(MRgFUS)treatment with an international remote online proctorship,and develop and evaluate the methodology of remote MRgFUS ***: This single-center,nonrandomized controlled prospective study included 94 patients:27 with essential tremor(ET)and 67 with tremor-dominant Parkinson's disease(PD).The coming of proctors was impossible,so we arranged for the remote participation of proctors from the United Kingdom,Spain,and Israel.A total of 38 patients(40.4%)received telemedicine-proctored treatment(proctor group)and 56 received their treatment independently(solo group).We used the Clinical Rating Scale for Tremor(CRST)for ET patients and the Unified Parkinson's Disease Rating Scale(UPDRS)Part III for PD ***: In patients with ET,success rates were 81.8%(proctor group)and 100%(solo group)(p=0.22).CRST reduction on the treated side was 71.43%[65.83%;80.56%](proctor group)versus 60.87%[53.99;79.58](solo group)(p=0.19).none of the patients showed worsening of tremors within 1 *** patients with PD,the success rates were 92.6%(proctor group)and 100%(solo group)(p=0.08).The UPDRS Part III improvement was 30.1%(proctor group)versus 39.9%(solo group)(p=0.003).The 1-year recurrence rate was 40%(proctor group)and 17.5%(solo group)(p=0.04).no complications were observed at 6 ***: We developed a feasible and safe methodology for telemedicine remote online-proctored MRgFUS *** significant difference was observed between the solo and developed remote proctor protocols in terms of complication rate,effect,and long-term results;however,UPDRS Part III improvement was better in the PD solo *** study demonstrated that the MRgFUS international proctorship can be performed successfully remotely.

关键词： essential tremor MRgFUS Parkinson's disease proctor telemedicine

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