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Particuology 2024年第2期85卷 252-267页

作者： junpeng Zhang Jingna sun Huagui Huang Zhenge Yuan National Engineering Research Center for Equipment and Technology of Cold Strip Rolling Yanshan UniversityQinhuangdao066004China Xingtai Naknor Technology Co. LtdXingtai054000China

Elucidating the intricate correlation between calendering,structure,and performance is crucial to comprehending the relationship between performance parameters and process steps of lithium-ion batteries(LIBs).Discrete element method(DEM)simulations were adopted in this work to calculate the interparticle force and stress tensor under incremental calendering process conditions,which revealed the effect of the anisotropy of complex contact force network on the anisotropy of heat transfer within porous electrode.The thermal conductivity of electrode was predicted using porosity to characterize the process-structure-performance correlation.The comprehensive influence of contact number and con-tact area between particles and current collector determines the magnitude of interfacial thermal resistance and interfacial heat transfer coefficient.For the first time,this work quantitatively analyzed the structural mechanics and heat transfer mechanism during calendering process of porous electrodes,and the results indicate a promising way to optimize and design battery electrode structures.

关键词： Li-ion battery electrode Structural mechanicsAnisotropy Thermal conductivity Discrete element method

X-ray-activated Bi^(3+)/Pr^(3+)co-doped LiYGeO_4 phosphor with UV and NIR dual-emissive persistent luminescence

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Journal of Rare Earths 2024年第5期42卷 955-961,I0005页

作者： Xianggui Yin Hongyun Zhong Lin Liu junpeng Shi Xia sun Yun Zhang State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou350002China Xiamen Key Laboratory of Rare Earth Photoelectric Functional Materials Xiamen Institute of Rare Earth MaterialsHaixi InstituteChinese Academy of SciencesXiamen361021China Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China

X-ray-activated luminescence materials have broad application prospects in photodynamic therapy of deep tissue.Among them,X-ray-activated persistent luminescence materials(PLMs)exhibiting multiple emission peaks have drawn extensive attention for the ir capacity to achieve a combination of bioimaging and therapeutic functions.Here,we developed a novel PLM,LiYGeO_4:Bi^(3+),Pr^(3+),that simultaneously exhibits UV and NIR dual persistent luminescence(PersL)emissions after irradiation by X-ray.The material can be re peatedly excited by X-ray and emits similar lumine scence intensity every time,which shows good PersL stability.In addition,LiYGeO_4:Bi^(3+),Pr^(3+)exhibits photostimulated PersL properties by stimulation with a red light-emitting diode(LED)or NIR laser after long-term decay.This work provides a new choice of X-ray-excited PLMs with UV and NIR dual emission and the novel phosphor shows promise as a potential candidate for the integration of treatment and diagnosis of deep tumors.

关键词： Co-doping X-ray-activated Dual emissions Persistent luminescence Rare earths

X-ray excited Mn^(2+)-doped persistent luminescence materials with biological window emission for in vivo bioimaging

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Journal of Rare Earths 2024年第1期42卷 28-35,I0001页

作者： Hanrun Zheng Lin Liu Yi’ang Li Rui Rong Liang Song junpeng Shi Jing Teng Xia sun Yun Zhang State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou350002China University of the Chinese Academy of Sciences Beijing100049China Xiamen Hospital of Traditional Chinese Medicine Xiamen361015China Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou350108China

In recent years,persistent luminescence materials(PLMs)excited by X-rays and emitting in biological windows have received extensive attention in the field of high-sensitivity bioimaging.Transition metal Mn^(2+)is an ideal emission center,but few studies focus on Mn^(2+)-doped PLMs with X-ray excitation and biological window emission.Here,we report a Mn^(2+)-doped PLM,LiYGeO_(4):Mn^(2+)(LYGM),with excellent biological window persistent luminescence emission.After excitation by UV,LYGM produces a durable biological window of persistent luminescence emission at 660 nm for up to 20 h.More importantly.LYGM can be repeatedly excited by X-rays,resulting in long-term biological window persistent luminescence emission.In addition,we obtain LYGM around 200 nm in diameter by ball milling and centrifugation and improve its biocompatibility by surface modification to apply it to in vivo imaging in mice.After LYGM are injected into mice through the tail vein,in situ excitation of X-rays can be achieved.After the persistent luminescence decays,LYGM can be re-excited for repeated imaging.Therefore,LYGM shows potential prospects for in vivo deep tissue and long-term bioimaging.

关键词： Persistent luminescence X-ray Biological window In vivo imaging Rare earths

Benzoselenol as an organic electrolyte additive in Li-S battery

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Nano Research 2023年第3期16卷 3814-3822页

作者： junpeng sun Kai Zhang Yongzhu Fu Wei Guo College of Chemistry Zhengzhou UniversityZhengzhou 450001China

Lithium-sulfur(Li-S)battery is one of the promising high-energy battery systems for future use.However,the shuttle effect due to the dissolved lithium polysulfides in ether electrolyte hampers its practical application.Applying electrolyte additives in Li-S battery has been widely acknowledged as an effective way to reduce the shuttle effect and improve cycling efficiency.In this work,benzoselenol(PhSeH)is used as an organic electrolyte additive in Li-S battery.It reacts with elemental sulfur to form phenyl selenosulfide,altering the redox pathway of the cathode with the regeneration of S8 at the end of charge and enabling new redox reactions with high reversibility.The Li-S coin cell with an optimized amount of PhSeH in the electrolyte delivers a high discharge capacity of 1,436 mAh·g^(−1)and a capacity retention of 92.86%in 200 cycles,and exhibits lower discharge overpotential in comparison to the cell with blank electrolyte.The Li-S pouch cell with a low electrolyte/sulfur(E/S)ratio of 4.0μL·mg^(−1)shows a discharge capacity of 1,398 mAh and excellent capacity retention for 20 cycles.

关键词： lithium-sulfur(Li-S)battery benzoselenol electrolyte additive sulfur-selenium bond electrochemical performance

Stable α-CsPbI3 with extremely red emission for expanding the color gamut

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Science China(Information Sciences) 2024年第5期67卷 311-317页

作者： Yong ZHANG Xin WEI Lei GAO Weijie ZHAO Changjiu sun Junli WEI Mingjian YUAN Zhenhua NI junpeng LU Hongwei LIU School of Physics and Key Laboratory of MEMS of the Ministry of Education Southeast University Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Renewable Energy Conversion and Storage Center (RECAST) College of Chemistry Nankai University Jiangsu Key Lab on Opto-Electronic Technology School of Physics and TechnologyNanjing Normal University

The wider color gamut represents the better reproducibility of the real natural colors. Perovskite materials exhibit promising potential in full-color wide-gamut displays because of the wide tunability and high saturability of their photon emission. However, the full-color wide gamut(>100% Rec.2020) has not been constructed due to the lack of the extreme red primary color(～700 nm). Herein, the widest color gamut is realized, whereinα-CsPbI3 is used to generate the extreme red primary color. An in-situ encapsulation approach is advised to stabilizeα-CsPbI3 at room temperature by means of polyvinylpyrrolidone(PVP).Theα-CsPbI3 encapsulated by PVP(denoted as P-CPI) shows highly saturated(FWHM(full width at half maximum) ～28 nm) and extremely(～697 nm) red emission. The green emission is provided by P-CPBr(CsPbBr3 with PVP) which is also synthesized using the universal in-situ encapsulation approach. With the assistance of a commercial Ga N chip, the RGB gamut is extended to the widest(151% NTSC, 113%Rec.2020).

关键词： all-inorganic perovskite wide color gamut LED display carrier recombination

锂离子电池极片辊压异质微结构演化与性能相关性研究进展

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中国有色金属学报 2024年第6期34卷 1809-1829页

作者：张俊鹏孙静娜黄华贵苑振革安徽建筑大学机械与电气工程学院合肥230601 燕山大学国家冷轧板带装备及工艺工程技术研究中心秦皇岛066004 邢台纳科诺尔精轧科技股份有限公司邢台054000

在力争实现“碳达峰、碳中和”的“双碳”战略目标背景下,电池储能技术已成为我国汽车产业转型和经济可持续增长的重要发展方向。极片作为锂离子电池(LIB)的核心部件,决定了电池能量密度和服役安全性,而辊压工序是确保极片达到所需压实... 详细信息

在力争实现“碳达峰、碳中和”的“双碳”战略目标背景下,电池储能技术已成为我国汽车产业转型和经济可持续增长的重要发展方向。极片作为锂离子电池(LIB)的核心部件,决定了电池能量密度和服役安全性,而辊压工序是确保极片达到所需压实密度、提高电池综合性能的关键。然而,由于极片为“涂层-集流体-涂层”的典型层状复合结构,具有异质性特征,其中涂层为多孔可压缩结构,在辊压时涉及活性颗粒间和颗粒-集流体间的相互作用,因此,辊压变形机理极为复杂,厚度控制难度大,对后续性能表现影响显著。本文概述了极片辊压工艺基础理论、基本机理及性能的研究进展,有助于深入理解正负极片辊压-微结构-性能表现之间的相关性,为预测极片正向性能、设计极片反向工艺与微结构、完善辊压工艺设定和提高极片产品质量提供指导。

关键词：电池极片辊压微结构性能工艺建模

Toward an accurate method renaming approach via structural and lexical analyses

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Frontiers of Information Technology & Electronic Engineering 2022年第5期23卷 732-748页

作者： junpeng LUO Jingxuan ZHANG Zhiqiu HUANG Yong XU Chenxing sun College of Computer Science and Technology Nanjing University of Aeronautics and AstronauticsNanjing 211106China Collaborative Innovation Center of Novel Software Technology and Industrialization Nanjing 211106China Tencent Technology(Shenzhen)Company Limited Shenzhen 518054China

Methods in programs must be accurately named to facilitate source code analysis and comprehension.With the evolution of software,method names may be inconsistent with their implemented method bodies,leading to inaccurate or buggy method names.Debugging method names remains an important topic in the literature.Although researchers have proposed several approaches to suggest accurate method names once the method bodies have been modified,two main drawbacks remain to be solved:there is no analysis of method name structure,and the programming context information is not captured efficiently.To resolve these drawbacks and suggest more accurate method names,we propose a novel automated approach based on the analysis of the method name structure and lexical analysis with the programming context information.Our approach first leverages deep feature representation to embed method names and method bodies in vectors.Then,it obtains useful verb-tokens from a large method corpus through structural analysis and noun-tokens from method bodies through lexical analysis.Finally,our approach dynamically combines these tokens to form and recommend high-quality and project-specific method names.Experimental results over 2111 Java testing methods show that the proposed approach can achieve a Hit Ratio,or Hit@5,of 33.62%and outperform the state-of-the-art approach by 14.12%in suggesting accurate method names.We also demonstrate the effectiveness of structural and lexical analyses in our approach.

关键词： Method renaming Code refactor Deep learning Convolutional neural networks

2,000,000 fps 2D and 3D imaging of periodic or reproducible scenes with single-pixel detectors

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Photonics Research 2022年第9期10卷 2157-2164页

作者： WENJIE JIANG YONGKAI YIN junpeng JIAO XIAN ZHAO BAOQING sun School of Information Science and Engineering Shandong UniversityQingdao 266237China Key Laboratory of Laser&Infrared System Ministry of EducationQingdao 266237China Center for Optics Research and Engineering Shandong UniversityQingdao 266237China

Single-pixel imaging(SPI)can capture 2D images of the target with only a nonpixelated detector,showing promising application potential in nonvisible spectral imaging,low-photon imaging,lidar,and other extreme imaging fields.However,the imaging mechanism of traditional SPI makes it difficult to achieve high imaging speed,which is a primary barrier for its widespread application.To address this issue,in this work,we propose and demonstrate a novel high-speed 2D and 3D imaging scheme based on traditional SPI,termed time-resolved single-pixel imaging(TRSPI).Previous SPI works mainly utilize correlation between a stable target and iterative illumination masks to reconstruct a single image.In TRSPI,by further exploiting correlation information between a dynamic scene and every static mask,we can reconstruct a series of time-varying images of the dynamic scene,given the dynamic scene is repetitive or reproducible.Experimentally,we conducted 2D and 3D imaging on a rotating chopper with a speed of 4800 revolutions per minute(rpm),and imaging speeds up to 2,000,000 fps.It is believed that this technology not only opens up a novel application direction for SPI,but also will provide a powerful solution for high-speed imaging.

关键词： SPI utilize scene

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均匀化制度对6014铝合金显微组织的影响

金属热处理 2024年第1期49卷 215-222页

作者：迟蕊李延成孟双徐志远于俊芃张德镇郭丰佳孙宁山东南山铝业股份有限公司国家铝合金压力加工工程技术研究中心山东烟台265700 山东南山铝业股份有限公司有色金属产业研究院山东烟台265700

借助光学显微镜的明暗场像、差示扫描量热法、扫描电镜及透射电镜等手段,研究了不同均匀化制度对6014铝合金的组织、富铁相转变、元素分布和弥散相均匀性的影响。结果表明,6014铝合金铸锭中存在枝晶偏析现象和非平衡共晶组织,合金元素... 详细信息

借助光学显微镜的明暗场像、差示扫描量热法、扫描电镜及透射电镜等手段,研究了不同均匀化制度对6014铝合金的组织、富铁相转变、元素分布和弥散相均匀性的影响。结果表明,6014铝合金铸锭中存在枝晶偏析现象和非平衡共晶组织,合金元素含量波动较大,晶粒为等轴晶。铸锭中的第二相含量明显高于单级和双级均匀化态,由于第二相形态和分布不同,可分为α-AlFeMnSi、β-AlFeSi、Mg_(2)Si和Q-AlCuMgSi相。采用560℃×4 h+540℃×6 h双级均匀化处理制度时,网状枝晶并未全部断裂,延长560℃一级均匀化保温时间至12 h时,较多的β-AlFeSi相转变为α-AlFeMnSi相。采用560℃×19 h单级均匀化处理时,枝晶基本由网状形态转变为链状形态。采用580℃×4 h+540℃×6 h双级均匀化制度时,弥散相α-AlFeMnSi分布较为均匀,延长580℃一级均匀化保温时间至12 h时,组织发生过烧,弥散相尺寸增大且在晶界周围富集。

关键词： 6014铝合金均匀化制度组织弥散相均匀性

台风期间盐沼消波效应的观测研究——以珠江口芒洲湿地为例

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广西科学 2024年第1期31卷 79-86页

作者：孙璐黄盛赵军鹏何薇周水华邓伟陈新平国家海洋局南海环境监测中心广东广州510300 海南南沙珊瑚礁生态系统国家野外科学观测研究站广东广州510300 国家海洋局南海预报中心广东广州510300 自然资源部海洋减灾中心北京100194

滨海盐沼可以减少风暴潮和台风浪的冲击,从而增强海岸抵御台风等自然灾害的能力,减少经济损失,在保护海岸和防灾减灾等方面起到重要作用。本研究利用2020年6月台风“鹦鹉”活动期间珠江口芒洲湿地的现场实测波浪数据来分析其消浪功能,... 详细信息

滨海盐沼可以减少风暴潮和台风浪的冲击,从而增强海岸抵御台风等自然灾害的能力,减少经济损失,在保护海岸和防灾减灾等方面起到重要作用。本研究利用2020年6月台风“鹦鹉”活动期间珠江口芒洲湿地的现场实测波浪数据来分析其消浪功能,以定量研究盐沼植被的消波效应。结果表明,台风“鹦鹉”期间,芒洲湿地测得风暴潮最大增水达0.43 m,漫滩时间大于6 h;实测波浪通过宽度100 m和230 m盐沼植被带的波高衰减率分别为90.5%和97.2%,植被减灾能力为优;根据波高衰减率经验公式的估算结果,波浪经过植被宽度100 m和200 m的波高衰减率分别为94.0%和97.0%,与实测结果基本一致。由于台风“鹦鹉”影响时间短、强度弱,现场测得水位均在1 m以下,而盐沼植被的平均株高约为2 m,植被冠顶未被淹没,因此可将植被看作透空式堤防,其茎叶的摩擦阻尼作用导致波能衰减;并且现场测得有效波高均在0.10 m以下,同时也未发生植被大量倒伏甚至茎秆断裂的情形,因此盐沼植被充分发挥了消波作用。综上,虽然芒洲盐沼面积仅为3.39 km 2,但是其消波效果仍然非常显著。

关键词：芒洲湿地台风“鹦鹉” 盐沼消浪减灾