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Fluoride passivation of ZnO electron transport layers for efcient PbSe colloidal quantum dot photovoltaics

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Frontiers of Optoelectronics 2023年第3期16卷 141-151页

作者： jungang he You Ge Ya Wang Mohan Yuan Hang Xia Xingchen Zhang Xiao Chen Xia Wang Xianchang Zhou Kanghua Li Chao Chen Jiang Tang Hubei Key Laboratory of Plasma Chemistry and Advanced Materials Hubei Engineering Technology Research Center of Optoelectronic and New Energy MaterialsSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205China Wuhan National Laboratory for Optoelectronics(WNLO) School of Optical and Electronic InformationSchool of Integrated CircuitsHuazhong University of Science and TechnologyWuhan 430074China

Lead selenide(PbSe)colloidal quantum dots(CQDs)are suitable for the development of the next-generation of photovoltaics(PVs)because of efcient multiple-exciton generation and strong charge coupling *** date,the reported high-efcient PbSe CQD PVs use spin-coated zinc oxide(ZnO)as the electron transport layer(ETL).However,it is found that the surface defects of ZnO present a difculty in completion of passivation,and this impedes the continuous progress of *** address this disadvantage,fuoride(F)anions are employed for the surface passivation of ZnO through a chemical bath deposition method(CBD).The F-passivated ZnO ETL possesses decreased densities of oxygen vacancy and a favorable band *** from these improvements,PbSe CQD PVs report an efciency of 10.04%,comparatively 9.4%higher than that of devices using sol-gel(SG)ZnO as *** are optimistic that this interface passivation strategy has great potential in the development of solution-processed CQD optoelectronic devices.

关键词： Zinc oxide Surface passivation Band alignment Quantum-dot solar cells

层次性的学案教学法——探索应对“三新”高考及新课标的教法

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基础教育研究 2010年第11期 25-27,29页

作者：何军刚百色高级中学广西百色533000

高考命题的“新情境、新问题、新材料”对师生提出了严峻的挑战。为了摆脱困境，破解“三新”之谜，教师们可谓“八仙过海，各显神通”。时下，新课改及其理念风靡全国，广西的高中课改已是在弦之箭。探索一条既适应当今“三新”高考又... 详细信息

高考命题的“新情境、新问题、新材料”对师生提出了严峻的挑战。为了摆脱困境，破解“三新”之谜，教师们可谓“八仙过海，各显神通”。时下，新课改及其理念风靡全国，广西的高中课改已是在弦之箭。探索一条既适应当今“三新”高考又能与新课标接轨的教学法，意义更为凸显。本文拟就层次性学案教学法作些探讨。

关键词：学案教学法高考命题层次性教法标的新情境新材料新课标

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铁电陶瓷基光子晶体发展现状及其应用

材料导报 2013年第21期27卷 1-6,13页

作者：姜胜林周莹易金桥何俊刚华中科技大学光学与电子信息学院武汉430070

铁电陶瓷基光子晶体在外场激励作用下发生铁电相变,可用于制备带隙可调光子晶体。主要介绍了不同维度铁电陶瓷基光子晶体的常用制备方法,总结了每种方法的特点及代表性的研究成果,阐述了铁电陶瓷基光子晶体的应用,最后提出了铁电陶瓷基... 详细信息

铁电陶瓷基光子晶体在外场激励作用下发生铁电相变,可用于制备带隙可调光子晶体。主要介绍了不同维度铁电陶瓷基光子晶体的常用制备方法,总结了每种方法的特点及代表性的研究成果,阐述了铁电陶瓷基光子晶体的应用,最后提出了铁电陶瓷基光子晶体的发展趋势。

关键词：铁电陶瓷光子晶体可调带隙光子禁带

Reconstructing forest and grassland cover changes in China over the past millennium

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Science China Earth Sciences 2025年第1期68卷 94-110页

作者： Fanneng he Fan YANG Yafei WANG Key Laboratory of Land Surface Pattern and Simulation Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences Key Research Institute of Yellow River Civilization and Sustainable Development Henan University University of Chinese Academy of Sciences

Historical forest and grassland cover changes not only are critical indicators for quantifying ecological and environmental change processes but also serve as fundamental data for long-term climate change simulations and terrestrial ecosystem carbon emission assessments. However, because of limitations in historical data, quantitative estimations and spatially gridded reconstructions of these changes remain challenging, necessitating further methodological exploration. This study focused on China's present-day land area over the past millennium, objectively capturing the characteristics and drivers of forest and grassland cover changes. On this basis, using the forest transition theory and the space-for-time substitution method, we depicted the historical deforestation process as an inverted “S” curve and developed a model to reconstruct historical forest area changes based on the functional relationship between the forest area and population size dynamics. Subsequently, a gridded forest allocation model was established on the basis of deforestation tendencies. For the grassland cover, we implemented regionspecific methods, such as the cropland area deduction method and the habitat constraint method, to quantitatively reconstruct historical changes. Consequently, we obtained provincial forest and grassland area changes over the past millennium and mapped 10-km-resolution gridded data of forest and grassland cover. The results indicated the following.(1) The methods developed using population data as a proxy objectively reproduced the spatiotemporal evolution of forest and grassland cover in China over the past millennium. These feasible methods offer a novel pathway for the quantitative reconstruction of historical forest and grassland cover changes.(2) The data indicated that China's forest area generally decreased over the past millennium, characterized by a “decrease-then-increase” pattern. The forest area experienced three distinct phases: a slow decline(AD 1000

关键词： Land use and land cover change Forest Grassland Quantitative reconstruction Gridded reconstruction China historical period

Recent progress in constructing fluorinated solid-electrolyte interphases for stable lithium metal anodes

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International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 270-291页

作者： Di Zhang Pengfei Lv Wei Qin Xin he Yuanhua he Civil Aircraft Fire Science and Safety Engineering Key Laboratory of Sichuan Province College of Civil Aviation Safety EngineeringCivil Aviation Flight University of ChinaGuanghan 618307China School of Chemical Engineering Sichuan UniversityChengdu 610065China

Lithium metal batteries(LMBs)are emerging as a promising energy storage solution owing to their high energy density and specific ***,the non-uniform plating of lithium and the potential rupture of the solid-electrolyte interphase(SEI)during extended cycling use may result in dendrite growth,which can penetrate the separator and pose significant short-circuit *** a stable SEI is essential for the long-term operation of the ***-rich SEI has garnered significant attention for its ability to effectively passivate electrodes,regulate lithium deposition,and inhibit electrolyte *** the structural components and preparation methods of existing fluorinated SEI is crucial for optimizing lithium metal anode *** paper reviews the research on optimizing LiF passivation interfaces to protect lithium metal *** focuses on four types of compositions in fluorinated SEI that work synergistically to enhance SEI *** instance,combining compounds with LiF can further enhance the mechanical strength and ionic conductivity of the *** metals with LiF significantly improves electrochemical performance at the SEI/anode interface,with a necessary focus on reducing electron tunneling ***,incorporating polymers with LiF offers balanced improvements in interfacial toughness and ionic conductivity,though maintaining structural stability over long cycles remains a critical area for future *** alloys combined with LiF increase surface energy and lithium affinity,challenges such as dendrite growth and volume expansion *** summary,this paper emphasizes the crucial role of interfacial structures in LMBs and offers comprehensive guidance for future design and development efforts in battery technology.

关键词： LiF lithium metal anodes solid-electrolyte interphase interface cycling stability

Breaking new ground in photocatalysis: lutetium texaphyrin as a trigger for pyroptosis through biomolecular photoredox reactions

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Science China Chemistry 2025年第1期68卷 1-2页

作者： Qihang Ding Mengrong he Meijia Gu Department of Chemistry Korea University Department of Ultrasound Medicine Union Hospital Tongji Medical College Huazhong University of Science and Technology Key Laboratory of Combinatorial Biosynthesis and Drug Discovery (MOE) School of Pharmaceutical Sciences Wuhan University

Malignant neoplasms consistently pose a significant threat to global public health [1,2]. In recent years, immunotherapy has demonstrated remarkable clinical success; however, its efficacy is limited by the scarcity of immune cell infiltration within tumor microenvironments. Cell pyroptosis, a gasdermin-mediated process characterized by cellular swelling,rupture, and the release of intracellular contents such as IL-1β, IL-18, ATP, HMGB1, plays a crucial role in this context[3,4].

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磁控溅射法制备Ag掺杂p型ZnO薄膜的研究

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半导体技术 2010年第3期35卷 225-227,232页

作者：王莉何俊刚陈环刘志宇傅刚广州大学物理电子工程学院广州510006

采用磁控溅射法在石英玻璃基片上生长ZnO和ZnO:Ag薄膜。借助于SEM、XRD、霍尔测试、透射谱测试等方法,分析了O2气氛下退火温度对薄膜结构和电学性能的影响。霍尔测试结果表明,Ag掺杂ZnO薄膜经过600℃的O2气氛中热处理转变为p型电导。薄... 详细信息

采用磁控溅射法在石英玻璃基片上生长ZnO和ZnO:Ag薄膜。借助于SEM、XRD、霍尔测试、透射谱测试等方法,分析了O2气氛下退火温度对薄膜结构和电学性能的影响。霍尔测试结果表明,Ag掺杂ZnO薄膜经过600℃的O2气氛中热处理转变为p型电导。薄膜的XRD测试表明晶粒大小随退火温度升高而增大,所有薄膜样品只出现(002)衍射峰,呈现c轴取向生长。薄膜对可见光的透过率大于83%,其吸收限为378nm。

关键词：氧化锌薄膜银掺杂 p型半导体磁控溅射霍尔测试

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ZnO薄膜紫外光敏特性及晶界势垒的研究

电子元件与材料 2009年第12期28卷 36-38页

作者：何俊刚陈环王莉刘志宇傅刚广州大学物理与电子工程学院广东广州510006

以二水合醋酸锌为原料,采用sol-gel法在石英衬底上制备了ZnO薄膜。用AFM观察表面形貌,通过测量真空条件下不同温度热处理后薄膜的I-V特性,拟合计算晶界势垒高度。研究了热处理温度对ZnO薄膜性能的影响。结果表明:经650℃热处理制备的Zn... 详细信息

以二水合醋酸锌为原料,采用sol-gel法在石英衬底上制备了ZnO薄膜。用AFM观察表面形貌,通过测量真空条件下不同温度热处理后薄膜的I-V特性,拟合计算晶界势垒高度。研究了热处理温度对ZnO薄膜性能的影响。结果表明:经650℃热处理制备的ZnO薄膜样品具有较佳性能,结构均匀致密,粒径分布为20～32nm。在10V偏压和1.24×10–3W/cm2光强下,紫外光灵敏度为43.95;无光照条件下晶界势垒高度为0.079eV。紫外光照使晶界势垒高度下降为0.011eV,薄膜的紫外光灵敏度与势垒高度的相对变化密切相关。

关键词： ZnO薄膜热处理温度紫外光灵敏度晶界势垒

Dip2a regulates stress susceptibility in the basolateral amygdala

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Neural Regeneration Research 2025年第6期20卷 1735-1748页

作者： Jing Li Zixuan he Weitai Chai Meng Tian Huali Yu Xiaoxiao he Xiaojuan Zhu Key Laboratory of Molecular Epigenetics Ministry of Education Institute of Genetics and CytologyNortheast Normal UniversityChangchunJilin ProvinceChina

Dysregulation of neurotransmitter metabolism in the central nervous system contributes to mood disorders such as depression, anxiety, and post–traumatic stress disorder. Monoamines and amino acids are important types of neurotransmitters. Our previous results have shown that disco-interacting protein 2 homolog A(Dip2a) knockout mice exhibit brain development disorders and abnormal amino acid metabolism in serum. This suggests that DIP2A is involved in the metabolism of amino acid–associated neurotransmitters. Therefore, we performed targeted neurotransmitter metabolomics analysis and found that Dip2a deficiency caused abnormal metabolism of tryptophan and thyroxine in the basolateral amygdala and medial prefrontal cortex. In addition, acute restraint stress induced a decrease in 5-hydroxytryptamine in the basolateral amygdala. Additionally, Dip2a was abundantly expressed in excitatory neurons of the basolateral amygdala, and deletion of Dip2a in these neurons resulted in hopelessness-like behavior in the tail suspension test. Altogether, these findings demonstrate that DIP2A in the basolateral amygdala may be involved in the regulation of stress susceptibility. This provides critical evidence implicating a role of DIP2A in affective disorders.

关键词： 5-hydroxytryptamine acute restraint stress basolateral amygdala CaMKII neurons DIP2A metabolomics neurotransmitters principal component analysis stress susceptibility tryptophan