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Nano-silica modified lightweight and high-toughness carbon fiber/phenolic ablator with excellent thermal insulation and ablation performance

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Defence Technology（防务技术） 2024年第1期31卷 192-199页

作者： Wenjie Xu Wenda Song Xianfeng Jia Cheng Ma jitong Wang Wenming Qiao Licheng Ling State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China School of Chemical Engineering and Materials Changzhou Institute of TechnologyChangzhou 213032China Key Laboratory of Specially Functional Polymeric Materials and Related Technology(Ministry of Education) School of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China

Lightweight and high-toughness carbon fiber/phenolic ablator(CFPA)is required as the Thermal Protection System(TPS)material of aerospace vehicles for next-generation space *** improve the ablative properties,silica sol with good particle size distribution prepared using tetramethoxysilane(TMOS)was blended with natural rubber latex and deposited onto carbon fiber felt,which was then integrated with phenolic aerogel matrix,introducing nano-silica into the framework of *** modified CFPA with a low density of 0.28—0.31.g/cm3exhibits strain-in-fracture as high as 31.2%and thermal conductivity as low as 0.054 W/(m·K).Furthermore,a trace amount of nano-silica could effectively protect CFPA from erosion of oxidizing atmosphere in different high-temperature *** oxyacetylene ablation test of 3000°C for 20 s shows a mass ablation rate of 0.0225 g/s,a linear ablation rate of 0.209 mm/s for the modified CFPA,which are 9.64%and 24.82%lower than the unmodified ***,the long-time butane ablation test of 1.00°C for 200 s shows an insignificant recession with mass and linear ablation rate of 0.079 g/s and 0.039 mm/s,1..84%and 1..33%lower than the unmodified ***,the fixed thermocouple in the test also demonstrates a good thermal insulation performance with a low peak back-face temperature of 207.7°C,1..25%lower than the unmodified ***,the nano-silica modified CFPA with excellent overall performance presents promising prospects in high-temperature aerospace applications.

关键词： Nano-silica Carbonfiber Phenolic aerogel Insulation Ablation

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Electron delocalization-enhanced sulfur reduction kinetics on an MXene-derived heterostructured electrocatalyst

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Nano Research 2024年第8期17卷 7153-7162页

作者： Yunmeng Li Yinze Zuo Xiang Li Yongzheng Zhang Cheng Ma Xiaomin Cheng Jian Wang jitong Wang Hongzhen Lin Licheng Ling State Key Laboratory of Chemical Engineering Key Laboratory of Specially Functional Polymeric Materials and Related Technology(Ministry of Education)East China University of Science and TechnologyShanghai 200237China Institute of New Energy Materials and Engineering College of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China Key Laboratory of Specially Functional Polymeric Materials and Related Technology(Ministry of Education) School of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China i-Lab&CAS Key Laboratory of Nanophotonic Materials and Device Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of SciencesSuzhou 215123China Helmholtz Institute Ulm(HIU) D89081 UlmGermany

Lithium-sulfur(Li-S)batteries mainly rely on the reversible electrochemical reaction of between lithium ions(Li^(+))and sulfur species to achieve energy storage and conversion,therefore,increasing the number of free Li^(+)and improving the Li^(+)diffusion kinetics will effectively enhance the cell ***,Mo-based MXene heterostructure(MoS_(2)@Mo_(2)C)was developed by partial vulcanization of Mo_(2)C MXene,in which the introduction of similar valence S into Mo-based MXene(Mo_(2)C)can create an electron delocalization *** theoretical simulations and electrochemical characterisation,it is demonstrated that the MoS_(2)@Mo_(2)C heterojunction can effectively promote ion desolvation,increase the amount of free Li^(+),and accelerate Li^(+)transport for more efficient polysulfide *** addition,the MoS_(2)@Mo_(2)C material is also capable of accelerating the oxidation and reduction of polysulfides through its sufficient defects and vacancies to further enhance the catalytic ***,the Li-S battery with the designed MoS_(2)@Mo_(2)C electrocatalyst performed for 500 cycles at 1.C and still maintained the ideal capacity(664.7 mAh·g^(−1.),and excellent rate performance(567.6 mAh·g^(−1.at 5 C).Under the extreme conditions of high loading,the cell maintained an excellent capacity of 775.6 mAh·g^(−1.after 1.0 *** also retained 838.4 mAh·g^(−1.for 70 cycles at a low temperature of 0℃,and demonstrated a low decay rate(0.063%).These results indicate that the delocalized electrons effectively accelerate the catalytic conversion of lithium polysulfide,which is more practical for enhancing the behaviour of Li-S batteries.

关键词： delocalized electron lithium sulfur batteries MXene-based heterostructures catalytic desolvation multi-catalytic sites

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Utilizing dual-pathway energy transfer in upconversion nanoconjugates for reinforced photodynamic therapy

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Nano Research 2024年第4期17卷 2941-2948页

作者： Ruohao Zhang Yu Lu Yifei Zhou Kehong Lv Xinyu Fu jitong Gong Shuang Yao Xiaozhen Wang Jing Feng Hongjie Zhang State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China College of Chemistry Jilin UniversityChangchun 130012China Department of Breast Surgery General Surgery Centerthe First Hospital of Jilin UniversityChangchun 130021China Department of Chemistry Tsinghua UniversityBeijing 100084China

Enhancing the therapeutic effect of existing treatments or developing new non-invasive treatments are important measures to achieve high-efficiency treatment of malignant *** therapy(PDT)is an emerging treatment modality,and the key for achieving high-efficiency PDT is to select light with strong tissue penetration depth and enhance the generation of reactive oxygen species(ROS).Although the upconversion nanoparticles(UCNPs)modified with the photosensitizers could achieve PDT with strong penetration depth under near-infrared light irradiation,the ROS generated by traditional single-pathway PDT is still ***,we developed a novel nanoconjugate(UCNP-Ce6/AIEgen)for dual-pathway reinforced PDT,in which the UCNPs were co-modified with chlorin e6(Ce6)and luminogen with aggregation-induced emission(AIEgen).Due to the presence of AIEgen,UCNP-Ce6/AIEgen could avoid aggregation-caused luminescence quenching in biological water environments and convert upconversion luminescence(UCL)of UCNPs to Ce6-activatable ***,under the irradiation of 808 nm laser,UCNP-Ce6/AIEgen can not only undergo direct lanthanide-triplet energy transfer to activate Ce6,but also convert the UCL of UCNPs to the light that can activate Ce6 through Fӧrster resonance energy transfer to generate more ROS,thus promoting tumor cell *** work broadens the applications of nanoconjugates of lanthanide-based inorganic materials and organic dyes,and provides a conception for reinforced PDT of tumors.

关键词： upconversion nanoparticle aggregation-induced emission direct lanthanide-triplet energy transfer Förster resonance energy transfer photodynamic therapy

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Genetic mechanisms of high-quality tight siliciclastic reservoirs:A case study from the Upper Triassic Xujiahe Formation in the Yuanba area,Sichuan Basin,China

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Energy Geoscience 2024年第3期5卷 151-162页

作者： Ai Wang Junlong Liu Zhongqun Liu Kaihua Xiao Yanqing Huang Lingxiao Fan jitong Li Petroleum Exploration and Production Research Institute SINOPECBeijing100083China

This study analyzed the petrological characteristics,diagenesis,pore types,and physical properties of the tight coarse-grained siliciclastic sequences in the third member of the Upper Triassic Xujiahe Formation(also referred to as the Xu-3 Member)in the western Yuanba area in the northeastern Sichuan Basin,China,based on the results of 242.61.m-long core description,292 thin-section observations,scanning electron microscopy(SEM),and 292 physical property *** types and genetic mechanisms of high-quality tight coarse-grained siliciclastic reservoirs in this member was determined *** research objective is to guide the exploration and development of the tight coarse-grained siliciclastic sequences in the Xu-3 *** results of this study are as *** types of high-quality reservoirs are developed in the coarse-grained siliciclastic sequences of the Xu-3 Member,namely the fractured fine-grained sandy conglomerate type and porous medium-grained calcarenaceous sandstone *** energy in the sedimentary environment is the key factor controlling the formation of high-quality *** high-quality reservoirs are developed mainly in the transitional zone with moderately high hydrodynamic energy between delta-plain braided channels and delta-front subaqueous distributary *** dolomitic debris(gravel)content is the main factor affecting the reservoirs’physical *** micritic algal debris and sandy debris in the dolomitic debris(or gravels)tend to recrystallize during burial,forming intercrystalline pores *** the medium-grained calcarenaceous sandstones,intercrystalline pores in the dolomitic debris are formed at the early diagenetic stage,and a pore system consisting of structural fractures connecting intergranular pores,intergranular dissolution pores,and kaolinite intergranular micropores is developed at the late stage of *** formation of intercrystalline pores in dolomite gravels and gravel-edge f

关键词： Tight siliciclastic rock High-quality reservoir Genetic mechanism Xujiahe Formation Northeast Sichuan

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Integration of HiBiT into enteroviruses:A universal tool for advancing enterovirus virology research

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Virologica Sinica 2024年第3期39卷 422-433页

作者： Rui Yu Xiaohong Li Peng Zhang Minghao Xu jitong Zhao Jingjing Yan Chenli Qiu Jiayi Shu Shuo Zhang Miaomiao Kang Xiaoyan Zhang Jianqing Xu Shuye Zhang School of Medicine Shanghai UniversityShanghai200444China Clinical Center for Biotherapy Zhongshan HospitalFudan UniversityShanghai200433China Guangzhou Institutes of Biomedicine and Health The Chinese Academy of SciencesGuangzhou510530China Institutes of Biomedical Sciences Fudan UniversityShanghai200032China Shanghai Geriatric Medical Center Shanghai201104China Clinical Center for Biotherapy Zhongshan Hospital/Zhongshan Hospital(Xiamen)Fudan University361015China Shanghai Public Health Clinical Center Fudan UniversityShanghai201508China

The utilization of enteroviruses engineered with reporter genes serves as a valuable tool for advancing our understanding of enterovirus biology and its applications,enabling the development of effective therapeutic and preventive *** this study,our initial attempts to introduce a NanoLuc luciferase(NLuc)reporter gene into recombinant enteroviruses were unsuccessful in rescuing viable *** hypothesized that the size of the inserted tag might be a determining factor in the rescue of the ***,we inserted the 1.-amino-acid HiBiT tag into the genomes of enterovirus A71.EV-A71.,coxsackievirus A1.(CVA1.),coxsackievirus A7(CVA7),coxsackievirus A1.(CVA1.),namely EV-A71.HiBiT,CVA1.-HiBiT,CVA1.-HiBiT,CVA7-HiBiT,and observed that the HiBiT-tagged viruses exhibited remarkably high rescue ***,the HiBiT-tagged enteroviruses displayed comparable characteristics to the wild-type viruses.A direct comparison between CVA1.-NLuc and CVA1.-HiBiT recombinant viruses revealed that the tiny HiBiT insertion had minimal impact on virus infectivity and replication ***,these HiBiT-tagged enteroviruses demonstrated high genetic stability in different cell lines over multiple *** addition,the HiBiT-tagged viruses were successfully tested in antiviral drug assays,and the sensitivity of the viruses to drugs was not affected by the HiBiT ***,our findings provide definitive evidence that the integration of HiBiT into enteroviruses presents a universal,convenient,and invaluable method for advancing research in the realm of enterovirus ***,HiBiT-tagged enteroviruses exhibit great potential for diverse applications,including the development of antivirals and the elucidation of viral infection mechanisms.

关键词： Enterovirus Infectious clones Reporter genes Luciferase Drug screening

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Effects of flue gas desulfurization gypsum and clover planting on qualities of soil and winter jujube in coastal saline-alkali orchard of north China

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Soil Ecology Letters 2024年第1期6卷 141-152页

作者： Qi Shao Xuejing Xia Guihua Li Hui Li jitong Lin Yanhong Lou Quangang Yang Hui Wang Zhongchen Yang Hong Pan Yuping Zhuge National Engineering Research Centerfor Efficient Utilization of Soil and Fertilizer Resources College of Resources and EnvironmentShandong Agricultural UniversityTai'an271018China Tai'an City Management Comprehensive Service Center Tai'an 271021China

Flue gas desulfurization gypsum and clover planting alleviated the soil salinization *** pH and total phosphorus affected the bacterial *** phosphorus affected the fungal *** gas desulfurization gypsum and clover planting improved jujube *** coastal area of Shandong Province,characterized by coastal saline tidal soil,is one of the main production areas of winter jujube in ***,the low soil fertility and poor soil structure in jujube orchard restricted the development of the jujube *** objectives of this study were to 1.evaluate the effect of application of flue gas desulfurization(FGD)gypsum and clover planting on soil quality improvement and soil microbial community structure of jujube orchard;2)investigate the effects of two measures on the nutrition and quality of winter *** results showed that FGD gypsum reduced the soil total salt content by 65.6%,and clover planting increased the soil organic matter content by 30.7%,which effectively alleviated the soil salinization stress and improved the soil *** pH and total phosphorus(TP)were the main determinants influencing bacterial community composition,and TP was the dominant factor of the fungal community composition in the saline-alkali ***,FGD gypsum addition and clover planting significantly increased the sugar degree and Vc content of winter jujube,thus improved jujube quality,and further contributed to the ecological sustainable development of winter jujube industry.

关键词： saline-alkali soils winter jujube bacterial community fungal community fue gas desulfurization gypsum clover planting

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Converting intercalation-type cathode in spent lithium-ion batteries into conversion-type cathode

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Nano Research 2024年第5期17卷 4602-4609页

作者： Dingding Zhu Yong Su Jingzhao Chen Xiangze Ou Xuedong Zhang Wen Xie Yuyan Zhou Yunna Guo Qiushi Dai Peng Jia jitong Yan Lin Geng Baiyu Guo Liqiang Zhang Yongfu Tang Qiao Huang Jianyu Huang School of Materials Science and Engineering Xiangtan UniversityXiangtan 411105China Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066000China

The widespread applications of lithium-ion batteries(LIBs)generate tons of spent ***,recycling LIBs is of paramount importance in protecting the environment and saving the *** commercialized LIBs mostly adopt layered oxides such as LiCoO_(2)(LCO)or LiNi_(x)Co_(y)Mn_(1.x-y)O_(2)(NMC)as the cathode *** the intercalation-type spent oxides into conversion-type cathodes(such as metal fluorides(MFs))offers a valid recycling strategy and provides substantially improved energy densities for ***,two typical Co-based cathodes,LCO and LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2)(NMC622),in spent LIBs were successfully converted to CoF_(2) and(Ni_(x)Co_(y)Mn_(z))F_(2) cathodes by a reduction and fluorination *** as converted CoF_(2) and(Ni_(x)Co_(y)Mn_(z))F_(2) delivered cell energy densities of 650 and 700 Wh/kg,*** atomic-level electron microscopy revealed that the used LCO and NMC622 were converted to highly phase pure Co metal and Ni_(0.6)Co_(0.2)Mn_(0.2) alloys in the used graphite-assisted reduction roasting,simultaneously producing the important product of Li_(2)CO_(3) using only environment friendly *** study provided a versatile strategy to convert the intercalation-type Co-based cathode in the spent LIBs into conversion-type MFs cathodes,which offers a new avenue to recycle the spent LIBs and substantially increase the energy densities of next generation LIBs.

关键词： spent lithium-ion batteries recycling energy densities conversion-type cathode

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产教融合背景下社会工作专业实践教学模式探索——以社区工作课程实习为例

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创新创业理论研究与实践 2024年第9期7卷 115-118页

作者：王吉彤苏州科技大学

新时期，我国地方普通高校社会工作专业创新型、应用型人才培养的目标定位，要求必须深化产教融合教育理念，以推动专业实践教学模式重构。当前，社会工作专业实践教学中专业教育与专业服务存在脱节。基于此，该文以苏州某大学社会工作... 详细信息

新时期，我国地方普通高校社会工作专业创新型、应用型人才培养的目标定位，要求必须深化产教融合教育理念，以推动专业实践教学模式重构。当前，社会工作专业实践教学中专业教育与专业服务存在脱节。基于此，该文以苏州某大学社会工作专业社区工作课程实习为例，从产教融合教育理念、课程目标设置、实践教学模式、实践学习成果评价4个方面分析社会工作专业产教融合模式构建路径。最后，结合社会工作专业人才培养目标定位和社区工作课程实习产教融合模式构建经验，提出加快推进社会工作专业产教融合实践教学模式构建的对策建议，以期达到社会工作专业应用型创新人才培养的目的。

关键词：社会工作专业产教融合实践教学应用型创新人才人才培养

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日本服务型老年公寓入住者的入住理由及位置选择分析——基于岐阜县、爱知县和东京都入住老人的调研数据

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西部人居环境学刊 2024年第1期39卷 75-80页

作者：王吉彤铃木博志苏州科技大学社会发展与公共管理学院日本名城大学理工学部

通过对日本岐阜县、爱知县、东京都三个区域的服务型老年公寓的入住老人进行问卷调研,解析老人的入住理由和服务型老年公寓位置选择模式,提出合理规划建设服务型老年公寓的策略建议。结果显示老人在选择服务型老年公寓时,重视离自己及... 详细信息

通过对日本岐阜县、爱知县、东京都三个区域的服务型老年公寓的入住老人进行问卷调研,解析老人的入住理由和服务型老年公寓位置选择模式,提出合理规划建设服务型老年公寓的策略建议。结果显示老人在选择服务型老年公寓时,重视离自己及子女居住地近的要素,并在实际入住时,呈现相同趋势。城市化水平不同的区域,入住老人的护理等级,入住理由和服务型老年公寓位置选择模式呈现差异性。根据区域特征差异,分别提出相应规划建设策略。在我国老龄化程度日益严峻的社会背景之下,探讨日本服务型老年公寓的规划建设策略,从中汲取经验,对完善我国老年公寓规划建设,实现老年人居住环境高质量发展具有重要的启示意义。

关键词：服务型老年公寓选址老人居住地子女居住地区域差异规划策略

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基于邻域向量主成分分析图像增强的旁瓣弱光信号检测方法

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中国激光 2024年第6期51卷 109-123页

作者：王拯洲王力段亚轩李刚魏际同中国科学院西安光学精密机械研究所先进光学仪器研究室陕西西安710119

针对基于旁瓣光束衍射反演的强激光远场焦斑测量无法提取旁瓣图像更外围最小可测信号的问题,笔者提出了基于邻域向量主成分分析(NVPCA)图像增强的旁瓣弱光信号区域波峰参数检测方法。采取的主要优化措施为:首先,将旁瓣图像中的每个像素... 详细信息

针对基于旁瓣光束衍射反演的强激光远场焦斑测量无法提取旁瓣图像更外围最小可测信号的问题,笔者提出了基于邻域向量主成分分析(NVPCA)图像增强的旁瓣弱光信号区域波峰参数检测方法。采取的主要优化措施为:首先,将旁瓣图像中的每个像素和它的8邻域像素看作一个列向量,构建一个9维数据立方体,选择主成分分析变换后的第1.数据为NVPCA图像;其次,通过角度变换转化检测对象,检测所有方向上一维旁瓣曲线的各个波峰参数,获得旁瓣弱光信号区域能量的量化分布;然后,搜索每个旁瓣波峰在所有方向上的极大值位置点,连接对应位置点生成每个旁瓣波峰的极大值圆环,计算各极大值圆环的灰度均值;最后,选择大于局域对比度方法(LCM)目标分离阈值且最小的极大值圆环的灰度均值作为整个旁瓣光束的最小可测信号。实验结果表明,采用基于NVPCA图像增强的旁瓣弱光信号检测方法能够从旁瓣图像的第5波峰环分离和提取最小可测信号,动态范围比值提升至原来的1.528倍,各旁瓣波峰参数满足精度要求,为未来大型激光装置强激光远场的精确测量奠定了基础。

关键词：远场测量邻域向量主成分分析旁瓣光束衍射反演角度变换旁瓣波峰参数检测

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