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Laser assisted phase transformation of carbon-based transition metal oxide electrode for high-performance supercapacitor application

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Science China Chemistry 2025年

作者： Mingzhen Xiu Jianghong Zhang yu Lu Xun Cao Kang Huang Siyu Zhu Bowei Zhang yu Liang Chunwang zhao Junsheng Wu Yizhong Huang School of Materials Science and Engineering Nanyang Technological University Energy Research Institute Interdisciplinary Graduate Programme Nanyang Technological University Institute of Sustainability for Chemicals Energy and Environment Agency for Science Technology and ResearchSingapore Institute of Advanced Materials and Technology University of Science and Technology Beijing School of Materials Science and Technology Shenyang University of Chemical Technology School of Materials Science and Hydrogen Energy Foshan University

Transitional metal oxides have a wide range of applications due to their superior *** enhanced performance of metal oxide relies on their desirable oxidation states,which is challenging to achieve and requires complex *** study demonstrates a facile strategy enabling rapid phase transformation of transition metal *** approach involves synthesis of a tetragonal Mn3O4/carbon cloth composite using the liquid plasma discharge deposition （LPDD） technique,followed by laser irradiation with the presence of ethylene glycol under an N2gas *** resulting face-centered cubic MnO/carbon cloth electrode exhibits an excellent capacitance of 1,125 F g-1at 2 A g-1,with remarkable capacitance retention of 95%after10,000 *** approach can be extended to other transition metals including Co,Cu,Cr,Fe,Ni,and *** simulations reveal the significance of ethylene glycol and the underlying mechanism associated with the phase transformation of transition metal *** present study offers a powerful technique for the phase transformation of transition metal oxide which can guide the development of new electrode materials with enhanced electrochemical properties for high-performance energy storage applications.

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动态回弹模量滞回曲线形态参数研究

公路交通科技 2017年第10期34卷 6-12页

作者：刘靖宇刘朝晖王旭东黄优长沙理工大学交通运输工程学院湖南长沙410004 交通运输部公路科学研究院北京100000

动态回弹模量的滞回曲线是动态加载作用下混合料的荷载和变形曲线,可反映沥青混合料内部应力应变状态随荷载和温度等的演变规律。基于黏弹理论可确定滞回曲线的3种形态参数:长轴斜率k、椭圆离心率e、滞回曲线面积S,分别表征沥青混合料... 详细信息

动态回弹模量的滞回曲线是动态加载作用下混合料的荷载和变形曲线,可反映沥青混合料内部应力应变状态随荷载和温度等的演变规律。基于黏弹理论可确定滞回曲线的3种形态参数:长轴斜率k、椭圆离心率e、滞回曲线面积S,分别表征沥青混合料的动态回弹模量、黏滞性及耗散能。并由此进行不同温度、荷载的动态回弹模量试验,结果发现:随温度升高SBS与70#沥青混合料形态参数存在较大差异,且其变化曲线均在15~20℃出现明显拐点;随荷载级位变大k,S呈一定的变化规律但e值基本不变。表明:(1)相对级配而言,沥青品质对混合料性能影响更大,而黏滞性与荷载大小无关;(2)在15~20℃间沥青混合料的力学性能差异较大,对温度的敏感性较高;(3)不同的滞回曲线形态参数取值体现了沥青混合料间的性能差异,可以采用3种形态参数对沥青混合料的黏滞性、耐疲劳性等基本力学性能进行评价。最后,基于试验曲线的变化规律,建立了回弹模量的应力依赖性模型,可反映不同应力水平条件下沥青混合料的响应行为,且预测结果较接近真实状态;基于Miner线性损伤准则,推导了变荷载累积耗散能预估方程,并建立了基于能量耗散理论的疲劳方程,可以通过动态模量试验得到的形态参数S对混合料疲劳性能进行预测。

关键词：道路工程形态参数动态模量试验滞回曲线长轴斜率离心率耗散能

Double [5]carbohelicene: facile synthesis, chiroptical properties,isomerization study, and lasing application

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Science China Chemistry 2025年第1期68卷 233-240页

作者： Peipei Liu Yantong Li Meng-Xiang Wu Hao Kang Xiao-Li zhao Lin Xu Linlin Liu Xiaodong Li Junfeng Fang Zhiwei Fang Ya Cheng Hai-Bo Yang Huakang yu Xueliang Shi State Key Laboratory of Petroleum Molecular & Process Engineering Shanghai Key Laboratory of Green Chemistry and Chemical ProcessesSchool of Chemistry and Molecular Engineering East China Normal University School of Physics and Optoelectronics South China University of Technology Institute of Polymer Optoelectronic Materials & Devices State Key Laboratory of Luminescent Materials & Devices South China University of Technology School of Physics and Electronic Science Engineering Research Center of Nanophotonics & Advanced Instrument Ministry of EducationEast China Normal University State Key Laboratory of Precision Spectroscopy School of Physics and Electronic Science East China Normal University

Double carbohelicenes have attracted considerable attention due to their aesthetic structures, distinct π-conjugation extension, inherent chirality, and intriguing optical and electronic properties. Herein, the concise de novo synthesis of a new double[5]carbohelicene 1 together with its chiroptical properties, isomerization process and lasing application is presented. 1 was synthesized by a simple protocol involving the formation of a 6,6′-bipentacene as the key intermediate. It is worth noting that1 existed as two diastereomers 1-PP/MM and 1-PM, which were successfully isolated and unambiguously confirmed by Xray crystallography. The optical resolution of the racemic 1-PP/MM was successfully achieved by chiral-phase highperformance liquid chromatography（HPLC）, and 1-PP and 1-MM were characterized by circular dichroism. Interestingly, it was found that 1-PP/MM could be completely isomerized to 1-PM upon heating, and the detailed thermodynamics and kinetics of the isomerization process were systematically investigated. 1-PM exhibited deep-red luminescence with emission maximum at 723 nm and fluorescence quantum yield as high as 32.95%. Consequently, we can showcase the lasing application of 1-PM by doping with epoxy resin to assemble a bottle microlaser spontaneously, which the lasing wavelength is 796.6 nm at a threshold of 0.8 m J cm-2. We believe that our studies, including the facile synthesis methodology, detailed isomerization studies, and lasing application, will shed some light on the design and synthesis of novel carbohelical systems with more functions.

关键词： double carbohelicene optical resolution organic laser isomerization X-ray diffraction

Dissecting the cell microenvironment of ovarian endometrioma through single-cell RNA sequencing

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Science China Life Sciences 2025年第1期68卷 116-129页

作者： Jiangpeng Wu Siyu Xia Wenting Ye Yan Sun jing Cai Fubing yu Haiping Wen Xiuwei Yi Taikang Li Mingwei Chen Jiayun Chen Ge Song Chuanbin Yang Yali Song Jigang Wang Department of Reproductive Medicine Dongguan Maternal and Child Health Care Hospital Department of Urology and Shenzhen Clinical Research Centre for GeriatricsShenzhen People's HospitalSouthern University of Science and Technology State Key Laboratory for Quality Ensurance and Sustainable Use of Dao-di Herbs Artemisinin Research Centerand Institute of Chinese Materia MedicaChina Academy of Chinese Medical Sciences Reproductive Medicine Center Foshan Women and Children Hospital State Key Laboratory of Antiviral Drugs School of PharmacyHenan University

Ovarian endometrioma（OE）, also known as “chocolate cysts,” is a cystic mass that develops in the ovaries due to endometriosis and is a common gynecological condition characterized by the growth of endometrial tissue outside the uterus, leading to symptoms such as dysmenorrhea, pelvic pain, and infertility. However, the precise molecular and cellular mechanisms driving this pathophysiology remain largely unknown, posing challenges for diagnosis and treatment. Here, we employed integrated single-cell transcriptomic profiling of over 52,000 individual cells from endometrial tissues of OE patients and healthy donors and identified twelve major cell populations. We identified notable alterations in cell type-specific proportions and molecular signatures associated with OE. Notably, the activation of IGFBP5+macrophages with pro-inflammatory properties, NK cell exhaustion, and aberrant proliferation of IQCG+and KLF2+epithelium are key features and may be the potential mechanisms underlying the pathogenesis of OE. Collectively, our data contribute to a better understanding of OE at the single cell level and may pave the way for the development of novel therapeutic strategies.

关键词： ovary high-throughput sequencing transcriptomics gene expression analysis ligand-receptor analysis

单片机牵引电磁铁参数测试系统中的多路显示器

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计算机技术与发展 1992年第5期14卷 34-36页

作者：贾景云赵可萍天津纺织工学院自动化系天津300160

本文主要介绍单片机在牵引电磁铁多数测试实验中如何实现多路显示,阐述了多路显示器遇到的一些特殊问题.

关键词：多路显示器牵引电磁铁操作频率极限温升

Experimental demonstration of 220-GHz terahertz signals wireless transmission over 4.6 km

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Science China(Information Sciences) 2025年第1期68卷 386-388页

作者： Yi WEI Jianjun yu Mingxu WANG Xiongwei YANG Qiutong ZHANG jingwen TAN Bing ZHANG Ying WU Yang HAN Peng TIAN Wen ZHOU Kaihui WANG Feng zhao State Key Laboratory of ASIC and System Key Laboratory for Information Science of Electromagnetic Waves (MoE)School of Information Science and Technology Fudan University School of Electronic Engineering Xi'an University of Posts and Telecommunications

The advancement of terahertz (THz) communication technology drives the evolution of wireless communication systems,offering novel pathways and technical means for the development of future 6G communication *** wireless communication systems are often constrained by bandwidth limitations of electronic devices in high frequency ***,THz communication technology leverages the characteristics of electromagnetic waves to transcend these limitations,enabling communication athigher frequencies and wider bandwidths.

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Experimental demonstration of D-band signals wireless transmission over 30 km

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Science China Technological Sciences 2025年

作者： Yi WEI Xiongwei YANG Jianjun yu Xianming zhao Mingxu WANG jingwen TAN Weiping LI Feng zhao Chengzhen BIAN Hansong MA Qinyi ZHANG Qiutong ZHANG Bing ZHANG Wen ZHOU Kaihui WANG Sicong XU Jianguo yu State Key Laboratory of ASIC and System Key Laboratory for Information Science of Electromagnetic Waves (MoE)and School of Information Science and Technology Fudan University Harbin Institute of Technology School of Automation Xi'an University of Posts and Telecommunications School of Electronic Engineering Beijing University of Posts and Telecommunications

Due to the rise of innovative technologies like artificial intelligence(AI),the Internet of Things(IoT), and telemedicine, the demand for internet traffic is rapidly increasing. In order to achieve ultra-high-speed wireless communication, many researchers are directing their efforts towards the Dband. The D-band, spanning the frequency band 110–170 GHz, has abundant spectrum resources and license-free characteristics [1,2].

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某医学专科学校毕业生就业情况调查分析

中华医学教育杂志 2011年第6期31卷 828-831页

作者：喻静昭胡昌军怀化医学高等专科学校临床医学系学生工作办公室 418000 医学检验系预防医学教研室

目的分析某医学专科学校毕业生就业现状，找出存在问题及其影响因素，以指导就业工作。方法采取自行设计问卷调查表，对某医学专科学校2007届343名毕业生进行为期6个月的追踪调查，采用SPSS10．0对调查结果进行统计分析。结果343名毕业... 详细信息

目的分析某医学专科学校毕业生就业现状，找出存在问题及其影响因素，以指导就业工作。方法采取自行设计问卷调查表，对某医学专科学校2007届343名毕业生进行为期6个月的追踪调查，采用SPSS10．0对调查结果进行统计分析。结果343名毕业生就业率达到97．1％。其中，52．6％的毕业生在国家事业单位工作，7．5％的毕业生在国有企业工作，33．4％的毕业生在私营企业工作，6．5％的毕业生无工作单位；68．5％的毕业生从事医学专业技术工作，58．8％的临床医学专业毕业生从事医学专业技术工作；60．0％的毕业生通过亲朋好友介绍找到工作，23．2％的毕业生自己找到工作，16．8％的毕业生通过学校提供的信息找到工作；90．3％的毕业生3个月内工作未变，9．7％的毕业生3个月内换岗。结论学校在学生就业方面发挥作用不大，临床医学专业学生从事医学专业技术工作比例较低，国家应当多方面采取有效措施，加强学校在学生就业方面的引导。

关键词：医学专科生就业调查分析

Printing perovskite and graphene parallel structure-based optical-mechanical sensors for human-machine interaction

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Science China Technological Sciences 2025年

作者： Sisi CHEN Jiemin ZHANG Nan CHENG Wenbo LI jing LIU Hongfei XIE Jie ZHANG yueying CHENG Xiaotong zhao Meng SU Yanlin SONG Key Laboratory of Green Printing CAS Research/Education Center for Excellence in Molecular Sciences Institute of ChemistryChinese Academy of Sciences (ICCAS) University of Chinese Academy of Sciences Weiyang College Tsinghua University Department of Cardiovascular Surgery First Medical Center PLA General Hospital AECC Beijing Institute of Aeronautical Materials Beijing Institute of Graphene Technology Beijing Engineering Research Centre of Graphene Application School of Integrated Circuit & Beijing National Research Center for Information Science and Technology (BNRist) Tsinghua University

Surgical robots are designed to provide enhanced precision and dexterity compared to manual surgical procedures,which mainly rely on multimodal sensing technologies for the surgeon to seamlessly operate the robotic arms and *** with single-mode sensors, optical and mechanical bi-modal sensors provide improved precision, enhanced safety,and robustness of human-machine interaction systems. Here, the template-guided and pneumatic printing technologies are combined to construct perovskite and graphene parallel structures with both optical and mechanical sensing capabilities. The printed uniformly crystallized perovskite microstructure exhibits fast and sensitive photoelectric response characteristics,enabling shadow recognition functionality. The combination of graphene and elastic rubber endows the great printability to prepare parallel structures near the perovskite arrays for force sensing capabilities. Thus, the printed perovskite and graphene structures possess non-contact optical sensing capabilities to detect hand position by recognizing shadows between the hand and the sensor, as well as contact mechanical sensing capabilities to detect touch force applied by the hand. It provides a synergistic platform for real-time and multidimensional feedback to improve human-machine interaction.

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