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Spontaneous Orientation Polarization of Anisotropic Equivalent Dipoles Harnessed by Entropy Engineering for Ultra‑Thin Electromagnetic Wave Absorber

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Nano-Micro Letters 2025年第1期17卷 424-438页

作者： Honghan Wang Xinyu Xiao Shangru Zhai Chuang Xue Guangping Zheng Deqing Zhang Renchao che Junye cheng Liaoning Key Lab of Lignocellulose chemistry and BioMaterials Liaoning Collaborative Innovation Center for Lignocellulosic BiorefinerySchool of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034People’s Republic of China School of Life Science and Biotechnology Dalian University of TechnologyDalian 116024People’s Republic of China Department of Mechanical Engineering Hong Kong Polytechnic UniversityHung HomKowloonHong Kong 999077People’s Republic of China School of Materials Science and Engineering Qiqihar UniversityQiqihar 161006People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Department of Materials Science Shenzhen MSU-BIT UniversityShenzhen 517182People’s Republic of China

The synthesis of carbon supporter/nanoscale high-entropy alloys(HEAs)electromagnetic response composites by carbothermal shock method has been identified as an advanced strategy for the collaborative competition engineering of conductive/dielectric *** migration modes within HEAs as manipulated by the electronegativity,valence electron configurations and molar proportions of constituent elements determine the steady state and efficiency of equivalent ***,enlightened by skin-like effect,a reformative carbothermal shock method using carbonized cellulose paper(CCP)as carbon supporter is used to preserve the oxygencontaining functional groups(O·)of carbonized cellulose fibers(CCF).Nucleation of HEAs and construction of emblematic shell-core CCF/HEAs heterointerfaces are inextricably linked to carbon metabolism induced by O·.Meanwhile,the electron migration mode of switchable electronrich sites promotes the orientation polarization of anisotropic equivalent *** virtue of the reinforcement strategy,CCP/HEAs composite prepared by 35%molar ratio of Mn element(CCP/HEAs-Mn_(2.15))achieves efficient electromagnetic wave(EMW)absorption of−51.35 dB at an ultra-thin thickness of 1.03 *** mechanisms of the resulting dielectric properties of HEAs-based EMW absorbing materials are elucidated by combining theoretical calculations with experimental characterizations,which provide theoretical bases and feasible strategies for the simulation and practical application of electromagnetic functional devices(e.g.,ultra-wideband bandpass filter).

关键词： High-entropy alloys Carbothermal shock Switchable electron migration modes Emblematic shell-core heterointerfaces Ultra-thin thickness

“Zero‑Strain” NiNb_(2)O_(6) Fibers for All‑Climate Lithium Storage

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Nano-Micro Letters 2025年第1期17卷 348-360页

作者： Yan Zhao Qiang Yuan Liting Yang Guisheng Liang Yifeng cheng Limin Wu Chunfu Lin Renchao che College of Physics Donghua UniversityShanghai 201620People’s Republic of China School of Materials Science and Engineering Institute of Materials for Energy and EnvironmentQingdao UniversityQingdao 266071People’s Republic of China Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative MaterialsAcademy for Engineering&TechnologyFudan UniversityShanghai 200438People’s Republic of China Zhejiang Laboratory Hangzhou 311100People’s Republic of China Inner Mongolia University Hohhot 010021People’s Republic of China

Niobates are promising all-climate Li^(+)-storage anode material due to their fast charge transport,large specific capacities,and resistance to electrolyte ***,their moderate unit-cellvolume expansion(generally 5%–10%)during Li^(+)storage causes unsatisfactory long-term ***,“zero-strain”NiNb_(2)O_(6) fibers are explored as a new anode material with comprehensively good electrochemical *** Li^(+)storage,the expansion of electrochemical inactive NiO_(6) octahedra almost fully offsets the shrinkage of active NbO_(6) octahedra through reversible O *** superior volume-accommodation capability of the NiO_(6) layers guarantees the“zero-strain”behavior of NiNb_(2)O_(6) in a broad temperature range(0.53%//0.51%//0.74%at 25//−10//60℃),leading to the excellent cyclability of the NiNb_(2)O_(6) fibers(92.8%//99.2%//91.1%capacity retention after 1000//2000//1000 cycles at 10C and 25//−10//60℃).This NiNb_(2)O_(6) material further exhibits a large reversible capacity(300//184//318 mAh g−1 at 0.1C and 25//−10//60℃)and outstanding rate performance(10 to 0.5C capacity percentage of 64.3%//50.0%//65.4%at 25//−10//60℃).Therefore,the NiNb_(2)O_(6) fibers are especially suitable for large-capacity,fast-charging,long-life,and all-climate lithium-ion batteries.

关键词： NiNb_(2)O_(6)porous fiber “Zero-strain”mechanism Electrochemical property Harsh-temperature operation Operando characterization

Influence of geological factors on coal permeability in the Sihe coal mine

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International Journal of Coal Science & Technology 2022年第1期9卷 58-70页

作者： Guangui Zou Qianhua Zhang Suping Peng Jiasheng She Deliang teng Chaochao jin Yuyan che State Key Laboratory of Coal Resources and Safe Mining BeijingChina College of Geoscience and Surveying Engineering China University of Mining&TechnologyBeijingChina

Permeability of coal reservoirs influence the extraction of coal gas from coal *** coal samples were collected at an anticline and a syncline of the No.3 coal seam in the Sihe coal ***,permeability,pore size,vitrinite reflectance,and liquid nitrogen adsorption of the samples were *** curvatures at the sample locations,and the distance between the sampling locations and the nearest faults were calculated based on seismic *** influences of the evaluated parameters on permeability were *** factors that influence permeability of the No.3 coal seam were extracted using principal component analysis(PCA).Based on the porosity–permeability model derived from the Archie formula and classic Kozeny–Carman equation,we deduced that the permeability of coal increased with an increase in *** an increase in average vitrinite reflectance,permeability decreases first and then *** results showed that coal permeability was regulated by three key components representing three *** first component included pore size,depth,and pore complexity accounting for 52.59%of the variability indicating that it was the most important in controlling *** second component included specific surface area,structural curvature,and porosity,and the third component comprised of specific surface area,porosity,and average vitrinite ***,pore diameter and complexity had significant effects on coal *** results show that researchers and stakeholders must consider the interactions among multiple factors rather than single factors to understand the influences on permeability to facilitate efficient utilization of coalbed methane resources.

关键词： Coal mine Permeability Geological factors Principal component analysis

Designing Electronic Structures of Multiscale Helical Converters for Tailored Ultrabroad Electromagnetic Absorption

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Nano-Micro Letters 2025年第1期17卷 439-455页

作者： Zhaobo Feng Chongbo Liu Xin Li Guangsheng Luo Naixin Zhai Ruizhe Hu jing Lin jinbin Peng Yuhui Peng Renchao che Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle School of Environmental and Chemical EngineeringNanchang Hangkong UniversityNanchang 330063People’s Republic of China School of Physics and Materials Nanchang UniversityNanchang 330031People’s Republic of China Key Laboratory of Nondestructive Testing Ministry of EducationNanchang Hangkong UniversityNanchang 330063People’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsAcademy for Engineering and TechnologyFudan UniversityShanghai 200438People’s Republic of China

Atomic-scale doping strategies and structure design play pivotal roles in tailoring the electronic structure and physicochemical property of electromagnetic wave absorption(EMWA)***,the relationship between configuration and electromagnetic(EM)loss mechanism has remained ***,drawing inspiration from the DNA transcription process,we report the successful synthesis of novel in situ Mn/N co-doped helical carbon nanotubes with ultrabroad EMWA *** calculation and EM simulation confirm that the orbital coupling and spin polarization of the Mn–N4–C configuration,along with cross polarization generated by the helical structure,endow the helical converters with enhanced EM *** a result,HMC-8 demonstrates outstanding EMWA performance,achieving a minimum reflection loss of−63.13 dB at an ultralow thickness of 1.29 *** precise tuning of the graphite domain size,HMC-7 achieves an effective absorption bandwidth(EAB)of 6.08 GHz at 2.02 mm ***,constructing macroscale gradient metamaterials enables an ultrabroadband EAB of 12.16 GHz at a thickness of only 5.00 mm,with the maximum radar cross section reduction value reaching 36.4 dB *** innovative approach not only advances the understanding of metal–nonmetal co-doping but also realizes broadband EMWA,thus contributing to the development of EMWA mechanisms and applications.

关键词： Metal-nonmetal co-doping 3d-2p orbital coupling Spin polarization Helical structure Broadband EM wave absorption

Characteristics of long period microtremor and validation of microtremor array measurements in inland areas of China

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Journal of Mountain Science 2016年第11期13卷 1910-1922页

作者： che Ai-lan ZHANG teng-yu FENG Shao-kong School of Naval Architecture Ocean and Civil Engineering Shanghai Jiaotong University 800 Dongchuan-Road Shanghai 200240 China

To study the characteristics of long period microtremor and applicability of microtremor survey,we have made microtremor observations using long period seismometers of the China's mainland from coastal cities like Shanghai and Tianjin through Beijing,Xi'an,to the far inland cities of Lanzhou and *** observation shows that the level of power spectrum of long period microtremors reduced rapidly from the coast to the inland ***,the energy of long period microtremors in Beijing,Xi'an,Lanzhou and Tianshui area are only approximately ten-thousandth to thousandth of that in *** at the complexity of the underground structure in the far inland,a series of underground structure models with different distributions were assessed using three-dimensional,dynamic finite element method(FEM) *** results were used to evaluate microtremor survey methods and their limitations with regard to aggregate variability and thickness ***-wave reflections between layers with the change of underground structure distribution occurred,which have significant effect on the performance of the different field *** over a broad spectrum from which velocity-depth profiles were produced via inversion *** the thickness nor the shear waveVelocity V of the subsurface layer inversion results appeared over a large evaluation with increasing slope *** particular,when the angle of the model reached 45°,it could not be accurately evaluated using one-dimensional inversion ***,the array microtremor survey(AMS) was carried out in Shanghai City,*** AMS techniques do not have the layer sensitivity or accuracy(velocity and layer thickness) of borehole techniques,the obtained shear wave velocity structure is especially useful for earthquake disaster prevention and seismic analysis.

关键词： Long period microtremor Array Microtremor survey Power spectrum Inversion S-wave velocity structure

3D trajectory inversion of an adjacent well using scattered P-wave

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Petroleum Science 2023年第2期20卷 857-865页

作者： Lu cheng Xiao-Hua che Wen-Xiao Qiao teng Zhao State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing102249China Key Laboratory of Earth Prospecting and Information Technology Beijing102249China

In oil and gas exploitation,cluster well technology can significantly reduce costs and improve *** effective adjacent well detection method can greatly reduce the risk of collision between adjacent *** study proposes a method to invert the 3D trajectory of an adjacent well using a scattered P-wave obtained by borehole azimuthal acoustic reflection *** obtaining the scattered P-wave from the raw data of the target well using the wave field separation technology,the waveform data in an imaging profile can be obtained by the downhole acoustic directional reception *** imaging technology is then used to obtain the image of the formation in the imaging ***,by analyzing the images of the formation in the imaging profile of the different azimuths,the well spacing and azimuth of the target well can be ***,the 3D trajectory of the target well can be obtained by solving the inversion *** method was validated by processing the field data from a deviated well in a deep *** comparison of the inversion and actual trajectories of the target well demonstrated that the maximum deviation of the inversion trajectory is 0.9 m in the north-south direction,0.78 m in the east-west direction,1.45 m in the well spacing,and 2.48°in the *** field data inversion result demonstrated that the method can effectively use the azimuth reflection acoustic data to invert the 3D trajectory of an adjacent well,which indicates that the borehole azimuthal acoustic reflection imaging technology has great potential within the context of adjacent well detection.

关键词： Acoustic imaging Acoustic reflection logging Directional reception Adjacent well

Crystal Structure of a Nickel(II) Complex with Asymmetric _L-Histidine Ligand

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Chinese Journal of Structural chemistry 2006年第9期25卷 1047-1050页

作者： jin Yi che Yun-Xia ZHENG Ji-Min Department of chemistry Nankai University Tianjin 300071 China

A novel nickel（Ⅱ） complex with L-histidine has been synthesized and solved by single-crystal X-ray diffraction analysis at physiological pH. The title complex （C7H16NiN4O6S, Mr = 343.01） crystallizes in monoclinic, space group P21 with a = 7.2194（7）, b = 7.5968（7）, c = 12.2797（11） A, β = 93.3110（10）°, V = 672.35（11） A^3, Z = 2, Dc= 1.694 g/cm^3, F（000） = 356, μ（MoKα） = 1.626 mm^-1, T = 293（2） K, the final R = 0.0184 and wR = 0.0426 for 2207 observed reflections with 1 〉 2σ（I）. The complex provides insights into a possible structural arrangement between nickel （Ⅱ） and L-histidine which may be physiologically important and abundantly present in biological systems.

关键词： crystal structure synthesis L-histidine nickel physiological pH

Monitoring the frozen duration of Qinghai Lake using satellite passive microwave remote sensing low frequency data

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Chinese Science Bulletin 2009年第13期54卷 2294-2299页

作者： che Tao LI Xin jin Rui Cold and Arid Regions Environment and Engineering Research Institute Chinese Academy of Sciences Lanzhou 710000 China

The Qinghai Lake is the largest inland lake in *** significant difference of dielectric properties between water and ice suggests that a simple method of monitoring the Qinghai lake freeze-up and break-up dates using satellite passive microwave remote sensing data could be *** freeze-up and break-up dates from the Qinghai Lake hydrological station and the MODIS L1B reflectance data were used to validate the passive microwave remote sensing *** validation shows that passive microwave remote sensing data can accurately monitor the lake *** uncertainty comes mainly from the revisit frequency of satellite *** data from 1978 to 2006 show that lake ice duration is reduced by about 14―15 *** freeze-up dates are about 4 days later and break-up dates about 10 days *** regression analyses show that,at the 0.05 significance level,the correlations are 0.83,0.66 and 0.89 between monthly mean air temperature(MMAT) and lake ice duration days,freeze-up dates,break-up dates,***,inter-annual variations of the Qinghai Lake ice duration days can significantly reflect the regional climate variation.

关键词：被动微波遥感遥感数据冻结卫星期限监测 MODIS数据低频

Dendrite Spacing Selection during Directional Solidification of Pivalic Acid-Ethanol System

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Journal of Materials Science & Technology 2008年第3期24卷 340-342页

作者： Myung-jin Suk Young-Min Park Youn-che Kim Department of Materials and-Metallurgical Engineering Kangwon National University

Unidirectional solidification of pivalic acid （PVA）-ethanol （Eth） mixture was performed to examine whether an allowable range of primary dendrite spacing definitely exists at a given growth velocity and how the range is history-dependent. PVA-0.59 wt pct Eth was unidirectionally solidified in the range of growth velocity 0.5-64 μm/s at the temperature gradient of 2.3 K/ram. Sequential change in growth velocity was imposed to determine the upper and lower limits for the allowable range of stable spacing. An allowable range of the steady state primary spacing was observed at a given growth velocity, and the extent of the range seems to be dependent on the degree to which step-increase or step-decrease in growth velocity is accomplished. As the degree of sequential change in growth velocity increases, the history-dependence of the selection for the primary dendrite spacing tends to disappear.

关键词： Dendrite spacing History-dependent Spacing selection Pivalic acid-ethanol