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AIEgens-lightened Functional Polymers: Synthesis, Properties and Applications

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Chinese Journal of Polymer Science 2019年第4期37卷 302-326,I0005页

作者： Shi-Yuan Zhou Hai-Bo Wan Feng Zhou Pei-Yang Gu Qing-Feng Xu jian-mei lu College of Chemistry Chemical Engineering and Materials ScienceCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow University

Recently, polymers with aggregation-induced emission(AIE) effects have attracted significant attention due to their broad applications in luminescence sensors, stimuli responsive materials, electroluminescence devices, etc. In this review, we summarize recent advances concerning AIE polymers. Four types of AIE polymers including end-functionalized polymers, side-chain polymers, main-chain polymers, and other polymers according to the location of AIEgens, are described. Their synthetic preparation, optical property, AIE effects, and applications are also illustrated in this review.

关键词： Aggregation-induced emission Functional polymers Synthetic method Application

N,O Co-Doping Enhanced Adsorption of Chloramphenicol for Highly Efficient and Robust Electrocatalytic Hydrodechlorination

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Chinese Journal of Chemistry 2024年第20期42卷 2445-2452页

作者： Xue-Feng Cheng Qiang Cao Qing Liu Hao-Yu Zhang Qing-Feng Xu jian-mei lu College of Chemistry Chemical Engineering and Materials ScienceCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhouJiangsu 215123China

Electrocatalysis technology can effectively promote the hydrodechlorination of chloramphenicol(CAP)to reduce the ***,there are still some challenges such as low degradation rate and poor ***,we prepared porous N,O co-doped carbon supported Pd nanoparticles composites(Pd NPs/NO-C)for electrocatalytic degradation of *** doping of N and O not only effectively enhanced the interaction between substrate and CAP,promoting the mass transfer process,but also enhanced the anchoring effect on Pd nanoparticles,avoiding the occurrence of *** prepared composites achieved removal efficiency of CAP over 99%within 1 h,and the rate constant was as high as 6.72 h^(–1),outperforming previous reported ***,Pd NPs/NO-C composites showed a wide range of pH tolerance,excellent ion interference resistance and long-term *** work unravels the importance of mass transfer processes in solution to electrocatalytic hydrodechlorination and provides new research ideas for catalysts design.

关键词： Chloramphenicol Hydrodechlorination Electrocatalysis N,O co-doped carbon Mass transfer Supported catalysts Nanoparticles Low-dimensionalmaterials

Graphene from microwave-initiated upcycling of waste polyethylene for electrocatalytic reduction of chloramphenicol

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Chinese Chemical Letters 2024年第4期35卷 187-192页

作者： Qiang Cao Xue-Feng Cheng Jia Wang Chang Zhou Liu-Jun Yang Guan Wang Dong-Yun Chen Jing-Hui He jian-mei lu College of Chemistry Chemical Engineering and Materials ScienceCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215123China

Waste polyolefin plastics, accounting for 50% of all plastic waste, represent a tremendously unexploited carbon source. Efficiently upcycling polyolefin waste into value-added carbon materials for waste water treatment avoiding using noble metals is challenging but economically and environmentally sustainable. In this work, MAX-Ti_(3)AlC_(2) supported Fe selectively catalyzes polyolefin into few-layered graphene in 5 min under microwave treatment. Graphene and MAX supported Fe(Fe@MLC) can completely(99.9%)degrade chloramphenicol(CAP) within 60 min, retain robust after 10 cycles and work efficiently at a wide p H range(3.87–13.03), avoiding the usage of noble metal. Moreover, the electrochemical active surface area(ECSA) of Fe@MLC is 2.7 times higher than that of commercial Pt/C. This work provides a cheap and efficient catalyst that promotes deconstruction of plastic wastes and indirectly degrades antibiotics thereby realizes the treatment of waste water with waste plastic.

关键词： Microwave Ti_(3)AlC_(2) Electrochemistry Dechlorination Chloramphenicol

One-dimensional π-d conjugated coordination polymers: synthesis and their improved memory performance

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Science China Chemistry 2019年第6期62卷 753-760页

作者： Xue-Feng Cheng Jie Li Xiang Hou Jin Zhou Jing-Hui He Hua Li Qing-Feng Xu Na-Jun Li Dong-Yun Chen jian-mei lu College of Chemistry Chemical Engineering and Materials Science Soochow University Shanghai Institute of Measurement and Testing Technology

Multilevel resistance random access memories(RRAMs) are intensively studied due to their potential applications in high density information storage. However, the low ternary device yields and high threshold voltages based on current materials cannot meet the requirement for applications. Improvement via material innovation remains desirable and challenging. Herein,five one-dimensional conjugated coordination polymers were synthesized via the reaction between metal ions(Zn^(2+), Cu^(2+), Ni^(2+),Pt^(2+) and Pd^(2+)) and 2,5-diaminobenzene-1,4-dithiol(DABDT) and fabricated into RRAM devices. The as-fabricated ternary memories have relatively low threshold voltages(V_(th1):-1 to-1.4 V, V_(th2):-1.8 to-2.2 V). Their ternary device yields were improved from 24% to 56%. The first and the second resistance switches are interpreted by the space charge limited current(SCLC) and grain boundary depletion limited current(GBLC) modes, respectively. The Pd-DABDT, which is of planar structure,smaller band gap and better crystallinity than others, shows the best performance among these five polymers. Our work paves a simple and efficient way to optimize the performance of ternary RRAM devices employing one-dimensional hybrid materials.

关键词： one-dimensional coordination polymer resistive random access memory ternary device yield low threshold voltages d-π conjugation

Description of two new species of Hemiphyllodactylus(Reptilia: Gekkonidae) from karst landscapes in Yunnan, China, highlights complex conservation needs

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Zoological Research 2022年第5期43卷 767-786页

作者： Ade Prasetyo Agung Ada Chornelia L.Lee Grismer Jesse L.Grismer Evan S.H.Quah jian-mei lu Kyle W.Tomlinson Alice C.Hughes Landscape Ecology Group Center for Integrative ConservationXishuangbanna Tropical Botanical GardenChinese Academy of SciencesMenglunMenglaYunnan 666303China University of Chinese Academy of Sciences Beijing 101408China Herpetology Laboratory Department of BiologyLa Sierra UniversityRiversideCalifornia 92515USA Institute for Tropical Biology and Conservation Universiti Malaysia SabahJalan UMSKota KinabaluSabah 88400Malaysia Lee Kong Chian Natural History Museum National University of SingaporeSingapore 117377Singapore Community Ecology and Conservation Group Center for Integrative ConservationXishuangbanna Tropical Botanical GardenChinese Academy of SciencesMenglunMenglaYunnan 666303China School of Biological Sciences University of Hong KongPokfulamHong Kong SARChina

Karst habitats are hotspots of diversity and endemism. Their naturally fragmented distributions across broad geographic landscapes have led to the complex array of smaller evolutionary ecosystems that present unique challenges from a conservation *** assessments of karst habitats have revealed that these ecosystems contain an almost unparalleled level of endemism, and many site-restricted species remain undescribed, thus posing considerable challenges for effective conservation *** rock-dwelling species, such as geckos, may be particularly prone to such isolation. In this paper, we discuss one such genus, i.e.,Hemiphyllodactylus, and explore its diversity across karst landforms in Yunnan Province, southwestern China. Based on morphological and genetic data, we describe two new species of Hemiphyllodactylus from karst habitats in Simao District and Yanshan County. A phylogenetic tree for Hemiphyllodactylus was constructed using 1?039 base pairs(bp) of the mitochondrial NADH dehydrogenase subunit 2 gene(ND2). The Simao and Yanshan specimens can be distinguished from all other congeners within their respective subclades based on uncorrected genetic pairwise distances greater than 6.3% and 4.3%respectively, as well as significant morphological differences. The discovery and description of these two new species brings the total number of described Hemiphyllodactylus species in China to 14and indicates many more undescribed species from unsurveyed karst regions await *** findings suggest that karst ecosystems in Yunnan support a higher diversity of Hemiphyllodactylus than previously *** study also highlights the importance of karst ecosystems as refugia for sitespecific endemic species and the need for heightened conservation efforts.

关键词： Discovery Endemism Geckos Reptiles South China

Lead-free perovskite MASnBr3-based memristor for quaternary information storage

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InfoMat 2020年第4期2卷 743-751页

作者： Wen-Hu Qian Xue-Feng Cheng Jin Zhou Jing-Hui He Hua Li Qing-Feng Xu Na-Jun Li Dong-Yun Chen Zhi-Gang Yao jian-mei lu National United Engineering Laboratory of Functionalized Environmental Adsorption Materials College of ChemistryChemical Engineering and Materials ScienceCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhouChina Testing and Analysis Center Soochow UniversitySuzhouChina

Memristors are a new type of circuit element with a resistance that is tunable to discrete levels by a voltage/current and sustainable after removal of power,allowing for low-power computation and multilevel information *** organic-inorganic lead perovskites are reported to demonstrate memristive behavior,but few have been considered for use as a multilevel memory;also,their potential application has been hindered by the toxicity of lead *** this article,lead-free perovskite MASnBr3 was utilized in memristors for quaternary information *** tin oxide(ITO)/MASnBr3/Au memristors were fabricated and showed reliable memristive switching with well-separated ON/OFF states of a maxima resistance ratio of 102 to *** importantly,four resistive states can be distinguished and repeatedly written/read/erased with a retention time of 104 seconds and an endurance of 104 *** investigating the current-electrode area relationship,Br distribution in the ON/OFF states by in situ Raman and scanning electron microscopy,and temperaturedependent current decay,the memristive behavior was explicitly attributed to the forming/breaking of conductive filaments caused by the migration of Br−under an electric *** addition,poly(ethylene terephthalate)-ITO/MASnBr3/Au devices were found to retain their multiresistance state behavior after being bent for 1000 times,thus demonstrating good device *** results will inspire more lead-free perovskite work for multilevel information storage,as well as other memristor-based electronics.

关键词： MASnBr3 memristor perovskite resistive memory RRAM

Recent progress in the applications of presynaptic dopaminergic positron emission tomography imaging in parkinsonism

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Neural Regeneration Research 2025年第1期20卷 93-106页

作者： Yujie Yang Xinyi Li Jiaying lu Jingjie Ge Mingjia Chen Ruixin Yao mei Tian jian Wang Fengtao Liu Chuantao Zuo Key Laboratory of Arrhythmias Ministry of EducationDepartment of Medical GeneticsShanghai East HospitalSchool of MedicineTongji UniversityShanghaiChina Department of Neurology National Research Center for Aging and MedicineNational Center for Neurological Disordersand State Key Laboratory of Medical NeurobiologyHuashan HospitalFudan UniversityShanghaiChina Department of Nuclear Medicine&PET Center National Center for Neurological Disordersand National Clinical Research Center for Aging and MedicineHuashan HospitalFudan UniversityShanghaiChina International Human Phenome Institutes(Shanghai) ShanghaiChina Human Phenome Institute Fudan UniversityShanghaiChina

Nowadays,presynaptic dopaminergic positron emission tomography,which assesses deficiencies in dopamine synthesis,storage,and transport,is widely utilized for early diagnosis and differential diagnosis of *** review provides a comprehensive summary of the latest developments in the application of presynaptic dopaminergic positron emission tomography imaging in disorders that manifest *** conducted a thorough literature search using reputable databases such as PubMed and Web of *** criteria involved identifying peer-reviewed articles published within the last 5 years,with emphasis on their relevance to clinical *** findings from these studies highlight that presynaptic dopaminergic positron emission tomography has demonstrated potential not only in diagnosing and differentiating various Parkinsonian conditions but also in assessing disease severity and predicting ***,when employed in conjunction with other imaging modalities and advanced analytical methods,presynaptic dopaminergic positron emission tomography has been validated as a reliable in vivo *** validation extends to screening and exploring potential neuropathological mechanisms associated with dopaminergic *** summary,the insights gained from interpreting these studies are crucial for enhancing the effectiveness of preclinical investigations and clinical trials,ultimately advancing toward the goals of neuroregeneration in parkinsonian disorders.

关键词： aromatic amino acid decarboxylase brain imaging dopamine transporter Parkinson’s disease parkinsonism positron emission tomography presynaptic dopaminergic function vesicle monoamine transporter type 2

Clinical value of combining epirubicin with mindfulness intervention in patients with urinary system tumors and depression

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World Journal of Psychiatry 2025年第1期15卷 54-62页

作者： Juan Liu Yan-Ping Guo Yan-mei lu Bei-Lin Wang Department of Urology Surgery Zhumadian Central HospitalZhumadian 463000Henan ProvinceChina Department of Psychiatry Zhumadian Mental HospitalZhumadian 463000Henan ProvinceChina

BACKGROUND Urinary system tumors often cause negative psychological symptoms,such as depression and dysphoria which significantly impact immune function and indirectly affect cancer *** epirubicin(EPI)is recommended by the European Association of Urology and can improve prognosis,its long-term use can cause toxic side effects,reduce treatment compliance,and increase psycho-logical ***,an appropriate intervention mode is *** This was a retrospective study including 110 patients with urinary system tumors and depression admitted to Zhumadian Central Hospital between March 2021 and July *** were divided into conventional(n=55)and joint inter-vention(n=55)*** conventional group received mitomycin and routine nursing,while the joint intervention group received EPI and mindfulness *** groups underwent three cycles of *** function(CD4+cells,CD8+cells,CD4+/CD8+ratio),tumor marker levels[urinary bladder cancer antigen(UBC),bladder tumor antigen(BTA)and nuclear matrix protein 22(NMP22)],quality of life questionnaire-core 30(QLQ-C30),17-item Hamilton depression scale(HAMD-17),and cancer-related fatigue[cancer fatigue scale(CFS)]were *** reactions and nursing satisfaction were recorded and *** Post-intervention,CD4+,CD8+,and CD4+/CD8+levels increased in both groups,with the joint intervention group showing more significant improvement(PluSION EPI combined with mindfulness intervention significantly improved clinical outcomes in patients with urinar

关键词： Urinary system tumor Bladder cancer Prostate cancer Depression Epirubicin

Synthesis of Unsymmetric Ureas by Selenium-Catalyzed Oxidative-Reductive Carbonylation with CO

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Synthesis of Unsymmetric Ureas by Selenium-Catalyzed Oxidati...