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Application of epoxy resin in cultural relics protection

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Chinese Chemical Letters 2024年第4期35卷 31-42页

作者： Zhaoru Chen Xiaoxu liu Haonan Chen jialong li Xiaofeng Wang Jianfeng Zhu Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials School of Material Science and EngineeringShaanxi University of Science and TechnologyXi'an 710021China College of Mechanical&Electrical Engineering Shaanxi University of Science and TechnologyXi'an 710021China

Cultural relics have their unique artistic, cultural and historical value, and the protection of important cultural relics is conducive to the inheritance of historical culture. As a kind of cementing agent and binder commonly seen in cultural relics protection, epoxy resin is widely used in the bonding and consolidation of various materials in cultural relics, which has important practical application value. In this review, a systematic classification of commonly used epoxy resins, including their molecular structures, synthesis reactions and properties are provided, the problems and solutions of epoxy resin in cultural relics protection are summarized. The solutions are classified into three aspects: functional epoxy resin, blending modification, and other modification. Representative application examples of epoxy resin are listed in the field of cultural relics protection, and the development direction of epoxy resin in cultural relics protection in the future is proposed, which provides useful guidance for the modification of epoxy resin and its application in cultural relics protection in the future.

关键词： Epoxy resin Cultural relics Modified UV resistance

Full T-cell activation and function in teleosts require collaboration of first and co-stimulatory signals

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Zoological Research 2024年第1期45卷 13-24页

作者： Wei liang Kang li Haiyou Gao Kunming li Jiansong Zhang Qian Zhang Xinying Jiao jialong Yang Xiumei Wei State Key Laboratory of Estuarine and Coastal Research School of Life SciencesEast China Normal UniversityShanghai 200241China Laboratory for Marine Biology and Biotechnology Qingdao National Laboratory for Marine Science and TechnologyQingdaoShandong 266237China

Mammalian T-cell responses require synergism between the first signal and co-stimulatory signal.However,whether and how dual signaling regulates the T-cell response in early vertebrates remains unknown.In the present study,we discovered that the Nile tilapia(Oreochromis niloticus)encodes key components of the LAT signalosome,namely,LAT,ITK,GRB2,VAV1,SLP-76,GADS,and PLC-γ1.These components are evolutionarily conserved,and CD3εmAb-induced T-cell activation markedly increased their expression.Additionally,at least ITK,GRB2,and VAV1 were found to interact with LAT for signalosome formation.Downstream of the first signal,the NF-κB,MAPK/ERK,and PI3K-AKT pathways were activated upon CD3εmAb stimulation.Furthermore,treatment of lymphocytes with CD28 mAbs triggered the AKT-mTORC1 pathway downstream of the co-stimulatory signal.Combined CD3εand CD28 mAb stimulation enhanced ERK1/2 and S6 phosphorylation and elevated NFAT1,c-Fos,IL-2,CD122,and CD44 expression,thereby signifying T-cell activation.Moreover,rather than relying on the first or co-stimulatory signal alone,both signals were required for T-cell proliferation.Full T-cell activation was accompanied by marked apoptosis and cytotoxic responses.These findings suggest that tilapia relies on dual signaling to maintain an optimal T-cell response,providing a novel perspective for understanding the evolution of the adaptive immune system.

关键词： Oreochromis niloticus CD3 CD28 T cells Adaptive immunity Evolution

Regulation of chloroplast protein degradation

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Journal of Genetics and Genomics 2023年第6期50卷 375-384页

作者： Yang Sun jialong li lixin Zhang Rongcheng lin State Key Laboratory of Crop Stress Adaptation and Improvement Schoolof Life SciencesHenan UniversityKaifengHenan 475001China Key Laboratory of Photobiology Institute of BotanyChinese Academy of SciencesBejing 100093China

Chloroplasts are unique organelles that not only provide sites for photosynthesis and many metabolic processes,but also are sensitive to various environmental stresses.Chloroplast proteins are encoded by genes from both nuclear and chloroplast genomes.During chloroplast development and responses to stresses,the robust protein quality control systems are essential for regulation of protein homeostasis and the integrity of chloroplast proteome.In this review,we summarize the regulatory mechanisms of chloroplast protein degradation refer to protease system,ubiquitin-proteasome system,and the chloroplast autophagy.These mechanisms symbiotically play a vital role in chloroplast development and photosynthesis under both normal or stress conditions.

关键词： Chloroplast Protein homeostasis Protease Ubiquitin-proteasome Chlorophagy

Modulating the alloying mode in the doping-induced synthesis of Au-Pd nanowires

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Nano Research 2024年第4期17卷 3334-3343页

作者： Hui Jin Xiaoliang Wei Lecheng Zhao jialong Yu Qiao Pan Shumin li Qian Wang Zhaotong Yuan Dan Yang Donghui Zhao Hongyu Chen Yawen Wang Institute of Advanced Synthesis School of Chemistry and Molecular EngineeringJiangsu National Synergistic Innovation Center for Advanced MaterialsNanjing Tech UniversityNanjing 211816China School of Science Westlake UniversityHangzhou 310064China Institute of Natural Sciences Westlake Institute for Advanced StudyHangzhou 310064China

Heterogeneous doping is one effective strategy for synthesizing metal alloy nanowires.Herein,the heterogeneous doping processes of Pd on the ultrathin Au nanowires were systematically modulated and investigated.Au-Pd alloy nanowires with various morphologies and lattice structures can be obtained by adjusting the morphology of the precursor Au nanowires and the kinetics of the heterogeneous doping processes.The effects of the rate of Pd reduction and the concentration of the ligand oleylamine(OAm)on the Pd deposition and alloying mode were articulated.Generally,as the Pd deposition rate decreases,the Pd deposition and alloying mode switches from the island-forming Stransky–Krastanov(SK)mode to the epitaxial Frank-van der Merwe(FM)mode,and eventually to an unconventional twisting alloying mode,where the interdiffusion of Pd and Au causes drastic rearrangement of the lattice structure and formation of helical structures.The kinetics-related variation of alloying mode could also be observed in the Au-Ag nanowires,demonstrating a general design principle for the synthesis of alloy nanostructures.In addition,the electrocatalytic performance of various Au-Pd nanowires was evaluated,and the alloy nanowire formed via the SK mode was found to be an excellent electrocatalyst for oxygen reduction and ethanol oxidation.

关键词： gold nanowires Au-Pd alloy oleylamine post-synthetic modification

Positive effects of biochar application and Rhizophagus irregularis inoculation on mycorrhizal colonization,rice seedlings and phosphorus cycling in paddy soils

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Pedosphere 2024年第2期34卷 361-373页

作者： Yixuan CHEN Zhonghua WEN Jun MENG Zunqi liU jialong WEI Xiyu liU Ziyi GE Wanning DAI li liN Wenfu CHEN National Biochar Institute Shenyang Agricultural UniversityShenyang 110866China Key Laboratory of Biochar and Soil Improvement Ministry of Agriculture and Rural AffairsShenyang 110866China

Phosphorus(P)is an essential element for plant growth but is often limiting in ecosystems;therefore,improving the P fertilizer use efficiency is important.Biochar and arbuscular mycorrhizal fungi(AMF)may enhance P cycling in paddy soils that contain high content of total P but low content of available P(AP).In this study,the effects of biochar addition and Rhizophagus irregularis inoculation on the organic and inorganic P contents and phosphatase activities in paddy soils,rice seedling growth,and AMF colonization were investigated.Compared with no biochar addition,biochar addition enhanced the percentage of spore germination at day 7,hyphal length,most probable number,and mycorrhizal colonization rate of R.irregularis by 32%,662%,70%,and 28%on average,respectively.Biochar and R.irregularis altered soil P cycling and availability.Biochar and R.irregularis,either individually or in combination,increased soil AP content by 2%–48%.Rice seedlings treated with biochar and R.irregularis produced greater biomass,improved root morphology,and increased nutrient uptake compared with those of the control without biochar and R.irregularis.The results suggest that combined application of biochar and R.irregularis is beneficial to rice cultivation in paddy soils with high content of total P but low content of AP.

关键词： arbuscular mycorrhizal fungi available P phosphorus fraction rice husk biochar seedling growth spore germination

PCDH17 restricts dendritic spine morphogenesis by regulating ROCK2-dependent control of the actin cytoskeleton,modulating emotional behavior

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Zoological Research 2024年第3期45卷 535-550页

作者： Laidong Yu Fangfang Zeng Mengshu Fan Kexuan Zhang Jingjing Duan Yalu Tan Panlin liao Jin Wen Chenyu Wang Meilin Wang jialong Yuan Xinxin Pang Yan Huang Yangzhou Zhang Jia-Da li Zhuohua Zhang Zhonghua Hu Hunan Key Laboratory of Molecular Precision Medicine Department of Critical Care MedicineXiangya HospitalCentral South UniversityChangshaHunan 410008China Center for Medical Genetics and Hunan Key Laboratory of Medical Genetics School of Life SciencesCentral South UniversityChangshaHunan 410008China National Clinical Research Center for Geriatric Disorders Xiangya HospitalCentral South UniversityChangshaHunan 410008China Hunan Provincial Clinical Research Center for Critical Care Medicine Xiangya HospitalCentral South UniversityChangshaHunan 410008China Hunan Key Laboratory of Animal Models for Human Diseases School of Life SciencesCentral South UniversityChangshaHunan 410008China MOE Key Lab of Rare Pediatric Diseases School of Life SciencesCentral South UniversityChangshaHunan 410008China Department of Neurosciences University of South China Medical SchoolHengyangHunan 421001China

Proper regulation of synapse formation and elimination is critical for establishing mature neuronal circuits and maintaining brain function.Synaptic abnormalities,such as defects in the density and morphology of postsynaptic dendritic spines,underlie the pathology of various neuropsychiatric disorders.Protocadherin 17(PCDH17)is associated with major mood disorders,including bipolar disorder and depression.However,the molecular mechanisms by which PCDH17 regulates spine number,morphology,and behavior remain elusive.In this study,we found that PCDH17 functions at postsynaptic sites,restricting the number and size of dendritic spines in excitatory neurons.Selective overexpression of PCDH17 in the ventral hippocampal CA1 results in spine loss and anxiety-and depression-like behaviors in mice.Mechanistically,PCDH17 interacts with actin-relevant proteins and regulates actin filament(F-actin)organization.Specifically,PCDH17 binds to ROCK2,increasing its expression and subsequently enhancing the activity of downstream targets such as liMK1 and the phosphorylation of cofilin serine-3(Ser3).Inhibition of ROCK2 activity with belumosudil(KD025)ameliorates the defective F-actin organization and spine structure induced by PCDH17 overexpression,suggesting that ROCK2 mediates the effects of PCDH17 on F-actin content and spine development.Hence,these findings reveal a novel mechanism by which PCDH17 regulates synapse development and behavior,providing pathological insights into the neurobiological basis of mood disorders.

关键词： Synapse development Dendritic spine Mood disorder Actin cytoskeleton Animal behavior

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Fabrication of C@MoxTi1-xO2-δ nanocrystalline with functionalized interface as efficient and robust PtRu catalyst support for methanol electrooxidation

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Journal of Energy Chemistry 2020年第1期29卷 7-14,I0001页

作者： jialong li Lei Zhao Xifei li Sue Hao Zhenbo Wang MIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyNo.92 West-Da Zhi StreetHarbin 150001HeilongjiangChina Institute of Advanced Electrochemical Energy&School of Materials Science and Engineering Xi'an University of TechnologyXi'an 710048ShaanxiChina

A core shell structured C@MoxTi1-xO2-δnanocrystal with a functionalized interface(C@MTNC-FI)was fabricated via the hydrothermal method with subsequent annealing derived from tetrabutyl orthotitanate.The formation of anatase TiO2 was inhibited by the simultaneous presence of the hydrothermal etching/regrowth process,infiltration of Mo dopants and carbon coating,which endows the C@MTNC-FI with an ultrafine crystalline architecture that has a Mo-functionalized interface and carbon-coated shell.Pt Ru nanoparticles(NPs)were supported on C@MTNC-FI by employing a microwave-assisted polyol process(MAPP).The obtained Pt Ru/C@MTNC-FI catalyst has 2.68 times higher mass activity towards methanol electrooxidation than that of the un-functionalized catalyst(Pt Ru/C@TNC)and 1.65 times higher mass activity than that of Pt Ru/C catalyst with over 25%increase in durability.The improved catalytic performance is due to several aspects including ultrafine crystals of TiO2 with abundant grain boundaries,Mofunctionalized interface with enhanced electron interactions,and core shell architecture with excellent electrical transport properties.This work suggests the potential application of an interface-functionalized crystalline material as a sustainable and clean energy solution.

关键词： Interface functionalization TiO2 Nanocrystalline Mo doping Core–shell PtRu catalyst Methanol electrooxidation

考虑混凝土弹塑性的植入式GFRP封装FBG传感器应变传递分析

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传感技术学报 2024年第2期37卷 216-223页

作者：彭涛李佳龙任东兴中冶成都勘察研究总院有限公司四川成都610023

工程化FBG传感器的封装层引入的应变传递损耗使其具有应变传递误差,需进行应变传递分析。已有研究多聚焦于基体处于线弹性时的应变传递分析,而混凝土结构发生弹塑性变形后的应变传递规律尚未明晰。以植入式GFRP封装FBG传感器为对象,在... 详细信息

工程化FBG传感器的封装层引入的应变传递损耗使其具有应变传递误差,需进行应变传递分析。已有研究多聚焦于基体处于线弹性时的应变传递分析,而混凝土结构发生弹塑性变形后的应变传递规律尚未明晰。以植入式GFRP封装FBG传感器为对象,在应变传递分析中引入混凝土的非线弹性本构关系,建立了基体与FBG的应变传递关系,通过有限元模拟验证了该理论推导的有效性。基于理论分析探讨了混凝土弹塑性演化、混凝土标号、传感器半径与标距等因素对应变传递效率的影响,并分析了传感器的尺寸设计。研究表明:平均应变传递率在混凝土弹性阶段变化较小,而到塑性阶段则显著降低,混凝土标号、半径与标距都会对应变传递效率产生较大影响。本研究可广泛用于植入式FBG传感器的应变传递误差修正及设计。

关键词：光纤传感植入式FBG传感器应变传递混凝土弹塑性理论分析

矿物微-纳尺度硫同位素分析及在东营凹陷油气成藏的应用示范

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岩石学报 2024年第1期40卷 313-322页

作者：郝佳龙张刘平李照阳杨蔚林杨挺中国科学院地质与地球物理研究所地球与行星物理院重点实验室北京100029 中国科学院地质与地球物理研究所油气资源研究院重点实验室北京100029 防灾科技学院三河市065201

黄铁矿等硫化物离子探针硫同位素分析已经广泛应用在成矿机理、古环境重建、大气环境硫源示踪及行星演化等研究中。纳米离子探针(CAMECA Nano SIMS 50L)的使用将硫化物硫同位素分析空间分辨率提升到微纳尺度(1μm~100nm),实现了分辨率1~... 详细信息

黄铁矿等硫化物离子探针硫同位素分析已经广泛应用在成矿机理、古环境重建、大气环境硫源示踪及行星演化等研究中。纳米离子探针(CAMECA Nano SIMS 50L)的使用将硫化物硫同位素分析空间分辨率提升到微纳尺度(1μm~100nm),实现了分辨率1~2μm、精度0.5‰(1SD)的硫同位素点分析方法,分辨率100nm、精度1‰的硫同位素图像分析方法。为了进一步优化分析流程拓展纳米离子探针硫同位素的应用,本文系统比较了纳米离子探针微纳尺度硫同位素点分析方法、图像分析方法的各自特点及分析流程;并以东营凹陷北带沙四段黄铁矿为研究对象,联合采用了纳米离子探针硫同位素点分析和硫同位素图像分析手段,对黄铁矿微细结构进行分析,从而揭示了储层中黄铁矿成因及其油气成藏的指示意义。

关键词：纳米离子探针硫同位素空间分辨率东营凹陷同位素图像