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Chinese Optics Letters 2022年第3期20卷 30-34页

作者： Jun Guo jan qiu Jie Xu Bin Xu Juchong Ding Xiaodan Wang Xiaodong Xu Jun Xu Jiangsu Key Laboratory of Advanced Laser Materials and Devices School of Physics and Electronic EngineeringJiangsu Normal UniversityXuzhou 221116China School of Physics Science and Engineering Institute for Advanced StudyTongji UniversityShanghai 200092China Department of Electronic Engineering Xiamen UniversityXiamen 361005China Research&Development Center of Material and Equipment 26th Research InstituteChina Electronics Technology Group CorporationChongqing 400060China School of Physics Science and Technology Suzhou University of Science and TechnologySuzhou 215009China

A good thermo-optic property of strontium dodeca-aluminum oxide[SrAl_(12)O_(12),SRA]host material is very advantageous to the development of high-performance lasers by doping rare-earth ions for gain *** this work,we report on diode-end-pumped high-performance continuous-wave and passively Q-switched Nd:SRA *** continuous-wave operation,a maximum output power of 6.45 W is achieved at 1049 nm with a slope eficiency of about 41.6%.Using a Y_(3)Al_(12)O_(19)etalon,we have firstly achieved a 1066 nm laser with a maximum output power of 4.15 W and a slope efficiency of about 27%,to the best of our *** passively Q switched operation,with Cr^(4+):YAG as a saturable absorber,a maximum average output power of 1.82 W was achieved with the shortest pulse width of 18.2 ns at pulse repetition rate of 22.9 *** single-pulse energy and pulse peak power were 79.4μJ and 4.3 *** work has further verified that the Nd:SRA crystal is very promising for high-performance laser generation.

关键词： diode pump Nd:SRA crystal continuous-wave operation passively Q-switched operation

Directly addressable GaN-based nano-LED arrays: fabrication and electro-optical characterization

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Microsystems & Nanoengineering 2020年第1期6卷 275-284页

作者： Daria D.Bezshlyakh Hendrik Spende Thomas Weimann Peter Hinze Steffen Bornemann jan Gulink Joan Canals Joan Daniel Prades Angel Dieguez Andreas Waag Institute of Semiconductor Technology Technische Universitat BraunschweigHans-Sommer Str.6638106 BraunschweigGermany Laboratory for Emerging Nanometrology Langer Kamp 6 a/b38106 BraunschweigGermany Epitaxy Competence Center ec2 Technische Universitat BraunschweigHans-Sommer Str.6638106 BraunschweigGermany Nanostructuring and Clean Room Center Infrastructure Physikalisch-Technische BundesanstaltBundesallee 10038116 BraunschweigGermany Department of Electronic and Biomedical Engineering University of BarcelonaCarrer Marti i Franques 108028 BarcelonaSpain

The rapid development of display technologies has raised interest in arrays of self-emitting,individually controlled light sources atthe *** nitride(GaN)micro-light-emitting diode(LED)technology meets this ***,the current technology is not suitable for the fabrication of arrays of submicron light sources that can be controlled *** approach is based on nanoLED arrays that can directly address each array element and a self-pitch with dimensions below the wavelength of *** design and fabrication processes are explained in detail and possess two geometries:a 6×6 array with 400 nm LEDs and a 2×32 line array with 200 nm *** nanoLEDs are developed as core elements of a novel on-chip super-resolution *** technology,based on its physical properties,is an ideal platform for such nanoLEDs.

关键词： arrays GaN optical

Magnetic Phase Transition in Two-Dimensional CrBr_(3) Probed by a Quantum Sensor

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Chinese Physics Letters 2022年第4期39卷 79-82页

作者： Haodong Wang Peihan Lei Xiaoyu Mao † Xi Kong Xiangyu Ye Pengfei Wang Ya Wang Xi Qin jan Meijer Hualing Zeng Fazhan Shi Jiangfeng Du Hefei National Laboratory for Physical Sciences at the Microscale and School of Physical Sciences University of Science and Technology of ChinaHefei 230026China CAS Key Laboratory of Microscale Magnetic Resonance University of Science and Technology of ChinaHefei 230026China CAS Center for Excellence in Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China National Laboratory of Solid State Microstructures and Department of Physics Nanjing UniversityNanjing 210093China Felix-Bloch Institute for Solid State Physics University LeipzigLinn´e Str.5D-04103 LeipzigGermany

Recently,magnetism in two-dimensional(2 D)van der Waals(vd W)materials has attracted wide *** is anticipated that these materials will stimulate discovery of new physical phenomena and novel *** capability to quantitatively measure the magnetism of 2 D magnetic vd W materials is essential to understand these *** we report on quantitative measurements of ferromagnetic-to-paramagnetic phase transition of an atomically thin(down to 11 nm)vd W magnet,namely Cr Br_(3),with a Curie point of 37.5 *** experiment demonstrates that surface magnetism can be quantitatively investigated,which is useful for a wide variety of potential applications.

关键词： materials Transition Probe

One droplet reaction for synthesis of multi-sized nanoparticles

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Nano Research 2023年第4期16卷 5850-5856页

作者： Bingda Chen Feifei Qin Meng Su Daixi Xie Zeying Zhang Qi Pan Huadong Wang Xu Yang Sisi Chen Jingwei Huang Dominique Derome jan Carmeliet Yanlin Song Key Laboratory of Green Printing Institute of ChemistryChinese Academy of SciencesBeijing Engineering Research Center of Nanomaterials for Green Printing TechnologyBeijing National Laboratory for Molecular Sciences(BNLMS)Beijing 100190China University of Chinese Academy of Sciences Beijing 100049China Chair of Building Physics Department of Mechanical and Process EngineeringETH Zürich(Swiss Federal Institute of Technology in Zürich)Zürich 8092Switzerland Department of Civil and Building Engineering Universitéde SherbrookeSherbrooke QC J1K 2R1Canada

Reaction kinetics of nanoparticles can be controlled by tuning the Peclet number(Pe)as it is an essential parameter in synthesis of multi-sized ***,we propose to implement a self-driven multi-dimension microchannels reactor(MMR)for the one droplet synthesis of multi-sized *** carefully controlling the Pe at the gas-liquid interface,the newly formed seed crystals selectively accumulate and grow to a specific *** the combination of microchannels of different widths and lengths,one droplet reaction in the same apparatus achieves the synchronous synthesis of diverse *** enables precise control of nanoparticle diameter at 5 nm precision in the range of 10-110 *** use of MMR can be extended to the synthesis of uniform Ag,Au,Pt,and Pd nanoparticles,opening towards the production and engineering of nanostructured *** approach gives the chance to regulate the accumulation probability for precise synthesis of nanoparticles with different diameters.

关键词： gas-liquid interface accumulation effect one droplet reaction multi-sized nanoparticles

Making the Genotypic Variation Visible:Hyperspectral Phenotyping in Scots Pine Seedlings

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Plant Phenomics 2023年第4期5卷 790-804页

作者： jan Stejskal Jaroslav Čepl Eva Neuwirthová Olusegun Olaitan Akinyemi Jiří Chuchlík Daniel Provazník Markku Keinänen Petya Campbell jana Albrechtová Milan Lstiburek Zuzana Lhotáková Department of Genetics and Physiology of Forest Trees Faculty of Forestry and Wood SciencesCzech University of Life Sciences PraguePragueCzech Republic Department of Environmental and Biological Sciences University of Eastern FinlandJoensuuFinland Department of Experimental Plant Biology Charles UniversityPragueCzech Republic Center for Photonic Sciences University of Eastern FinlandJoensuuFinland Department of Geography and Environmental Sciences University of Maryland Baltimore CountyBaltimoreMDUSA Biospheric Sciences Laboratory NASA Goddard Space Flight CenterGreenbeltMDUSA

Hyperspectral reflectance contains valuable information about leaf functional traits,which can indicate a plant's physiological ***,using hyperspectral reflectance for high-throughput phenotyping of foliar traits could be a powerful tool for tree breeders and nursery practitioners to distinguish and select seedlings with desired adaptation potential to local *** evaluated the use of 2 nondestructive methods(i.e.,leaf and proximal/canopy)measuring hyperspectral reflectance in the 350-to 2,500-nm range for phenotyping on 1,788 individual Scots pine seedlings belonging to lowland and upland ecotypes of 3 different local populations from the Czech ***-level measurements were collected using a spectroradiometer and a contact probe with an internal light source to measure the biconical reflectance factor of a sample of needles placed on a black background in the contact probe field of *** proximal canopy measurements were collected under natural solar light,using the same spectroradiometer with fiber optical cable to collect data on individual seedlings'hemispherical conical reflectance *** latter method was highly susceptible to changes in incoming *** spectral datasets showed statistically significant differences among Scots pine populations in the whole spectral ***,using random forest and support vector machine learning algorithms,the proximal data obtained from the top of the seedlings offered up to 83%accuracy in predicting 3 different Scots pine *** conclude that both approaches are viable for hyperspectral phenotyping to disentangle the phenotypic and the underlying genetic variation within Scots pine seedlings.

关键词： Scots forest reflectance

Hybrids of gold nanoparticles and oligo(p-phenyleneethynylene)s end-functionalized with alkynylruthenium groups:Outstanding two-photon absorption in the second biological window

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Nano Research 2020年第10期13卷 2755-2762页

作者： Cristóbal Quintana Mahbod Morshedi Jun Du Joseph P.L.Morrall jan K.Zaręba Marek Samoc Marie P.Cifuentes Mark G.Humphrey I Research School of Chemistry Australian National UnriversityCanberraACT 2601Australia Advanced Materials Engineering and Modelling Group Wroclaw University of Science and TechnologyWroclaw 50370Poland

Oligo(p-phenyleneethynylene)s(OPEs)end-capped with(alkynyl)bis(diphosphine)ruthenium and thiol/thiolate groups stabilize ca.2 nm diameter gold nanoparticles(AuNPs).The morphology,elemental composition and stability of the resultant organometallic OPE/AuNP hybrid materials have been defined using a combination of molecular-and nano-material chacterization *** hybrids display long-term stability in solution(more than a month),good solubility in organic solvents,reversible rutheniumcentered oxidation,and transparency beyond 800 nm,and possess very strong nonlinear absorption activity at the first biological window,and unprecedented two-photon absorption activity in the second biological window(σ2 up to 38,000 GM at 1,050 nm).

关键词： gold nanoparticles inorganic materials metal alkynyl complexes nonlinear optics organometallics

Microstructure and hydrogen storage properties of as-cast and rapidly solidified Ti-rich Ti-V alloys

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Transactions of Nonferrous Metals Society of China 2012年第8期22卷 1831-1838页

作者： Suwarno SUWARNO jan Ketil SOLBERG jan Petter MAEHLEN Bente KROGH Bφrre Tore BφRRESEN Esther OCHOA-FERNANDEZ Erling RYTTER Mario WILLIAMS Roman DENYS Volodymyr A.YARTYS Department of Materials Science and Engineering Norwegian University of Science and TechnologyNO-7491TrondheimNorway Institute for Energy Technology P.O.Box 40NO-2027KjellerNorway Statoil Research Centre RotvollN-7005TrondheimNorway University of the Western Cape Private Bag X17Bellville7535South Africa

The goal of the present work was to optimize the phase-structural composition and microstructure of binary Ti0.8-0.9V0.2-0.1 alloys with respect to their hydrogen sorption properties. Application of these alloys is for hydrogen absorption from gaseous mixtures containing substantial amounts of carbon monoxide （CO） at high temperatures. Irrespective of alloy composition, both α（HCP） and β（BCC） phases in Ti0.8-0.9V0.2-0.1 formed single phase FCC hydrides upon hydrogenation in pure H2. An in situ synchrotron X-ray diffraction study showed that only the β-phase transformed to the corresponding hydride when the alloy was hydrogenated in a mixture of H2＋10%CO. Rapid solidification （RS） of the alloy resulted in refined grain sizes both in the Ti0.8V0.2 and Ti0.9V0.1 alloys. Furthermore, RS was found to increase the β-phase fraction in Ti0.9V0.1, being twice larger than that of the as-cast alloy. Ti0.9V0.1 had a platelike microstructure as observed by scanning electron microscopy （SEM）, the plates were about 300 nm thick. The microstructure refinement resulted in a faster kinetics of H desorption as observed by temperature desorption spectroscopy （TDS）.

关键词： hydrogen storage Ti-V alloys rapid solidification synchrotron X-ray diffraction carbon monoxide

Size-dependent structural and magnetic properties of chemically synthesized Co-Ni-Ga nanoparticles

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Nano Research 2017年第10期10卷 3421-3433页

作者： Changhai Wang Aleksandr A. Levin Julie Karel Simone Fabbrici Jinfeng Qian Carlos E. ViolBarbosa Siham Ouardi Franca Albertini Walter Schnelle jan Rohlicek Gerhard H. Fecher Claudia Felser Max Planck Institute for Chemical Physics of Solids D-01187 Dresden Germany Institute of Materials for Electronics and Magnetism IMEM-CNRI-43124 Parma Italy MIST E-R Laboratory Via Gobetti 101 I-40129 Bologna Italy

Phase transitions and magnetic properties of shape-memory materials can be tailored by tuning the size of the constituent materials, such as nanoparticles. However, owing to the lack of suitable synthetic methods for size-controlled Heusler nanoparticles, there is no report on the size dependence of their properties and functionalities. In this contribution, we present the first chemical synthesis of size-selected Co-Ni-Ga Heusler nanoparticles. We also report the structure and magnetic properties of the biphasic Co-Ni-Ga nanoparticles with sizes in the range of 30-84 nm, prepared by a SBA-15 nanoporous silica- templated approach. The particle sizes could be readily tuned by controlling the loading and concentration of the precursors. The fractions and crystallite sizes of each phase of the Co-Ni-Ga nanoparticles are closely related to their particle size. Enhanced magnetization and decreased coercivity are observed with increasing particle size. The Curie temperature （To） of the Co-Ni-Ga nanoparticles also depends on their size. The 84 nm-sized particles exhibit the highest Tc （≈ 1,174 K） among all known Heusler compounds. The very high Curie temperatures of the Co-Ni-Ga nanoparticles render them promising candidates for application in high-temperature shape memory alloy-based devices.

关键词： Co-Ni-Ga nanoparticles chemical synthesis size magnetic properties

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铋基材料光催化还原水中六价铬的研究进展

Chinese Journal of Catalysis 2023年第12期55卷 20-43页

作者：孙阳 jan E.Szulejko Ki-Hyun Kim Vanish Kumar 李小伟汉阳大学土木与环境工程系首尔韩国国家农业食品生物技术研究所(NABI) 旁遮普邦纳加尔印度上海大学环境与化学工程学院有机化合物污染控制工程教育部重点实验室中国上海200444

光催化还原是处理水溶液体系中六价铬(Cr(VI))的一种新方法.层状铋(Bi)基材料具有增强的光捕获能力和可调的带隙能量,被认为是一种光催化还原去除Cr(VI)的有效材料.本文从修饰策略(如异质结、缺陷工程和掺杂)和工艺变量(如溶液p H和添... 详细信息

光催化还原是处理水溶液体系中六价铬(Cr(VI))的一种新方法.层状铋(Bi)基材料具有增强的光捕获能力和可调的带隙能量,被认为是一种光催化还原去除Cr(VI)的有效材料.本文从修饰策略(如异质结、缺陷工程和掺杂)和工艺变量(如溶液p H和添加剂的类型/数量)等方面,对用于光催化还原处理Cr(VI)的铋基材料的改进机制进行深入总结.此外,采用工业上用作关键指标的优值系数(FoM),对各种铋基材料的性能进行评估.结果发现,平均粒径为5-10 nm,具有shuriken形状的BiVO_(4)具有最高的FoM值(3.45×10^(-5) molg^(-1)Wh^(-1)),且其光催化还原性能最好.同时,与其他非铋基催化剂相比,BiVO_(4)的光催化还原Cr(VI)性能也具有很好的优势.但是,目前铋基催化剂成本较高,且光催化还原过程能耗较大,距离大规模实际应用还有一定的距离.未来,为实现铋基催化剂光催化还原处理含Cr(VI)废水的大规模应用,应大幅度降低催化剂的生产成本,并提高催化剂光子吸收效率从而进一步提高能源利用率.

关键词：光催化铬半导体铋优值系数

Intrinsic carrier multiplication in layered Bi_(2)O_(2)Se avalanche photodiodes with gain bandwidth product exceeding 1 GHz

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Nano Research 2021年第6期14卷 1961-1966页

作者： Vinod K.Sangwan Joohoon Kang David Lam J.Tyler Gish Spencer A.Wells jan Luxa James P.Male GJeffrey Snyder Zdenek Sofer Mark C.Hersam Department of Materials Science and Engineering Northwestern UniversityEvanstonIL60208USA Department of Inorganic Chemistry University of Chemistry and Technology PragueTechnicka 516628Prague 6Czech Republic Department of Chemistry Northwestern UniversityEvanstonIL60208USA Department of Electrical and Computer Engineering Northwestern UniversityEvanstonIL60208USA

Emerging layered semiconductors present multiple advantages for optoelectronic technologies including high carrier mobilities,strong light-matter interactions,and tunable optical absorption and ***,metal-semiconductor-metal avalanche photodiodes(APDs)are fabricated from Bi2O2Se crystals,which consist of electrostatically bound[Bi2O2]2+and[Se]2−*** resulting APDs possess an intrinsic carrier multiplication factor up to 400 at 7 K with a responsivity gain exceeding 3,000 A/W and bandwidth of~400 kHz at a visible wavelength of 515.6 nm,ultimately resulting in a gain bandwidth product exceeding 1 *** to exceptionally low dark currents,Bi2O2Se APDs also yield high detectivities up to 4.6×1014 Jones.A systematic analysis of the photocurrent temperature and bias dependence reveals that the carrier multiplication process in Bi2O2Se APDs is consistent with a reverse biased Schottky diode model with a barrier height of~44 meV,in contrast to the charge trapping extrinsic gain mechanism that dominates most layered semiconductor *** this manner,layered Bi2O2Se APDs provide a unique platform that can be exploited in a diverse range of high-performance photodetector applications.

关键词： layered semiconductor photodetector high-frequency Schottky diode impact ionization