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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan Ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju kim Wangyun Won Department of Chemical and Biological Engineering Korea University Department of Chemical Engineering (Integrated process) Kyung Hee University Department of Chemical Engineering and Materials Science Ewha Womans University Department of Chemical Engineering Pukyong National University Resources Engineering Plant Research Department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

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Stable immobilization of lithium polysulfides using three-dimensional ordered mesoporous Mn_(2)O_(3) as the host material in lithium-sulfur batteries

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Carbon Energy 2024年第6期6卷 99-112页

作者： Sung Joon Park Yun Jeong Choi hyun-seung kim Min Joo Hong Hongjun Chang Janghyuk Moon Young-Jun kim Junyoung Mun Ki jae kim Department of Energy Science Sungkyunkwan UniversitySuwonGyeonggi-doRepublic of Korea Department of Energy Engineering Konkuk UniversitySeoulRepublic of Korea Advanced Batteries Research Center Korea Electronic Technology InstituteSeongnamRepublic of Korea Department of Future Energy Engineering Sungkyunkwan UniversitySuwonRepublic of Korea Department of Energy Systems Engineering Chung-Ang UniversitySeoulRepublic of Korea SKKU Advanced Institute of Nanotechnology Sungkyunkwan UniversitySuwonGyeonggi-doRepublic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwonRepublic of Korea School of Advanced Materials Science and Engineering Sungkyunkwan UniversitySuwonRepublic of Korea

Lithium-sulfur batteries(LSBs)have drawn significant attention owing to their high theoretical discharge capacity and energy ***,the dissolution of long-chain polysulfides into the electrolyte during the charge and discharge process(“shuttle effect”)results in fast capacity fading and inferior electrochemical *** this study,Mn_(2)O_(3)with an ordered mesoporous structure(OM-Mn_(2)O_(3))was designed as a cathode host for LSBs via KIT-6 hard templating,to effectively inhibit the polysulfide shuttle ***-Mn_(2)O_(3)offers numerous pores to confine sulfur and tightly anchor the dissolved polysulfides through the combined effects of strong polar-polar interactions,polysulfides,and sulfur chain *** OM-Mn_(2)O_(3)/S composite electrode delivered a discharge capacity of 561 mAh g^(-1) after 250 cycles at 0.5 C owing to the excellent performance of OM-Mn_(2)O_(3).Furthermore,it retained a discharge capacity of 628mA h g^(-1) even at a rate of 2 C,which was significantly higher than that of a pristine sulfur electrode(206mA h g^(-1)).These findings provide a prospective strategy for designing cathode materials for high-performance LSBs.

关键词： host material lithium-sulfur battery ordered mesoporous structure shuttle effect transition-metal oxides

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Comparison of hepatic venous pressure gradient and endoscopic grading of esophageal varices

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World Journal of Gastroenterology 2016年第11期22卷 3212-3219页

作者： Eun Ji Lee Yong jae kim Dong Erk Goo Seung Boo Yang hyun-Joo kim jae Young Jang Soung Won Jeong Department of Radiology Soonchunhyang University Seoul Hospital Department of Radiology Soonchunhyang University Gumi Hospital Department of Gastroenterology Soonchunhyang University Seoul Hospital

AIM: To determine the correlation between the hepatic venous pressure gradient and the endoscopic grade of esophageal ***: From September 2009 to March 2013, a total of 176 measurements of hepatic venous pressure gradient (HVPG) were done in 146 patients. Each transjugular HVPG was measured twice, first using an end whole catheter (EH-HVPG), and then using a balloon catheter (B-HVPG). The HVPG was compared with the endoscopic grade of esophageal varices (according to the general rules for recording endoscopic findings of esophagogastric varices), which was recorded within a month of the measurement of ***: The study included 110 men and 36 women, with a mean age of 56.1 years (range, 43-76 years). The technical success rate of the pressure measurements was 100% and there were no complication related to the procedures. Mean HVPG was 15.3 mmHg as measured using the end hole catheter method and 16.5 mmHg as measured using the balloon catheter method. Mean HVPG (both EH-HVPG and B-HVPG) was not significantly different among patients with different characteristics, including sex and comorbid factors, except for cases with hepatocellular carcinoma (B-HVPG, P = 0.01; EH-HVPG, P = 0.02). Portal hypertension (> 12 mmHg HVPG) occurred in 66% of patients according to EH-HVPG and 83% of patients according to B-HVGP, and significantly correlated with Child’s status (B-HVPG, P < 0.000; EH-HVGP, P < 0.000) and esophageal varies observed upon endoscopy (EH-HVGP, P = 0.003; B-HVGP, P = 0.006). One hundred and thirty-five endoscopies were performed, of which 15 showed normal findings, 27 showed grade 1 endoscopic esophageal varices, 49 showed grade 2 varices, and 44 showed grade 3 varices. When comparing endoscopic esophageal variceal grades and HVPG using univariate analysis, the P value was 0.004 for EH-HVPG and 0.002 for ***: Both EH-HVPG and B-HVPG showed a positive correlation with the endoscopic grade of esophag

关键词： Hepatic venous pressure gradient Liver cirrhosis Esophageal varices Endoscopic grade of esophageal varices Balloon catheter measurement End hole catheter measurement

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Prolonged and highly efficient intracellular extraction of photosynthetic electrons from single algal cells by optimized nanoelectrode insertion

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Nano Research 2018年第1期11卷 397-409页

作者： Hyeonaug Hong Yong jae kim Myungjin Han Gu YOO hyun Woo Song Youngcheol Chae jae-Chul Pyun Arthur R. Grossman WonHyoung Ryu Department of Mechanical Engineering Yonsei University Seou103722 Republic of Korea Yonsei Institute of Convergence Technology and school of In tegrated Technology Yonsei University Incheon 21983 Republic of Korea Department of Materials Science & Engineering Yonsei University Seou103722 Republic of Korea Department of Electrical & Electronic Engineering Yonsei University Seou103722 Republic of Korea Deportment of Plant Biology Carnegie Institution for Science Department of Biology Stanford University Stanford CA 94305 USA

Harvesting photosynthetic electrons （PEs） from plant or algal cells can be a highly efficient and environmentally friendly way of generating renewable energy. Recent work on nanoelectrode insertion into algal cells has demonstrated the possibility to directly extract PEs from living algal cells with high efficiencies. However, the instability of the inserted cells limits the practicality of this technology. Here, the impact of nanoelectrode insertion on intracellular extraction of PEs is characterized with the goal of stabilizing algal cells after nanoelectrode insertion. Using nanoelectrodes 〈 500 nm in diameter, algal cells remained stable for over one week after insertion and continued to provide PEs through direct extraction by the inserted nanoelectrodes. After nanoelectrode insertion, a photosynthetic current density of 6 ***-2, which is several fold higher than the current densities attained using approaches based on isolated thylakoid membranes or photosystem I complexes, was observed in the dark and during illumination at various light intensities.

关键词： bio-solar energy photosynthetic electrons algal cells nanoelectrode cell insertion

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Presence of CCK-A, B receptors and effect of gastrin and cholecystokinin on growth of pancreatobiliary cancer cell lines

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World Journal of Gastroenterology 2005年第6期11卷 803-809页

作者： Jin-Young Jang Sun-Whe kim Ja-Lok Ku Yong-hyun Park jae-Gahb Park Department of Surgery

AIM: To investigate the effects of gastrin and cholecystokinin (CCK) and their specific antagonists on the growth of pancreatic and biliary tract cancer cell lines. METHODS: Five pancreatic and 6 biliary cancer cell lines with 2 conrtol cells were used in this study. Cell proliferation study was done using 3-[4,5-dimethylthiazol-2-yl]-2,5-diphenyl tetrazolium bromide (MTT) test and direct cell count method. Reverse transcription-polymerase chain reaction (RT-PCR) and slot blot hybridization were performed to examine and quantify the expression of hormonal receptors in these cell lines. RESULTS: SNU-308 showed a growth stimulating effect by gastrin-17, as did SNU-478 by both gastrin-17 and CCK-8. The trophic effect of these two hormones was completely blocked by specific antagonists (L-365, 260 for gastrin and L-364, 718 for CCK). Other cell lines did not respond to gastrin or CCK. In RT-PCR, the presence of CCK-A receptor and CCK-B/gastrin receptor mRNA was detected in all biliary and pancreatic cancer cell lines. In slot blot hybridization, compared to the cell lines which did not respond to hormones, those that responded to hormones showed high expression of receptor mRNA. CONCLUSION: Gastrin and CCK exert a trophic action on some of the biliary tract cancers.

关键词： Bile duct cancer Gallbladder cancer Pancreatic cancer Gastrin Cholecystokinin

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Risk factors of electrocoagulation syndrome after esophageal endoscopic submucosal dissection

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World Journal of Gastroenterology 2018年第10期24卷 1144-1151页

作者： Dae Won Ma Young Hoon Youn Da hyun Jung jae Jun Park Jie-hyun kim Hyojin Park Department of Internal Medicine Gangnam Severance Hospital Yonsei University College of Medicine

AIM To investigate post endoscopic submucosal dissection electrocoagulation syndrome(PEECS) of the *** We analyzed 55 consecutive cases with esophageal endoscopic submucosal dissection for superficial esophageal squamous neoplasms at a tertiary referral hospital in South Korea. Esophageal PEECS was defined as "mild" meeting one of the following criteria without any obvious perforation: fever(≥ 37.8 ℃), leukocytosis(> 10800 cells/μl), or regional chest pain more than 5/10 points as rated on a numeric pain intensity scale. The grade of PEECS was determined as "severe" when meet two or more of above *** We included 51 cases without obvious complications in the analysis. The incidence of mild and severe esophageal PEECS was 47.1% and 17.6%, respectively. Risk factor analysis revealed that resected area, procedure time, and muscle layer exposure were significantly associated with PEECS. In multivariate analysis, a resected area larger than 6.0 cm^2(OR = 4.995, 95%CI: 1.110-22.489, P = 0.036) and muscle layer exposure(OR = 5.661, 95%CI: 1.422-22.534, P = 0.014) were independent predictors of esophageal PEECS. All patients with PEECS had favorable outcomes with conservative management approaches, such as intravenous hydration or *** Clinicians should consider the possibility of esophageal PEECS when the resected area exceeds 6.0 cm^2 or when the muscle layer exposure is noted.

关键词： Electrocoagulation Endoscopic submucosal dissection Esophageal neoplasm Syndrome

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Mechanical characteristics of tensile strength ratio method compared to other parameters used for moisture susceptibility evaluation of asphalt mixtures

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Journal of Traffic and Transportation Engineering(English Edition) 2019年第6期6卷 621-630页

作者： Thanh Chung Do Van Phuc Tran Van Phuc Le hyun Jong Lee Won jae kim Department of Civil and Environmental Engineering Sejong UniversitySeoul 143-747South Korea Faculty of Civil Engineering University of Transport and CommunicationsHo Chi Minh CityVietnam

In this study,mechanical characteristics of tensile strength ratio(TSR)were evaluated by comparing it to other methods in evaluating moisture sensitivity of asphalt *** types of asphalt mixtures with and without anti-stripping additives were prepared and tested in the *** compressive strength(UCS)and indirect tensile(IDT)testing were conducted to determine the mixture’s tensile strength ratio and cohesion ratio(CR).Determining TSR alone was found to be insufficient when evaluating moisture *** is a need to consider both TSR and wet IDT strength to properly evaluate moisture behavior of asphalt ***,it was found that the cohesion and the IDT strength have a good relation in which the minimum condition of the slope,must be ***,it was observed thatβvalues change depending on material type and ***,there is a need to evaluate theseβvalues for varying material and testing *** addition,it was found that the TSR and CR results are highly correlated with an average difference of 1.5%.Furthermore,other tests such as Marshall stability and dynamic immersion were also *** was found that Marshall stability ratio(MSR)and Marshall stability to flow ratio(MSFR)values are less sensitive to moisture effect when measuring moisture resistance compared to TSR ***,the 48 h testing result of the dynamic immersion test showed better correlation with TSR values.

关键词： Asphalt mixtures Moisture damage Anti-stripping additives Tensile strength ratio Cohesion strength ratio

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Endoscopic stenting for recurrence-related colorectal anastomotic site obstruction:Preliminary experience

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World Journal of Gastroenterology 2014年第38期20卷 13936-13941页

作者： Jung Ho kim Jong Joon Lee jae Hee Cho Kyoung Oh kim Jun-Won Chung Yoon jae kim Kwang An Kwon Dong Kyun Park Ju hyun kim Department of Internal Medicine Gachon University Gil Medical Center

AIM: To evaluate the efficacy of stents in treating patients with anastomotic site obstructions due to cancer recurrence following colorectal surgery.

关键词： Colorectal neoplasms Endoscopy Intestinal obstruction Stents Surgical anastomosis

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Grasper type scissors for endoscopic submucosal dissection of gastric epithelial neoplasia

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World Journal of Gastroenterology 2013年第37期19卷 6221-6227页

作者： Woo-Chul Chung Byung-Wook kim Chul-hyun Lim Tae-Ho kim jae-Myung Park Joon-Sung kim Division of Gastroenterology Department of Internal MedicineSuwon St.Vincent’s HospitalThe Catholic University of Korea Division of Gastroenterology Department of Internal MedicineIncheon St.Mary’s HospitalThe Catholic University of Korea Division of Gastroenterology Department of Internal MedicineSeoul St.Mary’s HospitalThe Catholic University of Korea Division of Gastroenterology Department of Internal MedicineBucheon St.Mary’s HospitalThe Catholic University of Korea

AIM:To evaluate the efficacy and safety of grasper type scissors(GTS)for endoscopic submucosal dissection(ESD)of gastric epithelial ***:The study was performed by 4 endoscopists in 4 institutions affiliated to The Catholic University of *** was performed in 76 consecutive patients with gastric epithelial neoplasia by using the GTS(37 patients)or the hook knife plus coagrasper(HKC)(39 patients).The complete resection rate,complication rate,total time elapsed and elapsed time per square centimeter of the dissected specimen were analyzed between the GTS and HKC ***:The mean age of the GTS group was 62.3±11.4 years and mean age of the HKC group was 65.6±10.1 *** adenocarcinoma was found in32.4%in the GTS group and 33.3%in the HKC *** procedures were performed without interruption in every case in both *** en bloc resection rates of both groups were 100%.The total time elapsed during the procedure was 44.54±21.72 min in the GTS group and 43.77±21.84 min in the HKC group(P=0.88)and the time elapsed per square centimeter of the resected lesion was 7.53±6.35 min/cm2in the GTS group and 6.92±5.93 min/cm2in the HKC group(P=0.66).The overall complication rate was not significantly different between the two ***:GTS is a safe and effective device for ESD compared with *** can be performed with GTS alone,which can reduce the costs for ESD.

关键词： Gastric epithelial neoplasia Endoscopic submucosal dissection Grasper type scissors Hook knife Coagrasper

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Flow Characteristics in Compact Thermal Spray Coating Systems with Minimum Length Nozzle

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Plasma Science and Technology 2009年第5期11卷 550-554页

作者： Seung-hyun kim Youn-Jea kim School of Mechanical Engineering Sungkyunkwan University

In this study, numerical analysis is performed to adopt the equivalence ratio on the high velocity oxygen fuel （HVOF） thermal spray coating systems equipped with a minimum length nozzle. The analysis is applied to investigate the axisymmetric, steady-state, turbulent, and chemically combusting flow both within the torch and in a free jet region between the torch and the substrate to be coated. The combustion is modeled using a single-step and eddy-dissipation model which assumes that the reaction rate is limited by the turbulent mixing rate of the fuel and oxidant. As the diameter of the nozzle throat is increased, the location of the Mach shock disc moves backward from the nozzle exit. As the throat diameter and the divergent portion are 6 mm and 8 mm, respectively, the pressure in the HVOF system is the lowest at the chamber and the expanding gas is steadily maintained with both high velocity and high temperature for different equivalence ratios. Thus, relatively minor amendments of the equivalence ratio and the geometry of HVOF can lead to improved control over coating characteristics.

关键词： minimum length nozzle HVOF equivalence ratio

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