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Low-thermal-budget synthesis of monolayer MoS2

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Science China Materials 2024年第1期67卷 372-374页

作者： Zongmeng Yang Shibo fang jing Lu State Key Laboratory for Mesoscopic Physics and School of Physics Peking University Collaborative Innovation Center of Quantum Matter Beijing Key Laboratory for Magnetoelectric Materials and Devices (BKL-MEMD) Peking University Peking University Yangtze Delta Institute of Optoelectronics Key Laboratory for the Physics and Chemistry of Nanodevices Peking University Beijing Key Laboratory of Quantum Devices Peking University

Two-dimensional (2D) materials, such as MoS2, have been considered as a competitive coordinate for future electronics due to their excellent electrostatics and high mobility [1–3]. Moreover, the potential integration of 2D materials with silicon circuits can present increased density and multifunction in future heterogeneously integrated circuits [4,5]. However, the high thermal-budget during Mo S2 synthesis exceeds the temperature requirement of direct integration with Si in the back-end-of-line (BEOL) fabrication process [6–8].

关键词： FILMS

A transfer learning enhanced physics-informed neural network for parameter identification in soft materials

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Applied Mathematics and Mechanics(English Edition) 2024年第10期45卷 1685-1704页

作者： jing'ang ZHU Yiheng xue Zishun LIU International Center for Applied Mechanics State Key Laboratory for Strength and Vibration of Mechanical Structures School of Aerospace EngineeringXi'an Jiaotong University

Soft materials, with the sensitivity to various external stimuli, exhibit high flexibility and stretchability. Accurate prediction of their mechanical behaviors requires advanced hyperelastic constitutive models incorporating multiple parameters. However,identifying multiple parameters under complex deformations remains a challenge, especially with limited observed data. In this study, we develop a physics-informed neural network(PINN) framework to identify material parameters and predict mechanical fields,focusing on compressible Neo-Hookean materials and hydrogels. To improve accuracy, we utilize scaling techniques to normalize network outputs and material parameters. This framework effectively solves forward and inverse problems, extrapolating continuous mechanical fields from sparse boundary data and identifying unknown mechanical *** explore different approaches for imposing boundary conditions(BCs) to assess their impacts on accuracy. To enhance efficiency and generalization, we propose a transfer learning enhanced PINN(TL-PINN), allowing pre-trained networks to quickly adapt to new scenarios. The TL-PINN significantly reduces computational costs while maintaining accuracy. This work holds promise in addressing practical challenges in soft material science, and provides insights into soft material mechanics with state-of-the-art experimental methods.

关键词： 35Q74 74A20 74B20 74G75 inverse problem O242 O343 parameter identification physics-informed neural network (PINN) soft material transfer learning

A RAPID FLUORIMETRIC DETERMINATION OF TYROSINE IN SERUM BY THE REACTION WITH CERIUM (Ⅳ)

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Chinese Chemical Letters 1993年第5期4卷 435-438页

作者： Nian Qin JIE, jing He YANG and xue fang LIU Department of chemistry, Shandong University, Jinan, 250100

A fluorimetric method for the determination of tyrosine in serum was proposed. The fluoriscence intensity is a linear function of tyrosine content in the range 0-1. 44ug/ml. The percentage of recovery was satisfactory.

关键词： Th IV A RAPID FLUORIMETRIC DETERMINATION OF TYROSINE IN SERUM BY THE REACTION WITH CERIUM

Strengthening and control of second-phase particle precipitation in ferritic/austenitic/martensitic heat-resistant alloys:a review

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Journal of Iron and Steel Research International 2024年第1期31卷 3-23页

作者： xue-cheng Peng Han-jie Guo Xin-fang Zhang Yi-wa Luo Ye Sun jing Guo Rong-guang Yang Xiao-dan Zheng School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China Beijing Key Laboratory of Special Melting and Preparation of High-End Metal Materials University of Science and Technology Beijing(USTB)Beijing100083China Beijing Shougang Gitane New MATERIALS Co. Ltd.Beijing102206China

Heat-resistant alloys with excellent mechanical properties are widely used in various fields,and further improvement in their properties is essential to meet the requirements in new-generation advanced supercritical boilers,nuclear reactors,superheaters,and other new materials *** effectively enhance the comprehensive performance of heat-resistant alloys,second-phase particle strengthening has been widely studied,and in the face of different service envi-ronments of advanced heat-resistant steels,the selection of suitable second-phase particles is essential to maximize the performance of these *** this end,three major types of reinforcing phases in heat-resistant alloys such as carbides,rare earth oxides,and intermetallic compounds are summarized.A comparative analysis of the precipitation behavior of the reinforcing phases with different types as well as the risks and means of controlling their use in service,is *** parameters for the application of various types of second-phase particles in heat-resistant alloys are provided to support the design and preparation of new ultrahigh-performance heat-resistant alloys.

关键词： Heat-resistant alloy Second-phase particle Carbide Rare earth oxide Intermetallic compound Strengthening

A review on plasmonic enhancement of activity and selectivity in electrocatalytic CO_(2)reduction

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Frontiers in Energy 2024年第4期18卷 399-417页

作者： jing xue Zhenlin CHEN Yuchao ZHANG Jincai ZHAO Key Laboratory of Photochemistry Beijing National Laboratory for Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Utilizing plasmonic effects to assist electrochemical reactions exhibits a huge potential in tuning the reaction activities and product selectivity,which is most appealing especially in chemical reactions with multiple products,such as CO_(2)reduction reaction(CO_(2)RR).However,a comprehensive review of the development and the underlying mechanisms in plasmon-assisted electrocatalytic CO_(2)RR remains few and far ***,the fundamentals of localized surface plasmonic resonance(LSPR)excitation and the properties of typical plasmonic metals(including Au,Ag,and Cu)are ***,the potential mechanisms of plasmonic effects(such as hot carrier effects and photothermal effects)on the reaction performance in the field of plasmon-assisted electrocatalytic CO_(2)RR are summarized,which provides directions for the future development of this *** is concluded that plasmonic catalysts exhibit potential capabilities in enhancing CO_(2)RR while more in situ techniques are essential to further clarify the inner mechanisms.

关键词： localized surface plasmonic resonance(LSPR)effect plasmonic metals CO_(2)reduction reaction(CO_(2)RR) hot carrier effect photothermal effect

Lorentz violation induces isospectrality breaking in Einstein-bumblebee gravity theory

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Science China(Physics,Mechanics & Astronomy) 2024年第8期67卷 87-96页

作者： Wentao Liu Xiongjun fang Jiliang jing Jieci Wang Department of Physics Key Laboratory of Low Dimensional Quantum Structures and Quantum Control of Ministry of EducationSynergetic Innovation Center for Quantum Effects and ApplicationsHunan Normal UniversityChangsha 410081China

In this study,we investigate the quasinormal modes(QNMs)of a Lorentz-violating spacetime,factoring in a cosmological constant,within the framework of Einstein-bumblebee *** findings reveal that the interaction of spacetime with an anisotropic bumblebee field imparts distinct contributions to the axial and polar sectors of the vector *** subsequently breaks the isospectrality typically observed in vector *** evidence strongly indicates isospectral breaking in the vector modes of Einstein-bumblebee black holes:a pronounced breakage in the real part of the frequencies,while the imaginary component seems less *** isospectral breaking indicates the existence of two different waveforms in the Ringdown phase of the black hole,which provides a potential signal of quantum gravity observable in current experiments.

关键词： Lorentz-violating isospectral breaking quasinormal modes

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SETD2 in cancer: functions, molecular mechanisms, and therapeutic regimens

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Cancer Biology & Medicine 2024年第9期21卷 725-730页

作者： Yawen Weng jing xue Ningning Niu State Key Laboratory of Systems Medicine for Cancer Stem Cell Research Center Ren Ji Hospital Shanghai Cancer InstituteShanghai Jiao Tong University School of Medicine

In recent years, the histone methyltransferase SET domain containing 2 (SETD2) has garnered significant attention for its involvement in carcinogenesis. Herein we aim to summarize the research advances regarding SETD2 in tumors,elucidate the role in global epigenetic regulation, highlight potential therapeutic regimens for patients with SETD2 deficiency, and outline future research directions.

关键词： METHYLATION

Surface reconstruction of heterostructures in alkaline medium towards enhanced electrocatalytic hydrogen evolution

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Rare Metals 2024年第6期43卷 2636-2647页

作者： Ming-Yang Yang Ji Yuan xue-Lian Fu jing-jing Chen jing Hu Zhou-Guang Lu Chen Liu Guangdong Research Center for Interfacial Engineering of Functional Materials Shenzhen Key Laboratory of Polymer Science and TechnologyShenzhen Key Laboratory of Energy Electrocatalytic MaterialsCollege of Materials Science and EngineeringShenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Interfacial Science and Engineering of Materials Department of Materials Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China

Constructing heterostructures has proved to be a successful strategy to fabricate electrocatalysts with high efficiency for water ***,the structure evolution in alkaline hydrogen evolution reaction lacks investigation and the specific active center remains ***,we take the well-designed Ni_(3)S_(2)@VO_(2) heterostructures as a model to investigate the electrocatalytic activity and the surface reconstruction process of heterostructure catalysts in alkaline *** Ni_(3)S_(2)@VO_(2) heterostructures,with Ni_(3)S_(2) nanorods as the core and VO_(2) nanoflakes as the shell,coupled with the high conductive Ni_(3)S_(2),the hydrophilic VO_(2) and modulated electronic structures at the interfaces,exhibited prominent activity and superior stability at various current ***,the ex-situ characterizations confirmed that the surface reconstruction from Ni_(3)S_(2)@VO_(2) into Ni_(3)S_(2)@amorphous-Ni(OH)_(2) in alkaline media could optimize the water dissociation barrier and exposed large active area,thereby contributing to improved electrocatalytic *** study not only introduces novel high-performance electrocatalysts for hydrogen evolution reaction(HER),but also provides a new avenue for re-examining hetero-structural catalysts in alkaline solutions.

关键词： Heterostructures Ni_(3)S_(2)@VO_(2) Surface reconstruction Water dissociation Alkaline hydrogen evolution

Intensified warming suppressed the snowmelt in the Tibetan Plateau

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Advances in Climate Change Research 2024年第3期15卷 452-463页

作者： Xiang LI Peng CUI xue-Qin ZHANG fang ZHANG Key Lab of Land Surface Pattern and Simulation Institute of Geographic Sciences and Natural Resources ResearchBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China China‒Pakistan Joint Research Center on Earth Sciences Chinese Academy of Sciences and Higher Education CommissionIslamabad 45320Pakistan

Understanding how hydrological factors interrelate is crucial when examining the impact of climate warming on ***,these connections are often overlooked,leading to an unclear relationship between temperature and *** study investigates the complex interplay between temperature and snowmelt in the Tibetan Plateau from 1961 to 2020,focusing on how extreme high-temperature events affect the frequency of extreme *** a structural equation model,we detected three temperature-related factors that predominantly influenced snowmelt and extreme *** annual average temperature was found to have a significant indirect impact on snowmelt,mediated by changes in snowfall,snow depth and snow *** contrast,high-temperature days(daily maximum temperatures exceeding the 90th percentile)and heat waves(at least three consecutive high-temperature days)negatively affected extreme snowmelt directly or *** direct effect of increasing extreme temperature events was associated with an earlier onset of high-temperature periods,which accelerated snowmelt and shortened the duration of extreme snowmelt ***,the reduction in snow cover owing to warming emerged as a main factor suppressing snowmelt and extreme snowmelt *** also revealed spatiotemporal variations in the temperature‒snowmelt relationship that highly depended on changes in snowmelt *** study elucidated why warming suppresses snowmelt and extreme snowmelt events in the Tibetan Plateau,highlighting the mediating roles of snow-related and phenological *** findings will provide scientific support for climate simulation and water management policymaking in alpine regions worldwide.

关键词： Climate change Extreme temperature Snowmelt Structural equation model Tibetan Plateau