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Bromine and oxygen redox species mediated highly selective electro-epoxidation of styrene

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Organic Chemistry Frontiers 2022年第2期9卷 436-444页

作者： Yuchi Zhang Asma Iqbal Jiantao Zai Shu-Yu Zhang Hongran Guo Xuejiao Liu ibrahim ul islam Hira Fazal Xuefeng Qian Shanghai Electrochemical Energy Devices Research Center School of Chemistry and Chemical Engineering and State Key Laboratory of Metal Matrix CompositesShanghai Jiao Tong University Shanghai200240P.R.China

Olefin epoxidation is an essential transformation and arouses great interest among the scientific community for the key role of epoxide in the chemical *** methods suffer from harmful oxidants and require harsh operating conditions and complex separation ***-epoxidation through bromine redox reactions is an eco-friendly ***,the lack of efficient electrodes always limits the selectivity of epoxidation and results in massive energy ***,we found that GF-CoS_(2)/CoS heterostructures anchored on graphite felt(GF-CoS_(2)/CoS)can efficiently facilitate the generation of bromine redox species on the *** synergistic cooperation between the bromine redox species and oxygen redox species(generated on a graphite rod cathode)can establish a benign electro-epoxidation system for olefin substrates in an ambient *** the optimized reaction conditions,the epoxidation of styrene can achieve a yield of 97% at 30 mA cm^(-2).Importantly,the applied voltage(4-5 V)is roughly half of the Pt-based electrode system(7.8-9.3 V),hence,saving half of the *** demonstrated that our proposed strategy could also be applied to other *** of the simple,sustainable,and economic advantages of the epoxidation process,we believe this strategy is highly desirable for technical applications.

关键词： redox epoxidation styrene

高稳定性的三线态-三线态湮灭上转换发光无机有机复合材料及其在发光型太阳能聚光器上的应用

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高稳定性的三线态-三线态湮灭上转换发光无机有机复合材料及其在...

Classifying rockburst with confidence:A novel conformal prediction approach

中国化学会第十六届全国光化学学术讨论会（2019）

作者：杨雪婷 ibrahim ul islam 陆军北京化工大学

三线态-三线态湮灭上转换发光(TTA-UC)是一种重要的光谱转换现象。TTA-UC主要由光敏剂和湮灭剂组成。通过激发三线态光敏剂从基态跃迁到第一激发单线态,经系间窜越至激发三线态,再经过给受体分子间的三线态-三线态能量传递(TTET)过程产... 详细信息

三线态-三线态湮灭上转换发光(TTA-UC)是一种重要的光谱转换现象。TTA-UC主要由光敏剂和湮灭剂组成。通过激发三线态光敏剂从基态跃迁到第一激发单线态,经系间窜越至激发三线态,再经过给受体分子间的三线态-三线态能量传递(TTET)过程产生受体激发三线态,两个处于激发三线态的受体分子发生三线态三线态湮灭(TTA),一个受体分子弛豫到基态,而另一受体分子跃迁至单重激发态,发射出上转换荧光。本文将TTA-UC能量给受体蒽与菲分子引入到LDHs(层状复合金属氢氧化物,又称水滑石)纳米层间,成功构筑了Ac&Ph@PTBEM/LDHs组装复合薄膜,实现了上转换体系的固载化,利用LDHs的二维限域效应,有效的提高了体系的光化学稳定性、能量转移以及上转换发光效率。用770nm的光激发复合薄膜中的蒽分子,通过TTET将能量转移至菲分子,后者将有效的发射出389nm的光子,蓝移381nm。将制备的超薄膜作为发光型太阳能聚光器应用于硅太阳能电池,与无太阳能聚光器相比,硅太阳能电池的光电转化效率提高了16倍,体现了该组装复合薄膜作为太阳能转换器材料的潜在应用。

关键词：三线态三线态湮灭上转换发光 LDHs 发光型太阳能聚光器

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International Journal of Mining Science and Technology 2024年第1期34卷 51-64页

作者： Bemah ibrahim Isaac Ahenkorah University of South Australia UniSA STEMSA 5000Australia

The scientific community recognizes the seriousness of rockbursts and the need for effective mitigation *** literature reports various successful applications of machine learning(ML)models for rockburst assessment;however,a significant question remains unanswered:How reliable are these models,and at what confidence level are classifications made?Typically,ML models output single rockburst grade even in the face of intricate and out-of-distribution samples,without any associated confidence *** the susceptibility of ML models to errors,it becomes imperative to quantify their uncertainty to prevent consequential *** address this issue,we propose a conformal prediction(CP)framework built on traditional ML models(extreme gradient boosting and random forest)to generate valid classifications of rockburst while producing a measure of confidence for its *** proposed framework guarantees marginal coverage and,in most cases,conditional coverage on the test *** CP was evaluated on a rockburst case in the Sanshandao Gold Mine in China,where it achieved high coverage and efficiency at applicable confidence ***,the CP identified several“confident”classifications from the traditional ML model as unreliable,necessitating expert verification for informed *** proposed framework improves the reliability and accuracy of rockburst assessments,with the potential to bolster user confidence.

关键词： Rockburst Machine learning Uncertainty quantification Conformal prediction

Enhancing Canola Yield and Photosynthesis under Water Stress with Hydrogel Polymers

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Phyton-International Journal of Experimental Botany 2024年第7期93卷 1623-1645页

作者： Elham A.Badr Gehan Sh.Bakhoum Mervat Sh.Sadak ibrahim Al-Ashkar Mohammad Sohidul islam Ayman El Sabagh Magdi T.Abdelhamid Field Crops Research Department National Research CentreCairo12622Egypt Botany Department National Research CentreCairo12622Egypt Plant Production Department College of Food and Agriculture SciencesKing Saud UniversityRiyadh12271Saudi Arabia Department of Agronomy Hajee Mohammad Danesh Science and Technology UniversityDinajpur5200Bangladesh Department of Field Crops Faculty of AgricultureSiirt UniversitySiirt56100Turkey Department of Agronomy Faculty of AgricultureKafrelsheikh UniversityKafrelsheikh33516Egypt Department of Research Centers Montana State UniversityBozemanMT 59717USA

While Egypt’s canola production per unit area has recently grown,productivity remains low,necessitating increased *** are water-absorbent polymer compounds that can optimize irrigation schedules by increasing the soil’s ability to retain ***,twoﬁeld experiments were conducted to examine hydrogel application to sandy soil on canola growth,biochemical aspects,yield,yield traits,and nutritional quality of yielded seeds grown under water deﬁcit stress *** experiments were conducted by arranging a split-plot layout in a randomized complete block design(RCBD)with three times replications of each *** water stress at 75%or 50%of crop evapotranspiration(ETc)lowered chlorophyll a,chlorophyll b,caro-tenoids,and total pigments content,indole-3-acetic acid,plant development,seed yield,and oil and total carbo-hydrates of seed yield,hydrogel treatment enhanced all of the traits mentioned ***,hydrogel enhanced to gather compatible solutes(proline,amino acids,total soluble sugars),phenolics content in leaves,seed protein,and crop water productivity,which increased while the plants were under water *** results revealed that the full irrigation(100%ETc)along with hydrogel compared to water-stressed(50%ETc)led to enhanced seed yield(kg ha^(-1)),Oil(%),and Total carbohydrates(%)of rapeseed by 57.1%,11.1%and 15.7%,***,under water-stressed plots with hydrogel exhibited enhancement by 10.0%,3.2%and 5.1%in seed yield(kg ha^(-1)),oil(%),and total carbohydrates(%)of rapeseed by 57.1%,11.1%and 15.7%,respec-tively compared to *** a result,the use of hydrogel polymer will be a viable and practical solution for increasing agricultural output under water deﬁcit stress situations.

关键词： Hydrogel oil osmolytes rapeseed yield water stress

A numerical investigation into the effect of altering compression ratio, injection timing, and injection duration on the performance of a diesel engine fuelled with diesel-biodiesel-butanol blend

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Clean Energy 2024年第5期8卷 73-96页

作者： Abdulkarim Youssef Amr ibrahim Mechanical Engineering Department Beirut Arab University115020 BeirutLebanon Mechanical Engineering Department Alexandria UniversityAlex 21544Egypt

Using renewable fuels for diesel engines can reduce both air pollution and dependence on fossil fuels.A computer simulation was constructed to predict the performance,combustion characteristics,and NOx emissions of a diesel engine fuelled with diesel-biodiesel-butanol *** simulation was validated by comparing the modelling results against experimental data and a good agreement between the results was *** fuels used for the validation were diesel(B0),biodiesel(B100),diesel-biodiesel blend(B50),and two diesel-biodiesel-butanol blends with 45%diesel-45%biodiesel-10%butanol(Bu10)and 40%diesel-40%biodiesel-20%butanol(Bu20)by *** results showed that the addition of butanol reduced NOx emissions but deteriorated the engine *** aim of the current work was the numerical optimization of the different parameters to enhance the engine performance while using butanol to decrease NOx *** engine compression ratio(CR)varied from 14 to 24,in increments of *** injection timing(IT)was reduced from 30°before top dead centre(bTDC)to 5°bTDC in increments of 5°.Also,the fuel injection duration(IDur)was extended from 20°to 50°in increments of 10°.Results showed that the increase in the CR improved engine performance for the two investigated fuels,Bu10 and *** maximum engine brake power(BP),thermal efficiency(BTE),and minimum brake-specific fuel consumption(BSFC)of 1.46 kW,32.3%,and 0.273 kg/kWh respectively,were obtained when the Bu10 fuel was injected under the optimum conditions of 24 CR,15°bTDC IT,and 40°*** these optimum conditions,the BP,BTE,and BSFC improved by 3%-3.5%for Bu10 and Bu20 fuel blends compared with the base engine conditions of a CR of 22,30°IDur,and 10°bTDC *** heat release rate during the premixed phase increased when the IT was advanced,while the mixing-controlled combustion phase was enhanced when the IT was *** emissions increased with increasing CR,while both an increase in IDur at con

关键词： compression ratio injection timing injection duration butanol biodiesel diesel

New insights into astrocyte diversity from the lens of transcriptional regulation and their implications for neurodegenerative disease treatments

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Neural Regeneration Research 2024年第11期19卷 2335-2336页

作者： ibrahim Olabayode Saliu Guoyan Zhao Department of Genetics Washington University School of MedicineSt.LouisMOUSA Department of Neurology Department of Pathology and ImmunologyWashington University School of MedicineSt.LouisMOUSA

Astrocytes are a major glial cell type in the central nervous system,and they provide trophic and metabolic support to *** addition to these roles,they play crucial roles in modulating synaptic functions,development,and pruning(Brandebura et al.,2023).Astrocytes become reactive(activated)by undergoing morphological,molecular,and functional alterations in response to neuropathology such as in injuries and neurodegenerative diseases(NDs)(Escartin et al.,2021).

关键词： degenerative injuries

Enteric neuropathy in diabetes:Implications for gastrointestinal function

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World Journal of Gastroenterology 2024年第22期30卷 2852-2865页

作者： Mona Mohamed ibrahim Abdalla Department of Human Biology School of MedicineInternational Medical UniversityBukit Jalil 57000Kuala LumpurMalaysia

Diabetes,commonly known for its metabolic effects,also critically affects the enteric nervous system(ENS),which is essential in regulating gastrointestinal(GI)motility,secretion,and *** development of diabetes-induced enteric neuropathy can lead to various GI dysfunctions,such as gastroparesis and irregular bowel habits,primarily due to disruptions in the function of neuronal and glial cells within the ENS,as well as oxidative stress and *** editorial explores the pathophysiological mechanisms underlying the development of enteric neuropathy in diabetic ***,it discusses the latest advances in diagnostic approaches,emphasizing the need for early detection and intervention to mitigate GI complications in diabetic *** editorial also reviews current and emerging therapeutic strategies,focusing on pharmacological treatments,dietary management,and potential neuromodulatory ***,this editorial highlights the necessity of a multidisciplinary approach in managing enteric neuropathy in diabetes,aiming to enhance patient quality of life and address a frequently overlooked complication of this widespread disease.

关键词： Diabetic neuropathy Gastrointestinal Insulin resistance Diabetes Enteric nervous system Enteric neuropathy

Numerical modelling and simulation analysis of wind blades:a critical review

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Clean Energy 2024年第1期8卷 261-279页

作者： ibrahim Alrowwad Xiaojia Wang Ningling Zhou Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China

Wind energy has emerged as a promising renewable energy source and wind turbine technology has developed rapidly in recent *** wind turbine performance depends heavily on the design and optimization of wind *** work offers a critical evaluation of the state of the art in the field of numerical modelling and simulation analysis,which have become crucial for the design and optimization of wind *** evaluation of the literature includes considerable research on the application of numerical methods for the structural and aerodynamic performance of wind blades under various operating situations,as well as for analysis and optimization of wind *** article illustrates how numerical techniques can be used to analyse wind blade performance and maximize design *** study of blade performance under various wind conditions has also been made possible through the use of simulation analysis,thus enhancing the efficiency and dependability of wind *** in wind turbine efficiency and dependability,and ultimately the move towards a more sustainable energy future,will be greatly helpful for the development of numerical modelling and simulation techniques.

关键词： wind blades simulations optimization numerical analysis mathematical modelling performance

Relational Turkish Text Classification Using Distant Supervised Entities and Relations

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Computers, Materials & Continua 2024年第5期79卷 2209-2228页

作者： Halil ibrahim Okur Kadir Tohma Ahmet Sertbas Department of Computer Engineering Faculty of Engineering and Natural SciencesIskenderun Technical UniversityHatay31200Turkey Department of Computer Engineering Faculty of EngineeringIstanbul University-CerrahpasaIstanbul34310Turkey

Text classification,by automatically categorizing texts,is one of the foundational elements of natural language processing *** study investigates how text classification performance can be improved through the integration of entity-relation information obtained from the Wikidata(Wikipedia database)database and BERTbased pre-trained Named Entity Recognition(NER)*** on a significant challenge in the field of natural language processing(NLP),the research evaluates the potential of using entity and relational information to extract deeper meaning from *** adopted methodology encompasses a comprehensive approach that includes text preprocessing,entity detection,and the integration of relational *** conducted on text datasets in both Turkish and English assess the performance of various classification algorithms,such as Support Vector Machine,Logistic Regression,Deep Neural Network,and Convolutional Neural *** results indicate that the integration of entity-relation information can significantly enhance algorithmperformance in text classification tasks and offer new perspectives for information extraction and semantic analysis in NLP *** of this work include the utilization of distant supervised entity-relation information in Turkish text classification,the development of a Turkish relational text classification approach,and the creation of a relational *** demonstrating potential performance improvements through the integration of distant supervised entity-relation information into Turkish text classification,this research aims to support the effectiveness of text-based artificial intelligence(AI)***,it makes significant contributions to the development ofmultilingual text classification systems by adding deeper meaning to text content,thereby providing a valuable addition to current NLP studies and setting an important reference point for future research.

关键词： Text classification relation extraction NER distant supervision deep learning machine learning