检索结果-南通市图书馆

Spatial construction of ultrasmall Pt-decorated 3D spinel oxidemodified N-doped graphene nanoarchitectures as high-efficiency methanol oxidation electrocatalysts

引用

Rare Metals 2024年第1期43卷 186-197页

作者： Qi Zhang Min-Min Yan Wen-Fa Du Chen-Yu Yin Jian Zhang Lu Yang Yun-Qing Kang Hai-Yan He hua-jie huang College of Mechanics and Materials Hohai UniversityNanjing 210098China New Energy Technology Engineering Lab of Jiangsu Province College of ScienceNanjing University of Posts&Telecommunications(NUPT)Nanjing 210023China International Center for Materials Nanoarchitectonics(WPIMANA) National Institute for Materials ScienceTsukuba 305-0044IbarakiJapan

Direct methanol fuel cell technology recently becomes the focus of both academic and engineering circles,which stimulates the exploitation and utilization of advanced electrode catalysts with high activity and long ***,we demonstrate a robust bottom-up approach to the spatial construction of three-dimensional(3D) spinel manganese-cobalt oxide-modified N-doped graphene nanoarchitectures decorated with ultrasmall Pt nanoparticles(Pt/MnCo_(2)O_(4)-NG) via a controllable selfassembly *** incorporation of MnCo_(2)O_(4)nanocrystals provides abundant hydroxyl sources to promote the oxidative removal of CO-like byproducts on Pt sites,while the existence of 3D porous N-doped graphene networks facilitates the transportation of both ions and electrons in the hybrid system,thus giving rise to remarkable synergetic coupling effects during the methanol oxidation ***,the optimized Pt/MnCo_(2)O_(4)-NG nano architecture expres ses exceptional electrocatalytic properties with a large electrochemically active surface area of 99.5 m^(2)·g^(-1),a high mass activity of1508.3 mA·mg^(-1),strong toxicity resistance and reliable long-term durability,which have obvious competitive advantages over those of conventional Pt/carbon black,Pt/carbon nano tube,Pt/graphene,and Pt/N-doped graphene catalysts with the same Pt usage.

关键词： Platinum MnCo_(2)O_(4) 3D graphene Electrocatalysts Methanol oxidation

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Nanosized Rh grown on single-walled carbon nanohorns for efficient methanol oxidation reaction

引用

Rare Metals 2022年第6期41卷 2108-2117页

作者： Xiang-jie Guo Qi Zhang Ya-Nan Li Yang Chen Lu Yang Hai-Yan He Xing-Tao Xu hua-jie huang Collegeof Mechanics and Materials Hohai University Nanjing 210098China International Center for Materials Nanoarchitectonics(WPI-MANA) National Institute for Materials ScienceIbaraki 305-0044Japan

Reasonable design and controllable synthesis of non-Pt catalysts with high methanol oxidation activity are regarded as a valid way to promote the large-scale com-mercial applications of direct methanol fuel cells(DMFCs).Herein,we develop a convenient and cost-ef-fective approach to the successful fabrication of nanosized Rh grown on single-walled carbon nanohorns(Rh/SWCNH)as anode catalysts for *** unique architectural configuration endows the as-obtained hybrids with a series of intriguing structural merits,including large specific surface areas,abundant opened holes,optimized electronic structures,homogeneous Rh dispersion,and good electrical *** a consequence,the resulting Rh/SWCNH catalysts exhibit exceptional elec-trocatalytic properties in terms of a large electrochemically active surface area of 102.5 m^(2)·g^(-1),a high mass activity of 784.0 mA·mg^(-1),as well as reliable long-term durability towards the methanol oxidation reaction in alkaline media,thereby holding great potential as alternatives for com-mercial Pt/carbon black and Pd/carbon black catalysts.

关键词： Rhodium Carbon nanohorns Electrocatalysts Methanol oxidation Fuel cells

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Distributed Nash Equilibrium Seeking on Compact Action Sets over Jointly Strongly Connected Switching Networks

引用

Journal of Systems Science & Complexity 2024年第1期37卷 63-81页

作者： HE Xiongnan huang jie Department of Mechanical and Automation Engineering The Chinese University of Hong KongHong Kong 999077China.

This paper studies the distributed Nash equilibrium seeking(DNES)problem for games whose action sets are compact and whose network graph is switching satisfying the jointly strongly connected *** keep the actions of all players in their action sets all the time,one has to resort to the projected gradient-based *** the assumption that the unique Nash equilibrium is the unique equilibrium of the pseudogradient system,an algorithm is proposed that is able to exponentially find the Nash ***,the authors also consider the distributed Nash equilibrium seeking problem for games whose actions are governed by high-order integrator dynamics and belong to some compact *** examples are used to illustrate the proposed approach.

关键词： Compact action sets jointly strongly connected switching graphs Nash equilibrium seeking projected gradient-based algorithm.

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

Probabilistic back-analysis of rainfall-induced landslides for slope reliability prediction with multi-source information

引用

Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3575-3594页

作者： Shui-hua Jiang Hong-Hu jie Jiawei Xie Jinsong huang Chuang-Bing Zhou School of Infrastructure Engineering Nanchang UniversityXuefu Road 999Nanchang330031China Discipline of Civil Surveying and Environmental EngineeringFaculty of Engineering and Built EnvironmentThe University of NewcastleCallaghanNSW2308Australia

Probabilistic back-analysis is an important means to infer the statistics of uncertain soil parameters,making the slope reliability assessment closer to the engineering ***,multi-source information(including test data,monitored data,field observation and slope survival records)is rarely used in current probabilistic *** the probabilistic back-analysis of spatially varying soil parameters and slope reliability prediction under rainfalls by integrating multi-source information is a challenging task since thousands of random variables and high-dimensional likelihood function are usually *** this paper,a framework by integrating a modified Bayesian Updating with Subset simulation(mBUS)method with adaptive Conditional Sampling(aCS)algorithm is established for the probabilistic back-analysis of spatially varying soil parameters and slope reliability *** this framework,the high-dimensional probabilistic back-analysis problem can be easily tackled,and the multi-source information(*** pressure heads and slope survival records)can be fully used in the back-analysis.A real Taoyuan landslide case in Taiwan,China is investigated to illustrate the effectiveness and performance of the established *** findings show that the posterior knowledge of soil parameters obtained from the established framework is in good agreement with the field ***,the updated knowledge of soil parameters can be utilized to reliably predict the occurrence probability of a landslide caused by the heavy rainfall event on September 12,2004 or forecast the potential landslides under future rainfalls in the Fuhsing District of Taoyuan City,Taiwan,China.

关键词： Rainfall-induced landslide Spatial variability Probabilistic back-analysis Slope reliability analysis Bayesian updating

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Aberrant protamination in sperm correlates to anomalous nuclear and cytoplasmic architectures in infertile males with sperm dysmorphology

引用

Asian Journal of Andrology 2024年第2期26卷 183-188页

作者： huan Jiang Chu-jie huang Department of Reproductive Endocrinology Longgang District Maternity&Child Healthcare Hospital of Shenzhen City(Longgang Maternity and Child Institute of Shantou University Medical College)Shenzhen 518172China Institute of Reproductive Immunology College of Life Science and TechnologyJinan UniversityGuangzhou 510632China

Aberrant sperm protamination is linked to sperm dysmorphology and nuclear chromatin ***,its effects on sperm cytoplasmic maturation remain largely *** relationships of protamines,sperm morphology,DNA damage,and cytoplasmic remodeling were illustrated in this study to provide fresh perspectives on the mechanisms of male infertility.A total of 205 infertile males were allocated into 5 groups according to the percentage of spermatozoa exhibiting abnormal morphology within their *** concentration,motility,abnormal sperm morphology,cytoplasmic droplets(CDs),and excess residual cytoplasm(ERC)were analyzed according to the World Health Organization manual(2010).Sperm nuclear vacuoles(NVs)were determined by propidium iodide(PI)*** protamine expressions(P1 and P2)were detected by western *** damage was measured by acridine orange test(AOT)to calculate the proportion of sperm with single-strand DNA breaks(SSBs).Our data showed that sperm concentration and motility in infertile males significantly decreased with the severity of abnormal sperm morphology(both P<0.01).P1 level,P1/P2 ratio,and SSB rate increased with the severity of sperm dysmorphology,whilst the P2 level decreased(all P

关键词： abnormal sperm morphology excess residual cytoplasm male infertility protamines sperm DNA damage sperm nuclear vacuoles

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Fabrication and properties of lightweight zirconia with fine closed porosity

引用

Journal of Iron and Steel Research International 2024年第6期31卷 1449-1458页

作者： Yi-bo Zhang hua-zhi Gu Lv-ping Fu Ao huang Mei-je Zhang The State Key Laboratory of Refractories and Metallurgy Wuhan University of Science and TechnologyWuhan 430081HubeiChina

Lightweight refractory materials with thermal insulation properties and erosion resistance are advantageous for hightemperature *** zirconia refractories were prepared using starch as a pore-forming agent,basic magnesium carbonate as a stabilizer,and nano-zirconia as an *** effects of the nano-zirconia content on the pore and thermal insulation properties of the lightweight zirconia refractories were investigated based on the porosity,phase composition,microstructure,and thermal ***-zirconia was shown to have a high surface energy,and its addition effectively increased the driving force for sintering,reduced the sintering temperature,and promoted the sintering reaction,thereby reducing the apparent porosity and improving the density of the prepared *** to the superplasticity of nano-zirconia,the surface stress caused plastic deformation between particles,which increased the migration rate of grain boundaries and trapped more gas inside the material before it diffused to the surface,thereby enhancing the closed porosity of the *** presence of closed pores could extend the thermal conduction path,decrease the conduction rate,and hinder the conduction effect to effectively reduce the thermal conductivity of the *** a nano-zirconia content of 0.75 wt.%,the prepared lightweight zirconia had the highest closed porosity and the lowest thermal *** apparent porosity,closed porosity,and total porosity of the material were 2.8%,7.0%,and 9.8%,respectively,and the thermal conductivity at 800℃was 1.37 W m^(-1)k^(-1).

关键词： Sintering Nano-zirconia Closed pore:Thermal conductivity Refractory material

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

End-to-end data-driven modeling framework for automated and trustworthy short-term building energy load forecasting

引用

Building Simulation 2024年第8期17卷 1419-1437页

作者： Chaobo Zhang jie Lu Jiahua huang Yang Zhao Department of the Built Environment Eindhoven University of TechnologyEindhovenThe Netherlands Energy Efficient Cities Initiative Department of EngineeringUniversity of CambridgeCambridgeUK Institute of Refrigeration and Cryogenics Zhejiang UniversityHangzhouChina Institute of Green Building and Engineering Design Zhejiang Province Institute of Architectural Design and Research Co.Ltd.HangzhouChina Key Laboratory of Clean Energy and Carbon Neutrality of Zhejiang Province Jiaxing Research InstituteZhejiang UniversityJiaxingChina

Conventional automated machine learning(AutoML)technologies fall short in preprocessing low-quality raw data and adapting to varying indoor and outdoor environments,leading to accuracy reduction in forecasting short-term building energy ***,their predictions are not transparent because of their black box ***,the building field currently lacks an AutoML framework capable of data quality enhancement,environment self-adaptation,and model *** address this research gap,an improved AutoML-based end-to-end data-driven modeling framework is *** optimization is applied by this framework to find an optimal data preprocessing process for quality improvement of raw *** bridges the gap where conventional AutoML technologies cannot automatically handle missing data and outliers.A sliding window-based model retraining strategy is utilized to achieve environment self-adaptation,contributing to the accuracy enhancement of AutoML ***,a local interpretable model-agnostic explanations-based approach is developed to interpret predictions made by the improved *** overcomes the poor interpretability of conventional AutoML *** performance of the improved framework in forecasting one-hour ahead cooling loads is evaluated using two-year operational data from a real *** is discovered that the accuracy of the improved framework increases by 4.24%–8.79%compared with four conventional frameworks for buildings with not only high-quality but also low-quality operational ***,it is demonstrated that the developed model interpretation approach can effectively explain the predictions of the improved *** improved framework offers a novel perspective on creating accurate and reliable AutoML frameworks tailored to building energy load prediction tasks and other similar tasks.

关键词： building energy load forecasting end-to-end data-driven modeling automated machine learning Bayesian optimization model retraining model interpretation

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nanoforming of transferred metal contacts for enhanced twodimensional field effect transistors

引用

Nano Research 2024年第4期17卷 3210-3216页

作者： Shuoheng Xu Zheng huang jie Guan Yaowu Hu The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Physics Southeast UniversityNanjing 211189China

Two-dimensional transition metal chalcogenides(2D-TMDs)have attracted much attention because of their unique layered structure and physical properties for transistor *** transferred metal contacts on these low-dimensional materials or their homogeneous and heterogeneous multilayers have generated huge interest to avoid deposition *** this paper,we show that there are large physical gaps at both the edge contact and surface contact between the transferred electrodes and the 2D materials.A method called laser shock induced superplastic deformation(LSISD)is proposed to tackle this issue and enhance the performance of the *** enhancement mechanism was investigated by molecular dynamics(MD)simulations of the nanoforming process,atomic force microscopy(AFM),scanning electron microscopy(SEM),transmission electron microscopy(TEM)characterizations of the interfaces,and density functional theory(DFT)*** force effect of laser shock can reduce the contact gap between metals and *** electrical performances of the transistors before and after LSISD,along with MD simulations,are used to find the optimal process *** addition,this paper applies the LSISD method to the short-channel MoS_(2)/graphene vertical transistors to show potential improvement in interface contact and electrical *** paper demonstrates the first report on using mechanical force induced by laser shock to enhance metal–semiconductor interfaces and transistor performances.

关键词： laser shock nanoforming metal-semiconductor contact electronics two-dimensional transistors

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

A Bio-inspired Mutual-hook Strategy for the Soft Finger to Improve Load-bearing Capacity and Grasping Stability

引用

Journal of Bionic Engineering 2024年第3期21卷 1290-1304页

作者： jie huang Lingjie Gai Xiaofeng Zong Yunquan Li School of Automation China University of GeosciencesWuhan430074China Hubei Key Laboratory of Advanced Control and Intelligent Automation for Complex System Wuhan430074China The Shien-Ming Wu School of Intelligent Engineering South China University of TechnologyGuangzhou510641China

Soft grippers have great potential applications in daily life,since they can compliantly grasp soft and delicate ***,the highly elastic fingers of most soft grippers are prone to separate from each other while grasping objects due to their low stiffness,thus reducing the grasping stability and load-bearing *** tackle this problem,inspired from the venus flytrap plant,this work proposes a mutual-hook mechanism to restrain the separation and improve the grasping performance of soft *** novel soft gripper design consists of three modules,a soft finger-cot,two Soft Hook Actuators(SHAs)and two sliding ***,the soft finger-cot covers on the soft finger,increasing the contact area with the target object,two SHAs are fixed to the left and right sides of the finger-cot,and the sliding mechanisms are designed to make SHAs stretch *** demonstrate that the proposed design can restrain the separation of soft fingers substantially,and the soft fingers with the finger-cots can grasp objects three times heavier than the soft fingers without the proposed *** proposed design can provide invaluable insights for soft fingers to restrain the separation while grasping,thus improving the grasping stability and the load-bearing capacity.

关键词： Soft robotics Soft bionic finger-cot Soft hook actuator Grasping stability Load-bearing capacity

来源：

维普期刊数据库评论

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

A Mean-Field Game for a Forward-Backward Stochastic System With Partial Observation and Common Noise

引用

IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 746-759页

作者： Pengyan huang Guangchen Wang Shujun Wang hua Xiao the School of Control Science and Engineering Shandong University the School of Statistics and Mathematics Shandong University of Finance and Economics IEEE the School of Management Shandong University the School of Mathematics and Statistics Shandong University

This paper considers a linear-quadratic(LQ) meanfield game governed by a forward-backward stochastic system with partial observation and common noise,where a coupling structure enters state equations,cost functionals and observation ***,to reduce the complexity of solving the meanfield game,a limiting control problem is *** virtue of the decomposition approach,an admissible control set is *** a filter technique and dimensional-expansion technique,a decentralized control strategy and a consistency condition system are derived,and the related solvability is also ***,we discuss an approximate Nash equilibrium property of the decentralized control ***,we work out a financial problem with some numerical simulations.

关键词： Decentralized control strategy ϵ-Nash equilibrium forward-backward stochastic system mean-field game partial observation

来源：

维普期刊数据库

同方期刊数据库评论

在线全文

学校读者我要写书评

暂无评论

欢迎您,

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案：

请选择收藏分类：

通借通还

欢迎您,

建议与咨询 留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

时间限定

文献类型

馆藏选择

核心期刊

语言

文献类型

帮助

文字说明：

检索规则说明：

检索范例：

分类表

所选分类

限定检索结果

文献类型

馆藏范围

日期分布

学科分类号

主题

机构

作者

语言

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

在线全文

请选择保存的检索档案： 新增检索档案 确定 取消

请选择收藏分类： 新增自定义分类 确定 取消

通借通还

建议与咨询留下您的常用邮箱和电话号码，以便我们向您反馈解决方案和替代方法

请选择保存的检索档案：

请选择收藏分类：