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Temporal study of GRS 1915+105 with rms-flux relation:The importance of magnetic activities in the corona

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Science china(physics,Mechanics & Astronomy) 2010年第S1期53卷 120-124页

作者： han dong1,zhang ShuangNan2 & SONG LiMing2 1 department of engineering physics & center for astrophysics,tsinghua university,beijing 100084,china 2 Key Laboratory of Particle astrophysics,Institute of High Energy physics,Chinese Academy of Sciences,beijing 100049,china 1. department of engineering physics & center for astrophysics Tsinghua University Beijing 100084 China 2. Key Laboratory of Particle astrophysics Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 China

The rms-flux relations for some observations of GRS 1915+105 are *** rms-flux relations of the light curves in only one state,state C or state A,can be described by the simple non-linear model provided zhang;we thus interpret that such a linear relation reflects the relative importance of magnetic instability for X-ray emission in the corona of the system,compared to the thermal viscous instability for the X-ray emission in the accretion *** rms-flux relations for state B are very scattered,possibly because of the dominance of thermal viscous instability for the X-ray emission in the accretion *** complex rms-flux relations for the observations of transitions between two or three states are caused by the combination of the different rms-flux relations of these *** underlying physical processes are the combination of magnetic topology in the corona and thermal viscous instability in the accretion disk.

关键词： rms-flux relation data analysis GRS 1915+105 magnetic instability

Understanding the Thermal Impedance of Silicone Rubber/Hexagonal Boron Nitride Composites as Thermal Interface Materials

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Chinese Journal of Polymer Science 2024年第3期42卷 352-363,I0008页

作者： Yuan Ji Shi-Da han Hong wu Shao-Yun Guo Feng-Shun zhang Jian-Hui Qiu The State Key Laboratory of Polymer Materials engineering Sichuan Provincial Engineering Laboratory of Plastic/Rubber Complex Processing TechnologyPolymer Research InstituteSichuan UniversityChengdu 610065China Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China department of Mechanical engineering Faculty of Systems Science and TechnologyAkita Prefectural UniversityAkita 015-0055Japan

Silicone rubber(SR) composites are most widely used as thermal interface materials(TIMs) for electronics heat dissipation. Thermal impedance as the main bottleneck limiting the performance of TIMs is usually neglected. Herein, the thermal impedance of SR composites loaded with different levels of hexagonal boron nitride(h-BN) as TIMs was elaborated for the first time by the ASTM D 5470 standard test and finite element analysis. It was found that elastic modulus and surface roughness of SR composites increased with the increase of h-BN content, indicating that the conformity was reduced. When the assembly pressure was 0.69 MPa, there existed an optimal h-BN content at which the contact resistance was minimum(0.39 K·cm^(2)·W^(-1)). Although the decreased bond line thickness(BLT) by increasing the assembly pressure was beneficial to reduce the thermal impedance, the proper assembly pressure should be selected to prevent the warpage of the contact surfaces and the increase in contact resistance, according to the compression properties of the SR composites. This study provides valuable insights into fabrication of high-performance TIMs for modern electronic device applications.

关键词： Thermal interface materials Hexagonal boron nitride Thermal impedance Surfaces

Multistimuli-Responsive Luminescent Porous Organic Polymers with Chiroptical Properties and Acid-Induced Degradation

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Chinese Journal of Chemistry 2024年第16期42卷 1886-1894页

作者： Youling He dongyang Fan Liang zhang dong Wang Ting han Rongrong Hu Ben Zhong Tang center for AIE Research Shenzhen Key Laboratory of Polymer Science and TechnologyGuangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Materials Science and EngineeringShenzhen UniversityShenzhenGuangdong 518060China College of physics and Optoelectronic engineering Shenzhen UniversityShenzhenGuangdong 518060China department of Chemistry Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and ReconstructionThe Hong Kong University of Science and TechnologyClear Water BayKowloonHong Kong999077China State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Luminescence from Molecular AggregatesSouth China Universityof TechnologyGuangzhouGuangdong 510640China School of Science and engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhen(CUHK-Shenzhen)Guangdong 518172China

Porous organic polymers(POPs)have attracted great attention in past *** diverse functional POPs have been developed,multistimuli-responsive POPs with excellent aggregate-state luminescence together with good chiroptical properties have rarely been ***,two pairs of Salen-type enantiomeric PoPs with multistimuli-responsive luminescence and chiral features were designed and synthesized by facile polycondensation reactions between polyfunctional aggregation-induced emission luminogen(AlEgen)-containing salicylaldehyde derivatives and chiral *** Salen units in polymer backbones as tetradentate ligands,a series of POP-metal complexes were further *** obtained POPs and metal complexes show good porosity,high thermal stability,and obvious circular dichroism ***,benefiting from the coexistence of AlEgen and Salen units in polymer structures,these POPs exhibit excellent luminescence performance in aggregate states and tunable fluorescence behaviors in response to external stimuli of Zn^(2+)ion,mechanical forces,organic solvent,and *** to the dynamic feature of Schiff base C=N bonds,the present POPs can efficiently undergo hydrolysis reactions under strong acidic conditions to reproduce the AlEgencontaining monomers,and such an acid-induced degradation process can be directly visualized and dynamically monitored via fluorescence *** properties collectively make the POPs candidate materials for applications in heterogeneous asymmetric catalysis,fluorescence sensing,biomedicine,etc.

关键词： Polymers Stimuli-responsive luminescence Porous polymers Chirality Aggregation-induced emission Fluorescence Schiff bases Degradation

Study of the response of 10B-doped MCP to wide-energy range neutrons from eV to MeV

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Nuclear Science and Techniques 2024年第8期35卷 132-141页

作者： Qiang Li Li‑Jiao Wang Xiang‑Biao Qiu jing‑Wen Li Wei Xu Tao Li Ze‑Bin Lin Chang‑Jun Ning Yong‑Hao Chen Rui‑Rui Fan Kang Sun jing‑Yu Tang Rong zhang han‑Tao jing Bo mei Qi An Hao‑Fan Bai Jiang‑Bo Bai Jie Bao Ping Cao Qi‑Ping Chen Zhen Chen Zeng‑Qi Cui An‑Chuan Fan Chang‑Qing Feng Fan‑Zhen Feng Ke‑Qing Gao Min‑Hao Gu Chang‑Cai han Zi‑Jie han Guo‑Zhu He Yong‑Cheng He Yang Hong Yi‑Wei Hu han‑Xiong Huang Wei‑Hua Jia Hao‑Yu Jiang Wei Jiang zhi‑Jie Jiang Zheng‑Yao jin Ling Kang Bo Li Chao Li Gong Li Jia‑Wen Li Xiao Li Yang Li Jie Liu Rong Liu Shu‑Bin Liu Guang‑Yuan Luan Bin‑Bin Qi Jie Ren zhi‑Zhou Ren Xi‑Chao Ruan Zhao‑Hui Song zhi‑Xin Tan Sheng‑Da Tang Peng‑Cheng Wang Zhao‑Hui Wang Zhong‑Wei Wen Xiao‑Guang wu Xuan wu Li‑Kun Xie Yi‑Wei Yang han Yi Yong‑Ji Yu Guo‑Hui zhang Lin‑Hao zhang Mo‑han zhang Qi‑Wei zhang Xian‑Peng zhang Yu‑Liang zhang Yue zhang zhi‑Yong zhang Mao‑Yuan Zhao Lu‑Ping Zhou zhi‑Hao Zhou Ke‑Jun Zhu Institute of High Energy physics Chinese Academy of Sciences(CAS)Beijing 100049China Spallation Neutron Source Science center Dongguan 523803China State Key Laboratory of Particle Detection and Electronics Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China dongguan Songshan Lake Future School Dongguan 523808China North Night Vision Science&Technology(Nanjing)Research Institute Co.Ltd. Nanjing 211106China Sino‑French Institute of Nuclear engineering and Technology Sun Yat-sen UniversityZhuhai 519082China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230027China State Key Laboratory of Particle Detection and Electronics University of Science and Technology of ChinaHefei 230026China department of Modern physics University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Nuclear physics and Technology School of PhysicsPeking UniversityBeijing 100871China Institute of Nuclear physics and Chemistry China Academy of Engineering PhysicsMianyang 621900China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China USTC Archaeometry Lab University of Science and Technology of ChinaHefei 230026China Northwest Institute of Nuclear Technology Xi’an 710024China university of Chinese Academy of Sciences Beijing 100049China

Neutron-sensitive microchannel plates(nMCPs)have applications in neutron detection,including energy spectrum measurements,neutron-induced cross sections,and neutron imaging.10B-doped MCPs(B-MCPs)have attracted significant attention owing to their potential for exhibiting a high neutron detection efficiency over a large neutron energy *** spatial and temporal resolutions are useful for neutron energy-resolved ***,their practical applications still face many technical *** this study,a B-MCP with 10 mol%10B was tested for its response to wide-energy neutrons from eV to MeV at the Back-n white neutron source at the china Spallation Neutron *** neutron detection efficiency was calibrated at 1 eV,which is approximately 300 times that of an ordinary MCP and indicates the success of 10 B *** factors that caused the reduction in the detection efficiency were simulated and *** neutron energy spectrum obtained using B-MCP was compared with that obtained by other measurement methods,and showed very good consistency for neutron energies below tens of *** response is more complicated at higher neutron energy,at which point the elastic and nonelastic reactions of all nuclides of B-MCP gradually become *** is beneficial for the detection of neutrons,as it compensates for the detection efficiency of B-MCP for high-energy neutrons.

关键词： Neutron radiation image 10B-doped MCP Neutron response Wide-energy range neutrons

Atomic Dispersed Hetero‑Pairs for Enhanced Electrocatalytic CO_(2)Reduction

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Nano-Micro Letters 2024年第1期16卷 55-67页

作者： Zhaoyong jin meiqi Yang Yilong dong Xingcheng Ma Ying Wang Jiandong wu jinchang Fan Dewen Wang Rongshen Xi Xiao Zhao Tianyi Xu jingxiang Zhao Lei zhang David J.Singh Weitao Zheng Xiaoqiang Cui State Key Laboratory of Automotive Simulation and Control School of Materials Science and EngineeringKey Laboratory of Automobile Materials of MOEElectron Microscopy CenterJilin UniversityChangchun 130012People’s Republic of China Key Laboratory of Photonic and Electronic Bandgap Materials Ministry of Educationand College of Chemistry and Chemical EngineeringHarbin Normal UniversityHarbin 150025People’s Republic of China College of Chemistry Jilin UniversityChangchun 130012People’s Republic of China department of physics and Astronomy and department of Chemistry University of MissouriColumbiaMO 65211USA

Electrochemical carbon dioxide reduction reaction(CO_(2)RR)involves a variety of intermediates with highly correlated reaction and ad-desorption energies,hindering optimization of the catalytic *** example,increasing the binding of the*COOH to the active site will generally increase the*CO desorption *** this relationship may be expected to dramatically improve the intrinsic activity of CO_(2)RR,but remains an unsolved ***,we addressed this conundrum by constructing a unique atomic dispersed hetero-pair consisting of Mo-Fe di-atoms anchored on N-doped carbon *** system shows an unprecedented CO_(2)RR intrinsic activity with TOF of 3336 h−1,high selectivity toward CO production,Faradaic efficiency of 95.96%at−0.60 V and excellent *** calculations show that the Mo-Fe diatomic sites increased the*COOH intermediate adsorption energy by bridging adsorption of*COOH *** the same time,d-d orbital coupling in the Mo-Fe di-atom results in electron delocalization and facilitates desorption of*CO ***,the undesirable correlation between these steps is *** work provides a promising approach,specifically the use of di-atoms,for breaking unfavorable relationships based on understanding of the catalytic mechanisms at the atomic scale.

关键词： CO_(2)reduction reaction Atomic dispersed catalyst Hetero-diatomic pair Ad-desorption energy Linear scaling relation

Entropy-modulated and interlayer-doped transition metal layered oxides enable high-energy-density sodium-ion capacitors

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Nano Research 2024年第10期17卷 8785-8793页

作者： Tiansheng Wang Yadong Li Zhengyuan Chen Qingshan Liu Jian Lang Langyuan wu Wendi dong Zhengyu Ju Hongsen Li Xiaogang zhang Guihua Yu College of physics Qingdao UniversityQingdao 266071China Jiangsu Key Laboratory of Materials and Technologies for Energy Storage College of Materials Science and TechnologyNanjing University of Aeronautics and AstronauticsNanjing 210016China Materials Science and engineering Program and Walker department of Mechanical engineering The University of Texas at AustinAustin 78712USA

In recent years,sodium-ion capacitors have attracted attention due to their cost-effectiveness,high power density and similar manufacturing process to lithium-ion ***,the utilization of oxide electrodes in traditional sodium-ion capacitors restricts their further advancement due to the inherent low operating voltage and electrolyte consumption based on their energy storage *** address these challenges,we incorporated Zn,Cu,Ti,and other elements into Na_(0.67)Ni_(0.33)Mn_(0.67)O_(2) to synthesize P2-type Na_(0.7)Ni_(0.28)Mn_(0.6)Zn_(0.05)Cu_(0.02)Ti_(0.05)O_(2) with a modulated entropy and pillaring *** the synergistic interplay between the interlayer pillar and the entropy modulation within the layers,the material exhibits exceptional toughness,effectively shielding it from detrimental phase transitions at elevated voltage *** a result,the material showcases outstanding kinetic properties and long-term cycling stability across the voltage *** integrating these materials with hierarchical porous carbon nanospheres to form a"rocking chair"sodium-ion capacitor,the hybrid full device delivers a high energy density(171 Wh·kg^(-1))and high power density(5245 W·kg^(-1)),as well as outstanding cycling stability(77% capacity retention after 3000 cycles).This work provides an effective material development route to realize simultaneously high energy and power for next-generation sodium-ion capacitors.

关键词： sodium-ion capacitors entropy modulation high power density long-term cycling layered oxide

Understanding synergistic catalysis on Pt–Cu diatomic sites via operando X-ray absorption spectroscopy in sulfur redox reactions

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eScience 2024年第5期4卷 110-119页

作者： Shuai Xie Xingjia Chen Leilei Wang Guikai zhang Haifeng Lv Guolei Cai Ying-Rui Lu Ting-Shan Chan e jing zhang Juncai dong Hongchang jin Xianghua Kong Junling Lu Song jin Xiaojun wu Hengxing Ji Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Materials for Energy ConversionDepartment of Applied ChemistryUniversity of Science and Technology of ChinaHefei 230026China School of Chemistry and Material Sciences CAS Key Laboratory of Materials for Energy Conversionand CAS Center for Excellence in Nanoscience and Synergetic Innovation of Quantum Information and Quantum TechnologyUniversity of Science and Technology of ChinaHefei 230026China Hefei National Laboratory for Physical Sciences at the Microscale Department of Chemical PhysicsSchool of Chemistry and Materials ScienceUniversity of Science and Technology of ChinaHefei 230026China beijing Synchrotron Radiation Laboratory Institute of High Energy PhysicsChinese Academy of SciencesBeijing 100049China National Synchrotron Radiation Research center Hsinchu 300092China School of Chemistry and Chemical engineering Hefei University of TechnologyHefei 230009China

Sulfur redox reactions render lithium–sulfur(Li–S)batteries with an energy density of>500Whkg−1 but suffer a low practical capacity and fast capacity fade due to sluggish sulfur redox reaction(SRR)kinetics,which lies in the complex reaction process that involves a series of reaction intermediates and proceeds via a cascade ***,we present a Pt–Cu dual-atom catalyst(Pt/Cu-NG)as an electrocatalyst for sulfur redox ***/Cu-NG enabled the rapid conversion of soluble polysulfide intermediates into insoluble Li2S2/Li2S,and consequently,it prevented the accumulation and shuttling of lithium polysulfides,thus outperforming the corresponding single-atom catalysts(SACs)with individual Pt or Cu *** X-ray absorption spectroscopy and density functional theory calculations revealed that a synergistic effect between the paired Pt and Cu atoms modifies the electronic structure of the Pt site through d-orbital interactions,resulting in an optimal moderate interaction of the metal atom with the different sulfide *** optimal interaction enhanced charge transfer kinetics and promoted sulfur redox *** work thus provides important insights on the atomic scale into the synergistic effects operative in dual-atom catalysts and will thus pave the way to electrocatalysts with enhanced efficiency for high-performance Li–S batteries.

关键词： Dual-atom catalysts Sulfur redox reaction Lithium-sulfur batteries Synergistic interaction X-ray absorption spectroscopy

STUDIES ON ION BEAM APPLICATION TO IMPROVE AQUATIC MACROPHYTE REMEDIATION CAPACITY IN EUTROPHIC WATERS

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水生生物学报 2006年第6期30卷 711-717页

作者： LI Miao1, wu Yue-jin 1, zhang Jun 1, YU han-Qing 2, wu Xiao-Lei 3 and YU Zeng-Liang 1 (1. Key Laboratory of Ion Beam Bioengineering, Institute of Plasma physics, the Chinese Academy of Sciences, Hefei, china 230031 2. School of Chemistry and Material Science, the university of Science and Technology of china, Hefei, china 230026 3. department of Environmental Science and engineering, tsinghua university, beijing, china 100084 ) Institute of Plasma physics the Chinese Academy of Sciences Key Laboratory of Ion Beam Bioengineering CAS Hefei 230031 School of Chemistry and Material Science the University of Science and Technology of China Hefei 230026 department of Environmental Science and engineering Tsinghua University Beijing 100084

Using ion beam biotechnology in combination with soil-less plant cultivation on artificial substratum (floating beds), the experiments were conducted with Ipomoea aquatica Forsk. Plants were attached to floating-beds which were placed on the surface of artificially nutrient-enriched tank water, in order to study the purification and remediation efficiency of ion beam-treated I. aquatica cultivars. The results show that N + ion beams with 25keV energy and dosages of 0, 2.6, 3.9, 5.2, 6.5, 7.8, 9.1×10 13N +(ions)/cm 2 affected I. aquatica dry seeds differently, with the dose of 3.9×10 13N + (ions)/cm 2 improving effectively the performance as expressed by various biological indices. After ion beam application, I. aquatica cultivars grew well in nutrient-enriched water bodies, increasing the growth of leaves and stem, number of leaves, length and area of roots, plant height, and weight more remarkably than observed in the control. The net removing rates of TN, TP were as high as 75% and 82%, respectively. Especially under the dose of 3.9×10 13N +(ions)/cm 2, the net removing rates of TN, TP were highest, for 77% and 85%, respectively. It was proved that ion beam application improves phytoremediation and may be used to purify nutrient rich water bodies.

关键词： Ion beam treatment Aquatic macrophyte Ipomoea aquatica Forsk Nutrient-enriched waters Remediation capacity

Genome assembly of autotetraploid Actinidia arguta highlights adaptive evolution and enables dissection of important economic traits

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Plant Communications 2024年第6期5卷 173-192页

作者： Xue-mei Lu Xiao-Fen Yu Guo-Qiang Li Ming-Hao Qu Huan Wang Chuang Liu Yu-Ping Man Xiao-han Jiang Mu-Zi Li Jian Wang Qi-Qi Chen Rui Lei Cheng-Cheng Zhao Yun-Qiu Zhou Zheng-Wang Jiang Zuo-Zhou Li Shang Zheng Chang dong Bai-Lin Wang Yan-Xiang Sun Hui-Qin zhang Jie-Wei Li Quan-Hui Mo Ying zhang Xin Lou Hai-Xu Peng Ya-Ting Yi He-Xin Wang Xiu-Jun zhang Yi-Bo Wang Dan Wang Li Li Qiong zhang Wen-Xia Wang Yongbo Liu Lei Gao jin-Hu wu Yan-Chang Wang CAS Key Laboratory of Plant Germplasm Enhancement and Specialty Agriculture Wuhan Botanical GardenChinese Academy of SciencesWuhanHubeiChina Key Laboratory of Western china’s Environmental Systems(Ministry of Education) College of Earth and Environmental SciencesLanzhou UniversityLanzhouGansuChina College of Life Sciences University of Chinese Academy of SciencesBeijingChina wuhan Frasergen Bioinformatics Co. LtdWuhanHubeiChina Institute of Soil and Fertilizer Anhui Academy of Agricultural SciencesHefeiChina College of Agricultural Sciences Xichang UniversityXichangSichuanChina department of Horticulture Heilongjiang Academy of Agricultural SciencesHarbinHeilongjiangChina College of Life Sciences Langfang Normal UniversityLangfangHebeiChina Institute of Horticulture Zhejiang Academy of Agricultural SciencesHangzhouZhejiangChina Guangxi Institute of Botany Chinese Academy of SciencesGuilinGuangxiChina Xi’an Botanical Garden of Shaanxi Province Institute of Botany of Shaanxi ProvinceXi’anShaanxiChina Institute of Modern Agricultural Research Dalian UniversityDalianLiaoningChina Bioinformatics center College of Plant Science and TechnologyBeijing University of AgricultureBeijingChina College of Agriculture Eastern Liaoning UniversityDandongLiaoningChina Dalian Institute of Chemical physics Chinese Academy of SciencesDalianLiaoningChina State Environmental Protection Key Laboratory of Regional Eco-process and Function Assessment Chinese Research Academy of Environmental SciencesBeijingChina Hubei Hongshan Laboratory WuhanHubeiChina The New Zealand Institute for Plant and Food Research Limited AucklandNew Zealand

Actinidia arguta,the most widely distributed Actinidia species and the second cultivated species in the genus,can be distinguished from the currently cultivated Actinidia chinensis on the basis of its small and smooth fruit,rapid softening,and excellent cold *** evolution of tetraploid Actinidia species and the genetic basis of their important agronomic traits are still ***,we generated a chromosome-scale genome assembly of an autotetraploid male *** *** genome assembly was 2.77 Gb in length with a contig N50 of 9.97 Mb and was anchored onto 116 *** and clustering of 101 geographically representative accessions showed that they could be divided into two geographic groups,Southern and Northern,which first diverged 12.9 million years *** underwent two prominent expansions and one demographic bottleneck from the midPleistocene climate transition to the late *** genomics studies using paleoclimate data enabled us to discern the evolution of the species’adaptation to different historical *** genes(AaCEL1,AaPME1,and AaDOF1)related to flesh softening were identified by multi-omics analysis,and their ability to accelerate flesh softening was verified through transient expression assays.A set of genes that characteristically regulate sexual dimorphism located on the sex chromosome(Chr3)or autosomal chromosomes showed biased expression during stamen or carpel *** chromosome-level assembly of the autotetraploid *** genome and the genes related to important agronomic traits will facilitate future functional genomics research and improvement of ***.

关键词： kiwiberry dioecism adaptive evolution paleoclimate GEA rapid softening