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A strategy for designing stable nanocrystalline alloys by thermo-kinetic synergy

Journal of Materials Science & Technology 2020年第8期36卷 21-31页

作者： H.R.Peng B.S Liu F.Liu State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an710072China School of Materials and Chemical Engineering Xi’an Technological UniversityXi’an710021China Analytical and Testing Center Northwestern Polytechnical UniversityXi’an710072China

Aiming to design stable nanocrystalline(NC)materials,so far,it has been proposed to construct nanostructure stability maps in terms of thermodynamic parameters,while kinetic stabilization has seldom been considered,despite the synergy of thermodynamics and kinetics.Consequently,the thermodynamically stabilized NC materials may be easily subjected to grain growth at high temperatures due to the weakly kinetic stabilization.Starting from the thermo-kinetic synergy,a stabilization criterion is proposed as a function of intrinsic solute parameters(e.***.the activation energy for bulk diffusion and the segregation enthalpy),intrinsic solvent parameters(e.***.the intrinsic activation energy for GB migration and the GB energy)and processing parameters(e.***.the grain size,the temperature and the solute concentration).Using first-principles calculations for a series of combinations between fifty-one substitutional alloying atoms as solute atoms and Fe atom as fixed solvent atom,it is shown that the thermal stability neither simply increases with increasing the segregation enthalpy as expected by thermodynamic stabilization,nor monotonically increases with increasing the activation energy for bulk diffusion as described by kinetic stabilization.By combination of thermodynamic and kinetic contributions,the current stabilization criterion evaluates quantitatively the thermal stability,thus permitting convenient comparisons among NC materials involved by various combinations of the solute atoms,the solvent atoms,or the processing conditions.Validity of this thermo-kinetic stabilization criterion has been tested by current experiment results of Fe-Y alloy and previously published data of Fe-Ni,Fe-Cr,Fe-Zr and Fe-Ag alloys,etc.,which opens a new window for designing NC materials with sufficiently high thermal stability and sufficiently small grain size.

关键词： Thermo-kinetic Synergy Criterion Thermal stability Nanocrystalline materials

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Uncovering the softening mechanism and exploring the strengthening strategies in extremely fine nanograined metals:A molecular dynamics study

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Journal of Materials Science & Technology 2022年第14期109卷 186-196页

作者： H.R.Peng Z.Y.Jian C.X.Liu L.K.huang Y.M.ren F.Liu School of Materials and Chemical Engineering Xi’an Technological UniversityXi’an 710021China State Key Laboratory of Solidification Processing Northwestern Polytechnical UniversityXi’an 710072China

The strength of polycrystalline metals increases with decreasing grain size,following the classical hallPetch relationship.however,this relationship fails when softening occurs at very small grain sizes(typically less than 10 to 20 nm),which limits the development of ultrahigh-strength materials.In this work,using columnar-grained nanocrystalline Cu-Ag‘samples’,molecular dynamics simulations were performed to investigate the softening mechanism and explore the strengthening strategies(e.g.,formation of solid solution or grain boundary(GB)segregation)in extremely fine nanograined metals.Accordingly,the softening of pure metals is induced by atomic sliding in the GB layer,rather than dislocation activities in the grain interior,although both occur during deformation.The solid solution lowers the stacking fault energy and increases the GB energy,which leads to the softening of NC metals.GB segregation stabilizes GB structures,which causes a notable improvement in strength,and this improvement can be further enhanced by optimizing the solute concentration and GB excess.This work deepens the understanding of the softening mechanism due to atomic sliding in the GB layer and the strengthening mechanism arising from tailoring the GB stability of immiscible alloys and provides insights into the design of ultrahighstrength materials.

关键词： Softening Strengthening Cu-Ag alloy Molecular dynamics Nanocrystalline

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The molecular implications of a caspase-2-mediated site-specific tau cleavage in tauopathies

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Neural regeneration research 2021年第9期16卷 1774-1775页

作者： peng Liu Karen h.Ashe Department of Neurology University of MinnesotaMinneapolisMNUSA Department of Neuroscience University of MinnesotaMinneapolisMNUSA N.Bud Grossman Center for Memory research and Care University of MinnesotaMinneapolisMNUSA Geriatric research Educationand Clinical CentersVeterans Affairs Medical CenterMinneapolisMNUSA

A major focus of current experimental therapies for neurodegenerative diseases is on modulating post-translational modifications(PTMs)of the microtubule-associated protein tau.Tau is a highly soluble,neuronal protein that is comprised of four domains–the N-terminal projection domain,the proline-rich region,the microtubule-binding domain,and the C-terminal tail.As a scaffold protein,tau dynamically interacts with numerous structural and functional biomolecules,such as cytoskeleton and motor proteins,chaperones,enzymes,DNA,rNA,and lipids.Over a dozen types of PTMs,combined with alternative splicing,confer upon tau its enormous structural heterogeneity,which subserves its many(patho-)physiological functions.

关键词： tau structural cleavage

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Architecture modification and In^(3+)-doping of WO_(3) photoanodes to boost the photoelectrochemical water oxidation performance

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Science China Chemistry 2023年第11期66卷 3269-3279页

作者： peng Zeng Yang Zhou Lingling peng Shaochuan Wang Tianyou peng School of Food and Pharmaceutical Engineering Zhaoqing UniversityZhaoqing 526061China College of Chemistry and Molecular Sciences Wuhan UniversityWuhan 430072China

WO_(3) photoanodes have been widely utilized for the oxygen evolution reaction(OEr)in the photoelectrochemical water splitting system.herein,the effects of hydrazine hydrate modification and In^(3+)-doping on the physicochemical properties and photocurrent density of the WO_(3) photoanode prepared by hydrothermally treating at 160℃followed by calcining at 500℃are investigated.Among them,the hydrazine hydrate in the hydrothermal solution can serve as a texture regulator,resulting in the formation of WO_(3) films with the layered architecture stacked by nanosheets dominantly exposed(020)facets,which allows the WO_(3) films to have faster charge separation and larger specific surface area for OEr according to the characterization results of microstructures and photoelectrochemcial behaviors;while the In^(3+)-doping can optimize the energy band structure of WO_(3) and adjust the work function to increase the driving force of OEr based on the ultraviolet photoelectron spectroscopy,Mott–Schottky and open-circuit photovoltage plots.Under the simulated sunlight(AM1.5G)illumination,the designed In^(3+)–WO_(3)(N_2h_4)photoanode in Na_2SO_4 solution delivers amaximum incident photon-to-current efficiency of 38.6%at 410 nm and a photocurrent density of 1.93 mA cm^(-2)at 1.23 V vs.rhE,which is 2.8 and 3.0 times higher than the pristine WO_(3) photoanode,respectively.This study provides a promising strategy to improve the water splitting performance of nanostructured WO_(3) photoanodes by altering the architecture and introducing heteroatoms.

关键词： WO_(3)photoanode oxygen evolution reaction photoelectrochemical water splitting doping architecture modification

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Amino acid nutrition and metabolism in domestic cats and dogs

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畜牧与生物技术杂志:英文版 2023年第5期14卷 1777-1797页

作者： peng Li Guoyao Wu North American renderers Association AlexandriaVirginia 22314USA Department of Animal Science Texas A&M UniversityCollege StationTX 77843USA

Domestic cats and dogs are carnivores that have evolved differentially in the nutrition and metabolism of amino acids.This article highlights both proteinogenic and nonproteinogenic amino acids.Dogs inadequately synthesize citrulline(the precursor of arginine)from glutamine,glutamate,and proline in the small intestine.Although most breeds of dogs have potential for adequately converting cysteine into taurine in the liver,a small proportion(1.3%-2.5%)of the Newfoundland dogs fed commercially available balanced diets exhibit a deficiency of taurine possibly due to gene mutations.Certain breeds of dogs(e.g.,golden retrievers)are more prone to taurine deficiency possibly due to lower hepatic activities of cysteine dioxygenase and cysteine sulfinate decarboxylase.De novo synthesis of arginine and taurine is very limited in cats.Thus,concentrations of both taurine and arginine in feline milk are the greatest among domestic mammals.Compared with dogs,cats have greater endogenous nitrogen losses and higher dietary requirements for many amino acids(e.g.,arginine,taurine,cysteine,and tyrosine),and are less sensitive to amino acid imbalances and antagonisms.Throughout adulthood,cats and dogs may lose 34%and 21%of their lean body mass,respectively.Adequate intakes of high-quality protein(i.e.,32%and 40%animal protein in diets of aging dogs and cats,respectively;dry matter basis)are recommended to alleviate aging-associated reductions in the mass and function of skeletal muscles and bones.Pet-food grade animal-sourced foodstuffs are excellent sources of both proteinogenic amino acids and taurine for cats and dogs,and can help to optimize their growth,development,and health.

关键词： Animal-sourced foodstuffs Cats Dogs health Metabolism Nutrition

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Laser Erasing and rewriting of Flexible Copper Circuits

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Nano-Micro Letters 2021年第11期13卷 409-420页

作者： Xingwen Zhou Wei Guo peng peng School of Mechanical Engineering and Automation Beihang UniversityBeijing 100191People’s Republic of China Department of Mechanical and Mechatronics Engineering Centre for Advanced Materials JoiningUniversity of WaterlooWaterlooON N2L 3G1Canada

Integrating construction and reconstruction of highly conductive structures into one process is of great interest in developing and manufacturing of electronics,but it is quite challenging because these two involve contradictive additive and subtractive processes.In this work,we report an all-laser mask-less processing technology that integrates manufacturing,modifying,and restoring of highly conductive Cu structures.By traveling a focused laser,the Cu patterns can be fabricated on the flexible substrate,while these as-written patterns can be selectively erased by changing the laser to a defocused state.Subsequently,the fresh patterns with identical conductivity and stability can be rewritten by repeating the writing step.Further,this erasing–rewriting process is also capable of repairing failure patterns,such as oxidation and cracking.Owing to the high controllability of this writing–erasing–rewriting process and its excellent reproducibility for conductive structures,it opens a new avenue for rapid healing and prototyping of electronics.

关键词： Laser writing Laser erasing Copper electrodes Electronic repairing Flexible electronics

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Fenton metal nanomedicines for imaging-guided combinatorial chemodynamic therapy against cancer

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Asian Journal of Pharmaceutical Sciences 2022年第2期17卷 177-192页

作者： peng Liu Ying peng Jinsong Ding Wenhu Zhou Xiangya School of Pharmaceutical Sciences Central South UniversityChangsha 410013China henan Key Laboratory of Biomolecular recognition and Sensing Shangqiu Normal UniversityShangqiu 476000China

Chemodynamic therapy(CDT)is considered as a promising modality for selective cancer therapy,which is realized via Fenton reaction-mediated decomposition of endogenous h_(2)O_(2) to produce toxic hydroxyl radical(•Oh)for tumor ablation.While extensive efforts have been made to develop CDT-based therapeutics,their in vivo efficacy is usually unsatisfactory due to poor catalytic activity limited by tumor microenvironment,such as anti-oxidative systems,insufficient h_(2)O_(2),and mild acidity.To mitigate these issues,we have witnessed a surge in the development of CDT-based combinatorial nanomedicines with complementary or synergistic mechanisms for enhanced tumor therapy.By virtue of their bio-imaging capabilities,Fenton metal nanomedicines(FMNs)are equipped with intrinsic properties of imaging-guided tumor therapies.In this critical review,we summarize recent progress of this field,focusing on FMNs for imaging-guided combinatorial tumor therapy.First,various Fenton metals with inherent catalytic performances and imaging properties,including Fe,Cu and Mn,were introduced to illustrate their possible applications for tumor theranostics.Then,CDT-based combinatorial systems were reviewed by incorporating many other treatment means,including chemotherapy,photodynamic therapy(PDT),sonodynamic therapy(SDT),photothermal therapy(PTT),starvation therapy and immunotherapy.Next,various imaging approaches based on Fenton metals were presented in detail.Finally,challenges are discussed,and future prospects are speculated in the field to pave way for future developments.

关键词： combinatorial medicines equipped

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Applications of MXenes in human-like sensors and actuators

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Nano research 2023年第4期16卷 5767-5795页

作者： Jinbo Pang Songang peng Chongyang hou Xiao Wang Ting Wang Yu Cao Weijia Zhou Ding Sun Kai Wang Mark h.rümmeli Gianaurelio Cuniberti hong Liu Institute for Advanced Interdisciplinary research(iAIr) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongUniversity of JinanJinan 250022China Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresden 01069Germany Center for Advancing Electronics Dresden Technische Universität DresdenDresden 01069Germany Dresden Center for Computational Materials Science Technische Universität DresdenDresden 01062Germany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität DresdenDresden 01062Germany high-Frequency high-Voltage Device and Integrated Circuits r&D Center Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Microelectronic Devices&Integrated Technology Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Shenzhen Key Laboratory of Nanobiomechanics Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China State Key Laboratory of Biobased Material and Green Papermaking Qilu University of TechnologyShandong Academy of SciencesJinan 250353China School of Bioengineering Qilu University of TechnologyShandong Academy of ScienceJinan 250353China Key Laboratory of Modern Power System Simulation and Control&renewable Energy Technology(Ministry of Education) Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Weihai Innovation Research InstituteQingdao UniversityQingdao 266000China School of Electrical and Computer Engineering Jilin Jianzhu UniversityChangchun 130118China Institute for Complex Materials Leibniz Institute for Solid State and Materials Research Dresden(IFW Dresden)20 Helmholtz StrasseDresden 01069Germany College of Energy Soochow Institute for Energy and Materials Innovations Soochow UniversitySuzhou 215006China Key L

human beings perceive the world through the senses of sight,hearing,smell,taste,touch,space,and balance.The first five senses are prerequisites for people to live.The sensing organs upload information to the nervous systems,including the brain,for interpreting the surrounding environment.Then,the brain sends commands to muscles reflexively to react to stimuli,including light,gas,chemicals,sound,and pressure.MXene,as an emerging two-dimensional material,has been intensively adopted in the applications of various sensors and actuators.In this review,we update the sensors to mimic five primary senses and actuators for stimulating muscles,which employ MXene-based film,membrane,and composite with other functional materials.First,a brief introduction is delivered for the structure,properties,and synthesis methods of MXenes.Then,we feed the readers the recent reports on the MXene-derived image sensors as artificial retinas,gas sensors,chemical biosensors,acoustic devices,and tactile sensors for electronic skin.Besides,the actuators of MXene-based composite are introduced.Eventually,future opportunities are given to MXene research based on the requirements of artificial intelligence and humanoid robot,which may induce prospects in accompanying healthcare and biomedical engineering applications.

关键词： MXenes sensors actuators gas sensors biosensors tactile sensors sound sensors artificial retina

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Controllable vortex lasing arrays in a geometrically frustrated exciton-polariton lattice at room temperature

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National Science review 2023年第1期10卷 196-204页

作者： Jun Wang Yutian peng huawen Xu Jiangang Feng Yuqing huang Jinqi Wu Timothy C.h.Liew Qihua Xiong Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Department of Optical Science and Engineering and Shanghai Frontiers Science Research Base of Intelligent Optoelectronics and Perception Fudan University State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics Tsinghua University Beijing Academy of Quantum Information Sciences

Quantized vortices appearing in topological excitations of quantum phase transition play a pivotal role in strongly correlated physics involving the underlying confluence of superfluids,Bose-Einstein condensates and superconductors.Exciton polaritons as bosonic quasiparticles have enabled studies of non-e quilibrium quantum gases and superfluidity.Exciton-polariton condensates in artificial lattices intuitively emulate energy-band structures and quantum many-body effects of condensed matter,underpinning constructing vortex lattices and controlling quantum fluidic circuits.here,we harness exciton-polariton quantum fluids of light in a frustrated kagome lattice based on robust metal-halide perovskite microcavities,to demonstrate vortex lasing arrays and modulate their configurations at room temperature.Tomographic energy-momentum spectra unambiguously reveal massless Dirac bands and quenched kinetic-energy flat bands coexisting in kagome lattices,where polariton condensates exhibit prototypical honeycomb and kagome spatial patterns.Spatial coherence investigations illustrate two types of phase textures of polariton condensates carrying ordered quantized-vortex arrays and π-phase shifts,which could be selected when needed using lasing emission energy.Our findings offer a promising platform on which it is possible to study quantum-fluid correlations in complex polaritonic lattices and highlight feasible applications of structured light.

关键词： vortex lasing exciton–polariton lattice Bose–Einstein condensation the orbital angular momentum of light geometric frustration perovskite semiconductor

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A Note on the heat Kernel for the rescaled harmonic Oscillator from Two Step Nilpotent Lie Groups

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Acta Mathematica Sinica,English Series 2022年第9期38卷 1597-1611页

作者： Zhi peng YANG Department of Mathematics Yunnan Normal UniversityKunming 650500P.R.China

In this note,we use Schr?dinger representations and the Fourier transform on two step nilpotent Lie groups to compute the explicit formula of the sub-Laplacian operator and its symbol,which is associated with the rescaled harmonic oscillator.Then we can give an explicit formula for the heat kernel of the rescaled harmonic oscillator for the singularity at the origin.Our results are useful for the general two step nilpotent Lie groups,including the heisenberg group and h-type group.

关键词： Sub-Laplacian heat kernel nilpotent Lie groups

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