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Science China Chemistry 2024年第9期67卷 2941-2948页

作者： Yang-Ping Zhang Shao-Min Pei Wen-Fa Chen Bin-Wen Liu Xiao-Ming Jiang guo-Cong guo State Key Laboratory of Structural Chemistry Fujian Institute of Research on the Structure of MatterChinese Academy of SciencesFuzhou 350002China Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China School of Physical Science and Technology Shanghai Tech UniversityShanghai 201210China

Non-centrosymmetric(NCS)structure is an indispensable prerequisite for second-order nonlinear optical(NLO)***,the mainstream approach for designing new NCS structures still relies on chemical substitution,necessitating an urgent infusion of fresh *** this work,two isomorphic sulfides AeMn_(6)Ga_(6)S_(16)(Ae=Ca,1;Sr,2)are afforded by modifying the skeleton of centrosymmetric(CS)Mn_(2)Ga_(2)S_(5) via introducing strong electropositive alkaline-earth ***,the incorporation of Ca^(2+)/Sr^(2+)cations allows the elementary[MnGaS_(9)]_(∞)chains to reconfigure into bumpy[MnS_(6)]-[GaS_(4)]layers in a new engagement manner,thus enabling the conversion from CS to NCS *** modifications cause not only strong second-harmonic generation(SHG)responses(~1.5×benchmark AgGaS_(2)@1,700 nm),but also significantly feasible bandgaps(2.60-2.64 e V)compared to the sulfide Mn_(2)Ga_(2)S_(5)(1.36 e V),which ultimately facilitate ultrahigh laser-induced damage thresholds(4.4-6.6×AgGaS_(2)@1,064 nm for compounds 1 and 2).The present study offers an ingenious approach for the transformation of CS to NCS structure.

关键词： second-harmonic generation non-centrosymmetrical structure NLO functional motif solid-state method

Applications of genetic code expansion technology in eukaryotes

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Protein & Cell 2024年第5期15卷 331-363页

作者： Qiao-ru guo Yu J.Cao State Key Laboratory of Chemical Oncogenomic Guangdong Provincial Key Laboratory of Chemical GenomicsPeking University Shenzhen Graduate SchoolShenzhen 518055China Institute of Chemical Biology Shenzhen Bay LaboratoryShenzhen 518132China

Unnatural amino acids(UAAs)have gained significant attention in protein engineering and drug development owing to their ability to introduce new chemical functionalities to *** eukaryotes,genetic code expansion(GCE)enables the incorporation of UAAs and facilitates posttranscriptional modification(PTM),which is not feasible in prokaryotic *** is also a powerful tool for cell or animal imaging,the monitoring of protein interactions in target cells,drug development,and switch ***,there is keen interest in utilizing GCE in eukaryotic *** review provides an overview of the application of GCE in eukaryotic systems and discusses current challenges that need to be addressed.

关键词： genetic code expansion unnatural amino acid eukaryotes basic research therapeutic applications

Tailoring of a robust asymmetric aramid nanofibers/MXene aerogel film for enhanced infrared thermal camouflage and Joule heating performances

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Nano Research 2024年第3期17卷 1990-1998页

作者： Wanbin Dang Wei guo Wenting Chen Qiuyu Zhang Key Laboratory of Special Functional and Smart Polymer Materials of Ministry of Industry and Information Technology School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China

The development of infrared(IR)surveillance technology has led to a growing interest in thermal ***,the trade-off relationship between low IR-emissivity and thermal insulation hinders the advance of thermal camouflage ***,guided by multi-physics simulation,we show a design of asymmetric aramid nanofibers/MXene(ANF/MXene)aerogel film that realizes high-efficient thermal camouflage *** rationale is that the asymmetric structure contains a thermal-insulation three-dimensional(3D)network part to prevent effective heat transfer and a low IR-emissivity(~0.3)dense surface layer to suppress radiative heat *** is remarkable that the synergy mechanism in the topology structure contributes to over 40%reduction of target radiation ***,the tailored asymmetric ANF/MXene aerogel film also enables sound mechanical properties such as a Young’s modulus of 44.4 MPa and a tensile strength of 1.3 MPa,superior to most aerogel *** also exhibits great Joule heating performances including low driving voltage(4 V),fast thermal response(<10 s),and long-term stability,further enabling its versatile thermal camouflage *** work offers an innovative design concept to configure multifunctional structures for next-generation thermal management applications.

关键词： asymmetric aerogel film low infrared(IR)-emissivity thermal insulation IR thermal camouflage Joule heating performance

Dual-salt poly(tetrahydrofuran) electrolyte enables quasi-solid-state lithium metal batteries to operate at -30 ℃

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Journal of Energy Chemistry 2024年第9期96卷 456-463页

作者： Zhiyong Li Zhuo Li Rui Yu Xin guo School of Materials Science and Engineering State Key Laboratory of Material Processing and Die&Mould TechnologyHuazhong University of Science and TechnologyWuhan 430074HubeiChina The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and TechnologyWuhan 430081HubeiChina

The stable operation of solid-state lithium metal batteries at low temperatures is plagued by severe restrictions from inferior electrolyte-electrode interface compatibility and increased energy barrier for Li^(+)***,we prepare a dual-salt poly(tetrahydrofuran)-based electrolyte consisting of lithium hexafluorophosphate and lithium difluoro(oxalato)borate(LiDFOB).The Li-salt anions(DFOB−)not only accelerate the ring-opening polymerization of tetrahydrofuran,but also promote the formation of highly ion-conductive and sustainable interphases on Li metal anodes without sacrificing the Li^(+)conductivity of electrolytes,which is favorable for Li^(+)transport kinetics at low *** of this polymer electrolyte in Li||LiFePO_(4)cells show 82.3%capacity retention over 1000 cycles at 30℃and endow stable discharge capacity at−30℃.Remarkably,the Li||LiFePO4 cells retain 52%of their room-temperature capacity at−20℃and 0.1 *** rational design of dual-salt polymer-based electrolytes may provide a new perspective for the stable operation of quasi-solid-state batteries at low temperatures.

关键词： Poly(tetrahydrofuran) Dual-salt electrolyte Solidel ectrolyte interphase Low-temperature operation Quasi-solid-state battery

On the convergence of tracking differentiator with multiple stochastic disturbances

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Science China(Information Sciences) 2024年第2期67卷 157-169页

作者： Zehao WU Huacheng ZHOU Baozhu guo Feiqi DENG School of Mathematics and Big Data Foshan University School of Mathematics and Statistics Central South University Academy of Mathematics and Systems Science Chinese Academy of Sciences Systems Engineering Institute South China University of Technology

This paper investigates the convergence, noise-tolerance, and filtering performance of a tracking differentiator in the presence of multiple stochastic disturbances for the first time. We consider a general case wherein the input signal is corrupted by additive colored noise, and the tracking differentiator is disturbed by additive colored noise and white noise. The tracking differentiator is shown to track the input signal and its generalized derivatives in the mean square sense. Further, the almost sure convergence can be achieved when the stochastic noise affecting the input signal is vanishing. Herein, numerical simulations are performed to validate the theoretical results.

关键词： tracking differentiator convergence noise-tolerance filtering performance multiple stochastic disturbances

Experimental and numerical demonstration of hierarchical time-delay reservoir computing based on cascaded VCSELs with feedback and multiple injections

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Science China(Information Sciences) 2024年第2期67卷 279-290页

作者： Xingxing guo Shuiying XIANG Xingyu CAO Biling GU State Key Laboratory of Integrated Service Networks Xidian University State Key Discipline Laboratory of Wide Bandgap Semiconductor Technology School of MicroelectronicsXidian University

In this paper, we propose and demonstrate experimentally and numerically a hierarchical timedelay optical reservoir computing(RC) system based on cascaded vertical-cavity surface-emitting lasers(VCSELs) with feedback and multiple injections. The prediction performance characteristics of the hierarchical time-delay RC system based on cascaded VCSELs under different reservoir layers are ***, the prediction performance of the hierarchical time-delay RC system is first improved and saturates as the number of reservoir layers increases. Besides, the impacts of key factors on predicting the hierarchical time-delay RC system are also analyzed in detail experimentally and numerically. This proposed hierarchical time-delay RC system based on VCSELs is useful for the further development of RC systems and may be beneficial to improve the ability of RC systems to solve more complex problems.

关键词： vertical-cavity surface-emitting laser reservoir computing neuromorphic photonics time-delay system information processing

Vibration response and safety control for blasting vibration of the existing tunnel with defects

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Underground Space 2024年第2期15卷 76-89页

作者： Junying Xia Bo Wang Xinxin guo Zhuoxiong Xie Key Laboratory of Transportation Tunnel Engineering Ministry of EducationSouthwest Jiaotong UniversityChengdu 610031China College of Environment and Civil Engineering Chengdu University of TechnologyChengdu 610059China Guangdong Communication Planning&Design Institute Group Co. LtdGuangzhou 510507China

Current studies on blasting construction of small clear-distance tunnels have not considered the impact of existing tunnel lining defects when establishing safety *** paper offers a series of study results based on the blasting project of a new tunnel adjacent to the existing defect Xinling tunnel to thoroughly examine the dynamic response,safety control standards,and measures of the existing defect ***,structural models were developed to investigate the influence of the presence or absence of specific defects(like lining cracks and cavities behind the lining)on the dynamic response of the current tunnel lining to identify the most unfavorable defect ***,establish safety control standards for intact linings and those with the most unfavorable ***,two types of control measures,single safe charge and reasonable delay time,were studied based on the established safety control *** particular,the most adverse position of cracks was the wall facing the explosion,the rise in depth was more unfavorable for vibration response,and the impact of the longitudinal crack was restricted to the vicinity of the *** the vault was the most adverse cavity position,the rise in cavity area was more damaging,and the influence range varied with longitudinal cavity ***,the impact of cracks was mainly evident in the amplification effect of stress at the crack *** contrast,cavities had varied degrees of amplification effects on the vibration velocity and stress response and a relatively extensive influence *** control research was conducted,when the tunnel was intact,with a right wall crack,a vault cavity,and both vault cavity and crack for this project,the peak particle velocity(PPV)of the safety control standard for vibration velocity was 13,10,13,and 8 cm/s,respectively,and the respective single safe charge could be adjusted at 64,53,37,and 25 ***,the presence of different defects had a relati

关键词： Existing tunnel Defect Blasting construction Vibration response Control standards and measures

Design of an automated robotic microinjection system for batch injection of zebrafish embryos and larvae

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Microsystems & Nanoengineering 2024年第1期10卷 89-103页

作者： Zhongyi guo Nana Ai Wei Ge Qingsong Xu Department of Electromechanical Engineering Faculty of Science and TechnologyUniversity of MacaoMacaoChina Department of Biomedical Sciences and Centre of Reproduction Development and Aging(CRDA)Faculty of Health SciencesUniversity of MacaoMacaoChina

This paper presents the design of a vision-based automated robotic microinjection system for batch injection of both zebrafish embryos and larvae.A novel visual recognition algorithm based on an automatic threshold and excessive dilatation is introduced to accurately identify the center of zebrafish embryos and larval yolks.A corresponding software system is developed using the producer-consumer model as the framework structure,and a friendly user interface is designed to allow operators to choose from a range of desired functions according to their different *** addition,a novel microstructural agarose device is designed and fabricated to simultaneously immobilize mixed batches of embryos and ***,a prototype microinjection system is fabricated by integrating hardware devices with visual *** experimental study is conducted to verify the performance of the robotic microinjection *** results show that the reported system can accurately identify zebrafish embryos and larvae and efficiently complete batch microinjection tasks of the mixtures with an injection success rate of 92.05%in 13.88 s per *** with manual and existing microinjection systems,the proposed system demonstrates the merits of versatility,excellent efficiency,high success rate,high survival rate,and sufficient stability.

关键词： zebra automated hardware

Physical neural networks with self-learning capabilities

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Science China(Physics,Mechanics & Astronomy) 2024年第8期67卷 23-42页

作者： Weichao Yu Hangwen guo Jiang Xiao Jian Shen State Key Laboratory of Surface Physics and Institute for Nanoelectronic Devices and Quantum Computing Fudan UniversityShanghai 200433China Zhangjiang Fudan International Innovation Center Fudan UniversityShanghai 201210China Department of Physics Fudan UniversityShanghai 200433China Shanghai Research Center for Quantum Sciences Shanghai 201315China Collaborative Innovation Center of Advanced Microstructures Nanjing 210093China

Physical neural networks are artificial neural networks that mimic synapses and neurons using physical systems or *** networks harness the distinctive characteristics of physical systems to carry out computations effectively,potentially surpassing the constraints of conventional digital neural networks.A recent advancement known as“physical self-learning”aims to achieve learning through intrinsic physical processes rather than relying on external *** article offers a comprehensive review of the progress made in implementing physical self-learning across various physical *** learning strategies that contribute to the realization of physical self-learning are *** challenges in understanding the fundamental mechanism of learning,this work highlights the progress towards constructing intelligent hardware from the ground up,incorporating embedded self-organizing and self-adaptive dynamics in physical systems.

关键词： self-learning physical neural networks neuromorphic computing physical learning

Fast and Adaptive Multi-Agent Planning under Collaborative Temporal Logic Tasks via Poset Products

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Research 2024年第2期2024卷 81-94页

作者： Zesen Liu Meng guo Weimin Bao Zhongkui Li Deparment of Mechanics and Engineering Science College of EngineeringPeking UniversityBejing 0081 China Science and Technology Commission of China Aerospace Science and Technology Corporation Beijing 100048China

Efficient coordination and planning is essential for large-scale multi-agent systems that collaborate in a shared dynamic environment. Heuristic search methods or learning-based approaches often lack the guarantee on correctness and performance. Moreover, when the collaborative tasks contain both spatial and temporal requirements, e.g., as linear temporal logic (LTL) formulas, formal methods provide a verifiable framework for task planning. However, since the planning complexity grows exponentially with the number of agents and the length of the task formula, existing studies are mostly limited to small artificial cases. To address this issue, a new planning paradigm is proposed in this work for system-wide temporal task formulas that are released online and continually. It avoids two common bottlenecks in the traditional methods, i.e., (a) the direct translation of the complete task formula to the associated B點hi automaton and (b) the synchronized product between the B點hi automaton and the transition models of all agents. Instead, an adaptive planning algorithm is proposed, which computes the product of relaxed partially ordered sets (R-posets) on-the-fly and assigns these subtasks to the agents subject to the ordering constraints. It is shown that the first valid plan can be derived with a polynomial time and memory complexity with respect to the system size and the formula length. Our method can take into account task formulas with a length of more than 400 and a fleet with more than 400 agents, while most existing methods fail at the formula length of 25 within a reasonable duration. The proposed method is validated on large fleets of service robots in both simulation and hardware experiments.

关键词： hardware service system