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Projected changes in extreme snowfall events over the Tibetan Plateau based on a set of RCM simulations

Atmospheric and Oceanic Science Letters 2024年第5期17卷 3-9页

作者： Yuanhai Fu xuejie gao Climate Change Research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science&TechnologyNanjingChina University of Chinese Academy of Sciences BeijingChina

Extreme snowfall events over the Tibetan Plateau(TP)cause considerable damage to local society and natural *** this study,the authors investigate the projected changes in such events over the TP and its surrounding areas based on an ensemble of a set of 21st century climate change projections using a regional climate model,*** model is driven by five CMIP5 global climate models at a grid spacing of 25 km,under the RCP4.5 and RCP8.5 *** modified ETCCDI extreme indices-namely,SNOWTOT,S1mm,S10mm,and Sx5day-are employed to characterize the extreme snowfall ***4 generally reproduces the spatial distribution of the indices over the region,although with a tendency of *** the projected changes,a general decrease in SNOWTOT is found over most of the TP,with greater magnitude and better cross-simulation agreement over the eastern *** the simulations project an overall decrease in S1mm,ranging from a 25%decrease in the west and to a 50%decrease in the east of the *** S10mm and Sx5day are projected to decrease over the eastern part and increase over the central and western parts of the ***,S10mm shows a marked increase(more than double)with high cross-simulation agreement over the central *** increases in all four indices are found over the Tarim and Qaidam basins,and northwestern China north of the *** projected changes show topographic dependence over the TP in the latitudinal direction,and tend to decrease/increase in low-/high-altitude areas.

关键词： Extreme snowfall Regional climate model Tibetan plateau Climate change

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Long-lifespan thin Li anode achieved by dead Li rejuvenation and Li dendrite suppression for all-solid-state lithium batteries

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Chinese Chemical Letters 2024年第10期35卷 530-536页

作者： xuejie gao Xinyang Chen Ming Jiang Hanyan Wu Wenfeng Ren Xiaofei Yang Runcang Sun Center for Lignocellulosic Chemistry and Biomaterials College of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034China Division of Energy Storage Dalian National Laboratoryfor Clean EnergyDalian Institute of Chemical PhysicsChinese Academy of SciencesDalian116023 China Institute of Physical Science and Information Technology Anhui UniversityHefei 230601China

Solid polymer electrolytes(SPEs)are considered to be one of the most promising systems applied in all-solid-state lithium metal batteries(ASSLMBs)on account of their chemical and electrochemical ro bustness,mechanical stability,cost-effective and scalable manufacturing ***,significant en deavors have been directed towards mitigating the formation of the Li dendrite in SPE-based ASSLMBs while research on the inactive lithium in the forms of the solid-electrolyte interface has been rarely re ***,a bi-functional GaI3additive is developed for in-situ generating Li_(3)Ga alloy for suppressing Li dendrite growth,as well as I3-in recovering dead *** on the density functional theory(DFT)results,the Li atom prefers to deposit on the Li_(3)Ga surface and then guide uniform Li deposi tion,while the I3species features a relatively lower lowest unoccupied molecular orbital(LUMO)energy level(-2.12 e V),meaning a higher electron affinity,which is beneficial for reviving inactive lithium to counterbalance the loss of *** a result,in comparison to cells employing pure PEGDME-based electrolytes,the Li-Li symmetric cells utilizing GaI3-containing solid-state electrolyte exhibited a cycling life nearly 30 times longer at a current density/capacity of 0.2 mA/cm^(2),0.2 mAh/cm^(2).The full batterie of LFP//1%GaI3-SPE//40μm Li delivered a noteworthy capacity retention of 82%after 1300 cycles at a rate of 1 C.

关键词： Synergistic effect In-situ Li Ga alloy Suppress Lidendrite Dead lithium regeneration All-solid-state lithium metal batteries

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Dual-single-atoms of Pt-Co boost sulfur redox kinetics for ultrafast Li-S batteries

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Carbon Energy 2024年第3期6卷 53-63页

作者： Hanyan Wu xuejie gao Xinyang Chen Weihan Li Junjie Li Lei Zhang Yang Zhao Ming Jiang Runcang Sun Xueliang Sun Center for Lignocellulosic Chemistry and Biomaterials College of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalianChina Department of Mechanical and Materials Engineering University of Western OntarioLondonOntarioCanada Institute of Physical Science and Information Technology Anhui UniversityHefeiChina

Applications of lithium-sulfur(Li-S)batteries are still limited by the sluggish conversion kinetics from polysulfide to Li_(2)*** various single-atom catalysts are available for improving the conversion kinetics,the sulfur redox kinetics for Li-S batteries is still not ***,in this work,a catalyst with dual-single-atom Pt-Co embedded in N-doped carbon nanotubes(Pt&Co@NCNT)was proposed by the atomic layer deposition method to suppress the shuttle effect and synergistically improve the interconversion kinetics from polysulfides to Li_(2)*** X-ray absorption near edge curves indicated the reversible conversion of Li_(2)Sx on the S/Pt&Co@NCNT ***,density functional theory demonstrated that the Pt&Co@NCNT promoted the free energy of the phase transition of sulfur species and reduced the oxidative decomposition energy of Li_(2)*** a result,the batteries assembled with S/Pt&Co@NCNT electrodes exhibited a high capacity retention of 80%at 100 cycles at a current density of 1.3 mA cm^(−2)(S loading:2.5 mg cm^(−2)).More importantly,an excellent rate performance was achieved with a high capacity of 822.1 mAh g^(−1) at a high current density of 12.7 mA cm^(−2).This work opens a new direction to boost the sulfur redox kinetics for ultrafast Li-S batteries.

关键词： DFT calculation dual-single-atoms of Pt-Co fast Li-sulfur batteries sulfur redox kinetics XANES analysis

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Use of the RegCM System over East Asia： Review and Perspectives

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Engineering 2017年第5期3卷 766-772页

作者： xuejie gao Filippo Giorgi Climate Change Research Center Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China The Abdus Salam International Center.for Theoretical Physics Trieste 34151 Italy

The Abdus Salam International Center for Theoretical Physics （ICTP） RegCM system is one of the most commonly used regional climate models （RCMs） over the East Asia region, In this paper, we present a brief review of the RegCM system and its applications to the East Asia region. The model history and plans for future development are described, Previous and ongoing applications, as well as the advantages and biases found in the model system over the East Asia region, are summarized, The model biases that exist are mainly found in the cold seasons, and are characterized by a warm bias at high latitudes and underestimation of precipitation in the south. These biases are similar to those of most global climate models （GCMs）, Finally, future plans on the application and development of the model, and specifically on those within the context of the Coordinated Regional Climate Downscaling Experiment （CORDEX）, are introduced. This paper is intended to serve as a reference for future users of the RegCM system within the East Asia region.

关键词： Regional climate model China Climate change Community land model

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A high resolution simulation of climate change over China

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Science China Earth Sciences 2011年第3期54卷 462-472页

作者： gao xuejie SHI Ying Filippo GIORGI The Laboratory of Climate Study National Climate Center China Meteorological Administration Beijing 100081 China The Abdus Salam International Centre for Theoretical Physics Trieste Italy

Multi-decadal high resolution climate change simulations over East Asia were performed by using The Abdus Salam International Centre for Theoretical Physics (ICTP) Regional Climate Model (RegCM3), nested within the NASA/NCAR global model FvGCM/CCM3. Two sets of simulations were conducted at 20-km grid spacings, one for present day (1961-1990) and one for the future climate (2071-2100, IPCC A2 scenario). Simulations of present climate conditions over China by RegCM3 and FvGCM were compared against observations to assess the model performance. Results showed that both models repro- duced the observed spatial structure of 500 hPa height, surface air temperature and precipitation. Compared with FvGCM, RegCM3 provided increasing spatial detail of surface variables. Furthermore, RegCM3 improved the simulation of monsoon precipitation over the region. Changes in the mean temperature and precipitation were analyzed and compared between the two models. Significant warming in the end of the 21st century was simulated by both models in December-January-February (DJF), June-July-August (JJA), and the annual mean. In DJF, greater warming was simulated by FvGCM over Northeast and Northwest China, as well as the Tibetan Plateau, compared with RegCM. In JJA, RegCM3 simulated greater warming over northern China, Inner Mongolia, Northwest China, and the Tibetan Plateau. Simulated changes in DJF precipitation showed similar spatial patterns between the two models. In JJA, while FvGCM projected a prevailing increase of monsoon precipitation over China, which is in agreement with other global models, RegCM3 projected extended areas of decreased precipitation. Changes in the variability for annual mean temperature and precipitation also are presented.

关键词： climate change regional climate model China

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Projection of the Future Changes in Tropical Cyclone Activity Affecting East Asia over the Western North Pacific Based on Multi-RegCM4 Simulations

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Advances in Atmospheric Sciences 2022年第2期39卷 284-303页

作者： Jie WU xuejie gao Yingmo ZHU Ying SHI Filippo GIORGI School of Geography and Environmental Engineering Gannan Normal UniversityGanzhou 341000China Climate Change Research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China University of Chinese Academy of Sciences Beijing 100049China Department of Atmospheric Sciences Yunnan UniversityKunming 650504China National Climate Center China Meteorological AdministrationBeijing 100081China The Abdus Salam International Centre for Theoretical Physics Trieste 34100Italy

Future changes in tropical cyclone(TC)activity over the western North Pacific(WNP)under the representative concentration pathway RCP4.5 are investigated based on a set of 21 st century climate change simulations over East Asia with the regional climate model RegCM4 driven by five global *** RegCM4 reproduces the major features of the observed TC activity over the region in the present-day period of 1986-2005,although with the underestimation of the number of TC genesis and intensity.A low number of TCs making landfall over China is also *** the end of the 21st century(2079-98),the annual mean frequency of TC genesis and occurrence is projected to increase over the WNP by16%and 10%,*** increase in frequency of TC occurrence is in good agreement among the simulations,with the largest increase over the ocean surrounding Taiwan Island and to the south of *** TCs tend to be stronger in the future compared to the present-day period of 1986-2005,with a large increase in the frequency of strong *** addition,more TCs landings are projected over most of the China coast,with an increase of~18%over the whole Chinese territory.

关键词： regional climate model RegCM4 tropical cyclone western North Pacific

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Projected Changes in Temperature and Precipitation Extremes over China as Measured by 50-yr Return Values and Periods Based on a CMIP5 Ensemble

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Advances in Atmospheric Sciences 2018年第4期35卷 376-388页

作者： Ying XU xuejie gao Filippo GIORGI Botao ZHOU Ying SHI Jie WU Yongxiang ZHANG National Climate Center China Meteorological Administration Beijing 100081 China Climate Change Research Center Institute of Atmospheric Sciences Chinese Academy of Sciences Beijing 100029 China The Abdus Salam International Centre for Theoretical Physics PO Box 586 Trieste 34100 Italy CMA-NJU Joint Laboratory for Climate Prediction Studies ( LCPS/CMA-NJU) Nanjing 210023 China University of Chinese Academy of Sciences Beijing 100049 China

Future changes in the 50-yr return level for temperature and precipitation extremes over China's Mainland are investigated based on a CMIP5 multi-model ensemble for RCP2.6, RCP4.5 and RCP8.5 scenarios. The following indices are analyzed： TXx and TNn （the annual maximum and minimum of daily annual maximum consecutive 5-day precipitation） and CDD maximum and minimum surface temperature）, RX5day （the （maximum annual number of consecutive dry days）. After first validating the model performance, future changes in the 50-yr return values and return periods for these indices are investigated along with the inter-model spread. Multi-model median changes show an increase in the 50-yr return values of TXx and a decrease for TNn, more specifically, by the end of the 21st century under RCP8.5, the present day 50-yr return period of warm events is reduced to 1.2 yr, while extreme cold events over the country are projected to essentially disappear. A general increase in RX5day 50-yr return values is found in the future. By the end of the 21st century under RCP8.5, events of the present RX5day 50-yr return period are projected to reduce to 〈 10 yr over most of China. Changes in CDD-50 show a dipole pattern over China, with a decrease in the values and longer return periods in the north, and vice versa in the south. Our study also highlights the need for further improvements in the representation of extreme events in climate models to assess the future risks and engineering design related to large-scale infrastructure in China.

关键词： CMIP5 extremes return values and periods China

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Assessing the sensitivity of RegCM4 to cumulus and ocean surface schemes over the Southeast Asia domain of the coordinated regional climate downscaling experiment

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Atmospheric and Oceanic Science Letters 2020年第1期13卷 71-79页

作者： WANG Zhengqi gao xuejie HAN Zhenyu WU Jia XU Ying JUNENG Liew Climate Change Research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijingChina National Climate Center China Meteorological AdministrationBeijingChina Faculty of Science and Technology Universiti Kebangsaan MalaysiaUKM BangiMalaysia

Multi-year experiments are conducted using the most recent version of the Abdus Salam International Centre for Theoretical Physics regional climate model RegCM4(version 4.7) to customize its performance over Southeast Asia - a region with few RCMs applied to date. The model is driven by ERA-Interim reanalysis data at a grid spacing of 25 km using the CORDEX(Coordinated Regional Climate Downscaling Experiment) Southeast Asia domain. The authors focus on comparing the convection schemes of Emanuel and Tiedtke(Tiedtke-1) and Tiedtke with effects of sea surface evaporation introduced(Tiedtke-2). The authors find that, for temperature over land, the model shows reasonable performance in reproducing the present-day climatology in both December–January–February(DJF) and June–July–August(JJA) in all the experiments. Meanwhile, cold biases prevail in both seasons, although portions of warm bias exist in DJF. For precipitation, the spatial pattern and amount, as well as seasonal evolution, are in general reproduced well in the *** performances of Tiedtke-1 and Tiedtke-2 are evident compared to Emanuel, particularly over ocean. Thereby, the optimal configuration of Reg CM4.7 for future climate change simulations over the region is identified as using the Tiedtke scheme with spray effects considered, along with the default settings for other physical parameterizations.

关键词： RegCM coordinated regional climate downscaling experiment convective scheme Southeast Asia

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Performance of RegCM4 over Major River Basins in China

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Advances in Atmospheric Sciences 2017年第4期34卷 441-455页

作者： xuejie gao Ying SHI Zhenyu HAN Meili WANG Jia WU Dongfeng ZHANG Ying XU Filippo GIORGI Climate Change Research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China National Climate Center China Meteorological AdministrationBeijing 100081China China Meteorological News Press China Meteorological AdministrationBeijing 100081China Shanxi Climate Center Taiyuan 030006China The Abdus Salam International Centre for Theoretical Physics Trieste 34100Italy

A long-term simulation for the period 1990–2010 is conducted with the latest version of the International Centre for Theoretical Physics＇ Regional Climate Model（RegCM4）, driven by ERA-Interim boundary conditions at a grid spacing of 25 km. The Community Land Model（CLM） is used to describe land surface processes, with updates in the surface parameters,including the land cover and surface emissivity. The simulation is compared against observations to evaluate the model performance in reproducing the present day climatology and interannual variability over the 10 main river basins in China,with focus on surface air temperature and precipitation. Temperature and precipitation from the ERA-Interim reanalysis are also considered in the model assessment. Results show that the model reproduces the present day climatology over China and its main river basins, with better performances in June–July–August compared to December–January–February（DJF）.In DJF, we find a warm bias at high latitudes, underestimated precipitation in the south, and overestimated precipitation in the north. The model in general captures the observed interannual variability, with greater skill for temperature. We also find an underestimation of heavy precipitation events in eastern China, and an underestimation of consecutive dry days in northern China and the Tibetan Plateau. Similar biases for both mean climatology and extremes are found in the ERA-Interim reanalysis, indicating the difficulties for climate models in simulating extreme monsoon climate events over East Asia.

关键词： regional climate model RegCM4 China river basin CLM

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In-situ polymerized carbonate induced by Li-Ga alloy as novel artificial interphase on Li metal anode

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中国化学快报:英文版 2023年第9期34卷 294-299页

作者： Ziping Wang Shuyuan Xie xuejie gao Xinyang Chen Lina Cong Jun Liu Haiming Xie Chuang Yu Yulong Liu School of Chemistry Northeast Normal UniversityChangchun 130024China Center for Lignocellulosic Chemistry and Biomaterials College of Light Industry and Chemical EngineeringDalian Polytechnic UniversityDalian 116034China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China

Li metal is considered an ideal anode material because of its high theoretical capacity and low electrode ***,the practical usage of Li metal as an anode is severely limited because of inevitable parasitic side reactions with electrolyte and dendrites *** present,single-component artificial solid electrolyte interphase cannot simultaneously meet the multiple functions of promoting ion conduction,guiding lithium ion deposition,inhibiting dendrite growth,and reducing interface side ***,multi-component design on Li metal surface is widely investigated to achieve long-term ***,we report a Li_(2)Ga-carbonate polymer interphase layer to solve volume changes,Li dendrites formation and *** a result,the Li symmetric cell can be stabilized at 3.0 m A/cm^(2)in carbonate electrolyte with limited volume of 20μ*** with 13.6 mg/cm^(2)(loading of 2 mAh/cm^(2))LiFePO_(4)cathode,discharge capacity retains at 90%for over 150 cycles under limited electrolyte *** such an alloy-polymer interphase layer,higher energy density Li metal batteries become prominent in the near future.

关键词： Lithium metal Alloy Polymer film High energy density Self-healing

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