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Nanodiamond reinforced self-healing and transparent poly(urethane-urea)protective coating for scratch resistance

International Journal of Smart and Nano Materials 2024年第1期15卷 75-94页

作者： Zhuochao Wang Wenxin Cao Chunqiang Sun Dongchao ji Kunlong Zhao Gang gao Xingchun Xu Yingqi Liu Tianyu Zhang jiaqi Zhu jiecai Han National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbinChina School of future technology Harbin institute of TechnologyHarbinChina Key Laboratory of Micro-systems and Micro-structures Manufacturing Ministry of EducationHarbinChina

With increasing demand for scratch-resistant flexible electro-nics,the development of transparent coatings with good scratch resistance and self-healing properties has emerged as a key research *** this study,a high-strength self-healing poly(urethane-urea)(PUU)-based nanocomposite coating was prepared by introducing functionalized nanodiamond(ND)into a PUU matrix via solution *** PUU matrix had hard-segment repeating units and was constructed using iso-phorone diamine and isophorone *** ND particles were modifed using a silane coupling agent,3-aminopropyl-triethoxysilane,to obtain well-dispersed KH-ND ***-ND promoted microphase separation in the PU matrix,inducing the formation of dense and homogeneous hard domains that dissipated stress,prevented further crack devel-opment,and improved the mechanical properties and scratch resistance of the *** addition,the coating exhibited excellent self-healing ***-transform infrared spectroscopy,scanning electron microscopy,and atomic force microscopy were used to characterize the self-healing and hardening mechanisms of the *** environmentally friendly PUU/KH-ND coating is easy to prepare and has broad application prospects in transparent and anti-scratch coatings for flexible electronics,automobiles,and home appliances.

关键词： Nanocomposite coatings self-healing scratch resistance transparent poly(urethane-urea)

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Sedimentary environment shift and organic matter enrichment mechanism in response to volcanic ash influence: A case study of the Permian Lucaogou Formation, Santanghu Basin,NW China

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Journal of Palaeogeography 2024年第4期13卷 793-822页

作者： Miao Yu Gang gao Miao Liu Hui Liang ji-Lun Kang Xiong-Fei Xu Xin-Ying Zhao College of Geosciences China University of Petroleum (Beijing) National Key Laboratory of Petroleum Resources and Engineering China University of Petroleum (Beijing) Petro China Tuha Oilfield Company

The second member of the Lucaogou Formation （P2l2） in the Tiaohu and Malang Sags of the Santanghu Basin （study area） underwent periodic volcanic activity and frequent lithological *** study comprehensively analyzed the organic geochemistry,mineral composition,organic matter （OM） types,volcanic cycle,and palaeoenvironment of shale in the study *** such as total organic carbon （TOC）,rock pyrolysis （Rock-Eval）,organic petrology,scanning electron microscopy （SEM） with energydispersive spectrum （EDS） analysis,X-ray diffraction （XRD）,trace elements,and saturated hydrocarbon gas chromatography and mass spectrometry （GC-MS） were *** findings suggest that limited terrigenous input during the sedimentary period of the P2l2led to the deposition of a distinctive mixture of volcanic ash （felsic） and carbonate （dolomite and calcite）,with a low average clay mineral content of 6%.The P2l2shale emerged as a high-quality source rock,predominantly composed of type I and II kerogens,with moderate OM *** deposition environment was characterized by hot and arid conditions,high salinity,and intensive reducibility,which was favorable for algae development and conducive to OM ***,two lamalginite types,labeled as lamalginite“A”and lamalginite“B,”were ***“B”-rich shales were deposited in a hotter and drier climate compared to lamalginite“A”-rich ***“B”-rich shale inexhibited high levels of C28regular sterane and β-carotenes,distinguishing it from lamalginite“A”-rich shale.A comprehensive analysis involving organic petrology,SEM,sedimentary environment,and biomarker characteristics suggests that lamalginite“B”may be a salt-tolerant green alga,while lamalginite“A”may be a ***,an OM enrichment model for the P2l2shale was established.

关键词： Volcanic ash Geochemistry Petrology Palaeoenvironment Lamalginite

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Metallic Sb-stabilized porous silicon with stable SEI and high electron/ion conductivity boosting lithium-ion storage performance

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Rare Metals 2024年第9期43卷 4234-4242页

作者： jia-Guo Deng Hao-Qin Feng Yu-Long Xu Si-Guang Guo jian-Ping Li Kai-Fu Huo ji-jiang Fu Biao gao Pual-K.Chu The State Key Laboratory of Refractories and Metallurgy and Institute of Advanced Materials and Nanotechnology Wuhan University of Science and TechnologyWuhan 430081China Wuhan National Laboratory for Optoelectronics(WNLO) School of Optical and Electronic InformationHuazhong University of Science and TechnologyWuhan 430074China Department of Physics Department of Materials Science&Engineeringand Department of Biomedical EngineeringCity University of Hong KongHong Kong 999077China

Silicon(Si)has mild discharge potential and high theoretical capacity,making it a highly desirable material for lithium-ion batteries(LIBs).Nevertheless,the excessive volume expansion,poor ion/electron conductiv ity and unstable solid electrolyte interface(SEI)hinde practical application to ***,the metallic antimony(Sb)stabilized porous Si(SiDSb)composite was prepared by magnesiothermic reduction of Sb_(2)O_(3)and Mg_(2)Si and chemical etching to remove the by-product of *** highly conductive Sb nanodots embedded in the Si liga ments promote not only the formation of conductive and stable LiF-rich SEI,but also the electron/ion transpor ability of *** to the outstanding bulk/interface stability,excellent conductivity,as well as ideal porous structure,the SiDSb electrode demonstrates a capacity of820 mAh·g^(-1)after undergoing 320 turns at 1000 mA·g^(-1).Additionally,it exhibits a stable capacity of 675 m Ah·g^(-1)when tested at a higher current density of 5000 m A·g^(-1).The results reveal a viable solution to solve three problems at the same time,namely the poor conductivity,inferior SEI and excessive volume expansion of Si,boding well for the design of Si-based materials for high-energy LIBs.

关键词： Silicon Anodes Lithium-ion batteries Antimony Solid electrolyte interphase

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Highly Thermally Conductive and Structurally Ultra‑Stable Graphitic Films with Seamless Heterointerfaces for Extreme Thermal Management

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Nano-Micro Letters 2024年第3期16卷 383-397页

作者： Peijuan Zhang Yuanyuan Hao Hang Shi jiahao Lu Yingjun Liu Xin Ming Ya Wang Wenzhang Fang Yuxing Xia Yance Chen Peng Li Ziqiu Wang Qingyun Su Weidong Lv ji Zhou Ying Zhang Haiwen Lai Weiwei gao Zhen Xu Chao gao MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and EngineeringKey Laboratory of Adsorption and Separation Materials and Technologies of Zhejiang ProvinceZhejiang University38 Zheda RoadHangzhou 310027People’s Republic of China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030032People’s Republic of China Beijing Spacecrafts Manufacturing Co. LtdBeijing Friendship Road 104Haidian DistrictBeijing 100094People’s Republic of China Beijing Institute of Space Mechanics and Electricity Beijing Friendship Road 104Haidian DistrictBeijing 100094People’s Republic of China China Academy of Aerospace Aerodynamics Beijing 100074People’s Republic of China Hangzhou gaoxi Technol Co. LtdHangzhou 311113People’s Republic of China International Research Center for X Polymers International CampusZhejiang UniversityHaining 314400People’s Republic of China

Highly thermally conductive graphitic film(GF)materials have become a competitive solution for the thermal management of high-power electronic ***,their catastrophic structural failure under extreme alternating thermal/cold shock poses a significant challenge to reliability and ***,we present the first investigation into the structural failure mechanism of GF during cyclic liquid nitrogen shocks(LNS),which reveals a bubbling process characterized by“permeation-diffusion-deformation”*** overcome this long-standing structural weakness,a novel metal-nanoarmor strategy is proposed to construct a Cu-modified graphitic film(GF@Cu)with seamless *** well-designed interface ensures superior structural stability for GF@Cu after hundreds of LNS cycles from 77 to 300 ***,GF@Cu maintains high thermal conductivity up to 1088 W m^(−1)K^(−1)with degradation of less than 5%even after 150 LNS cycles,superior to that of pure GF(50%degradation).Our work not only offers an opportunity to improve the robustness of graphitic films by the rational structural design but also facilitates the applications of thermally conductive carbon-based materials for future extreme thermal management in complex aerospace electronics.

关键词： Highly thermally conductive Structurally ultra-stable Graphitic film Extreme thermal management Liquid nitrogen bubbling

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In vivo imaging reveals a synchronized correlation among neurotransmitter dynamics during propofol and sevoflurane anesthesia

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Zoological Research 2024年第3期45卷 679-690页

作者： gao-Lin Qiu Li-Jun Peng Peng Wang Zhi-Lai Yang ji-Qian Zhang Hu Liu Xiao-Na Zhu jin Rao Xue-sheng Liu Department of Anesthesiology First Affiliated Hospital of Anhui Medical UniversityHefeiAnhui 230022China School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China

General anesthesia is widely applied in clinical ***,the precise mechanism of loss of consciousness induced by general anesthetics remains ***,we measured the dynamics of five neurotransmitters,includingγ-aminobutyric acid,glutamate,norepinephrine,acetylcholine,and dopamine,in the medial prefrontal cortex and primary visual cortex of C57BL/6 mice through in vivo fiber photometry and genetically encoded neurotransmitter sensors under anesthesia to reveal the mechanism of general anesthesia from a neurotransmitter *** revealed that the concentrations of γ-aminobutyric acid,glutamate,norepinephrine,and acetylcholine increased in the cortex during propofol-induced loss of *** levels did not change following the hypnotic dose of propofol but increased significantly following surgical doses of propofol ***,the concentrations of the five neurotransmitters generally decreased during sevoflurane-induced loss of ***,the neurotransmitter dynamic networks were not synchronized in the non-anesthesia groups but were highly synchronized in the anesthetic *** findings suggest that neurotransmitter dynamic network synchronization may cause anesthetic-induced loss of consciousness.

关键词： General anesthesia Loss of consciousness In vivo neurotransmitter imaging Medial prefrontal cortex Primary visual cortex

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Cationic ordering transition in oxygen-redox layered oxide cathodes

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Carbon Energy 2024年第1期6卷 197-206页

作者： Xinyan Li Ang gao Qinghua Zhang Hao Yu Pengxiang ji Dongdong Xiao Xuefeng Wang Dong Su Xiaohui Rong Xiqian Yu Hong Li Yong-sheng Hu Lin Gu Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijingChina College of Materials Science and Opto-Electronic Technology University of Chinese Academy of SciencesBeijingChina Beijing National Center for Electron Microscopy and Laboratory of Advanced Materials School of Materials Science and EngineeringTsinghua UniversityBeijingChina Beijing Advanced Innovation Center for Materials Genome Engineering Huairou DivisionInstitute of PhysicsChinese Academy of SciencesBeijingChina

Understanding the structural origin of the competition between oxygen 2p and transition-metal 3d orbitals in oxygen-redox(OR)layered oxides is eminently desirable for exploring reversible and high-energy-density Li/Na-ion ***,we reveal the correlation between cationic ordering transition and OR degradation in ribbon-ordered P3-Na_(0.6)Li_(0.2)Mn_(0.8)O_(2) via in situ structural *** two different voltage windows,the OR capacity can be improved approximately twofold when suppressing the in-plane cationic ordering *** find that the intralayer cationic migration is promoted by electrochemical reduction from Mn^(4+)to Jahn–Teller Mn^(3+)and the concomitant NaO_(6) stacking transformation from triangular prisms to octahedra,resulting in the loss of ribbon ordering and electrochemical ***-principles calculations reveal that Mn^(4+)/Mn^(3+)charge ordering and alignment of the degenerate eg orbital induce lattice-level collective Jahn–Teller distortion,which favors intralayer Mn-ion migration and thereby accelerates OR *** findings unravel the relationship between in-plane cationic ordering and OR reversibility and highlight the importance of superstructure protection for the rational design of reversible OR-active layered oxide cathodes.

关键词： cationic ordering layered oxide cathodes oxygen redox sodium-ion batteries

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Atomic tracking of thermally-driven structural evolution in 2D crystals:Case of NbSe_(2)

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InfoMat 2024年第2期6卷 90-98页

作者： Baofei Hou Teng Zhang Tingting Wang Hongyan ji Huixia Yang Liangguang jia Xu Han jingsi Qiao Yu Zhang Liwei Liu Hong-Jun gao Yeliang Wang School of Integrated Circuits and Electronics&Yangtze Delta Region Academy Beijing Institute of TechnologyBeijingthe People's Republic of China Institute of Physics Chinese Academy of SciencesBeijingthe People's Republic of China

Advanced atomic tracking techniques play a critical role in characterizing structural evolution,elucidating fundamental mechanisms of exotic phenomena and tailoring delicate *** driven structural modulation in 2D crystals,such as the charge density wave(CDW),often leads to intriguing quantum properties,making them a valuable platform for exploring fundamental physics and potential device ***,despite their significance,experimental studies addressing atomic tracking of thermally-driven structural evolution in 2D crystals have been ***,we utilize high-accuracy variable-temperature atomic tracking measurements with scanning tunneling microscopy(STM)to directly observe a series of structural transitions in a model 2D crystal,namely NbSe_(2).With the atomic tracking technique,we confirm the existence of the universal thermally-driven CDW transition hysteresis between the heating and cooling *** transition hysteresis,characterized by a constant temperature offset,represents a new phenomenon of structural *** findings provide a feasible method to track CDW transitions at the atomic scale in 2D crystals,significantly contributing to a better understanding and the potential modulation of these materials'functions in nanodevices.

关键词： 2D crystal atomic tracking technique structural evolution temperature hysteresis

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Dimethylsulfoniopropionate (DMSP) Increases Longevity and Mitochondrial Function in Caenorhabditis elegans: Implications for the Role of the Global Sulfur Cycle in Terrestrial Ecosystems

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Environment & Health 2024年第8期2卷 572-585页

作者： Hongyuan Li Peng ji Yue Cao Zhitao Cui jingwei gao Hongshuang Wang Cong Lin Yibo Wang Xiaohui Wang Laboratory of Chemical Biology Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China The Key Laboratory of Molecular Epigenetics of the Ministry of Education Northeast Normal UniversityChangchun 130024China Department of Geriatrics The First Hospital of Jilin UniversityChangchun 130021China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026China Beijing National Laboratory for Molecular Sciences Beijing 100190China

Dimethylsulfoniopropionate(DMSP)is a compound synthesized by marine phytoplankton that contributes to the oceanic sulfur ***,DMSP has also been found in algal species and several terrestrial plants,forming part of the global sulfur ***,compared to its role in the marine environment,the impact of DMSP on terrestrial ecosystems remains relatively *** this study,DMSP was shown to promote longevity and prevent age-associated functional decline in Caenorhabditis elegans(***),a soil-dwelling *** decreased mitochondrial content and improved mitochondrial function in *** at the old stage,which was via enhancing autophagy *** was demonstrated that DMSP significantly increased the expression of autophagy and mitophagy genes during ***,DMSP protected against Parkinson’s disease(PD)induced byα-synuclein(α-syn)aggregation via *** studies showed that DMSP directly activated nuclear translocation of the Skinhead-1(SKN-1)transcription factor from the ***,SKN-1 was involved in DMSP-induced autophagy and played a key role in lifespan extension andα-syn clearance in *** conclusion,DMSP delays physiological aspects of aging in ***,providing insights into the interplay between the global sulfur cycle and terrestrial organisms.

关键词： DMSP C.elegans terrestrial ecosystem aging autophagy

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“两个结合”重要论断对中国特色社会主义发展规律的深化认识

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北京社会科学 2024年第5期 4-13页

作者：高继文山东师范大学马克思主义学院

“两个结合”重要论断以新的视野深化对中国特色社会主义的认识,深刻揭示了其形成发展规律。这主要表现为:丰富和发展“一个结合”“两个逻辑”思想,表明中国特色社会主义是科学社会主义中国化时代化的产物,同时是中华文明演进和中华优... 详细信息

“两个结合”重要论断以新的视野深化对中国特色社会主义的认识,深刻揭示了其形成发展规律。这主要表现为:丰富和发展“一个结合”“两个逻辑”思想,表明中国特色社会主义是科学社会主义中国化时代化的产物,同时是中华文明演进和中华优秀传统文化传承的结果,是中国历史发展的必由之路;坚定文化自信和历史自信,以“第二个结合”筑牢了中国特色社会主义道路的文化根基,凸显了新时代中国文化和中华民族现代文明建设的重要性;突出马克思主义与中华优秀传统文化相契合,阐明中国特色社会主义深深根植于中华优秀传统文化,充分彰显了中国道路的文化内涵和独特优势;明确了新征程党的理论创新方向,昭示坚持和发展新时代中国特色社会主义必须在理论上加强对中国式现代化、建设中华民族现代文明等重大课题的研究和创新。

关键词： “两个结合” “两个逻辑” 中国特色社会主义文化自信中华优秀传统文化

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Research paper Air atmosphere available fast one-pot synthesis of VO_(2)nanoparticles with excellent thermochromic properties by a novel liquid-shielding method

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Journal of Materiomics 2024年第1期10卷 17-26页

作者： Zhi Cao jin Li Chunhui Zhang Ke jiao Yunxiang Chen Yifei Liu Xinghui Hou Haipeng ji Liying Zhang Shasha Yi Yu Wang Zhang Chen Yanfeng gao Zongtao Zhang School of Materials Science and Engineering Zhengzhou UniversityKexue Ave 100Zhengzhou450001China School of Materials Science and Engineering Shanghai UniversityShangda Rd 99Shanghai200444China

As a typical strongly correlated transition oxide,vanadium dioxide(VO_(2))based nanomaterials have drawn many research attentions these years due to the giant metal-to-insulator phase transition(MIPT)at around 68℃.However,due to the complexities of the V-O system and interplays between various vanadium oxide phases,the synthesis of high-quality VO_(2)nanopowders is still fraught with many challenges,especially in air *** this paper,we report a novel air atmosphere available liquid-shielding synthesis method for thermochromic VO_(2)nanoparticles,by using low-eutectic molten-salt(LiCl-KCl)as the liquid-state air-insulation medium at elevated temperature and high-pressure pressed VOSO_(4)-KCl pillars immersed in these liquid salts as the *** amounts of glucose are added to introduce a slight reductive environment,and well dispersed VO_(2)nanoparticles with excellent ther-mochromic properties can be directly synthesized at an ultra-low temperature of 375℃.This feasible and atmosphere-available mass-production method is rarely reported in the related fields,which may provide a novel protocol strategy for the synthesis of high performance thermochromic VO_(2)and other functional oxide powders.

关键词： Vanadium dioxide Nanoparticle Molten salt Liquid shielding Thermochromic properties

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