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Polypyride intercalation boosting the kinetics and stability of V_(3)O_(7)·H_(2)O cathodes for aqueous zinc-ion batteries

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Journal of Energy Chemistry 2024年第10期97卷 361-370,I0007页

作者： Qingqing He Jie Bai Mengda Xue Yanxin liao Huayu Wang Mujun long Lingyun Chen Department of Applied Chemistry School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 41331China Laboratoryof Materials and Metallurgy Cllege of Materials Science and EngineeringChongqing UniversityChongqing 400044Chin

V_(3)O_(7)·H_(2)O(VO)is a high capacity cathode material in the field of aqueous zinc ion batteries(AZIBs),but it is limited by slow ion migration and low electrical *** this paper,polypyridine(PPyd)intercalated VO with nanoribbon structure was prepared by a simple in-situ pre-intercalation,which is noted *** total density of states(TDOS)shows that after the pre-intercalation of PPyd,an intermediate energy level appears between the valence band and conduction band,which provides a step that can effectively reduce the band gap and enhance the electron ***,the density functional theory(DFT)results found that Zn^(2+)is more easily de-intercalated from the V-O skeleton,which proves that the embeddedness of PPyd improves the diffusion kinetics of Zn^(2+).Electrochemical studies have shown that VO-PPyd cathode materials exhibit excellent rate performance(high specific capacity of 465 and 192 mA h g^(-1)at 0.2 and 10 A g^(-1),respectively)and long-term cycling performance(92.7%capacity retention rate after 5300 cycles),due to their advantages in structure and *** importantly,the energy density of VO-PPyd//Zn at 581 and 5806 W kg^(-1)is 375 and 247 W h kg^(-1),***-PPyd exhibits excellent electrochemical properties compared to previously reported vanadium based cathodes,which makes it highly competitive in the field of high-performance cathode materials of AZIBs.

关键词： V_(3)O_(7)·H_(2)O Polypyridine Ion migration Electrical conductivity Aqueous zinc ion batteries DFT calculation

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Analysis of the regional spectral properties in northwestern South China Sea based on an empirical orthogonal function

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Acta Oceanologica Sinica 2020年第7期39卷 107-114页

作者： Dongyang fu Yuye Huang Dazhao Liu Shan liao Guo Yu Xiaolong Zhang College of Electronic and Information Engineering Guangdong Ocean UniversityZhanjiang 524088China State Key Laboratory of Tropical Oceanography South China Sea Institute of OceanologyChinese Academy of SciencesGuangzhou 510301China University of Chinese Academy of Sciences Beijing 100049China

This study presents an analysis of the spectral characteristics of remote sensing reflectance(Rrs)in northwestern South China Sea based on the in situ optical and water quality data for August *** initially divided into four classes,classes A to D,using the max-classification algorithm,and the spectral properties of whole Rrs were characterized using the empirical orthogonal function(EOF)***,the dominant factors in each EOF mode were *** results indicated that more than 95%of the variances of Rrs are partly driven by the back-scattering characteristics of the suspended *** initial two EOF modes were well correlated with the total suspended matter and back-scattering ***,the first EOF modes of the four classes of Rrs(A-D Rrs-EOF1)significantly contributed to the total variances of each Rrs *** addition,the correlation coefficients between the amplitude factors of class A-D Rrs-EOF1 and the variances of the relevant water quality and optical parameters were better than those of the unclassified *** spectral shape of class ARrs-EOF1 was governed by the absorption characteristic of chlorophyll a and colored dissolved organic matter(CDOM).The spectral shape of class B Rrs-EOF1 was governed by the absorption characteristic of CDOM since it exhibited a high correlation with the absorption coefficient of CDOM(ag(λ)),whereas the spectral shape of class C Rrs-EOF1 was governed by the back-scattering characteristics but not affected by the suspended *** spectral shape of class D Rrs-EOF1 exhibited a relatively good correlation with all the water quality parameters,which played a significant role in deciding its spectral shape.

关键词： northwestern South China Sea remote sensing reflectance empirical orthogonal function analysis ocean color control factors

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The Measurement of the Software Ecosystem’s Productivity with GitHub

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Computer Systems Science & Engineering 2021年第1期36卷 239-258页

作者： Zhifang liao Yiqi Zhao Shengzong Liu Yan Zhang Limin Liu Jun long School of Computer Science and Engineering Central South UniversityChangsha410075China School of Information Technology and Management Hunan University of Finance and EconomicsChangsha410075China Department of Computing School of ComputingEngineering and Built EnvironmentGlasgow Caledonian UniversityGlasgowG40BAUK

Software productivity has always been one of the most critical metrics for measuring software ***,with the open-source community(e.g.,GitHub),new software development models are *** traditional productivity metrics do not provide a comprehensive measure of the new software development ***,it is necessary to build a productivity measurement model of open source software ecosystem suitable for the open-source community’s production *** on the natural ecosystem,this paper proposes concepts related to the productivity of open source software ecosystems,analyses influencing factors of open source software ecosystem productivity,and constructs a measurement model using these *** validation experiments show that the model is compatible with a large portion of open source software ecosystems in *** study can provide references for participants of the open-source software ecosystem to choose proper types of *** study also provides a basis for ecosystem health assessment for researchers interested in ecosystem quality.

关键词： Software ecosystem open-source software ecosystem OSSECO productivity productivity model

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An Overview of Research in Distributed Attitude Coordination Control

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IEEE/CAA Journal of Automatica Sinica 2015年第2期2卷 121-133页

作者： long Ma Haibo Min Shicheng Wang Yuan Liu Shouyi liao Second Artillery Engineering University

This paper provides an overview of attitude coordination problems of multi-rigid-body with the goal of promoting research in this area. Theoretical results regarding consensus seeking with different system models, different communication topologies, different control goals and different techniques are summarized. And applications of consensus protocols to multirigid- body coordination are investigated. Finally, some future research directions and open problems are also proposed. © 2014 Chinese Association of Automation.

关键词： Control systems Synchronization

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Performance of a thermally regenerative ammonia-based battery using gradient-porous copper foam electrodes

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Science China(Technological Sciences) 2021年第4期64卷 696-704页

作者： LU ZhiQiang ZHANG YongSheng ZHANG Liang LI Jun fu Qian ZHU Xun liao Qiang Key Laboratory of Low-Grade Energy Utilization Technologies and Systems Ministry of EducationChongqing 400030China Institute of Engineering Thermophysics School of Energy and Power EngineeringChongqing UniversityChongqing 400030China

Gradient-porous copper foam electrodes were applied to alleviate the adverse effects of the uneven current distribution of electrodes along the electrolyte flow direction in thermally regenerative ammonia-based batteries(TRABs).The results indicated that gradient-porous copper foam with a decreasing pore size(TRAB-LMS)provided the most uniform current distribution and generated the highest power density(15.5 W/m^(2)),total charge(1800 C)and energy density(1224 W h/m^(3)).With the increase in flow rate,the power density of the TRAB-LMS increased considerably within a certain range and then decreased slightly,with the optimal flowrate at 15 mL/*** the optimal flow rate,the performance of TRAB-LMS increased when the ammonia concentration rose from 0.5 to 2 M(1 M=1 mol L^(-1));however,it decreased slightly when the ammonia concentration further increased to 3 *** slight decrease in the cathode potential suggested that the flow and ammonia concentration beyond the optional values facilitated not only the transfer of ammonia into the porous anode,but also the crossover of ammonia from the anode to the cathode.

关键词： thermally regenerative ammonia-based battery gradient-porous electrode current distribution mass transfer

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Effect of operating parameters on the performance of thermally regenerative ammonia-based battery for low-temperature waste heat recovery

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Chinese Journal of Chemical Engineering 2021年第4期34卷 335-340页

作者： Yu Shi Liang Zhang Jun Li Qian fu Xun Zhu Qiang liao Yongsheng Zhang Key Laboratory of Low-grade Energy Utilization Technologies and Systems Ministry of EducationChongqing 400030China

This study investigated the important factors that affect the operating parameters of thermally regenerative ammoniabased batteries(TRABs),including the metal electrode type,membrane type,electrode surface area,electrode distance,electrolyte concentration,and ammonia *** experimental results showed that the maximum power density of TRABs with a Cu electrode was 40.0 W·m^(2),which was considerably higher than that with Ni(0.34 W·m^(2))and Co(0.14 W·m^(2))*** with an anion exchange membrane had a 28.6%higher maximum power density than those with a cation exchange *** increased electrode surface resulted in an increased maximum power but a decreased maximum power *** a certain range,TRAB performance was enhanced with decreased electrode distance and increased electrolyte *** increased ammonia concentration resulted in enhanced ammonia transfer and improved the TRAB performance.

关键词： Electrochemistry Thermally regenerative ammonia-based battery Recovery Renewable energy

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Probiotic cocktails accelerate baicalin metabolism in the ileum to modulate intestinal health in broiler chickens

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Journal of Animal Science and Biotechnology 2024年第2期15卷 779-794页

作者： Mingkun Gao Chaoyong liao Jianyang fu Zhonghua Ning Zengpeng Lv Yuming Guo State Key Laboratory of Animal Nutrition and Feeding College of Animal Science and TechnologyChina Agricultural UniversityBeijing 100193China National Engineering Laboratory for Animal Breeding College of Animal Science and TechnologyChina Agricultural UniversityBeijing 100193China

Background Baicalin and probiotic cocktails are promising feed additives with broad application *** probiotic cocktails are known to enhance intestinal health,the potential synergistic impact of combining baicalin with probiotic cocktails on the gut health of broiler chickens remains largely ***,this study aims to investigate the influence of the combined administration of baicalin and probiotic cocktails on the composition of ileal and cecal microbiota in broiler chickens to elucidate the underlying mechanisms responsible for the healthpromoting *** A total of 3201-day-old male Arbor Acres broilers were divided into 4 groups,each with 8 replicates of 10 chicks per *** a period of 42 d,the birds were fed a basal diet or the same diet supplemented with 37.5 g/t baicalin(BC),1,000 g/t probiotic cocktails(PC),or a combination of both BC(37.5 g/t)and PC(1,000 g/t).The results demonstrated that BC+PC exhibited positive synergistic effects,enhancing intestinal morphology,immune function,and barrier *** was evidenced by increased VH/CD ratio,sIgA levels,and upregulated expression of occludin and claudin-1(P<0.05).16S rRNA analysis indicated that PC potentiated the effects of BC,particularly in the ileum,where BC+PC significantly increased theα-diversity of the ileal microbiota,altered itsβ-diversity,and increased the relative abundance of Flavonifractor(P<0.05),a flavonoid-metabolizing ***,Flavonifractor positively correlated with chicken ileum crypt depth(P<0.05).While BC+PC had a limited effect on cecal microbiota structure,the PC group had a very similar microbial composition to BC+PC,suggesting that the effect of PC at the distal end of the gut overshadowed those of *** We demonstrated the synergistic enhancement of gut health regulation in broiler chickens by combining baicalin and probiotic *** cocktails enhanced the effects of baicalin and accelerated its metab

关键词： Baicalin Gut health Ileal microbiota Probiotic cocktails Synergistic effects

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A compilation of known QSOs for the Gaia mission

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Research in Astronomy and Astrophysics 2019年第2期19卷 151-160页

作者： Shi-long liao Zhao-Xiang Qi Su-Fen Guo Zi-Huang Cao Shanghai Astronomical Observatory Chinese Academy of Sciences School of Astronomy and Space Science University of Chinese Academy of Sciences National Astronomical Observatories Chinese Academy of Sciences

Quasars are essential for astrometry in the sense that they are spatially stationary because of their large distance from the Sun. The European Space Agency(ESA) astrometric satellite Gaia is scanning the whole sky with unprecedented accuracy up to the level of a few μas. However, Gaia's two-fields-ofview-observation strategy may introduce a parallax bias in the Gaia catalog. Since it presents no significant parallax, a quasar is the perfect natural object to detect such bias. More importantly, quasars can be used to construct a celestial reference frame in the optical wavelengths for the Gaia mission. In this paper, we compile a list of known quasars that have been published in the literatures. The final compilation(designated as Known Quasars Catalog for Gaia mission, KQCG) contains 1 842 076 objects, among which797 632 objects are found in Gaia DR1 after cross-identifications. Redshift, color information and position uncertainties of the objects are also provided if available. This catalog will be very useful for the Gaia mission.

关键词： quasars:general astrometry parallaxes proper motions reference systems catalogs

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Phenomenology of colored radiative neutrino mass model and its implications on cosmic-ray observations

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Chinese Physics C 2018年第10期42卷 1-18页

作者： Ran Ding Zhi-long Han Li Huang Yi liao Center for High Energy Physics Peking UniversityBeijing 100871China School of Physics and Technology University of JinanJinanShandong 250022China State Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China School of Physics Nankai UniversityTianjin 300071China

We extend the colored Zee-Babu model with a gauged U（1）B-L symmetry, and a scalar singlet dark matter （DM） candidate S. The spontaneous breaking of U（1）B-L leaves a residual Z2 symmetry that stabilizes the DM, and generates a tiny neutrino mass at the two-loop level with the color seesaw mechanism. After investigating the DM and flavor phenomenology of this model systematically, we further focus on its imprint on two cosmic-ray anomalies： The Fermi-LAT gamma-ray excess at the Galactic Center （GCE）, and the PeV ultra-high energy （UHE） neutrino events at the IceCube. We found that the Fermi-LAT GCE spectrum can be well-fitted by DM annihilation into a pair of on-shell singlet Higgs mediators while being compatible with the constraints from the relic density, direct detections, and dwarf spheroidal galaxies, in the Milky Way. Although the UHE neutrino events at the IceCube could be accounted for by the resonance production of a TeV-scale leptoquark, the relevant Yukawa couplings have been severely limited by the current low-energy flavor experiments. We subsequently derive the IceCube limits on the Yukawa couplings by employing its latest six-year data.

关键词： neutrino mass models gamma-ray excess at galactic center IceCube neutrinos dark matter

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ARCHER:a ReRAM-based accelerator for compressed recommendation systems

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Frontiers of Computer Science 2024年第5期18卷 147-160页

作者： Xinyang SHEN Xiaofei liao long ZHENG Yu HUANG Dan CHEN Hai JIN National Engineering Research Center for Big Data Technology and System Services Computing Technology and System LabClusters and Grid Computing LabSchool of Computer Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China

Modern recommendation systems are widely used in modern data *** random and sparse embedding lookup operations are the main performance bottleneck for processing recommendation systems on traditional platforms as they induce abundant data movements between computing units and ***-based processing-in-memory(PIM)can resolve this problem by processing embedding vectors where they are ***,the embedding table can easily exceed the capacity limit of a monolithic ReRAM-based PIM chip,which induces off-chip accesses that may offset the PIM ***,we deploy the decomposed model on-chip and leverage the high computing efficiency of ReRAM to compensate for the decompression performance *** this paper,we propose ARCHER,a ReRAM-based PIM architecture that implements fully yon-chip recommendations under resource ***,we make a full analysis of the computation pattern and access pattern on the decomposed *** on the computation pattern,we unify the operations of each layer of the decomposed model in multiply-and-accumulate *** on the access observation,we propose a hierarchical mapping schema and a specialized hardware design to maximize resource *** the unified computation and mapping strategy,we can coordinatethe inter-processing elements *** evaluation shows that ARCHER outperforms the state-of-the-art GPU-based DLRM system,the state-of-the-art near-memory processing recommendation system RecNMP,and the ReRAM-based recommendation accelerator REREC by 15.79×,2.21×,and 1.21× in terms of performance and 56.06×,6.45×,and 1.71× in terms of energy savings,respectively.

关键词： recommendation system ReRAM processing-in-memory embedding layer

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