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A review on plasma-based CO_(2) utilization:process considerations in the development of sustainable chemical production

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Plasma Science and Technology 2024年第9期26卷 1-16页

作者： Sirui LI Giulia De FELICE Simona EICHKORN Tao SHAO fausto gallucci Department of Chemical Engineering and Chemistry Eindhoven University of TechnologyEindhoven 5612 AZthe Netherlands Institute of Electrical Engineering Chinese Academy of SciencesBeijing 100190People’s Republic of China

Plasma-based processes,particularly in carbon capture and utilization,hold great potential for addressing environmental challenges and advancing a circular carbon *** significant progress has been made in understanding plasma-induced reactions,plasma-catalyst interactions,and reactor development to enhance energy efficiency and conversion,there remains a notable gap in research concerning overall process *** review emphasizes the critical need for considerations at the process level,including integration and intensification,to facilitate the industrialization of plasma technology for chemical *** centered on the development of plasma-based processes are made with a primary focus on CO_(2) conversion,offering insights to guide future work for the transition of the technology from laboratory scale to industrial *** of current research gaps,especially in upscaling and integrating plasma reactors with other process units,is the key to addressing critical *** review further delves into relevant research in process evaluation and assessment,providing methodological insights and highlighting key factors for comprehensive economic and sustainability ***,recent advancements in novel plasma systems are reviewed,presenting unique advantages and innovative concepts that could reshape the future of process *** review provides essential information for navigating the path forward,ensuring a comprehensive understanding of challenges and opportunities in the development of plasma-based CCU process.

关键词： non-thermal plasma carbon capture and utilization process integration process intensification techno-economic analysis life cycle analysis

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The significance of NO_(2) dimerization in plasma-based NO_(x) synthesis for nitrogen fixation

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Journal of Energy Chemistry 2024年第12期99卷 522-528页

作者： Thijs van Raak Huub van den Bogaard fausto gallucci Sirui Li Sustainable Process Engineering Department of Chemical Engineering and ChemistryEindhoven University of TechnologyDe Rondom 70Eindhoven 5612 APthe Netherlands Eindhoven Institute for Renewable Energy Systems(EIRES) Eindhoven University of TechnologyPO Box 513Eindhoven 5600 MBthe Netherlands

Plasma-based NO_(x) synthesis has been considered as a sustainable alternative to the conventional HaberBosch *** the advancements in research achieved in recent years,limited attention has been paid to the reversible dimerization reaction of NO_(2) to N_(2)O_(4).This reaction can significantly alter the parameters considered with the process’output,such as the concentration or volume fraction of products and the energy *** work aims to investigate the significance of dimerization through theoretical analysis and *** were conducted with a 2D-gliding arc reactor to evaluate the influence of dimerization in the case of plasma reactor *** was observed that the dimerization reaction reached equilibrium in microseconds,resulting in a maximum hypothetical NO_(2) equilibrium conversion of 48.8%.For plasma experiments,the dimerization could cause a maximum error of 14.1%in product detection,which needs to be carefully considered along with the influence of temperature variations on the measurement.

关键词： Nitrogen fixation N_(2)O_(4) Dimerization NO_(x)synthesis Non-thermal plasma Gliding arc reactor

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可持续能源转化的过程强化

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国外科技新书评介 2016年第7期 7-7页

作者： fausto gallucci 陈宏刚不详华北电力大学

过程强化是被产业界和学术界共同关注的热点，被广泛看作是改善化学工业竞争能力的关键。本质上过程强化的目标是创新性（反应器）的概念设计，以实现更小、更安全、更高效和更廉价的过程。

关键词：过程强化能源转化竞争能力化学工业概念设计学术界反应器

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Catalytic steam methane reforming enhanced by CO_2 capture on CaO based bi-functional compounds

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Journal of Energy Chemistry 2017年第5期26卷 1014-1025页

作者： Francesca Micheli Manuela Sciarra Claire Courson Katia gallucci Institut de Chimie et Procédés pour l'énergie l'Environnement et la Santé UMR CNRS 7515 ECPM University of Strasbourg Department of Industrial Engineering University of L'Aquila

Sorption enhanced steam methane reforming（SE-SMR） was performed to maximize hydrogen production and contemporary remove COfrom the product stream using bi-functional sorbent-catalyst *** were tested at two different scales: micro and laboratory. The CaO amount varied in the CaO-CaAlOsorbent system synthesized by wet mixing(CaO content of 100 wt%, 56 wt%, 30 wt%, or 0 wt% and balance of CaAlO) which were upgraded to bi-functional compounds by impregnation of 3 wt% of Ni. Nitrogen adsorption（BET/BJH）, X-Ray Diffraction（XRD）, Temperature-Programmed Reduction（TPR） and Scanning and Transmission Electronic Microscopy（SEM and TEM, respectively） analyses were performed to characterize structural and textural properties and reducibility of the bi-functional materials and evaluate their catalytic behavior. A fixed sorbent composition CaO-CaAlO(56 wt% of CaO and CaAlObalance), was chosen to study the effect of different weight hourly space times（WHST） and CHstream compositions in SE-SMR activity. Impregnated mayenite at both micro and laboratory scales showed stable Hcontent of almost 74%, with CHconversion of 72% similarly to the values reported by the sample containing 30 wt% of CaO in the *** with 30 wt% of CaO showed promisingly behavior, enhancing Hcontent up to almost 94.5%.When the sorption enhanced reaction is performed roughly 89% of CHconversion is achieved, and after the pre-breakthrough, the catalyst worked at the thermodynamic level. During cycling sorption/regeneration experiments, even if COremoval efficiency slightly decreases, CHconversion and Hyield remain stable.

关键词： Sorption enhanced steam methane reforming By-functional sorbent-catalyst compounds Calcium oxide Nickel catalyst Mayenite

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Preparation of Ampoules With B2O3 Coating on GaAs Surface for Space Experiments

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Journal of Semiconductors 1997年第1期18卷 61-63页

作者：周伯骏,E.Jensen,A.gallucci,R.Abbaschian University of Florida-Gainesuille 美国

A new B2O3 coating technique has been developed for the manufacture of liquidencapsulated float zone GaAs ampoules for on-orbit processing. The B2O3 coating is applied tothe surface of the GaAs rod in such a manner that it does not come into contact with thequartz tube. This eliminates problems encountered due to the differences in thermal expansionbetween quartz and boric oxide.

关键词： paste

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177个巨型储罐中的放射性污染淤泥该如何处理

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科技纵览 2020年第5期 26-35页

作者： Maria gallucci

这里有若干个“最”。记者称它为西半球污染最严重之地。这里也坐落着世界上最大的建筑项目之一。位于美国华盛顿州中南部的汉福德场区的沙质土壤下埋藏着177个巨型储罐,装满了过去44年间核材料生产残留的放射性物质。从第二次世界大战... 详细信息

这里有若干个“最”。记者称它为西半球污染最严重之地。这里也坐落着世界上最大的建筑项目之一。位于美国华盛顿州中南部的汉福德场区的沙质土壤下埋藏着177个巨型储罐,装满了过去44年间核材料生产残留的放射性物质。从第二次世界大战到冷战期间,汉福德生产的环装备了6万余件核武器,包括1945年8月将日本长崎夷为平地的原子弹。

关键词：放射性物质沙质土壤放射性污染美国华盛顿州日本长崎冷战期间储罐福德

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The influence of resistance training on adipokines in post-menopausal women:A brief review

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Sports Medicine and Health Science 2022年第4期4卷 219-224页

作者： Tomas Chapman-Lopez Dylan Wilburn Emma Fletcher Kathleen Adair Ahmed Ismaeel Jeffery Heileson Andrew gallucci LesLee Funderburk Panagiotis Koutakis Jeffrey S.Forsse Department of Health Human Performance and Recreation Baylor UniversityWacoTX76706USA Clinical Muscle Biology Lab Biology DepartmentBaylor UniversityWacoTX76798USA Department of Physiology University of Kentucky780 Rose St.MS508LexingtonKY40536USA Human Sciences and Design Baylor UniversityWacoTX76798USA

The onset of menopause elicits changes in body composition that negatively influence adipokine ***,various health risk factors(e.g.,cardiovascular disease,osteoporosis,physical inactivity,obesity,arterial hypertension,hypercholesterolemia,sarcopenia)are influenced by adipokines due to changes in body composition after ***,improvements in body composition are considered the primary influencer of *** several therapeutic interventions(e.g.,medication,diet,meditation,exercise)are employed to target changes in body composition,resistance training appears to be more effective in positively improving body composition through changes in lean-muscle mass/fat-mass ***,due to the lack of research,very little is known about adipokines'anti/inflammatory response in postmenopausal women after completing resistance *** resistance training studies in postmenopausal women have focused on leptin,adiponectin,and resistin,with limited research assessing other adipokines that are important in metabolic regulation and inflammatory ***,the consistency of resistance training protocols as an intervention is not standardized or fully ***,the focus of this review is to establish a more comprehensive understanding of the benefits of resistance training on influencing adipokine levels based on changes to total body composition in postmenopausal women.

关键词： Adipokines Post-menopause Resistance training Body composition

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