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Color and Gloss Changes of a Lignin-Based Polyurethane Coating under Accelerated Weathering

Journal of Renewable Materials 2024年第2期12卷 305-323页

作者： Fatemeh Hassani Khorshidi Saeed Kazemi najafi farhood najafi Antonio Pizzi Dick Sandberg Rabi Behrooz Department of Wood Science and Technology Faculty of Natural ResourcesTarbiat Modares UniversityTehranIran Department of Resin and Additives Institute for Color Science and TechnologyP.O.Box 16765-654TehranIran LERMAB University of LorraineBlvd des AiguillettesNancy54000France Wood Science and Engineering LuleåUniversity of TechnologySkellefteåSweden

The purpose of this research study was to investigate the properties of polyurethane coatings based on lignin *** this purpose,the prepared coatings were applied to pine wood surfaces and weathered ***,color and gloss of the coatings were measured before and after the weathering *** emission scanning electron microscopy(FE-SEM)micrographs prepared from the coatings showed that the average size of nano-particles in the polyurethane substrate was approximately 500 *** magnetic resonance(13C-NMR)spectroscopy showed that strong urethane bonds were formed in the nano-lignin-based *** calorimetric analysis(DSC)test revealed that the glass-transition temperature(Tg)of lignin nanoparticles modified with diethylenetriamine(DETA)was 112.8℃ and Tg of lignin nano-particles modified with ethylenediamine(EDA)was 102.5℃,which is lower than the Tg of un-modified lignin(114.6℃)and lignin modified with DETA(126.8℃)and lignin modified with EDA(131.3℃).The coatings modified with lignin nano-particles had a greater change in *** lignin nano-particles in the modified coating are trapping hydroxyl radicals which reduces photoactivity and yellowing of the polyurethane by about 3 times compared to unmodified polyurethane *** weathering test,the nano-lignin-based coating had a rougher surface with a lower contact angle(0.78°)compared to the unmodified polyurethane coating(0.85°).

关键词： Amination propylene carbonate lignin biopolymer polyurethane coating polyol UN SDG 13

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Effect of Amine Type on Lignin Modification to Evaluate Its Reactivity in Polyol Construction for Non-Isocyanate Polyurethanes(NIPU)

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Journal of Renewable Materials 2023年第5期11卷 2171-2190页

作者： Saeed Kazemi najafi farhood najafi Antonio Pizzi Fatemeh Hassani Khorshidi Rabi Behrooz Department of Wood Science and Technology Faculty of Natural ResourcesTarbiat Modares UniversityTehranIran Department of Resin and Additives Institute for Color Science and TechnologyTehranIran LERMAB University of LorraineBlvd des AiguillettesNancyFrance

Polyols are groups of organic compounds which contain carbon and are randomly linked to other atoms,especially carbon-carbon and *** compounds are mainly used as reactants to make other *** biopolymers,lignin is regarded as the base of a new polymer in polyol *** present study aimed to investigate the effects of amine type(diethylenetriamine and ethylenediamine)on the modification of lignin-based polyols,so as to provide an alternative to petroleum polyols and,in turn,increase functional groups and reduce their harm to humans’health and the *** this aim,first,lignin was extracted from raw ***,the extracted lignin was reacted with diethylenetriamine(DETA)and ethylenediamine(EDA).Finally,the Mannich method was used for the reaction between amine lignin and propylene *** results of the Fourier Transform Infrared(FTIR)spectroscopy analysis showed that modification with DETA led to more structural change in lignin and peak 1100 indicates the presence of C–O bond related to urethane bonds in modified ***,adding propylene carbonate to aminated lignin did not result in much change in the results of the FTIR ***,urethane bonds can be seen in the results of GPC at 400℃–500℃.Furthermore,a slight decrease in thermal stability was observed in lignin modified with amine and propylene carbonate,compared to the raw lignin sample.

关键词： Polyol lignin diethylenetriamine ethylenediamine propylene carbonate polyurethanes NIPU

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Radiation-induced inflammation and autoimmune diseases

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Military Medical Research 2018年第1期5卷 62-71页

作者： Rasoul Yahyapour Peyman Amini Saeed Rezapour Mohsen Cheki Abolhasan Rezaeyan Bagher farhood Dheyauldeen Shabeeb Ahmed Eleojo Musa Hengameh Fallah Masoud najafi School of Medicine Jiroft University of Medical Sciences Department of Radiology Faculty of ParamedicalTehran University of Medical Sciences Department of Radiologic Technology Faculty of ParamedicineAhvaz Jundishapur University of Medical Sciences Department of Medical Physics School of MedicineIran University of Medical Sciences Departments of Medical Physics and Radiology Faculty of Paramedical SciencesKashan University of Medical Sciences Department of Medical Physics and Biomedical Engineering Faculty of MedicineTehran University of Medical Sciences (International Campus) Department of Physiology College of MedicineUniversity of Misan Research center for molecular and cellular imaging Tehran University of Medical Sciences Department of Chemistry Faculty of ScienceIslamic Azad University Radiology and Nuclear Medicine Department School of Paramedical Sciences Kermanshah University of Medical Science

Currently,ionizing radiation(IR)plays a key role in the agricultural and medical industry,while accidental exposure resulting from leakage of radioactive sources or radiological terrorism is a serious *** to IR has various detrimental effects on normal *** an increased risk of carcinogenesis is the best-known long-term consequence of IR,evidence has shown that other diseases,particularly diseases related to inflammation,are common disorders among irradiated *** disorders are among the various types of immune diseases that have been investigated among exposed *** diseases and diabetes are two autoimmune diseases potentially induced by ***,the precise mechanisms of IR-induced thyroid diseases and diabetes remain to be elucidated,and several studies have shown that chronic increased levels of inflammatory cytokines after exposure play a pivotal ***,cytokines,including interleukin-1(IL-1),tumor necrosis factor(TNF-α)and interferon gamma(IFN-α),play a key role in chronic oxidative damage following exposure to ***,these cytokines change the secretion of insulin and thyroid-stimulating hormone(TSH).It is likely that the management of inflammation and oxidative damage is one of the best strategies for the amelioration of these diseases after a radiological or nuclear *** the present study,we reviewed the evidence of radiation-induced diabetes and thyroid diseases,as well as the potential roles of inflammatory *** addition,we proposed that the mitigation of inflammatory and oxidative damage markers after exposure to IR may reduce the incidence of these diseases among individuals exposed to radiation.

关键词： Radiation Inflammation Autoimmune diseases Thyroid Diabetes

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