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硫醇吸附挥发性有机气体(VOCs)的气敏机理

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原子与分子物理学报 2025年第3期42卷 35-44页

作者：张海燕李琦王梓臻文豪刘丹凤中国环境科学研究院北京100012 中国汽车工程研究院股份有限公司重庆401122 中国科学院微电子研究所北京100029

化学电阻气体传感器对于空气质量、食品检测和人体呼吸有着重要作用.传感器上修饰物硫醇与待测的VOCs之间吸附的气敏机理分析是选择硫醇、预测吸附能力与特异性的重要手段.本文选取了11-巯基-1-十一醇(MUD)和4-甲氧基苄硫醇(MTT)两种常... 详细信息

化学电阻气体传感器对于空气质量、食品检测和人体呼吸有着重要作用.传感器上修饰物硫醇与待测的VOCs之间吸附的气敏机理分析是选择硫醇、预测吸附能力与特异性的重要手段.本文选取了11-巯基-1-十一醇(MUD)和4-甲氧基苄硫醇(MTT)两种常见的硫醇与六种典型的VOCs(乙醇ETN、异丙醇IPA、丙酮ACN、正己烷HXN、甲苯TLN、苯甲醛BND),基于密度泛函理论(DFT),计算其表面静电势(ESP)并建立气体吸附模型.在气体吸附模型的基础上计算其吸附能,并分析其弱相互作用,从微观角度解释气体吸附的作用机理.实验结果表明,具有羟基的MUD分子对同样有羟基的气体(如ETN、IPA)能够以氢键的方式吸附,具有较强的选择效果;具有苯环的MTT分子与具有苯环结构的气体分子(如TLN、BND)吸附时会在苯环之间形成π-π堆积,基于色散作用进行吸附,这表明MTT分子对具有苯环结构的气体有着较强的吸附作用.研究发现其色散作用吸附的强弱与分子的表面ESP绝对值有关.本文对于传感器表面修饰物吸附气体的气敏机理进行了探究,并对表面修饰物的选择和实验结果预测提供了理论指导.

关键词：硫醇 VOCs DFT 表面静电势气体吸附模型弱相互作用分析

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Non-sequential striping encoder from replication to erasure coding for distributed storage system

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Frontiers of Computer Science 2019年第6期13卷 1356-1358页

作者： Yanwen XIE dan feng Fang WANG Lingling ZHANG Wuhan National Laboratory for Optoelectronics School of Computer Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Information Storage System Engineering Research Center of Data Storage Systems and TechnologyMinistry of Education of ChinaWuhan 430074China

1 Introduction and main contributions As so many machines are clustered in datacenters,failures occur frequently[1,2].Redundancy schemes,like replication and erasure coding,are deployed to store redundant data to tolerate *** distributed systems with these two redundancy schemes,new data are hot in replication,and usually turn cold as time goes *** encoder performing the conversion can cause large overheads on network and put data in low reliability when the encoder is not well designed.

关键词： strip redundant store

A lightweight data-voting strategy for triple-modular redundant control computers

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Science China(Technological Sciences) 2022年第2期65卷 419-431页

作者： LIU Bo YANG MengFei WANG Yong YUAN Li LIU ChaoWei XU Jian YU dan HU HongKai feng dan Beijing Institute of Control Engineering Beijing 100190China China Academy of Space Technology Beijing 100094China

Triple-modular redundancy(TMR), a well-known methodology for improving the reliability of computer systems, has been used for onboard control computers in many safety-critical space applications. In this paper, a lightweight data-voting strategy for TMR control computer is proposed, in which an additional straightforward input voting stage is added, so that determination of the maximum admissible deviation for output matching, as required by traditional strategies, can be avoided. The lightweight strategy is a practical data-voting solution for the TMR control computer that exploits the characteristics of the data of the control computer. The addition of input voting, in both the value and time domains, can ensure that the outputs of non-faulty machines are exactly equal, and the bitwise output matching of the TMR control computer can be performed. The new data-voting strategy has been optimized according to the actual application conditions in spacecraft control systems, and has been adopted for the TMR control computer of the Chang’e-5 Return Spacecraft. The results of the ground experiments and successful on-orbit application have demonstrated the advantages of the new data-voting strategy for TMR control computer.

关键词： TMR data-voting onboard control computer output matching

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A disk I/O optimized system for concurrent graph processing jobs

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Frontiers of Computer Science 2024年第3期18卷 13-29页

作者： Xianghao XU Fang WANG Hong JIANG Yongli CHENG dan feng Peng FANG School of Computer Science and Engineering Nanjing University of Science and TechnologyNanjing 210094China Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China Department of Computer Science&Engineering University of Texas at ArlingtonArlingtonTX 76019USA College of Computer and Data Science Fuzhou UniversityFuzhou 350108China Zhejiang Lab Hangzhou 311121China

In order to analyze and process the large graphs with high cost efficiency,researchers have developed a number of out-of-core graph processing systems in recent years based on just one commodity *** the other hand,with the rapidly growing need of analyzing graphs in the real-world,graph processing systems have to efficiently handle massive concurrent graph processing(CGP)***,due to the inherent design for single graph processing job,existing out-of-core graph processing systems usually incur unnecessary data accesses and severe competition of I/O bandwidth when handling the CGP *** this paper,we propose GraphCP,a disk I/O optimized out-of-core graph processing system that efficiently supports the processing of CGP *** proposes a benefit-aware sharing execution model to share the I/O access and processing of graph data among the CGP jobs and adaptively schedule the graph data loading based on the states of vertices,which efficiently overcomes above challenges faced by existing out-of-core graph processing ***,GraphCP adopts a dependency-based future-vertex updating model so as to reduce disk I/Os in the future *** addition,GraphCP organizes the graph data with a Source-Sorted Sub-Block graph representation for better processing capacity and I/O access *** evaluation results show that GraphCP is 20.5×and 8.9×faster than two out-of-core graph processing systems GridGraph and GraphZ,and 3.5×and 1.7×faster than two state-of-art concurrent graph processing systems Seraph and GraphSO.

关键词： graph processing disk I/O concurrent jobs

Knockout of cryptochrome 1 disturbs the locomotor circadian rhythm and development of Plutella xylostella

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Insect Science 2023年第4期30卷 1035-1045页

作者： Shao-Ping Chen dan-feng Wang Wei-feng Ma Xiao-Lu Lin Guang Yang State Key Laboratory of Ecological Pest ControlforFujan and Taiwan Crops Institute of Applied EcologyFujian Agriculture and Forestry UniversityFuzhouChina Joint International Research Laboratory of Ecological Pest Control Ministry of EducationFuzhouChina Ministerial and Provincial Joint Innovation Center for Safety Production of Cross-Strait Crops Fujian Agriculture and Forestry UniversityFuzhouChina Key Laboratory of Integrated Pest Management for Fujian-Taiwan Crops Ministry of AgricultureFuzhouChina Key Laboratory of Green Pest Control(Fujian Agriculture and Forestry University) Fujian Province UniversityFuzhouChina

Cryptochrome 1(CRY1)functions as a light-responsive photoreceptor,which is crucial for circadian *** identity and function of CRY1 in Plutella xylostella remain *** this study,cryl was cloned and identified in P ***,a cry1-knockout strain(Cry1-KO)of P xylostella with a 2-bp deletion was established from the strain Geneva 88(G88)using the CRISPR/Cas9 *** daily temporal os-cillation of cryl was observed in G88 and Cry1-KO,and cryl mean daily transcription of Cry1-KO was lower than that of *** G88 and Cry1-KO demonstrated rhythmic locomotion under the light/dark condition with Cryl-KO being more active than G88 in the daytime,whereas Cry1-KO completely lost rhythmicity under constant *** developmental period of pre-adult of Cry1-KO was longer than that of G88;the lifespan of the Cry1-KO male adult was shorter than that of G88;the fecundity of Cry1-KO was lower than that of G88;and Cry1-KO showed lower intrinsic rate of increase(r),net repro-duction rate(Ro),finite increase rate(a),and longer mean generation time(T)than *** results indicate that cryl is involved in the regulation of locomotor circadian rhythm and development in P xylostella,providing a potential target gene for controlling the pest and a basis for further investigation on circadian rhythms in lepidopterans.

关键词： circadian rhythm cryptochrome 1 lifespan locomotor activity Plutella xylostella reproduction

Metabolic Response of Pakchoi Leaves to Amino Acid Nitrogen

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Journal of Integrative Agriculture 2014年第4期13卷 778-788页

作者： WANG Xiao-li YU Wen-juan ZHOU Qian HAN Rui-feng HUANG dan-feng Department of Horticulture School of Agriculture and BiologyShanghai Jiao Tong University Instrumental Analysis Center Shanghai Jiao Tong University

Different nitrogen （N） forms may cause changes in the metabolic profiles of plants. However, few studies have been conducted on the effects of amino acid-N on plant metabolic profiles. The main objective of this study was to identify primary metabolites associated with amino acid-N （Gly, Gln and Ala） through metabolic profile analysis using gas chromatography- mass spectrometry （GC-MS）. Plants of pakchoi （Brassica campestris L. ssp. chinensis L.）, Huawang and Wuyueman cultivars, were grown with different nitrogen forms （i.e., Gly, Gln, Ala, NO3-N, and N starvation） applied under sterile hydroponic conditions. The fresh weight and plant N accumulation of Huawang were greater than those of Wuyueman, which indicates that the former exhibited better N-use efficiency than the latter. The physiological performances of the applied N forms were generally in the order of NO3-N〉Gln〉Gly〉Ala. The metabolic analysis of leaf polar extracts revealed 30 amino acid N-responsive metabolites in the two pakchoi cultivars, mainly consisting of sugars, amino acids, and organic acids. Changes in the carbon metabolism of pakchoi leaves under amino acid treatments occurred via the accumulation of fructose, glucose, xylose, and arabinose. Disruption of amino acid metabolism resulted in accumulation of endogenous Gly in Gly treatment, Pro in Ala treatment, and Asn in three amino acid （Gly, Gln and Ala） treatments. By contrast, the levels of endogenous Gln and Leu decreased. However, this reduction varied among cultivars and amino acid types. Amino acid-N supply also affected the citric acid cycle, namely, the second stage of respiration, where leaves in Gly, Gln and Ala treatments contained low levels of malic, citric and succinic acids compared with leaves in NO3-N treatments. No significant difference in the metabolic responses was observed between the two cultivars which differed in their capability to use N. The response of primary metabolites in pakchoi leaves to amino acid-N supply may

关键词： amino acid metabolite profile pakchoi

Iterative Detection and Decoding Algorithm in Dual Polarized Land Mobile Satellite MIMO Systems

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Journal of Harbin Institute of Technology(New Series) 2014年第2期21卷 28-32页

作者： Yang Wang dan-feng Zhao Xi Liao College of Information and Communication Engineering Harbin Engineering University

An iterative detection and decoding algorithm with outer code decision feedback is proposed for the dual polarized( DP) land mobile satellite( LMS) MIMO systems using concatenated codes. A feedback structure is added after the outer decoder in the proposed algorithm. The feedback information is exploited to control the detecting list in the MIMO detector and reduce the number of symbols which have to be processed at each iteration. As a result,the computational complexity is reduced. Meanwhile,the successfully decoded outer code words are used to calculate the more reliable initial information for the inner decoder and the system performance can be improved by this step. The simulation results show that the proposed algorithm can reduce the computational complexity compared to the traditional iterative detection and decoding algorithm and achieve better performance.

关键词： satellite communications multiple-input multiple-output(MIMO) dual polarization iterative detection and decoding

A New Solvent-free Synthesis of a, a'-Dibenzylidenecycloalkanones from Acetals with Cycloalkanones under Microwave Irradiation

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Chinese Chemical Letters 2003年第4期14卷 333-334页

作者： dan feng HUANG Jin Xian WANG Yu Lai HU College of Chemistry&Chemical Engineering Northwest Normal UniversityLanzhou 730070

A new rapid synthetic method is described for synthesis of a, a-dibenzylidene- cycloalkanones by the reaction of acetals and cycloalkanones without solvent using BF3稥t2O as catalyst under microwave irradiation.

关键词： Cycloalkanone acetal Lewis acid microwave irradiation.

Role of Substrate Roughness in ZnO Nanowire Arrays Growth by Hydrothermal Approach

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Acta Metallurgica Sinica(English Letters) 2016年第3期29卷 237-242页

作者： Qiu-Hong Wang Chao-Long Tang Cheng-Ming Jiang dan-feng Du feng Wang Jin-Hui Song Department of Metallurgical and Materials Engineering Center for Materials for Information Technology(MINT)University of Alabama Department of Mechanical Engineering Changzhou Institute of Mechatronic Technology

The role of substrate roughness in ZnO nanowire（NW） arrays hydrothermal growth has been systematically *** silicon substrates with different roughness by chemical etching have been selected to grow ZnO NW arrays hydrothermally after sputtering 5-nm-thick ZnO seed layer as *** as-grown samples reveal that average diameters and number densities of ZnO NW arrays are inversely proportional to the increasing substrate roughness observed by atomic-force microscopy and scanning electron ***,the theoretically derived equations based on nucleation with the Gibbs free energy to describe relations of substrate roughness versus average NW diameter and NW number density match well with experimental *** results in this paper can be used to control the number density and the average diameter of ZnO NW arrays by alternating substrate roughness.

关键词： ZnO nanowire Chemical synthesis Atomic-force microscopy Substrate roughness