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Near-zero-adhesion-enabled intact wafer-scale resist-transfer printing for high-fidelity nanofabrication on arbitrary substrates

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International Journal of Extreme Manufacturing 2024年第1期6卷 313-326页

作者： Zhiwen Shu Bo Feng peng Liu Lei Chen Huikang liang Yiqin Chen Jianwu Yu Huigao Duan College of Mechanical and Vehicle Engineering National Engineering Research Centre for High Efficiency GrindingHunan UniversityChangsha 410082People’s Republic of China Greater Bay Area Institute for Innovation Hunan UniversityGuangzhou 511300People’s Republic of China School of Mechanical Engineering Hunan University of Science and TechnologyXiangtan 411201People’s Republic of China Shenzhen Research Institute Hunan UniversityShenzhen 518000People’s Republic of China

There is an urgent need for novel processes that can integrate different functional nanostructures onto specific substrates,so as to meet the fast-growing need for broad applications in nanoelectronics,nanophotonics,and fexible *** direct-lithography methods are difficult to use on fexible,nonplanar,and biocompatible ***,this fabrication is usually accomplished by nanotransfer ***,large-scale integration of multiscale nanostructures with unconventional substrates remains challenging because fabrication yields and quality are often limited by the resolution,uniformity,adhesivity,and integrity of the nanostructures formed by direct ***,we proposed a resist-based transfer strategy enabled by near-zero adhesion,which was achieved by molecular modification to attain a critical surface energy *** approach enabled the intact transfer of wafer-scale,ultrathin-resist nanofilms onto arbitrary substrates with mitigated cracking and wrinkling,thereby facilitating the in situ fabrication of nanostructures for functional *** this approach,fabrication of three-dimensional-stacked multilayer structures with enhanced functionalities,nanoplasmonic structures with~10 nm resolution,and MoS2-based devices with excellent performance was demonstrated on specific *** results collectively demonstrated the high stability,reliability,and throughput of our strategy for optical and electronic device applications.

关键词： resist-based transfer printing near-zero adhesion critical surface energy wafer-scale nanofabrication in situ fabrication optoelectronic devices

Neurophysiological, histological, and behavioral characterization of animal models of distraction spinal cord injury: a systematic review

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Neural Regeneration Research 2024年第3期19卷 563-570页

作者： Bo Han Weishi liang Yong Hai Duan Sun Hongtao Ding Yihan Yang peng Yin Department of Orthopedics Beijing Chao-Yang HospitalCapital Medical UniversityBeijingChina

Distraction spinal cord injury is caused by some degree of distraction or longitudinal tension on the spinal cord and commonly occurs in patients who undergo corrective operation for severe spinal *** the increased degree and duration of distraction,spinal cord injuries become more serious in terms of their neurophysiology,histology,and *** few studies have been published on the specific characteristics of distraction spinal cord *** this study,we systematically review 22 related studies involving animal models of distraction spinal cord injury,focusing particularly on the neurophysiological,histological,and behavioral characteristics of this *** addition,we summarize the mechanisms underlying primary and secondary injuries caused by distraction spinal cord injury and clarify the effects of different degrees and durations of distraction on the primary injuries associated with spinal cord *** provide new concepts for the establishment of a model of distraction spinal cord injury and related basic research,and provide reference guidelines for the clinical diagnosis and treatment of this disease.

关键词： animal models behavior distraction heterogeneity histology mechanism neurophysiology spinal cord injury systematic review tension

Omics for deciphering oral microecology

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International Journal of Oral Science 2024年第2期16卷 197-207页

作者： Yongwang Lin Xiaoyue liang Zhengyi Li Tao Gong Biao Ren Yuqing Li Xian peng State Key Laboratory of Oral Diseases&National Center for Stomatology&National Clinical Research Center for Oral Diseases West China Hospital of StomatologySichuan UniversityChengduChina

The human oral microbiome harbors one of the most diverse microbial communities in the human body,playing critical roles in oral and systemic *** technological innovations are propelling the characterization and manipulation of oral ***-throughput sequencing enables comprehensive taxonomic and functional profiling of oral *** long-read platforms improve genome assembly from complex ***-cell genomics provides insights into uncultured *** imaging modalities including fluorescence,mass spectrometry,and Raman spectroscopy have enabled the visualization of the spatial organization and interactions of oral microbes with increasing *** techniques link phylogenetic identity with *** spectrometry imaging reveals metabolic niches and activities while Raman spectroscopy generates rapid biomolecular fingerprints for *** facilitates the isolation and cultivation of novel fastidious oral taxa using high-throughput *** integration of these technologies holds the promise of transforming our understanding of oral microbiome assembly,gene expression,metabolites,microenvironments,virulence mechanisms,and microbe-host interfaces in the context of health and ***,significant knowledge gaps persist regarding community origins,developmental trajectories,homeostasis versus dysbiosis triggers,functional biomarkers,and strategies to deliberately reshape the oral microbiome for therapeutic *** convergence of sequencing,imaging,cultureomics,synthetic systems,and biomimetic models will provide unprecedented insights into the oral microbiome and offer opportunities to predict,prevent,diagnose,and treat associated oral diseases.

关键词： insight holds oral

Covalent Organic Framework with 3D Ordered Channel and Multi-Functional Groups Endows Zn Anode with Superior Stability

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Nano-Micro Letters 2024年第4期16卷 350-363页

作者： Bin Li pengchao Ruan Xieyu Xu Zhangxing He Xinyan Zhu liang Pan Ziyu peng Yangyang Liu peng Zhou Bingan Lu Lei Dai Jiang Zhou School of Chemical Engineering North China University of Science and TechnologyTangshan 063009People’s Republic of China School of Materials Science and Engineering Central South UniversityChangsha 410083People’s Republic of China State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049People’s Republic of China Hunan Provincial Key Defense Laboratory of High Temperature Wear‑Resisting Materials and Preparation Technology Hunan University of Science and TechnologyXiangtan 411201People’s Republic of China School of Physics and Electronics Hunan UniversityChangsha 410082People’s Republic of China

Achieving a highly robust zinc(Zn)metal anode is extremely important for improving the performance of aqueous Zn-ion batteries(AZIBs)for advancing“carbon neutrality”society,which is hampered by the uncontrollable growth of Zn dendrite and severe side reactions including hydrogen evolution reaction,corrosion,and passivation,***,an interlayer containing fluorinated zincophilic covalent organic framework with sulfonic acid groups(COF-S-F)is developed on Zn metal(Zn@COF-S-F)as the artificial solid electrolyte interface(SEI).Sulfonic acid group(-SO_(3)H)in COF-S-F can effectively ameliorate the desolvation process of hydrated Zn ions,and the three-dimensional channel with fluoride group(-F)can provide interconnected channels for the favorable transport of Zn ions with ion-confinement effects,endowing Zn@COF-S-F with dendrite-free morphology and suppressed side ***,Zn@COF-S-F symmetric cell can stably cycle for 1,000 h with low average hysteresis voltage(50.5 m V)at the current density of 1.5 m A cm^(-2).Zn@COF-S-F|Mn O_(2)cell delivers the discharge specific capacity of 206.8 m Ah g^(-1)at the current density of 1.2 A g^(-1)after 800 cycles with high-capacity retention(87.9%).Enlightening,building artificial SEI on metallic Zn surface with targeted design has been proved as the effective strategy to foster the practical application of high-performance AZIBs.

关键词： Aqueous Zn ion batteries Covalent organic framework Interfacial modification Zn ion flux regulation Desolvation effect

A whole process damage constitutive model for layered sandstone under uniaxial compression based on Logistic function

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Journal of Central South University 2024年第7期31卷 2411-2430页

作者： LIU dong-qiao GUO Yun-peng LING Kai LI Jie-yu State Key Laboratory for Geomechanics and Deep Underground Engineering China University of Mining and Technology-BeijingBeijing 100083China School of Mechanics and Civil Engineering China University of Mining and Technology-BeijingBeijing 100083China

Bedding structural planes significantly influence the mechanical properties and stability of engineering rock *** study conducts uniaxial compression tests on layered sandstone with various bedding angles(0°,15°,30°,45°,60°,75°and 90°)to explore the impact of bedding angle on the deformational mechanical response,failure mode,and damage evolution processes of *** develops a damage model based on the Logistic equation derived from the modulus’s degradation considering the combined effect of the sandstone bedding dip angle and *** model is employed to study the damage accumulation state and its evolution within the layered rock *** research also introduces a piecewise constitutive model that considers the initial compaction characteristics to simulate the whole deformation process of layered sandstone under uniaxial *** results revealed that as the bedding angle increases from 0°to 90°,the uniaxial compressive strength and elastic modulus of layered sandstone significantly decrease,slightly increase,and then decline *** corresponding failure modes transition from splitting tensile failure to slipping shear failure and back to splitting tensile *** indicated by the modulus’s degradation,the damage characteristics can be categorized into four stages:initial no damage,damage initiation,damage acceleration,and damage deceleration *** theoretical damage model based on the Logistic equation effectively simulates and predicts the entire damage evolution ***,the theoretical constitutive model curves closely align with the actual stress−strain curves of layered sandstone under uniaxial *** introduced constitutive model is concise,with fewer parameters,a straightforward parameter determination process,and a clear physical *** study offers valuable insights into the theory of layered rock mechanics and holds implications for ensuring the safety of rock engineering.

关键词： layered sandstone uniaxial compression damage evolution Logistic function constitutive model

Enhanced thermoelectric performance enabled by compositing ZrO_(2)in n-type SiGe alloy with low thermal conductivity

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Rare Metals 2024年第3期43卷 1167-1176页

作者： Meng-Fei Wang Hua-Jun Lai Ji-Sheng liang Jun-liang Chen Wang-Yang Ding Qi Zhou Ying peng Cheng-Yan Liu Lei Miao Guangxi Key Laboratory for Relativity Astrophysics State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite StructuresSchool of Physical Science and TechnologyGuangxi UniversityNanning530004China Guangxi Academy of Sciences Nanning530007China Key Laboratory of Information Material Engineering Research Center of Electronic Information Materials and DevicesGuilin University of Electronic TechnologyMinistry of EducationGuilin541004China Guangxi Key Laboratory of Precision Navigation Technology and Application School of Information and CommunicationGuilin University of Electronic TechnologyGuilin541004China

SiGe-based thermoelectric(TE)materials have gained increasing interests due to their low maintenance costs,environmental friendliness and long ***,the intrinsically high thermal conductivity of Si-based materials also results in poor TE *** this investigation,a zirconia(ZrO_(2))composite strategy was applied to an n-type SiGe alloy,tremendously elevating its TE *** mechanical alloying and spark plasma sintering(SPS)processes,the ZrO_(2)induced the formation of nanopores in the SiGe matrix via phosphorus ***,such increase in porosity enhanced the phonon scattering and dramatically suppressed lattice thermal conductivity,from 2.83 to 1.59 W·m^(-1)·K^(-1)at 873 ***,reduced phosphorus doping led to an increase in Seebeck coefficients and a relatively minor decrease in electrical conductivity,The power factor didn't deteriorate significantly,either,as its maximum of~3.43 mW·m^(-1-)K^(-2)was achieved at 873 K with(Si_(0.8)Ge_(0.2))_(0.097)P_(0.03)(ZrO_(2))_(0.003).In short,a peak figure of merit(ZT)of~1.27 at 873 K and an average ZT~0.7 from 323 to 873 K were *** study demonstrates that the electrical and thermal transportation of SiGe material can be synergistically tuned by compositing ZrO_(2),illustrating a novel strategy to optimize the TE properties of bulk materials.

关键词： Thermoelectric SiGe alloy ZrO2 composting P element adsorption nanopores

Continuous gradient fusion class activation mapping: segmentation of laser-induced damage on large-aperture optics in dark-field images

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High Power Laser Science and Engineering 2024年第1期12卷 30-41页

作者： Yueyue Han Yingyan Huang Hangcheng dong Fengdong Chen Fa Zeng Zhitao peng Qihua Zhu Guodong Liu School of Instrumentation Science and Engineering Harbin Institute of TechnologyHarbinChina Research Center of Laser Fusion China Academy of Engineering PhysicsMianyangChina

Segmenting dark-field images of laser-induced damage on large-aperture optics in high-power laser facilities is challenged by complicated damage morphology, uneven illumination and stray light interference. Fully supervised semantic segmentation algorithms have achieved state-of-the-art performance but rely on a large number of pixel-level labels, which are time-consuming and labor-consuming to produce. LayerCAM, an advanced weakly supervised semantic segmentation algorithm, can generate pixel-accurate results using only image-level labels, but its scattered and partially underactivated class activation regions degrade segmentation performance. In this paper, we propose a weakly supervised semantic segmentation method, continuous gradient class activation mapping(CAM) and its nonlinear multiscale fusion(continuous gradient fusion CAM). The method redesigns backpropagating gradients and nonlinearly activates multiscale fused heatmaps to generate more fine-grained class activation maps with an appropriate activation degree for different damage site sizes. Experiments on our dataset show that the proposed method can achieve segmentation performance comparable to that of fully supervised algorithms.

关键词： class activation maps laser-induced damage semantic segmentation weakly supervised learning

A continuous and long-term in-situ stress measuring method based on fiber optic. Part I: Theory of inverse differential strain analysis

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Petroleum Science 2024年第2期21卷 1171-1189页

作者： Kun-peng Zhang Mian Chen Chang-Jun Zhao Su Wang Yong-dong Fan State Key Laboratory of Petroleum Resources and Prospecting China University of PetroleumBeijing102249China MOE Key Laboratory of Petroleum Engineering in China University of Petroleum Beijing102249China Beijing International Center for Gas Hydrate School of Earth and Space SciencesPeking UniversityBeijing100871China

A method for in-situ stress measurement via fiber optics was proposed. The method utilizes the relationship between rock mass elastic parameters and in-situ stress. The approach offers the advantage of long-term stress measurements with high spatial resolution and frequency, significantly enhancing the ability to measure in-situ stress. The sensing casing, spirally wrapped with fiber optic, is cemented into the formation to establish a formation sensing nerve. Injecting fluid into the casing generates strain disturbance, establishing the relationship between rock mass properties and treatment ***, an optimization algorithm is established to invert the elastic parameters of formation via fiber optic strains. In the first part of this paper series, we established the theoretical basis for the inverse differential strain analysis method for in-situ stress measurement, which was subsequently verified using an analytical model. This paper is the fundamental basis for the inverse differential strain analysis method.

关键词： In-situ stress Fiber optic Orthotropic elastic Differential evolution ABAQUS

Multiscale microstructural consideration of enhanced shear strength in TiAl intermetallic/K4169 alloy composite joints prepared by vacuum brazing with(Ti,Zr)-Ni-based amorphous filler metal

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Journal of Materials Science & Technology 2024年第5期172卷 51-70页

作者： liangliang Zhang Honggang dong peng Li Baosheng Wu Yueting Ma Libing Huang Chao Li Jiachen Li School of Materials Science and Engineering Dalian University of TechnologyDalian 116024China

TiAl intermetallic could be used to replace Ni-based alloy in assemblies to generate excellent specific strength.A(Ti,Zr)-Ni-based amorphous filler metal Ti_(21.25)Zr_(25)Ni_(25)Cu_(18.75)(at.%)was designed using a cluster-plus-glue-atom model to successfully vacuum braze K4169 and TiAl bimetallic *** various brazing temperatures and holding time,the quantitative relationships between lattice distortion,grain boundary,dislocation density,and hardness,elastic modulus,shear strength of the joints were ***,the fracture mechanism of the joints was *** brazed seam mainly consisted of solid diffusion reaction layers(ZonesⅠandⅢ)and filler metal residue zone(ZoneⅡ).When the brazing temperature increased to 1030℃,grain refinement occurred in the brazed ***Ⅰwas primarily composed of(Ni)ss[0-11]+TiNi[011]/(Cr,Fe,Ni)ss[0-11]/(Ti,Zr)Ni[0-1-1]+(Cr,Fe,Ni)ss[0-11].The(Ti,Zr)(Ni,Cu)[001]and(Ti,Zr)(Ni,Cu)[101]intermetallic compound-based solid solutions were formed in ZoneⅡ.And the lattice distortion of(Ti,Zr)(Ni,Cu)[101]and(Ti,Zr)(Ni,Cu)[001]was 32.05%and 14.82%,*** a result,the proportion of low angle grain boundaries(LAGBs)and deformed grains in ZoneⅡrose to 38.6%and 38.7%.In ZonesⅠandⅢ,the proportion of LAGBs reduced to 8%and 3.4%,*** the holding time increased,the long-range diffusion of Al in ZoneⅡcaused the(Ti,Zr)(Ni,Cu)[001]with cubic structure to transform into(Ti,Zr)(Ni,Cu,Al)[00-1]with hexagonal crystal system structure,where the lattice distortion was 4.42%and 10.49%for a and *** 1030℃/10 min,the average geometrically nec-essary dislocation densities(GNDs)in ZonesⅠ,ⅡandⅢwere 9.87×10^(14)m^(-2),8.55×10^(14)m^(-2)and 11.4×10^(14)m^(-2),***,the shear strength of joints reached 322 MPa due to the lattice distortion,dislocation strengthening and fine grain ***,the plastic and brittle hard phases were generated in ZoneⅡand displayed a mechanical interlocking structure tha

关键词： K4169/Ti_(21.25)Zr_(25)Ni_(25)Cu_(18.75)/TiAl composite joints Intermetallic compound-based solid solution Lattice distortion Elastic modulus