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High-Performance Perovskite Quantum Dot Solar Cells Enabled by Incorporation with Dimensionally Engineered Organic Semiconductor

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Nano-Micro Letters 2022年第12期14卷 272-285页

作者： Seyeong Lim Dae Hwan lee Hyuntae Choi Yelim Choi dong geon lee Sung Beom Cho Seonkyung Ko Jongmin Choi Younghoon Kim Taiho Park Department of Chemical Engineering Pohang University of Science and Technology(POSTECH)Pohang 37673Republic of Korea Department of Materials Science and Engineering Hanyang UniversitySeoul 04763Republic of Korea Center of Materials Digitalization Korea Institute of Ceramic Engineering and Technology(KICET)Jinju 52851Republic of Korea Department of Materials Science and Engineering Ajou UniversitySuwon 16499Republic of Korea Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology(DGIST)Daegu 42988Republic of Korea Department of Chemistry Kookmin UniversitySeoul 02707Republic of Korea

Perovskite quantum dots(PQDs)have been considered promising and effective photovoltaic absorber due to their superior optoelectronic properties and inherent material merits combining perovskites and ***,they exhibit low moisture stability at room humidity(20-30%)owing to many surface defect sites generated by inefficient ligand exchange *** surface traps must be re-passivated to improve both charge transport ability and moisture *** address this issue,PQD-organic semiconductor hybrid solar cells with suitable electrical properties and functional groups might dramatically improve the charge extraction and defect *** organic semiconductors are typically low-dimensional(1D and 2D)and prone to excessive self-aggregation,which limits chemical interaction with *** this work,we designed a new 3D star-shaped semiconducting material(Star-TrCN)to enhance the compatibility with *** robust bonding with Star-TrCN and PQDs is demonstrated by theoretical modeling and experimental *** Star-TrCN-PQD hybrid films show improved cubic-phase stability of CsPbI_(3)-PQDs via reduced surface trap states and suppressed moisture *** a result,the resultant devices not only achieve remarkable device stability over 1000 h at 20-30%relative humidity,but also boost power conversion efficiency up to 16.0%via forming a cascade energy band structure.

关键词： CsPbI3 quantum dots Star-shaped organic semiconductors Hybrid perovskite quantum dots Solar cell stability High-efficiency photovoltaics

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Chlorine-modified SnO2 electron transport layer for high-efficiency perovskite solar cells

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InfoMat 2020年第2期2卷 401-408页

作者： Xiaodong Ren Yucheng Liu dong geon lee Won Bin Kim Gill Sang Han Hyun Suk Jung Shengzhong(Frank)Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal UniversityXi'an710119China School of Advanced Materials Science and Engineering Sungkyunkwan UniversitySuwonKorea Dalian National Laboratory for Clean Energy Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian116023ChinaUniversity of the Chinese Academy of SciencesBeijing100039China

A high-quality electron transport layer(ETL)is a critical component for the realization of high-efficiency perovskite solar *** developed a controllable direct-contact reaction process to prepare a chlorinated SnO2(SnO2-Cl)*** is unique in that(a)102-dichlorobenzene is used to provide more reactive Cl radicals for more in-depth passivation;(b)it does not introduce any impurities other than *** is found that the chlorine modification significantly improves the electron ***,its associated solar cell efficiency is increased from 17.01%to 17.81%comparing to the pristine SnO2 ETL without the *** hysteresis index is significantly reduced to 0.017 for the SnO2-Cl ETL.

关键词： chlorine-modified SnO2 electron transport layer perovskite solar cell surface passivation

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Congestive ischemic colitis successfully treated with antiinflammatory therapy: A case report

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World Journal of Clinical Cases 2024年第1期12卷 142-147页

作者： geon Woo lee Su Bum Park Department of Internal Medicine Pusan National University School of Medicine and Research Institute for Convergence of Biomedical Science and TechnologyPusan National University Yangsan HospitalYangsan 50612South Korea

BACKGROUND Congestive ischemic colitis is a rare subtype of ischemic colitis with an unknown *** conservative management,such as fasting,no established treatment exists;therefore,surgical intervention should be considered in some cases if symptoms *** literature suggests that anti-inflam-matory agents may effectively treat congestive ischemic *** SUMMARY We present the case of a 68-year-old female patient who underwent laparoscopic left hemicolectomy for transverse colon cancer 3 years ***,follow-up included an annual colonoscopy and abdominal computed tomography(CT)at a local ***,progressive erythema and edema of the sigmoid colon were observed 1 year *** admission to our hospital,she complained of abdominal pain and *** CT showed thickening of the sigmoid colon walls,and colonoscopy revealed erythema,edema,and multiple ulcers with exudate in the sigmoid *** angiography showed engorgement of the sigmoid vasa recta without any vascular *** diagnosis was congestive ischemic colitis,and we treated the patient with anti-inflammatory *** 2 mo of glucocorticoid therapy(20 mg once daily)and 7 mo of 5-aminosalicylate therapy(1 g twice daily),the ulcers completely *** has not experienced any recurrence for 2 *** Anti-inflammatory therapy,specifically glucocorticoids and 5-aminosalicylate,has demonstrated promising efficacy and introduces potential novel treatment options for congestive ischemic colitis.

关键词： Ischemic colitis Glucocorticoids 5-aminosalicylate Colon cancer

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The association between C-reactive protein to albumin ratio and 6-month neurological outcome in patients with in-hospital cardiac arrest

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World Journal of Emergency Medicine 2024年第3期15卷 223-228页

作者： Ji Ho lee dong Hun lee Byung Kook lee Seok Jin Ryu Department of Emergency Medicine Chonnam National University HospitalGwangju 61469Republic of Korea Department of Emergency Medicine Chonnam National University Medical SchoolGwangju 61469Republic of Korea

The global incidence rates of in-hospital cardiac arrest(IHCA)range from1.2 to 9.0 per1,000 hospitalized patients,as per the National Cardiac Arrest Database.[1] While IHCAs tend to exhibit superior 30-day survival rates relative to out-of-hospital cardiac arrests (OHCA) due to situational advantages,such as immediate access to medical personnel and treatments.

关键词： patients cardiac IHC

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In situ infrared, Raman and X-ray spectroscopy for the mechanistic understanding of hydrogen evolution reaction

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Journal of Energy Chemistry 2024年第3期90卷 632-651,I0014页

作者： Andi Haryanto Kyounghoon Jung Chan Woo lee dong-Wan Kim Department of Chemistry Kookmin UniversitySeoul 02707Republic of Korea School of Civil Environmental and Architectural EngineeringKorea UniversitySeoul 02841Republic of Korea

Hydrogen production by water reduction reactions has received considerable attention because hydrogen is considered a clean-energy carrier,key for a sustainable energy *** methods have been widely used to study the reaction mechanism of the hydrogen evolution reaction(HER),but the calculation results need to be supported by experimental results and direct evidence to confirm the mechanistic *** this review,we discuss the fundamental principles of the in situ spectroscopic strategy and a theoretical model for a mechanistic understanding of the *** addition,we investigate recent studies by in situ Fourier transform infrared(FTIR),Raman spectroscopy,and X-ray absorption spectroscopy(XAS) and cover new findings that occur at the catalyst-electrolyte interface during *** spectroscopic strategies provide practical ways to elucidate catalyst phase,reaction intermediate,catalyst-electrolyte interface,intermediate binding energy,metal valency state,and coordination environment during HER.

关键词： Hydrogen evolution reaction Infrared spectroscopy Raman spectroscopy X-ray absorption spectroscopy Reaction mechanism

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An Experimental Study on Heat Thansfer Characteristics of Carbon Dioxide During Gas Cooling Process in A Horizontal Tube

An Experimental Study on Heat Thansfer Characteristics of Ca...

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第二届亚洲制冷空调大会

作者： Chang-Hyo Son dong-geon lee Si-Young Jeong Young-Lyoul Kim Hoo-Kyu Oh Dept. of Ref. Eng. Graduate school Pukyong Univ. Busan Korea Dept. of Refrigeration Eng. Graduate school Pukyong Univ. Busan Korea Dept. of Mech. Engineering. Sogang University Seoul Korea Cleaner Production Technology Center KITECH Chonan Korea Dept. of Refrigeration Eng. Pukyong University Busan Korea

The heat transfer coefficient and pressure drop during g as cooling process of CO(R-744)in a horizontal tube were investigated experimentally. The experiments were conducted withoutoil in the refrigerant loop. The main components of the refrigerant loop are a receiver, avariable-speed pump, a mass flow meter, a pre-heater and a gas cooler(test section). The waterloop consists of a variable speed pump, an isothermal tank, and a flow meter. The refrigerant,circulated by the variable-speed pump, condenses in the inner tube while water flows in theannulus. The gas cooler is 6000 mm in length, and it is divided into 12 subsections. The pressuredrop of CO in the gas cooler shows a relatively good agreement with those predicted byBlasius’s correlation. The local heat transfer coefficient of CO agrees well with the correlationby Bringer-Smith. However, at the region near Pseudo -critical temperature, the experimentsindicate higher values than the Bringer-Smith correlation. Based on the experimental datapresented in this paper, a new correlation to predict the heat transfer coefficient of supercriticalCO during in-tube cooling was developed. The deviation between the experimental values andthe values predicted by the new correlation is within 18%.

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CD200Rhigghh neutrophils with dysfunctional autophagy establish systemic immunosuppression by increasing regulatory T cells

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Cellular & Molecular Immunology 2024年第4期21卷 349-361页

作者： Ye Seon Kim Yu Sun Jeong geon Ho Bae Ji Hyeon Kang Mingyu lee Brian A.Zabel Yoe-Sik Bae Department of Biological Sciences Sungkyunkwan UniversitySuwon16419Republic of Korea Department of Health Science and Technology SAIHSTSungkyunkwan UniversitySeoul06351Republic of Korea Palo Alto Veterans Institute for Research Veterans Affairs HospitalPalo AltoCA94304USA

Distinct neutrophil populations arise during certain pathological *** generation of dysfunctional neutrophils during sepsis and their contribution to septicemia-related systemic immune suppression remain *** this study,using an experimental sepsis model that features immunosuppression,we identified a novel population of pathogenic CD200R^(high) neutrophils that are generated during the initial stages of sepsis and contribute to systemic immune suppression by enhancing regulatory T(T_(reg))*** to their CD200R^(low)counterparts,sepsis-generated CD200Rhigh neutrophils exhibit impaired autophagy and dysfunction,with reduced chemotactic migration,superoxide anion production,and TNF-α*** soluble CD200 blocks autophagy and neutrophil maturation in the bone marrow during experimental sepsis,and recombinant CD200 treatment in vitro can induce neutrophil dysfunction similar to that observed in CD200R^(high) *** administration of anα-CD200R antibody effectively reversed neutrophil dysfunction by enhancing autophagy and protecting against a secondary infection challenge,leading to increased *** analysis revealed that CD200R^(high) neutrophils expressed high levels of Igf1,which elicits the generation of Treg cells,while the administration of anα-CD200R antibody inhibited Treg cell generation in a secondary infection *** together,our findings revealed a novel CD200R^(high) neutrophil population that mediates the pathogenesis of sepsis-induced systemic immunosuppression by generating Treg cells.

关键词： Sepsis Neutrophils CD200R Autophagy IGF-1 Regulatory T cells

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Atomically Adjustable Rhodium Catalyst Synthesis with Outstanding Mass Activity via Surface-Li mi ted Cation Exchange

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Energy & Environmental Materials 2024年第2期7卷 83-92页

作者： Hak Hyeon lee dong Su Kim Swagotom Sarker Ji Hoon Choi Ho Seong lee Hyung Koun Cho Department of Advanced Materials Science&Engineering Sungkyunkwan University2066Seobu-roJangan-guSuwon-siGyeonggi-doSeoul 16419Korea Department of Advanced Materials Science&Engineering Kyungpook National University80Daehak-roBuk-guDaegu 41566Korea

Rh has been widely studied as a catalyst for the promising hydrazine oxidation reaction that can replace oxygen evolution reactions for boosting hydrogen production from hydrazine-containing *** Rh being expensive,only a few studies have examined its electrocatalytic mass ***,surface-limited cation exchange and electrochemical activation processes are designed to remarkably enhance the mass activity of *** atoms were readily replaced at the Ni sites on the surface of NiOOH electrodes by cation exchange,and the resulting RhOOH compounds were activated by the electrochemical reduction *** cation exchange-derived Rh catalysts exhibited particle sizes not exceeding 2 nm without agglomeration,indicating a decrease in the number of inactive inner Rh ***,an improved mass activity of 30 A mg_(Rh)^(-1)was achieved at 0.4 V versus reversible hydrogen ***,the two-electrode system employing the same CE-derived Rh electrodes achieved overall hydrazine splitting over 36 h at a stable low *** proposed surface-limited CE process is an effective method for reducing inactive atoms of expensive noble metal catalysts.

关键词： cation exchange synthesis electrochemical metallization hydrazine oxidation reaction mass activity rhodium catalyst

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Review on inorganic and polymeric materials-coordinated metal-organic-framework photocatalysts for green hydrogen evolution

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Journal of Energy Chemistry 2024年第5期92卷 322-356页

作者： dong-Eun lee Mohtaram Danish Umair Alam Wan-Kuen Jo School of Architecture CivilEnvironmental and Energy Engineering Kyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea School of Chemical Engineering Yeungnam UniversityGyeongsanGyeongbuk 38541Republic of Korea

Metal-organic frameworks(MOFs)possess a distinct advantage over conventional heterogeneous photocatalysts because of their carefully defined architecture and particular pores,which facilitate the targeted incorporation of other efficient cocatalysts or semiconductor *** integration of MOFs with other materials has resulted in significant breakthroughs,as the coupled materials improve the performance due to the combined *** unique MOF structures allow them to host foreign materials,which results in harvesting the visible region of the solar spectrum and effectively mitigating charge recombination by promoting charge *** review presents an evaluation of the latest developments in the utilization of surface and/or pore chemistry of MOF-supported heterojunctions for photocatalytic green-hydrogen generation with a basic understanding of the mechanism *** review begins with the basic principles of photocatalysis,the significance of MOFs,their optical properties,the methods used for synthesizing MOFs,and their coordination with other inorganic and polymeric ***,methods to increase photocatalytic H2 evolution using MOF-supported heterojunction have been proposed as standard ***,to address environmental challenges,we highlight the future potential of MOF-supported heterojunctions for use in green-energy *** hope that this review provides guidance to researchers in the development of effective heterojunctions based on MOFs to address challenges in energy applications and catalytic processes.

关键词： Renewable energy Environmental challenge Heterojunction Water splitting Photocatalysis

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Porously Reduced 2-Dimensional Bi2O2CO3 Petals for Strain-Mediated Electrochemical CO2 Reduction to HCOOH

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Energy & Environmental Materials 2024年第1期7卷 219-225页

作者： Won Seok Cho Dae Myung Hong Wan Jae dong Tae Hyung lee Chul Jong Yoo donghwa lee Ho Won Jang Jong-Lam lee Department of Materials Science and Engineering Pohang University of Science and Technology (POSTECH) Department of Materials Science and Engineering Research Institute of Advanced Materials Seoul National University

Here we introduce bismuth-based catalysts for the efficient electrochemical reduction of CO2to formic acid（HCOOH）,which are composed of petalshaped Bi2O2CO3（BOC） that spontaneously formed from Bi thin film in aqueous carbonate solution at room *** the electrochemical reduction process,the BOC petals transform to reduced BOC（R-BOC）consisting of individual BOC and Bi domains.

关键词： bismuth carbon dioxide reduction formic acid heterointerfaces strain

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