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Review on inorganic and polymeric materials-coordinated metal-organic-framework photocatalysts for green hydrogen evolution

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Journal of Energy Chemistry 2024年第5期92卷 322-356页

作者： dong-eun lee Mohtaram Danish Umair Alam Wan-Kuen Jo School of Architecture CivilEnvironmental and Energy Engineering Kyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea School of Chemical Engineering Yeungnam UniversityGyeongsanGyeongbuk 38541Republic of Korea

Metal-organic frameworks(MOFs)possess a distinct advantage over conventional heterogeneous photocatalysts because of their carefully defined architecture and particular pores,which facilitate the targeted incorporation of other efficient cocatalysts or semiconductor *** integration of MOFs with other materials has resulted in significant breakthroughs,as the coupled materials improve the performance due to the combined *** unique MOF structures allow them to host foreign materials,which results in harvesting the visible region of the solar spectrum and effectively mitigating charge recombination by promoting charge *** review presents an evaluation of the latest developments in the utilization of surface and/or pore chemistry of MOF-supported heterojunctions for photocatalytic green-hydrogen generation with a basic understanding of the mechanism *** review begins with the basic principles of photocatalysis,the significance of MOFs,their optical properties,the methods used for synthesizing MOFs,and their coordination with other inorganic and polymeric ***,methods to increase photocatalytic H2 evolution using MOF-supported heterojunction have been proposed as standard ***,to address environmental challenges,we highlight the future potential of MOF-supported heterojunctions for use in green-energy *** hope that this review provides guidance to researchers in the development of effective heterojunctions based on MOFs to address challenges in energy applications and catalytic processes.

关键词： Renewable energy Environmental challenge Heterojunction Water splitting Photocatalysis

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Porous g-C_(3)N_(4)-encapsulated TiO_(2) hollow sphere as a high-performance Z-scheme hybrid for solar-induced photocatalytic abatement of environmentally toxic pharmaceuticals

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Journal of Materials Science & Technology 2021年第23期82卷 21-32页

作者： dong-eun lee Satyanarayana Moru Wan-Kuen Jo Surendar Tonda School of Architecture CivilEnvironmental and Energy EngineeringKyungpook National University80 Daehak-roBuk-guDaegu41566Republic of Korea Department of Electrical and Computer Engineering Iowa State UniversityCoover HallOsborn DriveAmesIowa 50011USA Department of Physical Sciences Kakatiya Institute of Technology and ScienceWarangal506015TelanganaIndia

Herein,we rationally constructed a hybrid heterostructure comprising porous g-C_(3)N_(4)(CN)-encapsulated anatase TiO_(2) hollow spheres(TOHS)via a synthesis method that involves hydrothermal and calcination *** fabricated hybrid,termed CN/TOHS,demonstrated extraordinary activity toward the degradation of environmentally toxic pharmaceutical substances(acetaminophen and ciprofloxacin)in aqueous solutions under simulated sunlight irradiation;the activity of CN/TOHS was superior to that attained for individual TOHS and CN *** particular,the CN/TOHS hybrid containing 13.3 wt.%of CN on TOHS displayed the optimum degradation activity among the tested catalysts used in this study,and it also possessed exceptional recyclability and stability during consecutive degradation *** remarkable photocatalytic activity and stability of the hybrid were predominantly ascribed to the large solid interfacial contact between constituents,TOHS and CN,induced by effective hybrid structure,which boosted the interfacial charge transfer and impeded with the direct recombination of photo-induced ***,the results of the liquid chromatography-mass spectrometry analysis corroborated the effective mineralization of model pharmaceutical pollutants in the presence of the CN/TOHS *** simple interfacial engineering strategy presented in this study offers a potential route for the rational design of novel catalysts for application in environmental remediation and solar energy conversion.

关键词： TiO_(2)hollow sphere g-C3N4 Hybrid heterostructure Z-scheme charge transfer Pollutant degradation

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2D/2D BiOIO_(3)/g-C_(3)N_(4) S-scheme hybrid heterojunction with face-to-face interfacial contact for effective photocatalytic H_(2) production and norfloxacin degradation

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Journal of Materials Science & Technology 2023年第17期148卷 19-30页

作者： dong-eun lee Satyanarayana Moru KasalaPrabhakar Reddy Wan-Kuen Jo Surendar Tonda School of Architecture CivilEnvironmental and Energy EngineeringKyungpook National University80 Daehak-roBuk-guDaegu 41566Republic of Korea School of Advanced Sciences Vellore Institute of Technology-Andhra Pradesh(VIT-AP University)AmaravatiAndhra Pradesh 522237India Department of Chemistry and Biochemistry University of South Carolina631 Sumter StreetColumbiaSC 29208United States

A two-dimensional(2D)/2D hybrid heterojunction with face-to-face interfacial assembly is a desirable dimensionality design with significant potential for various photocatalytic applications due to the large interfacial contact area,which facilitates charge migration and ***,we developed an ef-ficient 2D/2D hybrid heterojunction consisting of BiOIO 3 nanoplates(BIO)and g-C_(3)N_(4) nanosheets(CN)using a simple but effective in situ growth method for photocatalytic aqueous antibiotic degradation and H_(2) *** face-to-face interfacial assembly of the BIO and CN components in the BIO/CN hy-brid heterojunction was verified using electron ***,the BIO/CN hybrid heterojunc-tion outperformed both the BIO and CN counterparts in terms of norfloxacin degradation and H_(2) gen-eration under simulated solar light ***,the photocatalytic performance of the hybrid catalyst remained nearly unchanged throughout five consecutive test *** exceptional performance and stability of the hybrid catalyst are attributable to its extended optical absorption range,large interfa-cial contact area provided by the face-to-face assembly in the 2D/2D hybrid configuration,and enhanced photoexcited charge separation efficiency and redox power of the separated charges,which are supported by an efficient S-scheme charge transfer *** study illuminates the rational construction of novel 2D/2D S-scheme hybrid heterojunction photocatalysts with practical applications in environmental remediation and sustainable energy generation.

关键词： g-C_(3)N_(4) BiOIO_(3) Face-to-face interface 2D/2D heterojunction S-scheme charge transfer Solar energy conversion

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Ileocolic intussusception caused by a lipoma in an adult

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World Journal of Clinical Cases 2017年第6期5卷 254-257页

作者： dong eun lee Jae Young Choe Department of Emergency Medicine School of Medicine Kyungpook National University Department of Pediatrics School of Medicine Kyungpook National University

Intussusception is rarely observed in adults. Adult cases account for only 5% of all cases of intussusceptions and almost 1%-5% of bowel obstruction cases. The etiology, presentation and management of intussusception in adults are different from those in children. The clinical presentation in adults often includes nonspecific signs and symptoms, thereby complicating differential diagnosis from other causes of abdominal pain. We report a 29-year-old Asian woman who visited our emergency department with complaints of fever associated with epigastric pain since one day. Abdominal computed tomography demonstrated ileocolic intussusception, and laparoscopic small bowel luminal mass resection was performed. Histopathology report confirmed a 3.5 cm × 2.7 cm submucosal lipoma in the terminal ileum. Sufficient vigilance and appropriate investigations are important for prompt diagnosis and surgical referral of patients to enable favorable outcomes. A computed tomography scan can be a helpful modality in establishing a diagnosis.

关键词： Adult intussusception ILeocolic Laparoscopic surgery Lipoma Computed tomography

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Bifunctional S-scheme hybrid heterojunction comprising CdS nanorods and BiOIO_(3) nanosheets for efficient solar-induced antibiotic degradation and highly-selective CO_(2) reduction

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Journal of Materials Science & Technology 2023年第30期161卷 74-87页

作者： dong-eun lee Naresh Mameda Kasala Prabhakar Reddy B.Moses Abraham Wan-Kuen Jo Surendar Tonda School of Architecture CivilEnvironmental and Energy EngineeringKyungpook National University80 Daehak-roBuk-guDaegu 41566South Korea Department of Chemistry Koneru Lakshmaiah Education FoundationVaddeswaramGunturAndhra Pradesh 522302India Department of Chemistry and Biochemistry University of South Carolina631 Sumter StreetColumbiaSC 29208United States Department of Chemical Engineering Indian Institute of Technology KanpurKanpur 208016India

The development of a bifunctional photocatalyst that can be utilized for both energy conversion and envi-ronmental remediation is of great practical *** addition,an S-scheme charge transfer process can assist a photocatalyst in efficiently separating photoexcited electrons and holes while maintaining the strong reducibility and oxidizability of the former and the latter,*** developed a bifunctional S-scheme hybrid photocatalyst comprising CdS nanorods and BiOIO_(3)(BIO) nanosheets for efficient antibi-otic degradation and cocatalyst-and sacrificial reagent-free CO_(2) *** combination of visible-light-responsive one-dimensional(1D)CdS and UV-light-responsive 2D BIO resulted in a CdS/BIO hybrid photocatalyst with effective 1D/2D(line)interfacial contact and a broadened optical absorption ***,the CdS/BIO hybrid exhibited exceptional diclofenac degradation and mineralization as well as outstanding CO_(2) reduction activity for CO production,with 95.4%CO selectivity over H_(2)*** exceptional performance of the hybrid catalyst is primarily attributed to the accelerated photoexcited charge transfer caused by the 1D/2D line interfacial contact and the high charge separation and strong redox power of the separated charges,both of which stem from the effective S-scheme charge transfer *** addition,photocorrosion of CdS was substantially mitigated,resulting in the high photocat-alytic performance of the hybrid catalyst even after repeated test *** study provides insight into the rational design of bifunctional S-scheme hybrid photocatalysts for CO_(2) reduction and pollutant degra-dation.

关键词： CdS BiOIO_(3) Bifunctional photocatalyst S-scheme mechanism Antibiotic degradation CO_(2)reduction

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Epidemiology and risk factors for sports-and recreation-related eye injury:a multicenter prospective observational study

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International Journal of Ophthalmology(English edition) 2021年第1期14卷 133-140页

作者： dong eun lee Hyun Wook Ryoo Sungbae Moon Jae Yun Ahn Jung Ho Kim Jong-Yeon Kim Department of Emergency Medicine Kyungpook National University Chilgok HospitalSchool of MedicineKyungpook National UniversityDaegu 41944Republic of Korea Department of Emergency Medicine Kyungpook National University HospitalSchool of MedicineKyungpook National UniversityDaegu 41944Republic of Korea Department of Emergency Medicine Yeungnam University College of MedicineDaegu 42415Republic of Korea Department of Public Health Kyungpook National University HospitalDaegu 41944Republic of Korea

AIM:To identify the epidemiologic characteristics of sportsand recreation-related eye injuries in a large metropolitan city and investigate risk factors associated with visual ***:We performed a multicenter prospective observational study on patients using the regional eye injury registry *** study included patients with sportsand recreation-related eye injury in four tertiary teaching hospitals in Daegu,Republic of Korea,from August 2016 to July *** primary outcome was visual impairment at the first hospital *** of sex,age,place,and causative materials were analyzed according to causative *** examine the association between causative activities and visual impairment,a Logistic regression analysis was ***:Of the 349 sports-and recreation-related eye injuries,soccer was the most common causative activity,with 21.8%(n=76).Sports-and recreation-related eye injuries occurred mainly in teenagers,individuals in their 20 s,and *** and soccer were significantly associated with visual impairment at the first hospital visit compared with combat sports[(adjusted odds ratio(AOR),5.18;95%confidence interval(CI),1.67-16.09 for badminton and AOR,3.87;95%CI,1.36-10.99 for soccer].CONCLUSION:Intervention efforts such as deployment of protective eyewear in sports facilities and schools and promotion of wearing protective eyewear during these activities in teenagers and individuals in their 20 s are mandatory.

关键词： epidemiology eye injury sports injury prevention

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Neural Wiskott-Aldrich syndrome protein(N-WASP)promotes distant metastasis in pancreatic ductal adenocarcinoma via activation of LOXL2

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Oncology Research 2024年第4期32卷 615-624页

作者： HYUNG SUN KIM YUN SUN lee SeunG MYUNG dong HYO JUNG KIM DA eun lee HYEON WOONG KANG MYEONG JIN KIM JOON SEONG PARK Department of Surgery Gangnam Severance HospitalYonsei University College of MedicineSeoulKorea Department of Surgery Graduate School of Medical ScienceBrain Korea 21 ProjectYonsei University College of MedicineSeoulKorea Gibiome Co. Ltd.Gyeonggi-doKorea

Pancreatic ductal adenocarcinoma(PDAC)is one of the most aggressive solid malignancies.A specific mechanism of its metastasis has not been *** this study,we investigated whether Neural Wiskott-Aldrich syndrome protein(N-WASP)plays a role in distant metastasis of *** found that N-WASP is markedly expressed in clinical patients with *** analysis showed a notably more distant metastatic pattern in the N-WASP-high group compared to the N-WASP-low group.N-WASP was noted to be a novel mediator of epithelialmesenchymal transition(EMT)via gene expression profile *** of N-WASP in pancreatic cancer cells significantly inhibited cell invasion,migration,and *** also observed positive association of lysyl oxidase-like 2(LOXL2)and focal adhesion kinase(FAK)with the N-WASP-mediated response,wherein EMT and invadopodia function were *** N-WASP and LOXL2 depletion significantly reduced the incidence of liver and lung metastatic lesions in orthotopic mouse models of pancreatic *** results elucidate a novel role for N-WASP signaling associated with LOXL2 in EMT and invadopodia function,with respect to regulation of intercellular communication in tumor cells for promoting pancreatic cancer *** findings may aid in the development of therapeutic strategies against pancreatic cancer.

关键词： Pancreatic cancer Neural Wiskott-Aldrich syndrome protein(N-WASP)signaling Metastasis Epithelial-mesenchymal transition(EMT) Lysyl oxidase-like 2(LOXL2)

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Experience of primary intestinal lymphangiectasia in adults: Twelve case series from a tertiary referral hospital

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World Journal of Clinical Cases 2024年第4期12卷 746-757页

作者： Ji eun Na Ji eun Kim Sujin Park eun Ran Kim Sung Noh Hong Young-Ho Kim dong Kyung Chang Department of Internal Medicine Inje University Haeundae Paik HospitalBusan 48108South Korea Department of Medicine Samsung Medical CenterSeoul 06351South Korea Department of Pathology Samsung Medical CenterSeoul 06351South Korea

BACKGROUND While primary intestinal lymphangiectasia(PIL)is considered a rare condition,there have been several reported cases in ***,the absence of clear guidance from diagnosis to treatment and prognosis poses challenges for both physicians and *** To enhance understanding by investigating clinical presentation,diagnosis,treatment,complications,and prognoses in adult PIL *** We enrolled adult patients diagnosed with PIL between March 2016 and September *** primary outcome involved examining the diagnosis and treatment process of these *** secondary outcomes included identifying complications(infections,thromboembolism)and assessing prognoses(frequency of hospitalization and mortality)during the follow-up *** Among the 12 included patients,peripheral edema(100%)and diarrhea(75%)were the main presenting *** tests showed that all the pati-ents exhibited symptoms of hypoalbuminemia and ***,the predominant findings were edema of the small intestine(67%)and ascites(58%).The typical endoscopic finding with a snowflake appearance was observed in 75%of *** the 12 patients,two responded positive-ly to octreotide and sirolimus,and eight who could undergo maintenance therapy discontinued *** due to PIL led to infection in half of the patients,thromboembolism in three patients,and one *** PIL can be diagnosed in adults across various age groups,with different severity and treatment responses among patients,leading to diverse complications and ***,tailored treatments will be *** anticipate that our findings will contribute to the management of PIL,an etiology of protein-losing enteropathy.

关键词： Primary intestinal lymphangiectasia in adults Protein-losing enteropathy Diagnosis Treatment Prognosis

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Trends in colorectal cancer incidence according to an increase in the number of colonoscopy cases in Korea

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World Journal of Gastrointestinal Oncology 2024年第1期16卷 51-60页

作者： Ga Hee Kim Yeong Chan lee Tae Jun Kim Sung Noh Hong dong Kyung Chang Young-Ho Kim dong-Hoon Yang Chang Mo Moon Kyunga Kim Hyun Gun Kim eun-Ran Kim Division of Gastroenterology Department of Internal MedicineAsan Medical CenterUniversity of Ulsan College of MedicineSeoul 05505South Korea Department of Digital Health Samsung Advanced Institute for Health Science and TechnologySungkyunkwan University School of MedicineSeoul 06351South Korea Division of Gastroenterology Department of Internal MedicineSamsung Medical CenterSungkyunkwan University School of MedicineSeoul 06351South Korea Division of Gastroenterology Department of Internal MedicineEwha Womans UniversitySeoul 07985South Korea Biomedical Statistics Center Samsung Medical CenterSeoul 06351South Korea Division of Gastroenterology Department of Internal MedicineSoonchunhyang University College of MedicineSeoul 04401South Korea

BACKGROUND The incidence of colorectal cancer(CRC)and preinvasive CRC(e.g.,early colon cancer and advanced adenoma)is gradually increasing in several *** To evaluate the trend in incidence of CRC and preinvasive CRC according to the increase in the number of colonoscopies performed in *** This retrospective cohort study enrolled Korean patients from 2002 to 2020 to evaluate the incidence of CRC and preinvasive CRC,and assess the numbers of diagnostic colonoscopies and colonoscopic ***-related complications by age group were also *** The incidence of CRC showed a rapid increase,then decreased after 2012 in the 50-75 year-age *** the study period,the rate of incidence of preinvasive CRC increased at a similar level in patients under 50 and 50-75 years of *** 2009,the increase has been rapid,showing a pattern similar to the increase in *** rate of colonoscopic polypectomy in patients aged under 50 was similar to the rate in patients over 75 years of age after *** rate of complications after colonoscopy and related deaths within 3 mo was high for those over 75 years of *** The diagnosis of preinvasive CRC increased with the increase in the number of colonoscopies *** the risk of colonoscopy-related hospitalization and death is high in the elderly,if early lesions at risk of developing CRC are diagnosed and treated under or at the age of 75,colonoscopy-related complications can be reduced for those aged 76 years or over.

关键词： Colorectal cancer Preinvasive colorectal cancer Colorectal polypectomy Colonoscopy

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Measurement of Gamma-Rays Induced Luminescence Generated in a Sapphire Based Fiber-Optic Radiation Sensor

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Journal of Applied Mathematics and Physics 2016年第8期4卷 1503-1506页

作者： Young Beom Song Kyoung Won Jang Hye Jin Kim dong eun lee Mingeon Kim Sang Hun Shin Wook Jae Yoo Bongsoo lee School of Energy Systems Engineering Chung-Ang University Seoul Korea School of Biomedical Engineering BK21 plus Research Institute of Biomedical Engineering Konkuk University Chungju-si Korea School of Biomedical Engineering BK21 plus Research Institute of Biomedical EngineeringKonkuk University Chungju-si Korea

In this study, we fabricated a sapphire based fiber-optic radiation sensor. To evaluate the fiber- optic radiation sensor, we measured the spectrum and intensity of the luminescence generated from the fiber-optic radiation sensor according to the thickness of the PMMA block by irradiation of gamma rays emitted from a Co-60 source. And the result was compared with the value calculated from the formula of Lambert-Beer.

关键词： Fiber-Optic Radiation Sensor Optical Glass Sapphire Luminescence Gamma Ray Source Spent Fuel

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