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Enhanced rate capability and cycle stability of Ti2C MXene for sodium storage through an aniline molecules welding strategy

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Tungsten 2025年第1期7卷 161-171页

作者： Hao Chen Ya-Qin Wang dong-Ting zhang Bei Zhao Min-Peng Li Chen-Yang Li Tian-Peng Xu Mao-Cheng Liu State Key Laboratory of Advanced Processing and Recycling of Non-Ferrous Metals Lanzhou University of Technology School of Materials Science and Engineering Lanzhou University of Technology School of Computer and Communication Technology Lanzhou University of Technology

MXenes obtained significant attention in the field of energy storage devices due to their characteristic layered structure,modifiable surface functional groups,large electrochemically active surface,and regulable interlayer ***,the self-restacking and sluggish ions diffusion kinetics performance of MXenes during the alkali metal ions insertion/extraction process severely impedes their cycle stability and rate *** paper proposes an aniline molecule welding strategy for welding p-phenylenediamine（PPDA） into the interlayers of Ti2C through a dehydration condensation *** welded PPDA molecules can contribute pillar effect to the layered structure of *** pillar effect effectively maintains the structural stability during the sodium ions insertion/extraction process and effectively expands the interlayer spacing of Ti2C from 1.16 to 1.38 nm,thereby enhancing ions diffusion kinetics performance and improving the long-term cycle *** Ti2C-PPDA demonstrates outstanding Na+storage capability,exhibiting a specific capacity of 100.2 mAh·g-1at a current density of 0.1 A·g-1over 960 cycles and delivering a remarkable rate capability 81.2 mAh·g-1at a current density of 5 A·*** study demonstrates that expanding interlayer spacing is a promising strategy to enhance the Na+storage capacity and improve long-term cycling stability,which provides significant guidance for the design of two-dimensional Na+storage materials with high-rate capability and cycle stability.

关键词： Diffusion kinetics Expanding interlayer spacing Rate capability Sodium ions storage Ti2C

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Analysis of the anti-T2DM components in dichloromethane fraction of Schisandra sphenanthera and its mechanism

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Traditional Medicine Research 2025年第1期10卷 27-43页

作者： Shi-Bo Feng Hai-Hui Jiang Hui-Li Kang Yi Jiang Hua-Wei zhang Xiao-Mei Song Yu-Ze Li Wen-Li Huang dong-dong zhang Chong Deng School of Pharmacy Shaanxi University of Chinese MedicineXianyang 712046China School of Pharmacy and Shaanxi Qinling Application Development and Engineering Center of Chinese Herbal Medicine Shaanxi University of Chinese MedicineXianyang 712046China Key Laboratory for Research and Development of“Qin Medicine”of Shaanxi Administration of Traditional Chinese Medicine Xianyang 712046China Shaanxi Key Laboratory of Research and Application of“Taibai Qi Yao” Xianyang 712046China

Background:The type 2 diabetes mellitus(T2DM)pharmacodynamic study of various parts of Schisandra sphenanthera was conducted in the previous stage,and it was found that dichloromethane extracted part(SDP)had a significant hypoglycemic ***,the components of SDP were analyzed,and the specific mechanism of its anti-T2DM was ***:We used a high-fat,high-sugar diet in combination with streptozotocin to induce a T2DM rat model,and the model rats were divided into two groups according to body weight and blood ***,oral glucose tolerance test,fasting blood glucose,low density lipoprotein cholesterol,superoxide dismutase,insulin,glycated hemoglobin,total cholesterol,nonesterified free fatty acids,alanine aminotransferase,high-density lipoprotein cholesterol,aspartate aminotransferase,malondialdehyde,and glutathione peroxidase were measured,organ indices were calculated,and pathological sections of pancreas and liver were *** 16S rRNA V3–V4 region of intestinal flora was sequenced to explore the effect of SDP on biochemical indicators and intestinal *** on the above indicators,the anti-T2DM mechanism of SDP in Schisandra sphenanthera was ***:After six weeks of administration,the biochemical indices of diabetic rats were diminished compared to the control *** SDP could significantly increase the gut microbialα-diversity index,resulting in significant changes in the flora of T2DM rats,with increased richness and diversity,reduced harmful flora,and significantly back-regulated the levels of acetic acid,propionic acid,and butyric ***:SDP can improve the symptoms associated with elevated blood glucose,dyslipidemia,elevated fasting insulin levels,and damaged glucose tolerance in *** against T2DM may be through the control of intestinal flora to normalize and exert anti-diabetic effect;its main active components may be lignans and terpenoids.

关键词： Schisandra sphenanthera T2DM intestinal flora HPLC

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基于质谱的脂质C=C和脂肪酰基位置鉴定方法及其在食品分析中的应用研究进展

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食品科学 2025年第1期46卷 293-303页

作者：滕蒙南段晓亮张东郭伟群浙江农林大学食品与健康学院浙江杭州311302 国家粮食和物资储备局科学研究院北京102629

脂质在生命体中发挥着重要作用,结构影响功能,脂质精细结构解析至关重要。但脂质结构的多样性和相似性对脂质分析提出了巨大挑战。质谱是脂质分析的重要技术之一,在脂质C=C和脂肪酰基位置结构解析中有着较好的应用。本文介绍脂质分析的... 详细信息

脂质在生命体中发挥着重要作用,结构影响功能,脂质精细结构解析至关重要。但脂质结构的多样性和相似性对脂质分析提出了巨大挑战。质谱是脂质分析的重要技术之一,在脂质C=C和脂肪酰基位置结构解析中有着较好的应用。本文介绍脂质分析的前处理方法,综述基于质谱的C=C位置和脂肪酰基位置鉴定方法,并讨论该方法在食品分析中的应用,最后展望质谱在脂质化合物精确结构解析方面的发展趋势,以期为不饱和脂质C=C位置和脂肪酰基位置鉴定以及异构体识别和定量分析技术发展和应用提供参考。

关键词：脂质质谱 C=C位置脂肪酰基位置应用

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Photodissociation Exploration for Near-Visible UV Absorption of Molecular Bromine

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Chinese Journal of Chemical Physics 2008年第1期21卷 12-20页

作者： dong-fang zhang Bing zhang State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics Wuhan Insti-tute of Physics and Mathematics Chinese Academy of Sciences Wuhan 430071 China Graduate School of Chinese Academy of Sciences Beijing 100039 China

The photodissociation of Br2 was investigated within the near-visible UV absorption band. Based on the potential curves for the ground and low-lying excited states, the optical cross-sections for the discrete transitions of C1^Пu,B^3Пou^＋, A^3П1u←X^1∑g＋ and their total energy absorption spectrum are derived, and the quantum yield of （Br＋Br6＊） channel are determined correspondingly. The one-dimensional Landau-Zener model is used to evaluate the behavior of curve crossing during photodissociation. The results indicate that the influence of nonadiabatic mechanism, which may be caused by the electronic-vibrational interplay between the 13 and C states, is negligibly small for the （Br＋Br^＊） channel. From the Landau-Zener modeling of the observed product recoil parameter β（Br＋Br）, the best-fit value of the coupling matrix elenment or coupling strength between the diabatic B and C state potentials is obtained.

关键词： Photodissociation Time-dependent wave packet Nonadiabatic mechanism Landau-Zener model

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Controlling microbiological interfacial behaviors of hydrophobic organic compounds by surfactants in biodegradation process

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Frontiers of Environmental Science & Engineering 2014年第3期8卷 305-315页

作者： dong zhang Department of Environmental Science Zhcjiang University Hangzhou 310058. China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou 310058 China

Bioremediation of hydrophobic organic compounds （HOCs） contanlinated soils involves several physicochemical and microbiological interracial processes among the soil-water-microorganism interfaces. The participation of surfactants facilitates the mass transport of HOCs in both the physicochemical and microbiological interfaces by reducing the interfacial tension. The effects and underlying mechanisms of surfactants on the physi-cochemical desorption of soil-sorbed HOCs have been widely studied. This paper reviewed the progress made in understanding the effects of surfactant on microbiological interlhcial transport of HOCs and the underlying mechanisms, which is vital for a better understanding and control of the mass transfer of HOCs in the biodegradation process. In summary, surfactants affect the microbiological interfacial behaviors of HOCs during three consecutive processes： the soil solution-microorganism sorption, the transmembrane process, and the intracellular metabolism. Surfactant could promote cell sorption of HOCs depending on the compatibility of surfactant hydrophile hydrophilic balance （HLB） with cell surface properties; while the dose ratio between surfactant and biologic mass （membrane lipids） determined the transmembrane processes. Although surfactants cannot easily directly affect the intracellular enzymatic metabolism of HOCs due to the steric hindrace, the presence of surfactants can indirectly enhanced the metabolism by increasing the substrate concentrations.

关键词： biodegradation sorption transmembrane transport microbiological interfaces surfactants

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Augmented FCN: rethinking context modeling for semantic segmentation

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Science China(Information Sciences) 2023年第4期66卷 193-211页

作者： dong zhang Liyan zhang Jinhui TANG School of Computer Science and Engineering Nanjing University of Science and Technology College of Computer Science and Technology Nanjing University of Aeronautics and Astronautics

The effectiveness of modeling contextual information has been empirically shown in numerous computer vision tasks. In this paper, we propose a simple yet efficient augmented fully convolutional network(AugFCN) by aggregating content-and position-based object contexts for semantic ***, motivated because each deep feature map is a global, class-wise representation of the input,we first propose an augmented nonlocal interaction(AugNI) to aggregate the global content-based contexts through all feature map interactions. Compared to classical position-wise approaches, AugNI is more efficient. Moreover, to eliminate permutation equivariance and maintain translation equivariance, a learnable,relative position embedding branch is then supportably installed in AugNI to capture the global positionbased contexts. AugFCN is built on a fully convolutional network as the backbone by deploying AugNI before the segmentation head network. Experimental results on two challenging benchmarks verify that AugFCN can achieve a competitive 45.38% mIoU(standard mean intersection over union) and 81.9% mIoU on the ADE20K val set and Cityscapes test set, respectively, with little computational overhead. Additionally, the results of the joint implementation of AugNI and existing context modeling schemes show that AugFCN leads to continuous segmentation improvements in state-of-the-art context modeling. We finally achieve a top performance of 45.43% mIoU on the ADE20K val set and 83.0% mIoU on the Cityscapes test set.

关键词： semantic segmentation context modeling long-range dependencies attention mechanism

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Numerical Simulation of the Distribution Function and Free Energy of a Single Wormlike Polymer Confined between Hard Walls

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Chinese Journal of Polymer Science 2020年第2期38卷 179-186,I0007页

作者： Yang Gu Hui zhang dong-Liang zhang School of Mathematics Sciences Beijing Normal UniversityBeijing 100875China Laboratory of Mathematics and Complex Systems Ministry of EducationSchool of Mathematics SciencesBeijing Normal UniversityBeijing 100875China The department of Orthodontics Beijing Stomatology Hospital Affiliated to Capital Medical UniversityBeijing 100006China

We focus on the distribution and free energy of a wormlike polymer confined between two parallel hard *** variation in the distribution and free energy of the wormlike chain as the spacing between the walls decreases(or as the total contour length of the wormlike chain increases or as the persistence length of the chain increases)is *** main reason for these changes is a degradation of the long wormlike chain into a Gaussian long chain under weak confinement.

关键词： Wormlike polymer Free energy Weak confinement

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Flexible single-electrode triboelectric nanogenerator with MWCNT/PDMS composite film for environmental energy harvesting and human motion monitoring

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Rare Metals 2022年第9期41卷 3117-3128页

作者： Hao zhang dong-Zhi zhang dong-Yue Wang Zhen-Yuan Xu Yan Yang Bao zhang College of Control Science and Engineering China University of Petroleum(East China)Qingdao266580China

With the rapid development of wearable electronic devices,modern portable energy sources pay more attention to lightweight,low cost,high flexibility and high *** paper proposed a flexible single-electrode triboelectric nanogenerator(S-TENG)composed of multi-walled carbon nanotube(MWCNT)/polydimethylsiloxane(PDMS)*** S-TENG has the advantages of high flexibility,high hydrophobicity,light weight,low cost,and high output *** peak-to-peak open circuit voltage can reach 435 V and the maximum short-circuit current density is 13μA·cm^(−2) under continuous *** the external load is 40 MΩ,the maximum output power density is 3.7 mW·cm^(−2).The S-TENG can not only harvest the mechanical energy generated by biological movement,but also can be used as a sensor to effectively detect human movement and handwriting *** addition,a 4×4 sensor array and a wireless transmission system were constructed to realize multi-point distributed detection and wireless transmission of portable smart *** S-TENG can harvest energy from falling water droplets,uninterrupted water flow,wind and percussion sounds,which demonstrates its broad application prospects in the field of flexible wearables.

关键词： Flexible Wearable Single-electrode Triboelectric nanogenerator(TENG) Environmental energy

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A SIMPLE ITERATIVE ALGORITHM FOR MAXCUT

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Journal of Computational Mathematics 2024年第5期42卷 1277-1304页

作者： Sihong Shao dong zhang Weixi zhang CAPT LMAM and School of Mathematical SciencesPeking UniversityBeijing 100871China LMAM and School of Mathematical Sciences Peking UniversityBeijing 100871China

We propose a simple iterative(SI)algorithm for the maxcut problem through fully using an equivalent continuous *** does not need rounding at all and has advantages that all subproblems have explicit analytic solutions,the cut values are monotonically updated and the iteration points converge to a local optima in finite steps via an appropriate subgradient *** experiments on G-set demonstrate the *** particular,the ratios between the best cut values achieved by SI and those by some advanced combinatorial algorithms in[***.,248(2017),365-403]are at least 0.986 and can be further improved to at least 0.997 by a preliminary attempt to break out of local optima.

关键词： Maxcut Iterative algorithm Exact solution Subgradient selection Fractional programming

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Effect of Heat Flux Distribution on Entropy Generation and Irreversibility of Lead-Bismuth Eutectic(LBE)Forced Convective Heat Transfer

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Journal of Thermal Science 2023年第1期32卷 223-236页

作者： zhang dong zhang Haochun WANG Qi SUN Wenbo School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China

Investigations on entropy generation and thermal irreversibility analysis are conducted for liquid lead-bismuth eutectic(LBE)in an annular *** find better performance in convective heat transfer,the computational fluid dynamics(CFD)code based on the finite volume method(FVM)is adopted to solve this *** elevated temperature LBE flows in the annular pipe,and four types of heat flux,including constant,linear increase and decrease,and parabolic distributions are imposed at the inside wall of the annular *** investigations are conducted for the specific average heat input of 200 kW/m^(2),and the different Peclet number Pe is set from 1200 to *** SST k-ωturbulent model and Cheng-Tak Prt model are *** mesh independence validation and models verification are also conducted and the maximum Nu error is 5.43%compared with previous experimental *** results from the local and system scales,respectively,including volumetric dimensionless entropy generation,Ns,Be,and Ep,are *** results indicate that the viscous friction and heat transfer caused by entropy generation can be found in the viscous sub-layer and buffer layer *** transfer is the primary factor that leads to irreversible ***,the results show that the best thermodynamic performance occurs under parabolic distributed heat flux in the research scope.

关键词： liquid lead-bismuth eutectic entropy generation analysis annular pipe CFD

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