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Enhanced visible-light photocatalytic hydrogen evolution using two-dimensional carbon nitride sheets with the removal of amine groups

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Chinese Chemical Letters 2024年第2期35卷 446-450页

作者： Yu Zhang Liting Wu Shaopeng Wang dingyi yang Huan Liang Yizhang Wu Jian Hao Youqing Wang Jianke Liu Yong Wang Department of Physics Shaanxi University of Science and TechnologyXi'an 710021China School of Advanced Materials and Nanotechnology Academy of Advanced Interdisciplinary ResearchXidian UniversityXi'an 710126China The State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology Xidian UniversityXi'an 710126China Collaborative Innovation Center of Advanced Microstructures National Laboratory of Solid State MicrostructuresNanjing UniversityNanjing 210093China State Key Laboratory of High-Efficiency Utilization of Coal and Green Chemical Engineering Ningxia UniversityYinchuan 750021China

Two-dimensional(2D)carbon nitride sheets(CNs)with atomically thin structures are regarded as one of the most promising materials for solar energy ***,due to their substantially enlarged bandgap caused by the strong quantum size effect and their incomplete polymerisation with a large number of non-condensed surface amino groups,the practical applicability of CNs in photocatalysis is *** this study,CNs with broad visible-light absorption were synthesised using a 5-min fast thermal *** removal of uncondensed amine groups reduces the bandgap of CNs from 3.06 eV to 2.60 eV,increasing their absorption of visible ***,the CNs were distorted after annealing,which can differentiate the spatial positions of electrons and holes,enhancing the visible-light absorption *** a result,when exposed to visible light,the photocatalytic hydrogen production activity of atomically thin 2D CNs rose by 8.38 *** research presents a dependable and speedy method for creating highly effective visible-light photocatalysts with narrowed bandgaps and improved visible-light absorption.

关键词： 2D carbon nitride sheets Rapid thermal annealing DFT calculations Visible-light absorption visible-light photocatalysis

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Room-temperature ferromagnetism and piezoelectricity in metalfree 2D semiconductor crystalline carbon nitride

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Nano Research 2024年第6期17卷 5670-5679页

作者： Yong Wang dingyi yang Wei Xu Yongjie Xu Yu Zhang Zixuan Cheng Yizhang Wu Xuetao Gan Wei Zhong Yan Liu Genquan Han Yue Hao Wide Bandgap Semiconductor Technology Disciplines State Key Laboratory School of MicroelectronicsAcademy of Advanced Interdisciplinary ResearchXidian UniversityXi’an 710071China Emerging Device and Chip Laboratory Hangzhou Institute of TechnologyXidian UniversityHangzhou 311200China INRS Centre for Energy Materials and Telecommunications1650 Boul.Lionel BouletVarennesQC J3X 1P7Canada National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures and Jiangsu Provincial Key Laboratory for NanotechnologyNanjing UniversityNanjing 210093China School of Education Jiangsu Open UniversityNanjing 210036China Department of Physics Shaanxi University of Science and TechnologyXi’an 710021China Department of Applied Physical Sciences The University of North Carolina at Chapel HillChapel HillNC 27514USA Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information Technologyand Shaanxi Key Laboratory of Optical Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical UniversityXi'an 710129 China

Two-dimensional(2D)materials that combine ferromagnetic,semiconductor,and piezoelectric properties hold significant potential for both fundamental research and spin electronic ***,the majority of reported 2D ferromagnetic-semiconductor-piezoelectric materials rely on d-electron systems,which limits their practical applications due to a Curie temperature lower than room temperature(RT).Here,we report a high-crystallinity carbon nitride(CCN)material based on sp-electrons using a chemical vapor deposition *** exhibits a band gap of 1.8 eV and has been confirmed to possess substantial in-plane and out-of-plane ***,we acquired clear evidences of ferromagnetic behavior at room *** structural characterizations combined with theoretical calculations reveal that incorporating structural oxygen into the highly ordered heptazine structure causes partial substitution of nitrogen sites,which is primarily responsible for generating room-temperature ferromagnetism and *** a result,the strain in wrinkles can effectively modulate the domain behavior and piezoelectric potential at room *** addition of RT ferromagnetic-semiconductor-piezoelectric material based on sp-electrons to the family of two-dimensional materials opens up numerous possibilities for novel applications in fundamental research and spin electronic devices.

关键词： crystallinity carbon nitride room-temperature ferromagnetism piezoelectricity magnetic force microscopy density functional theory(DFT)calculations

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基于图像法对自密实超高性能混凝土性能提升的研究

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硅酸盐通报 2024年第4期43卷 1398-1409页

作者：毛翔杨鼎宜曹忠露赵健陈龙祥王彤章扬州大学建筑科学与工程学院扬州225127 中交天津港湾工程研究院有限公司天津300222

为提升超高性能混凝土(UHPC)的性能,采用改进后的Andreasen&Andersen颗粒堆积模型设计UHPC基体配合比,利用图像法分析UHPC不同基体黏度对钢纤维分布的影响,并通过抗压强度结合纤维分布系数选择合适的基体黏度,研究不同形状、体积掺量的... 详细信息

为提升超高性能混凝土(UHPC)的性能,采用改进后的Andreasen&Andersen颗粒堆积模型设计UHPC基体配合比,利用图像法分析UHPC不同基体黏度对钢纤维分布的影响,并通过抗压强度结合纤维分布系数选择合适的基体黏度,研究不同形状、体积掺量的钢纤维对UHPC力学性能的影响,最终得到力学性能最佳的配合比。试验结果表明:良好的UHPC基体黏度在均匀分散钢纤维的同时可以避免内部出现过多气泡,进一步提升UHPC抗压强度;与端钩、长直形钢纤维相比,波纹形钢纤维在相同黏度下分散效果更佳,且对UHPC基体力学性能提升效果更好。UHPC最佳配合比为水胶比0.16,水泥、硅灰、矿渣质量比0.75∶0.2∶0.05,波纹形钢纤维体积掺量3%,减水剂质量分数0.8%,此时粉体颗粒最紧密堆积、钢纤维分布均匀,UHPC性能最佳。

关键词：超高性能混凝土颗粒紧密堆积理论钢纤维单丝拉拔抗压强度图像法

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Constructing metal-free heterophotocatalyst using two-dimensional carbon nitride sheets and violet phosphorene for highly efficient visible-light photocatalysis

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Journal of Materials Science & Technology 2023年第15期146卷 113-120页

作者： Yong Wang Chengxin Zeng Liting Wu Yalin Dong Yu Zhang dingyi yang Wen Hu Jian Hao Hongzhe Pan Rusen yang Academy of Advanced Interdisciplinary Research School of Advanced Materials and NanotechnologyXidian UniversityXi’an 710126China Department of Physics Shaanxi University of Science and TechnologyXi’an 710021China State Key Laboratory of High-Efficiency Utilization of Coal and Green Chemical Engineering Ningxia UniversityYinchuan 750021China School of Physics and Electronic Engineering Linyi UniversityLinyi 276005China

Two-dimensional(2D)carbon nitride sheets(CNs)with nanoscale thickness have great potential in solar energy conversion owing to their intrinsic ***,their photocatalytic efficiency falls far below the practical requirements because the generated electron-hole pairs rapidly *** construct a metal-free 2D p–n junction heterophotocatalyst from CNs and violet phosphorene(VP)using a simple electrostatic self-assembly *** experimental results and density functional theory calculations show that the built-in electric field of the p–n junction promotes photogenerated carrier transport at the heterojunction interface,thereby promoting the separation of photogenerated electron-hole *** visible-light illumination,the visible-light photocatalytic hydrogen and CO production rates of the CNs/VP heterojunction were increased by 5.85 and 1.51 times,respectively,when compared to that of *** study provides new insights into the design of metal-free heterogeneous photocatalysts with high catalytic activity。

关键词： Heterostructures DFT calculations Visible-light photocatalysis

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Designable heteronanocrystals via interface redox reaction

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Nano Research 2023年第4期16卷 5946-5952页

作者： Zhihua Li yang Li Nannan Luo Yuanyuan Qie dingyi yang Guowei Cao Yuxiang Liu Ying Fu Na Li Wen Hu Min Zhang Rusen yang Bo Tang College of Chemistry Chemical Engineering and Materials ScienceKey Laboratory of Molecular and Nano ProbesMinistry of EducationCollaborative Innovation Center of Functionalized Probes for Chemical Imaging in Universities of ShandongInstitute of Molecular and Nano ScienceShandong Normal UniversityJinan 250014China School of Advanced Materials and Nanotechnology Xidian UniversityXi'an 710126China

The synergistic interaction of different components in heteronanocrystals induces interfacial phenomena and novel ***,effective technologies to design and fabricate heteronanocrystals with materials on demand are still *** heterostructures in a copper patina are known to form at room temperature and under atmospheric *** redox process of copper tarnish inspired the discovery of a simple strategy to achieve heteronanocrystals that contained elements from group 3-11 and group *** interface redox-induced method is self-regulating at ambient conditions and applicable for metal,semiconductor,and dielectric *** enhanced interface bonding endows the heteronanocrystals with outstanding stability and catalytic performance,while the modular approach enables the design and fabrication of heteronanocrystals with intended materials to meet different purposes.

关键词： heteronanocrystals interface redox-induced synthesis modular approach

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混掺纤维水泥砂浆的高温性能研究

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硅酸盐通报 2024年第3期43卷 851-865页

作者：郭子荣杨鼎宜曹忠露贾向锋赵健陈龙祥毛翔扬州大学建筑科学与工程学院扬州225127 中交天津港湾工程研究院有限公司天津300222 扬州华运新材料科技有限公司扬州225000

火灾产生的高温会对水泥基复合材料造成严重损伤,而混掺玄武岩纤维可一定程度上提高水泥基复合材料的耐高温性能。为研究不同种类玄武岩纤维与聚丙烯纤维混掺水泥砂浆经高温作用后的性能变化规律,测试了混掺纤维水泥砂浆高温后的基本力... 详细信息

火灾产生的高温会对水泥基复合材料造成严重损伤,而混掺玄武岩纤维可一定程度上提高水泥基复合材料的耐高温性能。为研究不同种类玄武岩纤维与聚丙烯纤维混掺水泥砂浆经高温作用后的性能变化规律,测试了混掺纤维水泥砂浆高温后的基本力学性能,并借助扫描电子显微镜(SEM)和压汞试验对混掺纤维水泥砂浆的微观结构进行分析。结果表明:不同种类的玄武岩纤维与聚丙烯纤维混掺后均能改善水泥砂浆的耐高温性能;温度在200℃时由于水泥砂浆内部发生二次水化,混掺纤维水泥砂浆的抗压强度和抗折强度显著提高。随着温度升高至800℃,水泥砂浆内部结构被破坏,孔隙率逐渐增大,力学性能逐渐下降,但混掺纤维水泥砂浆性能仍高于基准组,这是因为聚丙烯纤维高温熔化后留下大量的孔道,缓解水泥砂浆内部孔隙压力,且玄武岩纤维在水泥砂浆内部起到桥接作用,缓解了高温裂纹的扩展。

关键词：聚丙烯纤维玄武岩纤维高温力学性能孔隙率微观结构

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High Permeability of Boron along the Transverse Direction of Wood under High-Voltage Electrostatic Field (HVEF) Treatment

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Journal of Renewable Materials 2022年第3期10卷 721-734页

作者： Daiyuan Zhang Qian He Baocong Du Junbao Yu Xudong Zhu dingyi yang Shengcai Li Tianyi Zhan Liming Shen Zhiqiang Wang Xiaoning Lu College of Materials Science and Engineering Nanjing Forestry UniversityNanjing210037China College of Civil Science and Engineering Yangzhou UniversityYangzhou225127China yangzhou Polytechnic Institute Yangzhou225100China

Permeability of wood preservative is one of the most significant factors for protection of wood ***-sotropic flow permeability was involved in different directions of wood with higher flow resistance in the trans-verse and lower longitudinal *** this study,boron acid solution was brushed onto the tangential section of air-dried wood cubes and boron penetration along wood transverse direction was investigated under free dif-fusion,vacuum and HVEF ***-scale boron distribution,FTIR measurement,leaching property,mechanical properties and fungistatic characteristic were investigated for free diffusion,vacuum and HVEF trea-ted samples *** results revealed that boron exhibited high permeability along the transverse direc-tion with the penetration depth of≈35 mm for HVEF treated samples and≈1 mm for free diffusion and vacuum treated *** HVEF treated samples,no significant decrease of hardness,compression modulus of elasti-city and strength were found in the treated *** fungistatic characteristic was showcased in HVEF trea-ted samples exposed to white rot ***,HVEF treatment has a positive effect on boron permeability and the improvement of penetration depth of preservatives hence playing a significant role in wood protection and prolonging the service life of wood construction.

关键词： Wood permeability boron distribution transverse direction HVEF treatment mechanical property fungistatic property

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MD Simulation of Diffusion Behaviors in Collision Welding Processes of Al-Cu, Al-Al, Cu-Cu

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Computers, Materials & Continua 2024年第6期79卷 3455-3468页

作者： dingyi Jin Guo Wei School of Intelligent Manufacturing Hunan First Normal UniversityChangsha410082China School of Physics and Technology Center for Ion Beam ApplicationHubei Nuclear Solid Physics Key LaboratoryWuhan UniversityWuhan430072China

To investigate the effects of material combinations and velocity conditions on atomic diffusion behavior near collision interfaces,this study simulates the atomic diffusion behavior near collision interfaces in Cu-Al,Al-Al and Cu-Cu combinations fabricated through collision welding using molecular dynamic(MD)*** atomic diffusion behaviors are compared between similar metal combinations(Al-Al,Cu-Cu)and dissimilar metal combinations(Al-Cu).By combining the simulation results and classical diffusion theory,the diffusion coefficients for similar and dissimilar metal material combinations under different velocity conditions are *** effects of material combinations and collision velocity on diffusion behaviors are also *** diffusion behaviors of dissimilar material combinations strongly depend on the transverse velocity,whereas those of the similar material combinations are more dependent on the longitudinal *** findings can provide guidance for optimizing welding parameters.

关键词： Atomic diffusion behavior molecular dynamics collision welding

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Rational Design of Biological Crystals with Enhanced Physical Properties by Hydrogen Bonding Interactions

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Research 2023年第3期2023卷 659-668页

作者： Hui Yuan Bin Xue dingyi yang Sigal Rencus-Lazar Yi Cao Ehud Gazit Dan Tan Rusen yang School of Advanced Materials and Nanotechnology Xidian UniversityXi’an 710126China The Shmunis School of Biomedicine and Cancer Research George S.Wise Faculty of Life SciencesDepartment of Materials Science and EngineeringThe Iby and Aladar Fleischman Faculty of EngineeringTel Aviv UniversityTel Aviv 6997801Israel National Laboratory of Solid State Microstructure Department of PhysicsNanjing UniversityNanjing 210093JiangsuChina

Hydrogen bonds are non-covalent interactions and essential for assembling supermolecules into ordered structures in biological systems,endowing crystals with fascinating physical properties,and inspiring the construction of eco-friendly electromechanical ***,the interplay between hydrogen bonding and the physical properties is not fully understood at the molecular ***,we demonstrate that the physical property of biological crystals with double-layer structures could be enhanced by rationally controlling hydrogen bonding interactions between amino and carboxyl *** hydrogen bonding interactions result in various thermal,mechanical,electronic,and piezoelectric *** particular,the weak interaction between O and H atoms contributes to low mechanical strength that permits important ion displacement under stress,giving rise to a strong piezoelectric *** study not only reveals the correlation between the hydrogen bonding and physical properties in double-layer structures of biological crystals but also demonstrates the potential of these crystals as functional biomaterials for high-performance energy-harvesting *** calculations and experimental verifications in this work provide new insights into the rational design of biomaterials with desirable physical properties for bioelectrical devices by modulating intermolecular interactions.

关键词： bonding rational biomaterials

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Tensile Behavior of Strain Hardening Cementitious Composites (SHCC) Containing Reactive Recycled Powder from Various C&D Waste

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Journal of Renewable Materials 2021年第4期9卷 743-765页

作者： Ruixue Wu Tiejun Zhao Peng Zhang dingyi yang Miao Liu Zhiming Ma College of Civil Engineering Qingdao University of TechnologyQingdao266033China College of Civil Science and Engineering Yangzhou UniversityYangzhou225127China

This work investigates the feasibility of utilizing reactive recycled powder(RP)from construction and demolition(C&D)waste as supplementary cementitious material(SCM)to achieve a ductile strain hardening cementitious composites(SHCC).The recycled mortar powder(RMP)from mortar waste,recycled concrete powder(RCP)from concrete waste and recycled brick powder(RBP)from clay brick waste were first prepared,and the micro-properties and tensile behavior of SHCC containing various types and replacement ratios of RPs were *** incorporated RP promotes pozzolanic and filler effects,while the hydration products in cementitious materials decrease with RP incorporation;therefore,the incorporated RP decreases the compressive strength of *** to the reduction in the matrix strength,the incorporated RP increases the crack-bridging extent and ductility of SHCC;the irregular micro-structure and high reactivity of RP also help the strain-hardening performance of the prepared *** addition,the strainhardening performance of SHCC containing RMP and RBP is surperior to that of SHCC with RCP and is slightly lower than that of SHCC with fly ash(FA);for instance,the ultimate strain of SHCC containing 54%FA,RMP,RCP and RBP is 3.67%,3.61%,2.52%and 3.53%,*** addition,the strain-hardening behavior of an SHCC doubled mix with FA and RMP or RBP has a similar ultimate strain and a higher ultimate stress than SHCC containing only FA.

关键词： Construction and demolition waste recycled powder strain hardening cementitious composites tensile behavior

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