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Aluminum exposure impairs oocyte quality via subcellular structure disruption and DNA da.age-related apoptosis in mice

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Journal of Environmental Sciences 2024年第5期139卷 308-319页

作者： Hongge Li Jingcai Liu Weihua Nong Mengying Shen Sheng dou Shaochen Sun Junli Wang The Affiliated Hospital of Youjiang Medical University for Nationalities Guangxi 533000China College of Animal Science and Technology Nanjing Agricultural UniversityNanjing 210095China School of Medical Laboratory Youjiang Medical University for NationalitiesGuangxi 533000China Industrial College of Biomedicine and Health Industry Youjiang Medical University for NationalitiesGuangxi 533000China Reproductive Medicine Guangxi Medical and Health Key Discipline Construction ProjectThe Affiliated Hospital of Youjiang Medical University for NationalitiesGuangxi 533000China

Aluminum(Al)can lead to an exposure of creature in varieties ways for its universality,and it could disturb normal physiological metabolism,with the da.age to multisystem including *** the oocyte quality is critical for female reproduction,we inspected the toxicity of Al on mouse oocyte *** constructed in vitro exposure mouse model,and we found that 5 mmol/L Al had adverse effects on oocyte maturation by impairing organelle and *** spindle and misaligned chromosomes which might be considered to be caused by elevated levels of acetylation,as well as abnormal distribution of actin dynamics could hinder normal meiosis of *** dysfunction indicated that Al affected proteins synthesis,transport and digestion,which would further da.age oocyte *** order to explore the mechanism of Al toxicity,our further investigation demonstrated that Al caused mitochondrial dysfunction and imbalance calcium homeostasis,resulting in limited energy ***,high level of reactive oxygen species,DNA da.age and apoptosis caused by oxida.ive stress were also the manifestation of Al toxicity on *** conclusion,our study provided the evidence that Al exposure affected oocyte quality through its effects on spindle organization,actin dynamics,organelle function and the induction of DNA da.age-related apoptosis with mouse model.

关键词： Aluminum Oocyte Cytoskeleton Organelle DNA da.age

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Unraveling the mechanism of potassium metal capacitor for highly efficient charge storage

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Science China Chemistry 2024年第5期67卷 1578-1588页

作者： Qianqian Yao Pei Tang Kunyao Peng Zhenyuan Miao Yuecong Chen Qingyun dou Xingbin Yan Department of Materials Science and Engineering Sun Yat-sen UniversityGuangzhou 510275China South China Academy of Advanced Optoelectronics South China Normal UniversityGuangzhou 510006China

Although hybrid metal ion capacitors(MICs) are highly desired to achieve both high power density of supercapacitors and high energy density of rechargeable batteries, the mismatch problem of electrochemical kinetics of negative and positive electrodes in MICs hampers the realization of this goal. Here, a new hybrid capacitor concept-potassium metal capacitor(PMC) is proposed for the first time, where potassium metal and commercial activated carbon(AC) without any modification are applied as negative and positive electrodes, respectively, and the electrolyte is the same as that of non-aqueous potassium ion batteries. The simplest PMC prototype exhibits a good combination of high energy density(184.9 Wh kg^(-1)) and power density(12.4 kW kg^(-1)), which benefits from the synergistic effect of potassium metal and AC electrode. The former experiences fast potassium plating/striping during charging and discharging, and the later possesses complex multiple charge behaviors driven by low potential of potassium metal. Specifically, below open-circuit voltage, transportation of solvated cations in AC pores plays an important role;beyond this voltage, synergy actions of cations and anions, including adsorption/desorption of solvated cations and anions, and ions exchange between them, dominate the capacitance contribution. This work enriches the types of MICs, and deepens the understanding of the energy storage mechanism of non-aqueous hybrid metal capacitors.

关键词： hybrid capacitor potassium metal activated carbon charge storage mechanism

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EMPSI:Efficient multiparty private set intersection(with cardinality)

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Frontiers of Computer Science 2024年第1期18卷 199-213页

作者： Yunbo YANG Xiaolei DONG Zhenfu CAO Jiachen SHEN Ruofan LI Yihao YANG Shangmin dou Shanghai Key Laboratory of Trustworthy Computing East China Normal UniversityShanghai 200062China Kunyao Academy of Shanghai Kunyao Network Technology Co. Ltd.Shanghai 201203China PwC US Advisory Shanghai AC Shanghai 200233China

Multiparty private set intersection(PSI)allows several parties,each holding a set of elements,to jointly compute the intersection without leaking any additional *** the development of cloud computing,PSI has a wide range of applications in privacy ***,it is complex to build an efficient and reliable scheme to protect user *** address this issue,we propose EMPSI,an efficient PSI(with cardinality)protocol in a multiparty *** avoids using heavy cryptographic primitives(mainly rely on symmetric-key encryption)to achieve better *** addition,both PSI and PSI with the cardinality of EMPSI are secure against semi-honest adversaries and allow any number of colluding clients(at least one honest client).We also do experiments to compare EMPSI with some state-of-the-art *** experimental results show that proposed EMPSI(-CA)has better performance and is scalable in the number of clients and the set size.

关键词： intersection cardinal primitive

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Co-aromatization of methane and hexane over Pt encapsulated in ZSM-5 zeolite and the electronic effect of K promoters

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Science China Chemistry 2024年第3期67卷 1017-1027页

作者： Bei Liu Fan Wang Xiaomeng dou Pengfei Li Hongwei Xiang Yong Yang Peng He State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001China Department of Chemistry Tsinghua UniversityBeijing 100084China National Energy R&D Center for Coal to Liquid Fuels Synfuels China Technology Co.Ltd.Beijing 101407China University of Chinese Academy of Sciences Beijing 101408China Leibniz-Institut für Katalyse e.V.an der Universitat Rostock Rostock 18059Germany

The co-aromatization of methane with higher hydrocarbons represents a promising route to valorize methane, an abunda.t but underexploited carbon resource. In this study, we elucida.e a novel approach to enhance the catalytic co-aromatization of hexane and methane by confining Pt within zeolite catalysts and modulating its electron density. Our findings show that encapsulating Pt within MFI structure is pivotal for activating the feedstock and fostering the formation of aromatic products. Interaction between K atoms and the silanol nest forms siloxy groups which are critical for the stabilization of Pt species. Tuning the K content in PtSn@MFI catalysts adeptly alters the electronic configuration of Pt clusters. This modification is corroborated by infrared and X-ray photoelectron spectroscopy analysis, and density functional theory calculations. Remarkably, the catalyst with 0.8 wt% K exhibits an optimal Pt electron density, driving its superior efficacy in the co-aromatization reaction, converting 0.78 mol of methane for each mole of hexane processed. By employing ~(13)C isotopic labeling and solid-state NMR studies, we demonstrate the participation of methane in the adsorbed species inside the zeolite channel and its incorporation to the benzyl site of the substitute group and phenyl rings in aromatic compounds, underscoring the importance of Pt encapsulation.

关键词： Pt encapsulation MFI zeolite methane activation co-aromatization ^(13)C solid-state NMR

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Catalytic effect in lithium metal batteries: From heterogeneous catalyst to homogenous catalyst

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Journal of Energy Chemistry 2024年第3期90卷 305-326,I0008页

作者： Haining Fan Xuan-Wen Gao Hailong Xu Yichun Ding Shi-Xue dou Wen-Bin Luo School of Fashion and Textiles The Hong Kong Polytechnic UniversityHong Kong 100872China Institute for Energy Electrochemistry and Urban Mines Metallurgy School of MetallurgyNortheastern UniversityShenyang 110819LiaoningChina Institute of Energy Materials Science University of Shanghai for Science and TechnologyShanghai 200000China State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi'an 710000ShaanxiChina

Lithium metal batteries are regarded as prominent contenders to address the pressing needs owing to the high theoretical *** the broader implementation,the primary obstacle lies in the intricate multi-electron,multi-step redox reaction associated with sluggish conversion kinetics,subsequently giving rise to a cascade of parasitic *** order to smooth reaction kinetics,catalysts are widely introduced to accelerate reaction rate via modulating the energy *** past decades,a large amount of research has been devoted to the catalyst design and catalytic mechanism exploration,and thus the great progress in electrochemical performance has been ***,it is necessary to make a comprehensive review toward key progress in catalyst design and future development *** this review,the basic mechanism of lithium metal batteries is provided along with corresponding advantages and existing challenges detailly *** main catalysts employed to accelerate cathode reaction with emphasis on their catalytic mechanism are summarized as ***,the rational design and innovative direction toward efficient catalysts are suggested for future application in metal-sulfur/gas battery and *** review is expected to drive and benefit future research on rational catalyst design with multi-parameter synergistic impacts on the activity and stability of next-generation metal battery,thus opening new avenue for sustainable solution to climate change,energy and environmental issues,and the potential industrial economy.

关键词： Energy storage and conversion Metal battery Sulfur battery Air battery Catalytic effect Heterogeneous catalyst Homogeneous catalyst

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XRL-SHAP-Cache:an explainable reinforcement learning approach for intelligent edge service caching in content delivery networks

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Science China(Information Sciences) 2024年第7期67卷 46-71页

作者： Xiaolong XU Fan WU Muhammad BILAL Xiaoyu XIA Wanchun dou Lina YAO Weiyi ZHONG School of Software Nanjing University of Information Science and Technology School of Computing and Communications Lancaster University School of Computing Technologies Royal Melbourne Institute of Technology State Key Laboratory for Novel Software Technology Nanjing University School of Computer Science and Engineering University of New South Wales da.a 61 Commonwealth Scientific and Industrial Research Organization School of Computer Science Qufu Normal University

Content delivery networks(CDNs) play a pivotal role in the modern internet infrastructure by enabling efficient content delivery across diverse geographical regions. As an essential component of CDNs, the edge caching scheme directly influences the user experience by determining the caching and eviction of content on edge servers. With the emergence of 5G technology, traditional caching schemes have faced challenges in ada.ting to increasingly complex and dynamic network environments. Consequently, deep reinforcement learning(DRL) offers a promising solution for intelligent zero-touch network governance. However, the blackbox nature of DRL models poses challenges in understanding and making trusting decisions. In this paper,we propose an explainable reinforcement learning(XRL)-based intelligent edge service caching approach,namely XRL-SHAP-Cache, which combines DRL with an explainable artificial intelligence(XAI) technique for cache management in CDNs. Instead of focusing solely on achieving performance gains, this study introduces a novel paradigm for providing interpretable caching strategies, thereby establishing a founda.ion for future transparent and trustworthy edge caching solutions. Specifically, a multi-level cache scheduling framework for CDNs was formulated theoretically, with the D3QN-based caching scheme serving as the targeted interpretable model. Subsequently, by integrating Deep-SHAP into our framework, the contribution of each state input feature to the agent's Q-value output was calculated, thereby providing valuable insights into the decision-making process. The proposed XRL-SHAP-Cache approach was evaluated through extensive experiments to demonstrate the behavior of the scheduling agent in the face of different environmental *** results demonstrate its strong explainability under various real-life scenarios while maintaining superior performance compared to traditional caching schemes in terms of cache hit ratio, quality of service(QoS),a

关键词： deep reinforcement learning (DRL) explainable artificial intelligence (XAI) multi-level cache content delivery network (CDN) D3QN algorithm Deep-SHAP

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Semiannual oscillation,annual oscillation,quasibiennial oscillation,and solar cycle variation of the OH airglow emission in the mesopause region

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Earth and Planetary Physics 2024年第3期8卷 479-496页

作者： Sheng-Yang Gu Dong Wang YuSong Qin Liang Tang YaFei Wei XianKang dou Electronic Information School Wuhan UniversityWuhan 430072China School of Optoelectronic Engineering Chongqing University of Posts and TelecommunicationsChongqing 400065China

The vertically integrated emission rate,centroid altitude,peak emission rate,and peak height of the hydroxyl(OH)airglow were calculated from Thermosphere Ionosphere Mesosphere Energetics and Dynamics(TIMED)/Sounding of the Atmosphere using Broadband Emission Radiometry(SABER)observations to study the seasonal and interannual variations in the intensity and location of the OH *** emission rate is inversely proportional to the height of the emission,with the semiannual oscillation dominating at low latitudes and the annual oscillation dominating at higher *** OH emission is modulated by the quasibiennial oscillation at the equator,and the quasibiennial oscillation signal is weak at other *** represented the vertical transport of atomic oxygen by using atomic oxygen concentrations obtained from a global atmospheric model,the Specified Dynamics Whole Atmosphere Community Climate Model with thermosphere and ionosphere eXtension *** with the amplitudes of the migrating diurnal tide(DW1)calculated from temperature da.a observed by TIMED/SABER,we found that both the vertical transport of atomic oxygen and DW1 amplitudes in the equatorial region exhibit semiannual oscillation and quasibiennial oscillation,which have a strong correlation with the variations in the amplitude and phase of semiannual oscillation and quasibiennial oscillation in OH *** is likely that the DW1 affects the vertical transport of atomic oxygen that is involved in the reaction to produce O3,thus affecting the OH *** analyzed the relationship between OH emission and solar activity by using the solar radio flux at 10.7 cm as a proxy for solar *** results showed that the OH emission is well correlated with solar activity,and the modulation of OH emission by solar activity has a significant latitudinal *** small correlation between emission height and solar activity indicates that solar activity modulates OH emission mainly thr

关键词： OH airglow semiannual oscillation quasibiennial oscillation solar activity diurnal tide

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Effects of biodegrada.ion on diamondoid distribution in crude oils from the Bongor Basin,Chad

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Energy Geoscience 2024年第2期5卷 120-128页

作者： Huanxin Song Menghan Chen Lirong dou Dingsheng Cheng Zhigang Wen Cooperative Innovation Center of Unconventional Oil and Gas Yangtze UniversityWuhanHubei430100China College of Resources and Environment Yangtze UniversityWuhanHubei430100China PetroChina Research Institute of Petroleum Exploration&Development Beijing100083China

The sensitivity of biodegrada.ion on diamondoids was investigated using a series of biodegraded oil samples from the Ronier tectonic unit of Bongor Basin,*** results suggest that diamondoids,including ada.antanes(As)and diamantanes(Ds),are relatively resistant to biodegrada.ion and obvious biodegrada.ion was observed in oils with a Peters-Moldowan(PM)biodegrada.ion rank of 6 or ***,the sensibility of biodegrada.ion on diamondoids is generally similar to hopanes and regular *** biodegrada.ion evolves,the changes in concentration and components of diamondoids show that the biodegrada.ion process is selective and *** significant increase of MD/MA and DMD/DMA for oils with a PM ranking 6^(+) indicates that diamantanes are generally more resistant to biodegrada.ion than *** similar trends of DMA/MA,EA/MA,MD/D,DMD/MD and other relevant indexes,show that higher alkylation homologs are more resistant to *** commonly used diamondoid ratios,such as MAI,EAI,MDI and DMID-1,are obviously affected by biodegrada.ion at the stage of high-level biodegrada.ion,which may indicate that these ratios should be used with caution in case of severely degraded oils.

关键词： Diamondoids Biodegrada.ion Sensitivity Crude oil Bongor Basin Chad

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DynIceda.a:a gridded ice-water classification da.aset at short-time intervals based on observations from multiple satellites over the marginal ice zone

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Big Earth da.a 2024年第2期8卷 249-273页

作者： Lin Huang Yubao Qiu Yang Li Shuwen Yu Wanyang Zhong Changyong dou Key Laboratory of Digital Earth Science Aerospace Information Research InstituteChinese Academy of SciencesBeijingChina International Research Center of Big da.a for Sustainable Development Goals BeijingChina University of Chinese Academy of Sciences BeijingChina School of Resources and Geosciences China University of Mining and TechnologyXuzhouChina

High-resolution observations of short-term changes in sea ice are critical to understanding ice dynamics and also provide important information used in advice to shipping,especially in the *** individual satellite sensors provide periodic sea ice obser-vations with spatial resolutions of tens of meters,information regarding changes that occur over short time intervals of minutes or hours is *** this study,a gridded ice-water classification da.aset with a high temporal resolution was developed based on observations acquired by multiple satellite sensors in the Marginal Ice Zone(MIZ).This da.aset-DynIceda.a-which combines Sentinel-1 Synthetic Aperture Rada.(SAR)da.a with Gaofen-3(GF-3)SAR and SDGSAT-1 thermal infrared imagery was used to obtain observations of the MIZ with a range of temporal resolutions ran-ging from minutes to tens of *** areas of the Arctic covered include the Kara Sea,Beaufort Sea,and Greenland Sea during the period from August 2021 to August ***-oriented segmen-tation and thresholding were used to obtain the ice-water classifi-cation map from Sentinel-1 and GF-3 SAR image pairs and Sentinel-1 SAR and SDGSAT-1 thermal image *** time interval between the images in each pair ranged from 1 minute to 68 ***-kilometer grid sample granules with a spatial resolution of 25 m for the GF-3 SAR da.a and 30 m for the SDGSAT-1 thermal da.a were *** classification was verified as having an overall accuracy of at least 95.58%.The DynIceda.a da.aset consists of 7338 samples,which could be used as reference da.a for further research on rapid changes in sea ice patterns at different short time scales and provide support for research on thermodynamic and dynamic models of sea ice in combination with other environmen-tal da.a,thus potentially improving the accuracy of sea ice forecast-ing using Artificial *** da.aset can be accessed at https://***/10.57760/sciencedb.j00001.00784.

关键词： Sea ice dynamics ice-water classification GF-3 SDGSAT-1 marginal ice zone

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A systematic understanding of microbial reductive dechlorination towards an improved “one health” soil bioremediation: A review and perspective

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Science China Technological Sciences 2024年第10期67卷 3009-3031页

作者： HE Yan LI ShuYao YUAN Jing CHENG Jie dou JiBo YANG XueLing XU JianMing Zhejiang Provincial Key Laboratory of Agricultural Resources and Environment Institute of Soil and Water Resources and Environmental ScienceCollege of Environmental and Resource SciencesZhejiang University Key Laboratory of Environment Remediation and Ecological Health Ministry of Education Microbiome Network and Department of Agricultural Biology Colorado State University Departments of Chemistry and Chemical & Biomolecular Engineering Institute for Functional Intelligent Materials (I-FIM)National University of Singapore

Chlorinated organic pollutants(COPs), both emerging and traditional, are typical persistent pollutants that harm soil health worldwide. Dechlorinators mediated reductive dechlorination is the optimal way to completely remove COPs from anaerobic soil through a redox reaction driven by electron transfer during microbial anaerobic respiration. Generally, the dechlorinated depletion of COPs in situ often interacts with multiple element biogeochemical activities, e.g., methanogenesis, sulfate reduction, iron reduction, and denitrification. Elucida.ing the relevance of biogeochemical cycles between COPs and multiple elements and the coupled mechanisms involved, thus, helps to develop effective pollution control strategies with the balance between pollution degrada.ion and element cycles in heterogeneous soil, ultimately contributing to “one health” goal. In this review, we summarized the microbial-chemical coupling redox processes and the driving factors, elucida.ed the interspecies metabolites exchange and electron transfer mechanisms within COP-dechlorinating communities, and further proposed a detailed design, construction, and analysis framework of engineering COP-dechlorinating microbiomes via “top-down” selfassembly and “bottom-up” synthesis to pave the way from laboratory to practical field application. Especially, we delve into the major challenges and perspectives surrounding the design of state-of-the-art synthetic microbial communities. Our goal is to improve the understanding of the microbial-mediated coupling between reductive dechlorination and element biogeochemical cycling, with a particular focus on the implications for health-integrated soil bioremediation under the “one health” concept.

关键词： reductive dechlorination biogeochemical redox processes interspecies interaction synthetic microbiomes, anaerobic soils

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