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Flexural behavior of textile reinforced mortar-autoclaved lightweight aerated concrete composite panels

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Frontiers of Structural and Civil Engineering 2024年第5期18卷 776-787页

作者： Liying GUO Mingke DENG Wei zhang Tong LI Yangxi zhang Mengyu CAO Xian hu Department of Civil Engineering Xi’an University of Architecture and TechnologyXi’an 710055China Key Lab of Structural Engineering and Earthquake Resistance Ministry of Education(XAUAT)Xi’an 710055China Scene engineering design institute Xi’an 710016China dahua Group Shang hai 200062China

To improve the deficiencies of prefabricated autoclaved lightweight aerated concrete(ALC)panel such as susceptibility to cracking and low load-bearing capacity,a textile-reinforced mortar-autoclaved lightweight aerated concrete(TRM-ALC)composite panel was developed in this *** group of reference ALC panels and five groups of TRM-ALC panels were fabricated and subjected to four-point flexural *** was applied on the tensile side of the ALC panels to create *** variable parameters were the plies of textile(one or two),type of textile(basalt or carbon),and whether the matrix(without textile)was applied on the compression side of *** results showed that a bonding only 8-mm-thick TRM layer on the surface of the ALC panel could increase the cracking load by 180%−520%.The flexural capacity of the TRM-ALC panel increased as the number of textile layers *** reinforcement of the matrix on the compressive side could further enhance the stiffness and ultimate loadbearing capacity of the TRM-ALC *** panels with basalt textile failed in flexural mode,with the rupture of fabric *** with carbon textile failed in shear mode due to the ultra-high tensile strength of *** addition,analytical models related to the different failure modes were presented to estimate the ultimate load-carrying capacity of the TRM-ALC panels.

关键词： prefabricated autoclaved lightweight aerated concrete panel textile-reinforced mortar cracking load flexural capacity stiffness

Magnetic Co-doped 1D/2D structuredγ-Fe_(2)O_(3)/MoS_(2) effectively activated peroxymonosulfate for efficient abatement of bisphenol A via both radical and non-radical pathways

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Frontiers of Environmental Science & Engineering 2024年第3期18卷 143-159页

作者： Junge Xu Dong Wang Die hu Ziwei zhang Junhong Chen Yingmu Wang Yifeng zhang College of Civil Engineering Fuzhou UniversityFuzhou 350116China China Nuclear Power Engineering Co. Ltd.Shenzhen 518120China Department of Environmental&Resource Engineering Technical University of DenmarkLyngby DK-2800Denmark

Iron-based catalysts have been widely used to treat refractory organic pollutants in *** this paper,magnetic Co-γ-Fe_(2)O_(3)was synthesized by a facile tartaric acid-assisted hydrothermal method,and Co-γ-Fe_(2)O_(3)/MoS_(2) nanocomposite catalyst was obtained via in situ growth of MoS_(2) nanosheets on Co-γ-Fe_(2)O_(3)*** nanocomposite catalysts were used to decompose bisphenol A(BPA)by activating peroxymonosulfate(PMS).It was shown that only 0.15 g/L catalyst and 0.5 mmol/L PMS degraded 10 mg/L of BPA(99.3%within 10 min)in the pH range of 3–*** was activated due to redox cycling among the pairs Co(III)/Co(II),Fe(III)/Fe(II),and Mo(VI)/Mo(IV).Quenching experiments and electron paramagnetic resonance spectroscopy demonstrated that both radical and non-radical pathways were involved in BPA degradation,in which active radical sulfate radical and non-radical singlet oxygen were the main reactive oxygen *** intermediates were identified by liquid chromatography-coupled mass spectrometry,and three possible BPA degradation pathways were *** toxicity of several degradation intermediates was lower,and Co-γ-Fe_(2)O_(3)/MoS_(2) exhibited excellent reusability and could be magnetically recovered.

关键词： Magnetic Co-γ-Fe_(2)O_(3) /MoS_(2) Hydrothermal method Bisphenol A Degradation pathways Toxicity analysis

Mg-Al-hydrotalcite with alkaline sites protects Ni/KIT-6 from formation of amorphous coke in glycerol steam reforming via tailoring reaction intermediates

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Frontiers of Chemical Science and Engineering 2024年第4期18卷 25-39页

作者： Yunyu Guo Yiran Wang Yuewen Shao Shu zhang Yi Wang Song hu Jun Xiang Xun hu School of Material Science and Engineering University of JinanJinan 250022China Joint International Research Laboratory of Biomass Energy and Materials College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037China State Key Laboratory of Coal Combustion Huazhong University of Science and TechnologyWuhan 430074China

During steam reforming,the performance of a catalyst and amount/property of coke are closely related to reaction intermediates reaching surface of a ***,modification of reaction intermediates by placing Mg-Al-hydrotalcite above Ni/KIT-6 catalyst in steam reforming of glycerol was conducted at 300 to 600°*** results revealed that the catalytic activity of Ni/KIT-6 in the lower bed was enhanced with either Mg1-Al5-hydrotalcite(containing more acidic sites)or Mg5-Al1-hydrotalcite(containing more alkaline sites)as upper-layer *** in situ infrared characterization of steam reforming demonstrated that Mg-Al-hydrotalcite catalyzed the deoxygenation of glycerol,facilitating the reforming of the partially deoxygenated intermediates over Ni/***-Al-hydrotalcite as protective catalyst,however,did not protect the Ni/KIT-6 from formation of more ***,this did not lead to further deactivation of Ni/KIT-6 while Mg5-Al1-hydrotalcite even substantially enhanced the catalytic stability,even though the coke was much more significant than that in the use of single Ni/KIT-6(52.7%vs.28.6%).The reason beneath this was change of the property of coke from more aliphatic to more ***5-Al1-hydrotalcite catalyzed dehydration of glycerol,producing dominantly reaction intermediates bearing C=C,which formed the catalytic coke of with carbon nanotube as the main form with smooth outer walls as well as higher aromaticity,C/H ratio,crystallinity,crystal carbon size,thermal stability,and resistivity toward oxidation on Ni/KIT-6 in the lower *** comparison,the abundance of acidic sites on Mg1-Al5-hydrotalcite catalyzed the formation of more oxygen-containing species,leading to the formation of carbon nanotubes of rough surface on Ni/KIT-6.

关键词： steam reforming of glycerol Mg-Alhydrotalcite sacrificial catalyst reaction intermediates property of coke

How the surface Cu layer affected the activity of Ni foil for alkaline hydrogen evolution

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Journal of Materials Science & Technology 2024年第2期169卷 11-18页

作者： Qingfeng hu Yuan Liu Xuerong Zheng Jinfeng zhang Jiajun Wang Xiaopeng Han Yida Deng Wenbin hu School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityBinhai New CityFuzhou 350207China

Synthesizing bimetallic nanomaterials,with noble metals as the surface layers and inert metals as the substrates,has been proven to be an effective way to reduce the use of noble metals with maintained catalytic ***,an atomic diffusion from the inert substrate to the surface during the long-term operation has been reported to significantly decrease the *** this work,a series of catalysis-inert Cu-coated Ni foil were fabricated through electrodeposition and their activities for alkaline hydrogen evolution were ***,the Ni/Cu-60 sample showed a similar catalytic property with pure Ni foil and only a slight decrease in HER activity was *** X-ray photoelectron spectroscopy(XPS)results indicated a decreased electron concentration of Cu in Ni/Cu-60,and theoretical calculations further demonstrated the electron transfer between the Ni substrate and Cu *** results reveal that a specific composition or structure of an inert metal layer might not significantly decrease the electrocatalytic activity of active ***,there are more possibilities for the rational design of metal-based catalysts for electrocatalysis.

关键词： Bimetallic heterostructure Charge redistribution Water splitting Alkaline hydrogen evolution

Steam reforming of acetic acid over Ni/biochar of low metal-loading:Involvement of biochar in tailoring reaction intermediates renders superior catalytic performance

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Chinese Journal of Chemical Engineering 2024年第4期68卷 241-252页

作者： Yunyu Guo Yiran Wang Shu zhang Yi Wang Song hu Jun Xiang Walid Nabgan Xun hu School of Material Science and Engineering University of JinanJinan 250022China Joint International Research Laboratory of Biomass Energy and Materials College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037China State Key Laboratory of Coal Combustion Huazhong University of Science and TechnologyWuhan 430074China Departament d'Enginyeria Química Universitat Rovira i VirgiliTarragona 43007Spain

Biochar is a reactive carrier as it may be partially gasified with steam in steam reforming,which could influence the formation of reaction intermediates and modify catalytic ***,the Ni/biochar as well as two comparative catalysts,Ni/Al_(2)O_(3) and Ni/SiO_(2),with low nickel loading(2%(mass))was conducted to probe involvement of the varied carriers in the steam *** results indicated that the Ni/biochar performed excellent catalytic activity than Ni/SiO_(2) and Ni/Al_(2)O_(3),as the biochar carrier facilitated quick conversion of the -OH from dissociation of steam to gasify the oxygen-rich carbonaceous intermediates like C=O and C-O-C,resulting in low coverage while high exposure of nickel species for maintaining the superior catalytic *** converse,strong adsorption of aliphatic intermediates over Ni/Al_(2)O_(3) and Ni/SiO_(2) induced serious coking with polymeric coke as the main type(21.5%and 32.1%,respectively),which was significantly higher than that over Ni/biochar(3.9%).The coke over Ni/biochar was mainly aromatic or catalytic type with nanotube morphology and high *** high resistivity of Ni/biochar towards coking was due to the balance between formation of coke and gasification of coke and partially biochar with steam,which created developed mesopores in spent Ni/biochar while the coke blocked pores in Ni/Al_(2)O_(3) and Ni/SiO_(2) catalysts.

关键词： Steam reforming Acetic acid Ni/biochar catalyst Property of coke Reaction intermediates

Circ_0003855 involvement of esophageal cancer progression through miR-622/FLOT1

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Oncology Research 2024年第5期32卷 925-931页

作者： JINGJING TIAN XIBAO hu XINRONG zhang Department of Gastroenterology Tianjin Nankai HospitalTianjin300100China Department of Digestive Medicine First Teaching Hospital of Tianjin University of Traditional Chinese MedicineTianjin300100China

To confirm the relationship between Circ_0003855 and EC,we purchased the human esophageal carcinoma cell line Eca109 and normal human esophageal epithelial cells HEEC,and the expression levels of Circ_0003855,miR-622,and FLOT1 were *** results show that Circ_0003855 and FLOT1 were highly expressed in Eca109 cells,while miR-622 was lowly expressed(p0.05).Synthesizing the results of these experiments above,we believe that interfering with the expression of Circ_0003855 can inhibit the activity of EC cells,and its mechanism is related to miR-622 and FLOT1.

关键词： Circ_0003855 miR-622 FLOT1 Esophageal cancer Cell proliferation

Evidence of ancient rock-ice avalanches along the China-Bhutan Chomolhari Range,and their implications for demise of the summit

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Journal of Mountain Science 2024年第9期21卷 2876-2890页

作者： hu Kaiheng zhang Qiyuan LI Pu zhang Xiaopeng LIU Shuang LI Hao Institute of Mountain Hazards and Environment Chinese Academy of SciencesChengdu 610299China University of Chinese Academy of Sciences Beijing 100149China

Large-scale rock-ice avalanches resulting from the interaction of tectonics and climate are characterized with high mobility,huge volumes of sediment,and rapid denudation,being a major agent of landscape evolution in high altitude mountainous ***,the extreme glaciated slope failures often transform into extraordinarily large and mobile debris flows,resulting in disastrous consequences such as sedimentation and *** to a dearth of on-site observation data and experimental data collection,our comprehension of the geomorphic and kinematic characteristics of rock-ice avalanches remains *** we report a cluster of ancient rock-ice avalanches spreading along the Chomolhari range of the China-Bhutan *** integrating remote sensing image interpretation with detailed field investigations,we demonstrate the geomorphic and sedimentary characteristics of four events among the *** estimated volumes of the four are 23.73 Mm³,39.69 Mm³,38.43 Mm³,and 38.25 Mm³,*** presence of pre-existing moraines or alluvial fans constrained their movement,resulting in deposition features such as marginal digitated lobes at higher elevations and large depressed areas in the *** the Savage-hutter theory,we calculate the basal friction angle and travel angle of these ancient rock-ice avalanches that are both less than 10°,affirming the similarity of these avalanches in the study area to those occurring in other *** study significantly contributes to understanding the geomorphic and kinematic characteristics of rock-ice avalanches in high-altitude mountainous regions,providing valuable insights into their response to the disproportionate growth of Himalayan peaks.

关键词： Rock-ice avalanche Himalayas Southern Yadong-Gulu rift Vertical slip-rate Landscape evolution

Control of slope-pattern on the deposition of fan-delta systems:a case study of the Upper Karamay Formation,Junggar Basin

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Frontiers of Earth Science 2024年第2期18卷 384-399页

作者： Mingxuan GAO Xinghe YU Shunli LI Wenmiao zhang Songhao hu Menglu zhang School of Energy Resource China University of GeosciencesBeijing 100083China Key laboratory of marine reservoir evolution and hydrocarbon enrichment mechanism(Ministry of Education) China University of GeosciencesBeijing 100083China College of Geosciences China University of PetroleumBeijing 102249China No.1 Oil Production Plant Xinjang Oilfield CompanyKaramay 834099China

The Mesozoic fan deltas in the north-west margin of the Junggar Basin,as important petroleum reservoirs,exhibited complex facies change and internal structures with strong heterogeneity which were controlled by the transformation of slope-patterns,bringing great challenges to the study of sedimentary *** Upper Karamay Formation at north-west margin of the Junggar Basin was the objective in this paper which attempts to clarify the mechanism of sedimentary response and sand-body distribution of fan delta systems under the control of slope-pattern *** on a data set of cores,well logs and seismic,two types of slope-pattern were identified in the study area,which include steep-to-gentle in the south and gentle-to-steep in the *** control of difference slope-patterns on the sand-body distribution was clarified based on the analysis of the sedimentary dynamics,facies characteristics,and depositional evolution of the fan *** study shows that the transport mechanism of sediments on the steep-slope was dominated by debris flows,developing coarse-grained,thick-bedded lobes with poor structural maturity of *** the gentle-slope,the deposition was dominated by hyperconcentrated-traction currents,forming relatively fine-grained,thin-bedded lobes with increased sandy *** sand-bodies show frequent bar-channel transformation and channel down-cutting under the steep slope setting,which exhibit migration of isolated river channels on the gentle *** the steep-to-gentle pattern,the coase-grained sediments were mainly accumulated at slope toe,generally developed equiaxial ***,the coarse-grained clasts were preserved both at proximal and distal lobes on the gentle-to-steep slopes,showing obvious lateral extension of the fan *** slope patterns controlled sedimentary respond rates of the fan deltas during lake level *** comparing the modern cases of fan systems worldwide,the control of slope patterns on deposit

关键词： fan delta slope-pattern sedimentary characteristics the Upper Karamay Formation

Dynamic Characteristics of Functionally Graded Timoshenko Beams by Improved Differential Quadrature Method

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Computer Modeling in Engineering & Sciences 2024年第8期140卷 1647-1668页

作者： Xiaojun huang Liaojun zhang Hanbo Cui Gaoxing hu School of Architecture and Civil Engineering Anhui Polytechnic UniversityWuhu241000China College of Water Conservancy and Hydropower Engineering Hohai UniversityNanjing210098China

This study proposes an effective method to enhance the accuracy of the Differential Quadrature Method(DQM)for calculating the dynamic characteristics of functionally graded beams by improving the form of discrete node ***,based on the first-order shear deformation theory,the governing equation of free vibration of a functionally graded beam is transformed into the eigenvalue problem of ordinary differential equations with respect to beam axial displacement,transverse displacement,and cross-sectional rotation angle by considering the effects of shear deformation and rotational inertia of the beam ***,ignoring the shear deformation of the beam section and only considering the effect of the rotational inertia of the section,the governing equation of the beam is transformed into the eigenvalue problem of ordinary differential equations with respect to beam transverse *** on the differential quadrature method theory,the eigenvalue problem of ordinary differential equations is transformed into the eigenvalue problem of standard generalized algebraic ***,the first several natural frequencies of the beam can be *** feasibility and accuracy of the improved DQM are verified using the finite element method(FEM)and combined with the results of relevant literature.

关键词： Timoshenko beams functionally graded materials dynamic characteristics natural frequency improved differential quadrature method