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上海交通大学学报 2008年第S1期42卷 93-96页

作者：吕学勤刘刚郑小霞吴毅雄上海电力学院信控系上海200090 上海交通大学材料科学与工程学院上海200240

阐述了锅炉水冷壁发生高温腐蚀的机制与条件,介绍了用于火力发电站的锅炉水冷壁检测机器人的发展情况,以及各种爬壁机器人的本体结构、磁路设计及控制系统等。由此得出水冷壁检测机器人能够缩短作业周期、提高电站的经济效益、降低劳动... 详细信息

阐述了锅炉水冷壁发生高温腐蚀的机制与条件,介绍了用于火力发电站的锅炉水冷壁检测机器人的发展情况,以及各种爬壁机器人的本体结构、磁路设计及控制系统等。由此得出水冷壁检测机器人能够缩短作业周期、提高电站的经济效益、降低劳动强度并提高检测精度.

关键词：水冷壁高温腐蚀爬壁机器人

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钢铁生产动态调度理论研究与工程应用综述

信息与控制 2003年第6期32卷 531-537页

作者：常春光胡琨元汪定伟郑秉霖李慧莹东北大学信息科学与工程学院

本文以钢铁企业生产为背景 ,为了更进一步研究有效的动态调度方案 ,首先论述了钢铁生产的动态调度问题的种类、特点 .其次 ,从理论与实践应用两方面分析了该领域的研究方法 .具体介绍了基于模型、智能、人机交互方法 .并分析了各种方法... 详细信息

本文以钢铁企业生产为背景 ,为了更进一步研究有效的动态调度方案 ,首先论述了钢铁生产的动态调度问题的种类、特点 .其次 ,从理论与实践应用两方面分析了该领域的研究方法 .具体介绍了基于模型、智能、人机交互方法 .并分析了各种方法间交叉组合的方式 .进而研究工程实现模式。

关键词：钢铁企业钢铁生产动态调度理论生产管理集成制造系统

Cavity-enhanced metrology in an atomic spin-1 Bose−Einstein condensate

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Frontiers of physics 2024年第3期19卷 185-196页

作者： Renfei zheng Jieli Qin Bing Chen Xingdong Zhao Lu Zhou school of Physics Hefei University of TechnologyHefei 230009China State Key Laboratory of Precision Spectroscopy Department of PhysicsSchool of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241China school of Physics and materials science Guangzhou University230 Wai Huan Xi RoadGuangzhou Higher Education Mega CenterGuangzhou 510006China Department of Physics Henan Normal UniversityXinxiang 453007China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China

Atom interferometer has been proven to be a powerful tool for precision metrology. Here we propose a cavity-aided nonlinear atom interferometer, based on the quasi-periodic spin mixing dynamics of an atomic spin-1 Bose−Einstein condensate trapped in an optical cavity. We unravel that the phase sensitivity can be greatly enhanced with the cavity-mediated nonlinear interaction. The influence of encoding phase, splitting time and recombining time on phase sensitivity are carefully studied. In addition, we demonstrate a dynamical phase transition in the system. Around the criticality, a small cavity light field variation can arouse a strong response of the atomic condensate, which can serve as a new resource for enhanced sensing. This work provides a robust protocol for cavity-enhanced metrology.

关键词： nonlinear atom interferometer spin-1 Bose−Einstein condensate spin-mixing dynamics quantum Fisher information parameter estimation

Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

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Frontiers in Energy 2024年第2期18卷 128-140页

作者： Junwen CAO Yikun HU Yun zheng Wenqiang ZHANG Bo YU Institute of Nuclear and New Energy technology(INET) Collaborative Innovation Center of Advanced Nuclear Energy TechnologyTsinghua UniversityBeijing 100084China Department of Chemical Engineering University of WaterlooWaterlooOntario N2L 3G1Canada Institute of New Energy materials and Engineering School of Materials Science and EngineeringFuzhou UniversityFuzhou 350108China

The Haber-Bosch process is the most widely used synthetic ammonia technology at *** its invention,it has provided an important guarantee for global food ***,the traditional Haber-Bosch ammonia synthesis process consumes a lot of energy and causes serious environmental *** the serious pressure of energy and environment,a green,clean,and sustainable ammonia synthesis route is urgently *** synthesis of ammonia is a green and mild new method for preparing ammonia,which can directly convert nitrogen or nitrate into ammonia using electricity driven by solar,wind,or water energy,without greenhouse gas and toxic gas ***,the basic mechanism of the nitrogen reduction reaction(NRR)to ammonia and nitrate reduction reaction(NO_(3)^(-))to ammonia were *** representative approaches and major technologies,such as lithium mediated electrolysis and solid oxide electrolysis cell(SOEC)electrolysis for NRR,high activity catalyst and advanced electrochemical device fabrication for(NO_(3)^(-))RR and electrochemical ammonia synthesis were *** on the above discussion and analysis,the main challenges and development directions for electrochemical ammonia synthesis were further proposed.

关键词： electrochemical ammonia synthesis nitrogen nitrate nitrogen reduction reaction(NRR)to ammonia nitrate reduction reaction(NO_(3)^(-))RR

Emergent symmetry in quantum phase transition:From deconfined quantum critical point to gapless quantum spin liquid

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science Bulletin 2024年第2期69卷 190-196页

作者： Wen-Yuan Liu Shou-Shu Gong Wei-Qiang Chen zheng-Cheng Gu Department of Physics The Chinese University of Hong KongHong KongChina Division of Chemistry and Chemical Engineering California Institute of TechnologyPasadena CA 91125USA school of Physical sciences Great Bay UniversityDongguan 523000China Great Bay Institute for Advanced Study Dongguan 523000China Department of Physics and Shenzhen Institute for Quantum science and Engineering Southern University of Science and TechnologyShenzhen 518055China Shenzhen Key Laboratory of Advanced Quantum Functional materials and Devices Southern University of Science and TechnologyShenzhen 518055China

The emergence of exotic quantum phenomena in frustrated magnets is rapidly driving the development of quantum many-body physics,raising fundamental questions on the nature of quantum phase *** we unveil the behaviour of emergent symmetry involving two extraordinarily representative phenomena,i.e.,the deconfined quantum critical point(DQCP)and the quantum spin liquid(QSL)*** large-scale tensor network simulations,we study a spatially anisotropic spin-1/2 square-lattice frustrated antiferromagnetic(AFM)model,namely the J1x-J1y-J2 model,which contains anisotropic nearestneighbor couplings J1x,J1y and the next nearest neighbor coupling *** small J1y/J1x,by tuning J2,a direct continuous transition between the AFM and valence bond solid phase is *** growing J1y/J1x,a gapless QSL phase gradually emerges between the AFM and VBS *** observe an emergent O(4)symmetry along the AFM–VBS transition line,which is consistent with the prediction of DQCP *** surprisingly,we find that such an emergent O(4)symmetry holds for the whole QSL–VBS transition line as *** findings reveal the intrinsic relationship between the QSL and DQCP from categorical symmetry point of view,and strongly constrain the quantum field theory description of the QSL *** phase diagram and critical exponents presented in this paper are of direct relevance to future experiments on frustrated magnets and cold atom systems.

关键词： Tensor network Quantum phase transition Emergent symmetry Quantum spin liquid Deconfined quantum critical point Anisotropic

Designing metal-organic framework fiber network reinforced polymer electrolytes to provide continuous ion transport in solid state lithium metal batteries

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Nano Research 2024年第4期17卷 2719-2727页

作者： Wanqing Fan Ying Huang Meng Yu Kaihang She Jingren Gou zheng Zhang MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions School of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China beijing Key Laboratory of Membrane materials and Engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084China

Polyethylene oxide(PEO)-based solid-state electrolytes are considered ideal for electrolyte materials in solid-state lithium metal batteries(SSLMBs).However,practical applications are hindered by the lower conductivity and poor interfacial ***,we propose a strategy to construct a three-dimensional(3D)fiber network of metal-organic frameworks(MOFs).Composite solid electrolytes(CSEs)with continuous ion transport pathways were fabricated by filling a PEO polymer matrix in fibers containing interconnected *** 3D fiber network provides a fast Li+transport path and effectively improves the ionic conductivity(1.36×10^(-4) S·cm^(-1),30℃).In addition,the network of interconnected MOFs not only effectively traps the anions,but also provides sufficient mechanical strength to prevent the growth of Li *** from the advantages of structural design,the CSEs stabilize the Li/electrolyte interface and extend the cycle life of the Li-symmetric cells to 3000 *** assembled SSLMBs exhibit excellent cycling performance at both room and high *** addition,the constructed pouch cells can provide an areal capacity of 0.62 mA·h·cm^(-2),which can still operate under extreme *** work provides a new strategy for the design of CSEs with continuous structure and stable operation of SSLMBs.

关键词： polyethylene oxide(PEO) solid-state lithium metal batteries(SSLMBs) three-dimensional fiber network composite solid electrolytes(CSEs)

Supported Atomically Dispersed Pd Catalyzed Direct Alkoxylation and Allylic Alkylation

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Chinese Journal of Chemistry 2024年第7期42卷 719-724页

作者： Ruixuan Qin Ziwen Chen Qingyuan Wu Nanfeng zheng Pengxin Liu New Cornerstone science Laboratory State Key Laboratory for Physical Chemistry of Solid SurfacesCollaborative Innovation Center of Chemistry for Energy Materialsand National&Local Joint Engineering Research Center of Preparation Technology of NanomaterialsCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenFujian 361005China Innovation Laboratry for Scences and Technoogies of Energy materials of Fujan Province(IKKM) Xiamen Fujian 361102China school of Physical science and technology Shanghai Tech UniversityShanghai 201210China Fujian Key Laboratory of Rare-earth Functional materials Fujian Shanhai Collaborative Innovation Center of Rare-earth Functional MaterialsLongyanFujian 366300China

A new approach to allylic alkylation is realized using an atomically dispersed palladium catalyst(Pd1/TiO2-EG).Unlike conventional methods that require derivation of substrates and utilization of additives,this method allows for direct allylic alkylation from allylic alcohols,producing H2O as the sole *** catalyst's high efficiency is attributed to the local hydrogen bonding at the or-ganic-inorganic interface(Pd-EG interface),facilitating hydroxyl group activation forη3π-allyl complex *** system demonstrates successful direct C—O and C—C coupling reactions with high selectivity,requiring no *** study highlights the potential of supported atomically dispersed catalysts for greener and more efficient catalysis,meanwhile,offers unique insights into the distinct behavior of atomically dispersed catalysts in comparison to homogeneous or nanoparticle-based catalysts.

关键词： Atomically dispersed catalyst Alkylation C—C coupling Organic-inorganic Interface Hydrogen bond Tsuji-Trost reaction Green catalysis

Occurrence and vertical distribution of aluminum and rare earths in weathered crust elution-deposited rare earth ore:Effect of soil solution pH and clay minerals

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Journal of Rare Earths 2024年第7期42卷 1394-1402,I0007页

作者： Jiaxin Pan Longsheng Zhao zheng Li Xiaowei Huang Zongyu Feng Jun Chen National Engineering Research Center for Rare Earth China GRINM Group Co.Ltd.Beijing100088China school of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing100083China GRIREM Hi–Tech Co. Ltd.Langfang065201China GRIREM Advanced materials Co. Ltd.Beijing100088China GRIMAT Engineering Institute Co. Ltd.Beijing101407China

Weathered crust elution-deposited rare earth ore is crucial source of medium and heavy rare earths,with in-situ leaching being the most common mining *** high contents of impurity of aluminum in the leach solution are a significant challenge for the subsequent enrichment process of rare earths.A comprehensive understanding of the occurrences and vertical distribution of aluminum and rare earths within typical vertical profiles can provide valuable insights into entire design of the in-situ *** paper improves a five-step sequential extraction method to analyze the occurrence and vertical distribution of rare earths and aluminum in vertical profiles from Chongzuo and *** results demonstrate that soil solution pH is the main factor affecting the vertical distribution of ionexchangeable rare *** samples have distinct areas of enrichment for ion-exchangeable rare earths or ***-exchangeable rare earths are primary concentrated in the middle and lower parts of the ore layer(4-13 m in Chongzuo,14-22 m in Longyan),while the ion-exchangeable aluminum is mainly enriched in the upper part of the ore layer(1-5 m in Chongzuo,and 2-14 m in Longyan).The vertical distribution of inorganic hydroxy aluminum is likely influenced by the micromorphology and particle size of the clay *** inorganic hydroxy aluminum concentration in Chongzuo samples decreases continuously from 415.65 to 120.95 mg/kg with increasing sampling depth,whereas the concentration in Longyan samples(110.55-171.27 mg/kg)is almost independence with sampling *** results provide direct guidance for the entire design of the injection well depth and the leaching parameters,thereby inhibiting the leaching of impurity of aluminum and lower the consumption of leaching agent.

关键词： Weathered crust elution-deposited rare earth ore Sequential extraction Occurrence Aluminum Rare earth elements

Review on the plastic instability of medium -Mn steels for identifying the formation mechanisms of Lüders and Portevin -Le Chatelier bands

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International Journal of Minerals,Metallurgy and materials 2024年第6期31卷 1285-1297页

作者： Bin Hu Han Sui Qinghua Wen zheng Wang Alexander Gramlich Haiwen Luo school of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China Steel Institute RWTH Aachen UniversityIntzestraße 152072 AachenGermany

Plastic instability,including both the discontinuous yielding and stress serrations,has been frequently observed during the tensile deformation of medium-Mn steels(MMnS)and has been intensively studied in recent ***,research results are controversial,and no consensus has been achieved regarding the ***,we first summarize all the possible factors that affect the yielding and flow stress serrations in MMnS,including the morphology and stability of austenite,the feature of the phase interface,and the deformation ***,we propose a universal mechanism to explain the conflicting experimental *** conclude that the discontinuous yielding can be attributed to the lack of mobile dislocation before deformation and the rapid dislocation multiplication at the beginning of plastic ***,the results show that the stress serrations are formed due to the pinning and depinning between dislocations and interstitial atoms in ***-induced martensitic transformation,influenced by the mechanical stability of austenite grain and deformation parameters,should not be the intrinsic cause of plastic ***,it can intensify or weaken the discontinuous yielding and the stress serrations by affecting the mobility and density of dislocations,as well as the interaction between the interstitial atoms and dislocations in austenite grains.

关键词： medium manganese steel discontinuous yielding stress serrations retained austenite dislocations