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Deciphering Water Oxidation Catalysts: The Dominant Role of Surface Chemistry over Reconstruction Degree in Activity Promotion

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NANO-MICRO LETTERS 2025年第1期17卷 1-15页

作者： An, Li Li, Jianyi Sun, Yuanmiao Zhu, Jiamin Seow, Justin Zhu Yeow Zhang, Hong Zhang, Nan Xi, Pinxian Xu, Zhichuan J. yan, chun-Hua Lanzhou Univ Frontiers Sci Ctr Rare Isotopes Key Lab Nonferrous Met Chem & Resources Utilizat G State Key Lab Appl Organ ChemColl Chem & Chem Eng Lanzhou 730000 Peoples R China Nanyang Technol Univ Sch Mat Sci & Engn Singapore 639798 Singapore Chinese Acad Sci Fac Mat Sci & Energy Engn Shenzhen Inst Adv Technol Inst Technol Carbon Neutral Shenzhen 518055 Peoples R China Yunnan Univ Natl Ctr Int Res Photoelect & Energy Mat Electron Microscopy Ctr Sch Mat & EnergyKey Lab Electromagnet Mat & Devic Kunming 650091 Peoples R China Baotou Res Inst Rare Earths State Key Lab Baiyunobo Rare Earth Resource Res & Baotou 014030 Peoples R China Peking Univ Beijing Natl Lab Mol Sci State Key Lab Rare Earth Mat Chem & Applicat PKU HKU Joint Lab Rare Earth Mat & Bioinorgan Chem Beijing 100871 Peoples R China

Demonstrate that the key factor to determine the activity of reconstructed surfaces is the surface chemistry, instead of reconstruction degree using the popular perovskite LaNi1-xFexO3 oxides as model *** content can influence both the surface reconstruction degree, the activation degree, and the activity of reconstructed *** oxygen evolution reaction activity of reconstructed catalysts is primarily governed by the chemistry of the reconstructed surface species. Water splitting hinges crucially on the availability of electrocatalysts for the oxygen evolution reaction. The surface reconstruction has been widely observed in perovskite catalysts, and the reconstruction degree has been often correlated with the activity enhancement. Here, a systematic study on the roles of Fe substitution in activation of perovskite LaNiO3 is reported. The substituting Fe content influences both current change tendency and surface reconstruction degree. LaNi0.9Fe0.1O3 is found exhibiting a volcano-peak intrinsic activity in both pristine and reconstructed among all substituted perovskites in the LaNi1-xFexO3 (x = 0.00, 0.10, 0.25, 0.50, 0.75, 1.00) series. The reconstructed LaNi0.9Fe0.1O3 shows a higher intrinsic activity than most reported NiFe-based catalysts. Besides, density functional theory calculations reveal that Fe substitution can lower the O 2p level, which thus stabilize lattice oxygen in LaNi0.9Fe0.1O3 and ensure its long-term stability. Furthermore, it is vital interesting that activity of the reconstructed catalysts relied more on the surface chemistry rather than the reconstruction degree. The effect of Fe on the degree of surface reconstruction of the perovskite is decoupled from that on its activity enhancement after surface reconstruction. This finding showcases the importance to customize the surface chemistry of reconstructed catalysts for water oxidation.

关键词： Oxygen evolution reaction Perovskite oxides Doping Activation and reconstruction

Advances in ethnopharmacology,phytochemistry and pharmacology of Erigerontis Herba and its Chinese medicine prescriptions

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Traditional Medicine Research 2025年第1期10卷 44-61页

作者： yang Zhou Yuan-yan Huang Ding-Yue Shang Ying Chen Meng Tian Cheng-Yu Jin Xin Lu Bing-chun yan Han-Qing Pang Institute of Translational Medicine School of MedicineYangzhou UniversityYangzhou 225009China Jiangsu Key Laboratory of Integrated Traditional Chinese and Western Medicine for Prevention and Treatment of Senile Diseases Yangzhou UniversityYangzhou 225009China School of Medicine Nanjing University of Chinese MedicineNanjing 210023China State Key Laboratory for Chemistry and Molecular Engineering of Medicinal Resources Guangxi Normal UniversityGuiling 541004China.

Erigerontis Herba(EH),the dried whole plant of Erigeron breviscapus,is well-known for circulating blood,activating meridians to alleviate pain,expelling wind,and clearing away *** has been extensively utilized in southern China for the treatment of stroke hemiplegia,chest stuffiness and pains,rheumatic arthralgia,headache,and *** review focuses on the botany,ethnopharmacology,phytochemistry,pharmacology and toxicity of EH and its related prescriptions to offer new insights for prospective research of *** information about EH was retrieved from ancient records and books,PubMed,China National Knowledge Infrastructure,Chinese Pharmacopoeia,Web of Science,Doctoral and Master’s Theses,and various electronic *** is a member of Compositae family and is mainly grown in southern *** Chinese medicine records that EH has the effects of circulating blood and removing blood stasis,expelling wind,and removing cold,as well as relieving rigidity of muscle and relieving *** now,nearly 200 ingredients have been characterized from EH,including flavonoids,caffeoyls,aromatic acids,coumarins,pentacyclic terpenoids,volatile oil and other *** extracts,EH related prescriptions(Dengzhan Xixin injection,Dengzhan Shengmai capsules,etc.)or compounds(scutellarin,scutellarein,etc.)possessed obvious therapeutic effects of ischemic stroke,cerebral hemorrhage,myocardial infarction,Alzheimer’s disease,diabetes and its complications,gastric cancer,bone,and joint degenerative ***,the major active compound of EH,has been used as a quality *** no obvious toxicity of EH has been *** to its traditional applications,ethnopharmacology,phytochemistry,pharmacology,and toxicity,EH was applied as a valuable herb for clinical application in food and medicine *** several compounds have been shown to possess diverse biological activities,the underlying mechanisms of their actions remain *** fully exploi

关键词： Erigeron breviscapus traditional applications ethnopharmacology phytochemistry pharmacology

Molecular ferroelectrics for efficient perovskite solar cells

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Science China Chemistry 2021年第2期64卷 169-170页

作者： chun-Hua yan Beijing National Laboratory for Molecular Sciences State Key Laboratory of Rare Earth Materials Chemistry and ApplicationsPKU-HKU Joint Laboratory in Rare Earth Materials and Bioinorganic ChemistryCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China College of Chemistry and Chemical Engineering Lanzhou UniversityLanzhou 730000China

During the past decade,the power conversion efficiencies(PCEs)of organic-inorganic hybrid perovskite solar cells(PSCs)have exceeded 25%[1],which is expected to be one of the candidates for the next generation of thin-film photovoltaic *** speaking,the performance of PSCs mainly depends on the light absorption capacity,defect passivation and photo-induced exciton separation and extraction of perovskite *** the light illumination,photo-induced excitons were separated and extracted by the built-in electric field of PSCs.

关键词： perovskite illumination inorganic

Recent development of hydrodynamic modeling in heavy-ion collisions

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Nuclear Science and Techniques 2020年第12期31卷 88-121页

作者： chun Shen Li yan Department of Physics and Astronomy Wayne State UniversityDetroitMI 48201USA RIKEN BNL Research Center Brookhaven National LaboratoryUptonNY 11973USA Key Laboratory of Nuclear Physics and Ion-Beam Application(MOE) Institute of Modern PhysicsFudan University220 Handan RoadShanghai 200433China

We present a concise review of the recent development of relativistic hydrodynamics and its applications to heavy-ion *** progress on the extended formulation of hydrodynamics toward out-ofequilibrium systems is addressed,with emphasis on the socalled attractor ***,recent phenomenological improvements in the hydrodynamic modeling of heavy-ion collisions with respect to the ongoing beam energy scan program,the quantitative characterization of transport coefficients in three-dimensionally expanding quark–gluon plasma,the fluid description of small colliding systems,and certain other interdisciplinary connections are discussed.

关键词： Heavy-ion collisions Hydrodynamics QCD

Analysis of sliding electric contact characteristics in augmented railgun based on the combination of contact resistance and sliding friction coefficient

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Defence Technology（防务技术） 2020年第4期16卷 747-752页

作者： chun-yan Zhu Bao-ming Li National Key Laboratory of Transient Physics Nanjing University of Science and TechnologyChina

The contact resistance between the armature and rails is an important indicator of the contact characteristics in electromagnetic *** the contact resistance depends not only on the contact state but also on the contact stress and temperature,there are some limitations in analyzing the contact characteristics using only the contact *** this paper,the contact characteristics of the augmented railgun are analyzed by the combination of contact resistance and sliding friction ***,the theoretical calculation model of the contact resistance and friction coefficient of the augmented electromagnetic railgun is *** the contact resistance and friction coefficient are calculated by the measured values of the muzzle voltage,rail current and armature ***,the contact characteristics are analyzed according to the features of the waveforms of the contact resistance and the friction coefficient,and the analysis conclusions are verified by experimental rail *** results showed that:the aluminum melt film gradually formed on the contact surface reduces the contact resistance and the friction coefficient;the wear and erosion of the armature cause deterioration of the contact state;after the transition,the reliability of the sliding contact between the armature and rails decreases,resulting in an increase in contact resistance.

关键词： Augmented railgun Contact resistance Friction coefficient Contact characteristics

Impact of community public health care on treatment effect,health cognition,and self-management in patients with type 2 diabetes

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World Journal of Clinical Cases 2025年第5期13卷 22-29页

作者： Hong Shi chun Liu Hong-yan Luo Department of Infrastructure Operation West China Hospital of Sichuan UniversityChengdu 610041Sichuan ProvinceChina Department of Public Health Minzu Street Community Health Service CenterWuhan 430000Hubei ProvinceChina Caotang Community Health Service Center Chengdu 610031Sichuan ProvinceChina

BACKGROUND At present,China has become the country with the largest number of individuals with diabetes mellitus(DM)in the world,with a total of approximately 140 million patients,the majority of whom have type 2 DM(T2DM).Based on conven-tional nursing methods,community home care has important clinical significance in controlling blood sugar and disease *** To explore the impact of community public health nursing on treatment effect,health cognition,and self-management in patients with *** One hundred patients with T2DM were selected as the research *** patients were divided into either a conventional nursing group or community nursing(CN)group using the random number table *** conventional nursing group(50 cases)received routine care,while the CN group(50 cases)received community public health care in addition to routine care as that for the conventional nursing *** rate of excellent and good blood glucose control,fasting blood glucose before and after care,2-h postprandial blood glucose,health cognition,and self-management ability,and patient satisfaction were compared between the two *** The CN group had a higher rate of excellent blood sugar control than the conventional nursing group(88%vs 70%,P0.05).After nursing,fasting blood glucose and 2-h postprandial blood glucose were reduced to varying degrees in both groups,and both blood glucose levels in the CN group were lower than those of the conventional nursing group(P<0.05).Compared with the scores before care,the cognitive level score for diabetes and self-management ability score improved after care in both *** cognitive level and self-management ability of patients in the CN group were higher than those of the conventional nursing group(P<0.05).The overall satisfaction of the CN group was better than

关键词： Community public health care Type 2 diabetes Blood sugar control Self-management ability Cognition level

Common Properties of the Operator Products in Local Spectral Theory

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Acta Mathematica Sinica,English Series 2015年第11期31卷 1715-1724页

作者： Kai yan Xiao chun FANG Department of Mathematics Tongji University

Let X,Y be Banach spaces, A,D ： X - Y and B,C ： Y - X be the bounded linear operators satisfying operator equation set ACD=DBD DBA=ACAIn this paper, we show that AC and BD share some basic operator properties such as the injectivity and the invertibility. Moreover, we show that AG＇ and BD share many common local spectral properties including SVEP, Bishop property （β） and Dunford property （C）.

关键词： Jacobson's lemma operator equation set common property local spectral theory

Fault-Tolerate Three-Party Quantum Secret Sharing over a Collective-Noise Channel

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Chinese Physics Letters 2011年第2期28卷 35-38页

作者： LI chun-yan LI yan-Song Key Laboratory for Atomic and Molecular Nanosciences and Department of Physics Tsinghua UniversityBeijing 100084 Tsinghua National Laboratory for Information Science and technology Beijing 100084

We present a fault-tolerate three-party quantum secret sharing(QSS)scheme over a collective-noise ***-free subspaces are used to tolerate two noise modes,a collective-dephasing channel and a collective-rotating channel,*** this scheme,the boss uses two physical qubits to construct a logical qubit which acts as a quantum channel to transmit one bit information to her two *** agents can get the information of the private key established by the boss only if they *** boss Alice encodes information with two unitary *** single-photon measurements are required to rebuilt Alice's information and detect the security by the agents Bob and Charlie,not Bell-state ***,Almost all of the photons are used to distribute information,and its success efficiency approaches 100%in theory.

关键词： theory collective quantum

Quantum Key Distribution Based on a Weak-Coupling Cavity QED Regime

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Chinese Physics Letters 2011年第12期28卷 28-31页

作者： LI chun-yan LI yan-Song State Key Laboratory of Low-dimensional Quantum Physics and Department of PhysicsTsinghua UniversityBeijing 100084 Tsinghua National Laboratory for Information Science and Technology Beijing 100084 Department of Physics National University of Defense TechnologyChangsha 410073

We present a quantum key distribution scheme using a weak-coupling cavity QED regime based on quantum dense *** entanglement statesof photons and electrons are used to distribute *** just need to transmit photons without storing them in the *** electron confined in a quantum dot,which is embedded in a microcavity,is held by one of the legitimate users throughout the whole communication *** the polarization of a single photon and spin of electron measurements are applied in this protocol,which are easier to perform than collective-Bell state *** optical apparatus,such as a special polarizing beam splitter in a circular basis and single photon operations,make it more flexible to realize under current *** efficiency will approach 100%in the ideal *** security of the scheme is also discussed.

关键词： process quantum scheme