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A General Strategy for Ordered Carrier Transport of Quasi‑2D and 3D Perovskite Films for Giant Self‑Powered Photoresponse and Ultrahigh Stability

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Nano-Micro Letters 2023年第8期15卷 128-140页

作者： Fei Zhu Gang Lian Deliang Cui Qilong Wang Haohai Yu Huaijin Zhang Qingbo Meng ching‑ping wong State Key Laboratory of Crystal Materials Shandong UniversityJinan 250100People’s Republic of China Key Laboratory for Special Functional Aggregated Materials of Education Ministry School of Chemistry&Chemical EngineeringShandong UniversityJinan 250100People’s Republic of China Key Laboratory for Renewable Energy Chinese Academy of Sciences(CAS)BeijingPeople’s Republic of China Key Laboratory for New Energy Materials and Devices Beijing National Laboratory for Condensed Matter PhysicsInstitute of PhysicsCASBeijing 100190People’s Republic of China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

Organic–inorganic hybrid perovskite materials have been focusing more attention in the field of self-powered photodetectors due to their superb photoelectric properties.However,a universal growth approach is required and challenging to realize vertically oriented growth and grain boundary fusion of 2D and 3D perovskite grains to promote ordered carrier transport,which determines superior photoresponse and high stability.Herein,a general thermal-pressed(TP)strategy is designed to solve the above issues,achieving uniaxial orientation and single-grain penetration along the film thickness direction.It constructs the efficient channel for ordered carrier transport between two electrodes.Combining of the improved crystal quality and lower trap-state density,the quasi-2D and 3D perovskite-based self-powered photodetector devices(with/without hole transport layer)all exhibit giant and stable photoresponse in a wide spectrum range and specific wavelength laser.For the MAPbI_(3)-based self-powered photodetectors,the largest R_(λ) value is as high as 0.57 A W^(−1)at 760 nm,which is larger than most reported results.Meanwhile,under laser illumination(532 nm),the FPEA_(2)MA_(4)Pb_(5)I_(16)-based device exhibits a high responsivity(0.4 A W^(−1)) value,which is one of the best results in 2DRP self-powered photodetectors.In addition,fast response,ultralow detection limit,and markedly improved humidity,optical and heat stabilities are clearly demonstrated for these TP-based devices.

关键词： Perovskites Thermal-pressed strategy Uniaxial orientation Self-powered photodetectors Stability

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Tailorable,Lightweight and Superelastic Liquid Metal Monoliths for Multifunctional Electromagnetic Interference Shielding

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Nano-Micro Letters 2022年第2期14卷 136-150页

作者： Yadong Xu Zhiqiang Lin Krishnamoorthy Rajavel Tao Zhao Pengli Zhu Yougen Hu Rong Sun ching-ping wong Shenzhen Institute of Advanced Electronic Materials Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055People’s Republic of China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

Liquid metal(LM)has become an emerging material paradigm in the electromagnetic interference shielding field owing to its excellent electrical conductivity.However,the processing of lightweight bulk LM composites with finite package without leakage is still a great challenge,due to high surface tension and pump-out issues of LM.Here,a novel confined thermal expansion strategy based on expandable microsphere(EM)is proposed to develop a new class of LM-based monoliths with 3D continuous conductive network.The EM/LM monolith(EM/LMm)presents outstanding performance of lightweight like metallic aerogel(0.104 g cm^(-1)),high strength(3.43 MPa),super elasticity(90%strain),as well as excellent tailor ability and recyclability,rely on its unique gas-filled closed-cellular structure and refined LM network.Moreover,the assembled highly conducting EM/LMm exhibits a recorded shielding effectiveness(98.7 dB)over a broad frequency range of 8.2-40 GHz among reported LM-based composites at an ultra-low content of LM,and demonstrates excellent electromagnetic sealing capacity in practical electronics.The ternary EM/LM/Ni monoliths fabricated by the same approach could be promising universal design principles for multifunctional LM composites,and applicable in magnetic responsive actuator.

关键词： Liquid metal Elastic monolith Confined thermal expansion Electromagnetic interference shielding Magnetic actuation

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Crosstalk between degradation and bioenergetics: how autophagy and endolysosomal processes regulate energy production

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Neural Regeneration Research 2025年第3期20卷 671-681页

作者： Angelid Pabon Jagannatham Naidu Bhupana ching-On wong Department of Biological Sciences Rutgers UniversityNewarkNJUSA

Cells undergo metabolic reprogramming to adapt to changes in nutrient availability, cellular activity, and transitions in cell states. The balance between glycolysis and mitochondrial respiration is crucial for energy production, and metabolic reprogramming stipulates a shift in such balance to optimize both bioenergetic efficiency and anabolic requirements. Failure in switching bioenergetic dependence can lead to maladaptation and pathogenesis. While cellular degradation is known to recycle precursor molecules for anabolism, its potential role in regulating energy production remains less explored. The bioenergetic switch between glycolysis and mitochondrial respiration involves transcription factors and organelle homeostasis, which are both regulated by the cellular degradation pathways. A growing body of studies has demonstrated that both stem cells and differentiated cells exhibit bioenergetic switch upon perturbations of autophagic activity or endolysosomal processes. Here, we highlighted the current understanding of the interplay between degradation processes, specifically autophagy and endolysosomes, transcription factors, endolysosomal signaling, and mitochondrial homeostasis in shaping cellular bioenergetics. This review aims to summarize the relationship between degradation processes and bioenergetics, providing a foundation for future research to unveil deeper mechanistic insights into bioenergetic regulation.

关键词： autophagy bioenergetics endolysosome energy production glycolysis metabolic reprogramming mitochondria

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Artificial solid electrolyte interface layer based on sodium titanate hollow microspheres assembled by nanotubes to stabilize zinc metal electrodes

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Journal of Energy Chemistry 2022年第8期31卷 539-546,I0015页

作者： Minfeng Chen Weijun Zhou Qinghua Tian Xiang Han Yanjun Tan Jizhang Chen ching-ping wong Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Materials Science and EngineeringNanjing Forestry UniversityNanjing 210037JiangsuChina Department of Chemistry School of SciencesZhejiang Sci-Tech UniversityHangzhou 310018ZhejiangChina Nanjing Sanle Group Co. Ltd.Nanjing 211800JiangsuChina School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

Recently,aqueous zinc-ion batteries with intrinsic safety,low cost,and environmental benignity have attracted tremendous research interest.However,zinc dendrites,harmful side reactions,and zinc metal corrosion stand in the way.Herein,we use lepidocrocite-type sodium titanate hollow microspheres assembled by nanotubes to constitute an artificial solid electrolyte interface layer on the zinc metal electrode.Thanks to the hierarchical structure with abundant open voids,negative-charged layered framework,low hydrophilicity,electrically insulting nature,and large ionic conductivity,the sodium titanate coating layer can effectively homogenize the electric field,promote the Zn^(2+)ion transfer,guide the Zn^(2+)ion flux,reduce the desolvation barrier,improve the exchange current density,and accommodate the plated zinc metal.Consequently,this coating layer can effectively suppress zinc dendrites and other unfavorable effects.With this coating layer,the Zn//Zn symmetric cell is able to provide an impressive cumulative zinc plating capacity of 1375 m Ah cm^(-2) at a current density of 5 m A cm^(-2).This coating layer also contributes to significantly improved electrochemical performances of Zn//MnO_(2) battery and zincion hybrid capacitor.This work offers new insights into the modifications of zinc metal electrodes.

关键词： Artificial SEI layers Hierarchical sodium titanates Interfacial stability Dendrite inhibition Aqueous Zn-ion batteries

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Rational design and evaluation of UV curable nano-silver ink applied in highly conductive textile-based electrodes and flexible silver-zinc batteries

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Journal of Materials Science & Technology 2022年第6期101卷 294-307页

作者： Hong Hong Lihong Jiang Huating Tu Jiyong Hu Kyoung-Sik Moon Xiong Yan ching-ping wong Key Laboratory of Textile Science&Technology Ministry of EducationDonghua UniversityShanghai 201620China Key Laboratory of High Performance Fibers&Products Ministry of EducationDonghua UniversityShanghai 201620China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332United States

The possibility of printing conductive ink on textiles is progressively researched due to its potential benefits in manufacturing functional wearable electronics and improving wearing comfort.However,few studies have reported the effect of conductive ink formulation on electrodes directly screen-printed on flexible substrates,especially printing UV curable conductive ink on common textiles.In this work,a novel UV curable nano-silver ink with short-time curing and low temperature features was developed to manufacture the fully flexible and washable textile-based electrodes by screen printing.The aim of this study was to determine the influence of ink formulation on UV-curing speed,degree of conversion,morphology and electrical properties of printed electrodes.Besides,the application demonstration was highlighted.The curing speed and adhesion of ink was found depending dominantly on the type of prepolymer and the functionality of monomer,and the type of photoinitiator had a decisive effect on the curing speed,degree of double bond conversion and morphology of printed patterns.The nano-silver content is key to guarantee the suitable screen-printability of conductive ink and therefore the uniformity and high conductivity of textile-based electrodes.Optimally,an ink formulation with 60 wt%nano-silver meets the potential application requirements.The electrode with 1.0 mm width showed significantly high electrical conductivity of 2.47×10^(6)S/m,outstanding mechanical durability and satisfactory washability.The high-performance of electrodes screen-printed on different fabrics proved the feasibility and utility of UV curable nano-silver ink.In addition,the application potential of the conductive ink in fabricating electronic textiles(e-textiles)was confirmed by using the textile-based electrodes as the cathodes of silverzinc batteries.We anticipate the developed UV curable conductive ink for screen-printing on textiles can provide a novel design opportunity for flexible and wearable e-textile applications.

关键词： Nano-silver ink formulation UV curing Textile-based electrodes High conductivity Mechanical durability Washability

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Assembly of flower-like VS_(2)/N-doped porous carbon with expanded(001)plane on rGO for superior Na-ion and K-ion storage

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Nano Research 2022年第5期15卷 4108-4116页

作者： Junwei Sun Gang Lian Laiying Jing Di Wu Deliang Cui Qilong Wang Haohai Yu Huaijin Zhang ching-ping wong State Key Lab of Crystal Materials Shandong UniversityJinan 250100China School of Materials Science and Engineering Qilu University of Technology(Shandong Academy of Sciences)Jinan 250353China Key Laboratory for Special Functional Aggregated Materials of Education Ministry School of Chemistry&Chemical EngineeringShandong UniversityJinan 250100China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGeorgia 30332USA

VS2 with natural layered structure and metallic conductivity is a prospective candidate for sodium-ion batteries(SIBs)and potassium-ion batteries(PIBs).However,due to large radius of Na+and K+,the limited interlayer spacing(0.57 nm)of VS2 generally determines high ion diffusion barrier and large volume variation,resulting in unsatisfactory electrochemical performance of SIBs and PIBs.In this work,flower-like VS_(2)/N-doped carbon(VS_(2)/N-C)with expanded(001)plane is grown on reduced graphene oxide(rGO)via a solvothermal and subsequently carbonization strategy.In the VS_(2)/N-C@rGO nanohybrids,the ultrathin VS2"petals"are alternately intercalated by the N-doped porous carbon monolayers to achieve an expanded interlayer spacing(1.02 nm),which can effectively reduce ions diffusion barrier,expose abundant active sites for Na+/K+intercalation,and tolerate large volume variation.The N-C and rGO carbonous materials can significantly promote the electrical conductivity and structural stability.Benefited from the synergistic effect,the VS2/N-C@rGO electrode exhibits large reversible capacity(Na+:407 mAh·g^(-1) at 1 A·g^(-1);K^(+):334 mAh·g^(-1) at 0.2 A·g^(-1)),high rate capacity(Na+:273 mAh·g^(-1) at 8 A·g^(-1);K+:186 mAh·g^(-1) at 5 A·g^(-1)),and remarkable cycling stability(Na+:316 mAh·g^(-1) at 2 A·g^(-1) after 1,400 cycles;K^(+):216 mAh·g^(-1) at 1 A·g^(-1) after 500 cycles).

关键词： VS_(2) N-doped porous carbon,graphene substrate expanded interlayer spacing sodium-ion batteries potassium-ion batteries

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Regulating the Electrical and Mechanical Properties of TaS_(2) Films via van der Waals and Electrostatic Interaction for High Performance Electromagnetic Interference Shielding

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Nano-Micro Letters 2023年第7期15卷 278-292页

作者： Fukang Deng Jianhong Wei Yadong Xu Zhiqiang Lin Xi Lu Yan-Jun Wan Rong Sun ching-ping wong Yougen Hu Shenzhen Institute of Advanced Electronic Materials Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055People’s Republic of China Shenzhen Geim Graphene Center Institute of Materials ResearchShenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055People’s Republic of China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332USA

Low-dimensional transition metal dichalcogenides(TMDs) have unique electronic structure, vibration modes, and physicochemical properties, making them suitable for fundamental studies and cutting-edge applications such as silicon electronics, optoelectronics, and bioelectronics. However, the brittleness, low toughness,and poor mechanical and electrical stabilities of TMD-based films limit their application. Herein, a TaS_(2) freestanding film with ultralow void ratio of 6.01% is restacked under the effect of bond-free van der Waals(vdW) interactions within the staggered 2H-TaS_(2) nanosheets.The restacked films demonstrated an exceptionally high electrical conductivity of 2,666 S cm^(-1), electromagnetic interference shielding effectiveness(EMI SE) of 41.8 dB, and absolute EMI SE(SSE/t) of 27,859 dB cm^(2) g^(-1), which is the highest value reported for TMD-based materials. The bond-free vdW interactions between the adjacent 2H-TaS_(2) nanosheets provide a natural interfacial strain relaxation, achieving excellent flexibility without rupture after 1,000 bends. In addition, the TaS_(2) nanosheets are further combined with the polymer fibers of bacterial cellulose and aramid nanofibers via electrostatic interactions to significantly enhance the tensile strength and flexibility of the films while maintaining their high electrical conductivity and EMI SE.This work provides promising alternatives for conventional materials used in EMI shielding and nanodevices.

关键词： 2D transition metal dichalcogenides 2H-TaS_(2) Flexibility Electromagnetic interference shielding

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Interfacial nitrogen engineering of robust silicon/MXene anode toward high energy solid-state lithium-ion batteries

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Journal of Energy Chemistry 2022年第4期31卷 727-735页

作者： Xiang Han Weijun Zhou Minfeng Chen Jizhang Chen Guanwen Wang Bo Liu Linshan Luo Songyan Chen Qiaobao Zhang Siqi Shi ching-ping wong College of Materials Science and Engineering Nanjing Forestry UniversityNanjing 210037JiangsuChina School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaUSA College of Mathematics and Physics Jinggangshan UniversityJi'an 343009JiangxiChina Department of Physics Jiujiang Research Institute and Collaborative Innovation Center for Optoelectronic Semiconductors and Efficient DevicesXiamen UniversityXiamen 361005FujianChina Department of Materials Science and Engineering College of MaterialsXiamen UniversityXiamen 361005FujianChina School of Materials Science and Engineering Shanghai UniversityShanghai 200444China

Replacing the conventional carbonate electrolyte by solid-state electrolyte (SSE) will offer improved safety for lithium-ion batteries.To further improve the energy density,Silicon (Si) is attractive for next generation solid-state battery (SSB) because of its high specific capacity and low cost.High energy density and safe Si-based SSB,however,is plagued by large volume change that leads to poor mechanical stability and slow lithium ions transportation at the multiple interfaces between Si and SSE.Herein,we designed a self-integrated and monolithic Si/two dimensional layered T_(3)C_(2)T_(x)(MXene,T_(x) stands for terminal functional groups) electrode architecture with interfacial nitrogen engineering.During a heat treatment process,the polyacrylonitrile not only converts into amorphous carbon (a-C) that shells Si but also forms robust interfacial nitrogen chemical bonds that anchors Si and MXene.During repeated lithiation and delithiation processes,the robust interfacial engineered Si/MXene configuration enhances the mechanical adhesion between Si and MXene that improves the structure stability but also contributes to form stable solid-electrolyte interphase (SEI).In addition,the N-MXene provides fast lithium ions transportation pathways.Consequently,the Si/MXene with interfacial nitrogen engineering (denoted as Si-N-MXene) deliveres high-rate performance with a specific capacity of 1498 m Ah g^(-1) at a high current of 6.4 A g^(-1).A Si-N-MXene/NMC full cell exhibited a capacity retention of 80.5%after 200 cycles.The Si-N-MXene electrode is also applied to SSB and shows a relative stable cycling over 100 cycles,demonstrating the versatility of this concept.

关键词： Solid-state lithium-ion battery Monolithic Si/MXene anode Interfacial nitrogen engineering Lithium ions transportation

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Surface-modified barium titanate by MEEAA for high-energy storage application of polymer composites

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High Voltage 2016年第4期1卷 175-180页

作者： Yanbin Shen Suibin Luo Shuhui Yu Rong Sun ching-ping wong Center for Advanced Materials Research Shenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhenPeople’s Republic of China Department of Nano Science and Technology Institute Nano Science and Technology InstituteUniversity of Science and Technology of ChinaSuzhouPeople’s Republic of China Faculty of Engineering The Chinese University of Hong KongHong KongPeople’s Republic of China

In this study,2-[2-(2-methoxyethoxy)ethoxy]acetic acid(MEEAA)was used to modify the surface of barium titanate nanoparticles(BT NPs)to enhance the compatibility and dispersion of the BT ceramic fillers in polymer matrix.A uniform coating layer with a thickness about 2 nm was formed on the surface of BT after modification.The poly(vinylidene fluoride)-hexafluoropropene[P(VDF-HFP)]composites filled with MEEAA-modified BT NPs achieved higher permittivity(∼13 at 3.0 vol%filler)and discharged energy density than that of the untreated BT filled composite.The maximum discharge energy density of 7.8 J/cm^(3)was obtained in the nanocomposites with 3 vol%MEEAA-modified BT NPs at electric field of 425 kV/mm,which is 77%higher than that of 4.4 J/cm^(3)of pure P(VDF-HFP)film at electric field of 420 kV/mm.

关键词： composites barium modified

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Rheological properties and screen printability of UV curable conductive ink for flexible and washable E-textiles

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Journal of Materials Science & Technology 2021年第8期67卷 145-155页

作者： Hong Hong Jiyong Hu Kyoung-Sik Moon Xiong Yan ching-ping wong Key Laboratory of Textile Science STechnology Ministry of EducationDong hua UniversityShanghai 201620China Key Laboratory of High Performance Fibers&Products Ministry of EducationDonghua UniversityShanghai 201620China School of Materials Science and Engineering Georgia Institute of TechnologyAtlantaGeorgia 30332United States

As a critical component for the realization of flexible electronics,multifunctional electronic textiles(etextiles)still struggle to achieve controllable printing accuracy,excellent flexibility,decent washability and simple manufacturing.The printing process of conductive ink plays an important role in manufacturing e-textiles and meanwhile is also the main source of printing defects.In this work,we report the preparation of fully flexible and washable textile-based conductive circuits with screen-printing method based on novel-developed UV-curing conductive ink that contains low temperature and fast cure features.This work systematically investigated the correlation between ink formulation,rheological properties,screen printability on fabric substrates,and the electrical properties of the e-textile made thereafter.The rheological behaviors,including the thixotropic behavior and oscillatory stress sweep of the conductive inks was found depending heavily on the polymer to diluent ratio in the formulation.Subsequently,the rheological response of the inks during screen printing showed determining influence to their printability on textile,that the proper control of ink base viscosity,recovery time and storage/loss modulus is key to ensure the uniformity of printed conductive lines and therefore the electrical conductivity of fabricated e-textiles.A formulation with 24 wt%polymer and 10.8 wt%diluent meets all these stringent requirements.The conductive lines with 1.0 mm width showed exceptionally low resistivity of 2.06×10^(-5)Ωcm Moreover,the conductive lines presented excellent bending tolerance,and there was no significant change in the sample electrical resistance during 10 cycles of washing and drying processes.It is believed that these novel findings and the promising results of the prepared product will provide the basic guideline to the ink formulation design and applications for screen-printing electronics textiles.

关键词： Conductive ink Rheology Screen printing UV curing Washable E-textiles

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