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A generalized nonlinear three-dimensional Hoek‒brown failure criterion

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3149-3164页

作者： Jiaxin Wang Shunchuan Wu Haiyong cheng Junlong Sun Xiaolong Wang yaxi Shen Faculty of Land Resource Engineering Kunming University of Science and TechnologyKunming650093China Key Laboratory of Geohazard Forecast and Geoecological Restoration in Plateau Mountainous Area Ministry of Natural ResourcesKunming650093China yunnan Key Laboratory of Geohazard Forecast and Geoecological Restoration in Plateau Mountainous Area Kunming650093China

To understand the strengths of rocks under complex stress states,a generalized nonlinear threedimensional(3D)Hoek‒brown failure(NGHb)criterion was proposed in this *** criterion shares the same parameters with the generalized Hb(GHb)criterion and inherits the parameter advantages of *** new parameters,b,and n,were introduced into the NGHb criterion that primarily controls the deviatoric plane shape of the NGHb criterion under triaxial tension and compression,*** NGHb criterion can consider the influence of intermediate principal stress(IPS),where the deviatoric plane shape satisfies the smoothness requirements,while the Hb criterion *** criterion can degenerate into the two modified 3D Hb criteria,the Priest criterion under triaxial compression condition and the Hb criterion under triaxial compression and tension *** criterion was verified using true triaxial test data for different parameters,six types of rocks,and two kinds of in situ rock *** comparison,three existing 3D Hb criteria were selected for performance comparison *** result showed that the NGHb criterion gave better prediction performance than other *** prediction errors of the strength of six types of rocks and two kinds of in situ rock masses were in the range of 2.0724%-3.5091%and 1.0144%-3.2321%,*** proposed criterion lays a preliminary theoretical foundation for prediction of engineering rock mass strength under complex in situ stress conditions.

关键词： Rock mechanics Hoekebrown criterion Failure criterion Intermediate principal stress True triaxial test Smoothness and convexity

Degradation of Rhodamine b by MnFe-LDH/PMS/O_(3) three-phase catalytic system: performance, mechanism and ecotoxicity studies

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Frontiers of Environmental Science & Engineering 2024年第1期18卷 111-127页

作者： ying Han ying yang Weibao Liu yilong Hou Ce Wang Jiangwei Shang Xiuwen cheng Key Laboratory of Pollutant Chemistry and Environmental Treatment College of Chemistry and Environmental ScienceYili Normal UniversityYining 835000China Key Laboratory for Environmental Pollution Prediction and Control of Gansu Province College of Earth and Environmental SciencesLanzhou UniversityLanzhou 730000China

This study developed a novel MnFe-LDH/PMS/O3 three-phase catalytic system to degrade the organic dye Rhb, which was used to address the drawbacks of persulfate oxidation and ozonation techniques. The structure, ionic and elemental composition, specific surface area, and magnetic properties of the LDHs were investigated using a variety of physicochemical characterization tools. The results showed that MnFe-LDH had a large specific surface area, a rich crystalline phase composition, and a functional group structure. The Rhb degradation rate of MnFe-LDH/PMS/O3 was 0.34 min−1, which was much higher than that of other comparative systems. Rhb could be completely degraded in 10 min after optimization and had a significant effect on TOC removal. The system was found to be effective over a wide pH range. Common anions were largely unaffected and humic acid acted as an inhibitor. At the same time, the system had generally effective degradation performance for different dyes. Combined with quenching experiments and EPR, it was found that SO4•−, •OH, O_(2)•−, and 1O_(2) all participated in the reaction, and •OH contributed more. The degradation pathway of Rhb was derived by LC-MS, and the T.E.S.T. evaluation found that the toxicity of the intermediate product was significantly reduced. Finally, the stability and availability of LDHs were verified using cycling experiments and metal ion leaching. This work provides a theoretical basis and data support for the synergistic catalysis of PMS/O3 and the deep treatment of dye wastewater.

关键词： Rhodamine b Layered double hydroxides Peroxymonosulfate Ozonation

Molecular simulation study on the evolution process of hydrate residual structures into hydrate

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Chinese Journal of Chemical Engineering 2024年第5期69卷 79-91页

作者： Liwei cheng yunfei Li Jinlong Cui Huibo Qin Fulong Ning bei Liu Guangjin Chen Faculty of Engineering China University of GeosciencesWuhan 430074China State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China College of Science Nanchang Institute of TechnologyNanchang 330099China School of Chemical Engineering Guangdong University of Petrochemical TechnologyMaoming 525000China National Center for International Research on Deep Earth Drilling and Resource Development China University of Geosciences(Wuhan)Wuhan 430074China

The clathrate hydrate memory effect is a fascinating phenomenon with potential applications in carbon capture,utilization and storage(CCUS),gas separation,and gas storage as it can accelerate the secondary formation of clathrate ***,the underlying mechanism of this effect remains *** gain a better understanding of the mechanism,we conducted molecular dynamic simulations to simulate the initial formation and reformation processes of methane *** this work,we showed the evolution process of hydrate residual structures into hydrate *** simulation results indicate that the residual structures are closely related to the existence of hydrate memory effect,and the higher the contribution of hydrate dissociated water to the hydrate nucleation process,the faster the hydrate *** hydrate dissociation,the locally ordered structures still exist after hydrate dissociation and can promote the formation of cluster structures,thus accelerating hydrate ***,the nucleation process of hydrate and the formation process of clusters are *** size of clusters composed of cup-cage structures is critical for hydrate *** residence time at high temperature after hydrate decomposition will affect the strength of the hydrate memory *** simulation results provide microscopic insights into the occurrence of the hydrate memory effect and shed light on the hydrate reformation process at the molecular scale.

关键词： Memory effect Molecular simulation Hydrate reformation Residual structures

Decomposition solutions and bäcklund transformations of the b-type and C-type Kadomtsev-Petviashvili equations

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Communications in Theoretical Physics 2024年第6期76卷 34-44页

作者： Xiazhi Hao S y Lou College of Science Zhejiang University of TechnologyHangzhou 310014China School of Physical Science and Technology Ningbo UniversityNingbo 315211China

This paper introduces a modified formal variable separation approach,showcasing a systematic and notably straightforward methodology for analyzing the b-type Kadomtsev-Petviashvili(bKP)*** the application of this approach,we successfully ascertain decomposition solutions,bäcklund transformations,the Lax pair,and the linear superposition solution associated with the aforementioned ***,we expand the utilization of this technique to the C-type Kadomtsev-Petviashvili(CKP)equation,leading to the derivation of decomposition solutions,bäcklund transformations,and the Lax pair specific to this *** results obtained not only underscore the efficacy of the proposed approach,but also highlight its potential in offering a profound comprehension of integrable behaviors in nonlinear ***,this approach demonstrates an efficient framework for establishing interrelations between diverse systems.

关键词： decomposition solution backlund transformation Lax pair linear superposition solution

binding SnO2 Nanoparticles with MoS2 Nanosheets Toward Highly Reversible and Cycle-Stable Lithium/Sodium Storage

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Energy & Environmental Materials 2024年第4期7卷 135-142页

作者： Deliang cheng Wenbiao Zhang yi Tang Qingsheng Gao Renzong Hu Lichun yang Min Zhu Institute of Advanced Materials Jiangxi Normal University School of Materials Science and Engineering Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials South China University of Technology College of Chemistry and Materials Science Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications Jinan University Department of Chemistry Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials Laboratory of Advanced Materials and Collaborative Innovation Center of Chemistry for Energy Materials Fudan University

SnO2,with its high theoretical capacity,abundant resources,and environmental friendliness,is widely regarded as a potential anode material for lithium-ion batteries （LIbs）.Nevertheless,the coarsening of the Sn nanop... 详细信息

关键词： 1 T-MoS2 heterostructure lithium-ion batteries Sn coarsening SnO2

Development of sustainable and efficient recycling technology for spent Li-ion batteries: Traditional and transformation go hand in hand

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Green Energy & Environment 2024年第5期9卷 802-830页

作者： Zejian Liu Gongqi Liu Leilei cheng Jing Gu Haoran yuan yong Chen yufeng Wu Guangzhou Institute of Energy Conversion Chinese Academy of Sciences(CAS)Guangzhou510640China School of Engineering Science University of Science and Technology of ChinaHefei230026China Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development Guangzhou510640China Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing100124China

Clean and efﬁcient recycling of spent lithium-ion batteries(LIbs)has become an urgent need to promote sustainable and rapid development of human ***,we provide a critical and comprehensive overview of the various technologies for recycling spent LIbs,starting with lithium-ion power *** research on raw material collection,metallurgical recovery,separation and puriﬁcation is highlighted,particularly in terms of all aspects of economic efﬁciency,energy consumption,technology transformation and policy *** and pathways for transformative full-component recovery of spent LIbs are explored,revealing a clean and efﬁcient closed-loop recovery *** methods are proposed for future recycling technologies,with a focus on how future research directions can be ***,based on life-cycle assessment,the challenges of future recycling are revealed from the LIbs supply chain and stability of the supply chain of the new energy.b.ttery industry to provide an outlook on clean and efﬁcient short process recycling *** work is designed to support the sustainable development of the new energy power industry,to help meet the needs of global decarbonization strategies and to respond to the major needs of industrialized recycling.

关键词： Spent LIbs Transformative recycling LCA analysis Policy guidance High value utilization

Nano-silica modified lightweight and high-toughness carbon fiber/phenolic ablator with excellent thermal insulation and ablation performance

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Defence Technology（防务技术） 2024年第1期31卷 192-199页

作者： Wenjie Xu Wenda Song Xianfeng Jia cheng Ma Jitong Wang Wenming Qiao Licheng Ling State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai 200237China School of Chemical Engineering and Materials Changzhou Institute of TechnologyChangzhou 213032China Key Laboratory of Specially Functional Polymeric Materials and Related Technology(Ministry of Education) School of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China

Lightweight and high-toughness carbon fiber/phenolic ablator(CFPA)is required as the Thermal Protection System(TPS)material of aerospace vehicles for next-generation space *** improve the ablative properties,silica sol with good particle size distribution prepared using tetramethoxysilane(TMOS)was blended with natural rubber latex and deposited onto carbon fiber felt,which was then integrated with phenolic aerogel matrix,introducing nano-silica into the framework of *** modified CFPA with a low density of 0.28—0.31 g/cm3exhibits strain-in-fracture as high as 31.2%and thermal conductivity as low as 0.054 W/(m·K).Furthermore,a trace amount of nano-silica could effectively protect CFPA from erosion of oxidizing atmosphere in different high-temperature *** oxyacetylene ablation test of 3000°C for 20 s shows a mass ablation rate of 0.0225 g/s,a linear ablation rate of 0.209 mm/s for the modified CFPA,which are 9.64%and 24.82%lower than the unmodified ***,the long-time butane ablation test of 1200°C for 200 s shows an insignificant recession with mass and linear ablation rate of 0.079 g/s and 0.039 mm/s,16.84%and 13.33%lower than the unmodified ***,the fixed thermocouple in the test also demonstrates a good thermal insulation performance with a low peak back-face temperature of 207.7°C,12.25%lower than the unmodified ***,the nano-silica modified CFPA with excellent overall performance presents promising prospects in high-temperature aerospace applications.

关键词： Nano-silica Carbonfiber Phenolic aerogel Insulation Ablation

Enhanced thermoelectric and mechanical properties of bi_(0.5)Sb_(1.5)Te_(3) alloy with dispersed yttrium oxide ceramic nanoparticles

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Rare Metals 2024年第4期43卷 1758-1768页

作者： Cun-cheng Li Ming-Wei Zhang Ji-Wu Xin Lei Wei Wen-yu Zhao School of Materials Science and Engineering Shandong University of TechnologyZibo255000China School of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore639798Singapore State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Reducing thermal conductivity while avoiding adverse interfacial reactions during sintering is crucial for improving the thermoelectric performance of bi_(2)Te_(3)based *** ceramic nanoparticles are good candidates for achieving this *** this study,we designed and prepared a series of p-type bi_(0.5)Sb_(1.5)Te_(3)nanocomposites decorated with y_(2)O_(3)ceramic nanoparticles via ball-milling dispersion and spark-plasma *** to the chemical stability of the ceramics,no traces of atomic doping or interfacial reactions were *** measurements revealed that the y_(2)O_(3)nanoparticles distributed along the grain boundaries acted as energy-dependent carrier-filtering centers to improve the scattering parameter and Seebeck coefficient,contributing to the elevated power factor even with a decreased electrical ***,the incorporated y_(2)O_(3)nanoparticles and various defect structures they induced effectively strengthened the phonon scattering and suppressed the lattice thermal ***,a peak figure of merit(ZT)of 1.23 at 313 K was achieved for 0.4%y_(2)O_(3)/bi_(0.5)Sb_(1.5)Te_(3),which is 13%higher than that of the *** addition,the Vickers hardness of the composite material was 35%higher than that of the *** study demonstrates the effectiveness of ceramic nanoparticles in synergistic ally improving the thermoelectric and mechanical properties,which may.b. further extended to other thermoelectric systems.

关键词： bi_(0.5)Sb_(1.5)Te_3 alloy y_(2)O_(3) ceramic nanoparticles Microstructures Thermoelectric performance Mechanical properties

A numerical model study on the spatial and temporal variabilities of dissolved oxygen in Qinzhou bay of the northern beibu Gulf

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Acta Oceanologica Sinica 2024年第6期43卷 49-59页

作者： Gaolei cheng Shiqiu Peng bin yang Dongliang Lu State Key Laboratory of Tropical Oceanography South China Sea Institute of OceanologyChinese Academy of SciencesGuangzhou 510301China Laboratory for Regional Oceanography and Numerical Modeling Qingdao National Laboratory for Marine Science and TechnologyQingdao 266237China Guangxi Key Laboratory of Marine Environmental Change and Disaster in the beibu Gulf Beibu Gulf UniversityQinzhou 535011China

Oxygen facilitates the breakdown of the organic material to provide energy for *** concentration of dissolved oxygen(DO) in the water must exceed a certain threshold to support the normal metabolism of marine *** in the northern b eibu Gulf,Qinzhou b ay receives abundant freshwater and nutrients from several rivers which significantly influence the level of the dissolved ***,the spatial-temporal variations of DO as well as the associated driving mechanisms have been rarely studied through field *** this study,a three-dimension al coupled physical-biogeochemical model is used to investigate the spatial and seasonal variations of the DO and the associated driving mechanisms in Qinzhou b *** validation against observations indicates that the model can capture the seasonal and inter-annual variability of the DO concentration with the range of 5-10 mg/*** experiments show that the river discharges,winds and tides play crucial roles in the seasonal variability of the DO by changing the vertical mixing and stratification of the water column and the circulation *** winter,the tide and wind forces have strong effects on the DO distribution by enhancing the vertical mixing,especially near the bay *** summer,the river discharges play a dominant role in the DO distribution by inhibiting the vertical water exchange and delivering more nutrients to the bay,which increases the DO depletion and results in lower DO on the bottom of the estuary salt *** findings can contribute to the preservation and management of the coastal environment in the northern beibu Gulf.

关键词： river plume dissolved oxygen stratification physical-biological model