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A highly stable zinc anode protected by a corrosion inhibitor for seawater-based zinc-ion batteries

Journal of Energy Chemistry 2024年第10期97卷 332-341,I0006页

作者： Bowei Shi Rongwei Meng Xin Jiang Yingxin Liu Huaiyuan Wang Quanjun Tang Li Wang chen zhang Guowei Ling Quan-Hong Yang Nanoyang Group Tianjin Key Laboratory of Advanced Carbon and Electrochemical Energy StorageState Key Laboratory of Chemical EngineeringSchool of Chemical Engineering and TechnologyNational Industry-Education Integration Platform of Energy StorageCollaborative Innovation Center of Chemical Science and Engineering(Tianjin)TianjinUniversityTianjin 300072China School of Marine Science and Technology Tianjin UniversityTianjin 300072China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityBinhai New CityFuzhou 350207FujianChina

The island-based energy storage is of urgent need for the grid construction combined with renewable energy for offshore *** direct use of seawater as a substitute of deionized water shows its great promise for aqueous zinc-ion batteries in such a specific ***,the metal corrosion,dendrite growth,and hydrogen evolution stand out in the harsh seawater *** address these challenges,we proposed a corrosion inhibitor that was effective in the field of metal anti-corrosion,2-phosphonobutane-1,2,4-tricarboxylic acid(PBTCA),to inhibit anode corrosion caused by Cl-and active H_(2)O molecules by forming a stable solid electrolyte interphase(SEI)film in the seawater-based ***,PBTCA can chelate with other cations present in seawater,such as Ca^(2+)and Mg^(2+),thereby preventing the aggregation and precipitation of sparingly soluble *** a current density of5 mA cm^(-2),the seawater-based zinc-ion battery exhibited an exceptional cycle life exceeding 2000 h and maintained a Coulombic efficiency of over 99.6%after 2000 ***,the performance of the Zn||ZVO full battery was significantly enhanced with the addition of *** study provides a simple,low-cost,and efficient approach for making the seawater-based zinc-ion batteries useable.

关键词： Zinc-ion batteries Anti-corrosion Seawater Solid electrolyte interphase

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基于边界点估计与稀疏卷积神经网络的三维点云语义分割

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浙江大学学报（工学版） 2024年第6期58卷 1121-1132页

作者：杨军张琛兰州交通大学电子与信息工程学院甘肃兰州730070 兰州交通大学测绘与地理信息学院甘肃兰州730070

针对大规模点云具有稀疏性,传统点云方法提取上下文语义特征不够丰富,并且语义分割结果存在物体边界模糊的问题,提出基于边界点估计与稀疏卷积神经网络的三维点云语义分割算法,主要包括体素分支与点分支.对于体素分支,将原始点云进行体... 详细信息

针对大规模点云具有稀疏性,传统点云方法提取上下文语义特征不够丰富,并且语义分割结果存在物体边界模糊的问题,提出基于边界点估计与稀疏卷积神经网络的三维点云语义分割算法,主要包括体素分支与点分支.对于体素分支,将原始点云进行体素化后经过稀疏卷积得到上下文语义特征;进行解体素化得到每个点的初始语义标签;将初始语义标签输入到边界点估计模块中得到可能的边界点.对于点分支,使用改进的动态图卷积模块提取点云局部几何特征;依次经过空间注意力模块与通道注意力模块增强局部特征;将点分支得到的局部几何特征与体素分支得到的上下文特征融合,增强点云特征的丰富性.本算法在S3DIS数据集和SemanticKITTI数据集上的语义分割精度分别达到69.5%和62.7%.实验结果表明,本研究算法能够提取到更丰富的点云特征,可以对物体的边界区域进行准确分割,具有较好的三维点云语义分割能力.

关键词：点云数据语义分割注意力机制稀疏卷积体素化

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Energy band modulation of N-doped rutile/anatase TiO_(2) photoanode promoting charge separation toward prominent photoelectrochemical performance

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Rare Metals 2024年第8期43卷 3784-3797页

作者： Juan Gao Shi-Xuan Wang Jia-Le Deng Ping-Ping Wei Fu-zhang chen Ling-cheng Zheng Yue-Qin Wang Yang Li Yin Liu Gang He School of Mechanics and Photoelectric Physics Anhui University of Science and TechnologyHuainan 232001China School of Materials Science and Engineering Anhui UniversityHefei230039China Tianneng Battery(Wuhu)Co. Ltd.Wuhu 241000China School of Materials Science and Engineering Anhui University of Science and TechnologyHuainan 232001China

To solve the problem of high photogenerated carrier recombination rate and low photoelectric conversion efficiency of TiO_(2)-based materials,a simple N-doped anatase/rutile TiO_(2) heterophase nanorod film was designed by a low-temperature hydrothermal method in this *** enhanced separation and transport of photogenerated charges were facilitated by the smaller contact barrier and appropriate band matching between anatase TiO_(2)nanoparticles and rutile TiO_(2) *** introduction of N doping in anatase TiO_(2) resulted in an upward shift of the valence band and a narrowing of the band gap,consequently enhancing the efficiency of visible light *** combination of the heterophase junction and N-doping exhibited a synergistic effect,effectively suppressing the recombination of photogenerated charges and enhancing the photoelectric conversion efficiency of the *** AM 1.5G irradiation,the photocurrent density(J)of the A-TO(N)@R-TONR photoanode reached2.19 mA·cm^(-2)(V_(RHE,1.23 eV)).Additionally,the incident photon-electron conversion efficiency(IPCE)and the charge injection efficiency(η)reached 81.4%and 51.6%at320 ***,the J,IPCE,andηvalues of the A-TO(N)@R-TONR photoanode were 2.96,2.1 and 3.2times those of pure R-TONR photoanode,*** work presents a rational strategy for designing efficient TiO_(2)-based photoanodes.

关键词： TiO_(2) Heterophase junction Photoanode

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Space advanced technology demonstration satellite

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Science China(Technological Sciences) 2024年第1期67卷 240-258页

作者： zhang XiaoFeng chen Wen ZHU Xiaocheng MENG Na HE JunWang BI XingZi zhang YongHe SHI Qi LI Fei LIU Rui FENG ZhengGong LIU Liu LI JinSong WU Haichen XU DongXiao LI TaiJie HUANG JiangJiang LIU Shuo LI TianTong YU XianSheng GAO Yang ZHOU Heng BAN HanYu zhang YanLi zhang YueTing YANG YingQuan HE Tao DUAN XuLiang chen Xin WANG YaMin SUN AnTai zhang KuoXiang SUN Ying WANG YaoBin FAN chengcheng XIONG ShaoLin LI XinQiao WEN XiangYang LING ZhiXing SUN XiaoJin zhang chen BAI XianYong WANG ZhanShan DENG YuanYong TIAN Hui YANG JianFeng XUE HongBo SANG Peng LIU JinGuo ZHENG HuiLong ZHU Xiang HE JianWu LI Hui XU LuXiang XU ShuYan chen WenWu LIU ZhenDong WANG ZhaoLi MAO XiangLong GAO Rong LI ZongXuan DING GuoPeng WANG XinYu DOU RunJiang WENG LuBin LUO Hao WANG YaPing LIANG XianFeng FANG ZiRuo Innovation Academy for Microsatellites Chinese Academy of SciencesShanghai 201203China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China National Astronomical Observatory of China Beijing 100101China Shanghai Institute of Technical Physics Chinese Academy of SciencesShanghai 200083China Institute of Precision Optical Engineering School of Physics Science and EngineeringTongji UniversityShanghai 200092China School of Earth and Space Sciences Peking UniversityBeijing 100871China Xi’an Institute of Optics and Precision Mechanics Chinese Academy of SciencesXi’an 710119China National Space Science Center Chinese Academy of SciencesBeijing 100190China Shenyang Institute of Automation Chinese Academy of SciencesShenyang 110016China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China Institute of Mechanics Chinese Academy of SciencesBeijing 100190China Shanghai Institute of Organic Chemistry Chinese Academy of SciencesShanghai 200032China Hangzhou Institute for Advanced Study University of Chinese Academy of SciencesHangzhou 310024China Nanyang Technological University Singapore 569830Singapore Dalian Institute of Chemical Physics Chinese Academy of SciencesDalian 116023China Technical Institute of Physics and Chemistry Chinese Academy of SciencesBeijing 100049China Changchun Institute of Optics Fine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Institute of Semiconductors Chinese Academy of SciencesBeijing 100083China Institute of Automation Chinese Academy of SciencesBeijing 100190China School of Aeronautics and Astronautics Zhejiang UniversityHangzhou 310058China

The Space Advanced Technology demonstration satellite(SATech-01),a mission for low-cost space science and new technology experiments,organized by Chinese Academy of Sciences(CAS),was successfully launched into a Sun-synchronous orbit at an altitude of~500 km on July 27,2022,from the Jiuquan Satellite Launch *** as an experimental platform for space science exploration and the demonstration of advanced common technologies in orbit,SATech-01 is equipped with 16 experimental payloads,including the solar upper transition region imager(SUTRI),the lobster eye imager for astronomy(LEIA),the high energy burst searcher(HEBS),and a High Precision Magnetic Field Measurement System based on a CPT Magnetometer(CPT).It also incorporates an imager with freeform optics,an integrated thermal imaging sensor,and a multi-functional integrated imager,*** paper provides an overview of SATech-01,including a technical description of the satellite and its scientific payloads,along with their on-orbit performance.

关键词： SATech-01 spacecraft design scientific instruments on-orbit performance

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Catalytic Asymmetric Diastereodivergent Synthesis of 2-Alkenylindoles Bearing both Axial and Central Chirality

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Precision Chemistry 2024年第5期2卷 208-220页

作者： Shuang Yang Jia-Bo Huang Da-Hua Wang Ning-Yi Wang Yu-Yu chen Xin-Yan Ke Hao chen Shao-Fei Ni Yu-chen zhang Feng Shi Research Center of Chiral Functional Heterocycles School of Chemistry and Materials ScienceJiangsu Normal UniversityXuzhou 221116China Department of Chemistry Key Laboratory for Preparation and Application of Ordered Structural Materials of Guangdong ProvinceShantou UniversityShantou 515063China Department of Otolaryngology Xuzhou First People’s HospitalAffiliated Xuzhou Municipal Hospital of Xuzhou Medical UniversityXuzhou 221002China School of Petrochemical Engineering Changzhou UniversityChangzhou 213164China

The catalytic asymmetric diastereodivergent synthesis of axially chiral 2-alkenylindoles was established via chiral phosphoric acid-catalyzed addition reactions of C3-unsubstituted 2-alkenylindoles with o-hydroxybenzyl alcohols under different reaction *** this strategy,two series of 2-alkenylindoles bearing both axial and central chirality were synthesized in a diastereodivergent fashion with moderate to high yields and good stereoselectivities(up to 99%yield,95:5 er,>95:5 dr).Moreover,theoretical calculations were performed on the key transition states leading to different stereoisomers,which provided an in-depth understanding of the origin of the observed stereoselectivity and diastereodivergence of the products under different reaction *** importantly,these 2-alkenylindoles were utilized in asymmetric catalysis as chiral organocatalysts and in medicinal chemistry for evaluation of their cytotoxicity,which demonstrated their potential *** study has not only established the catalytic atroposelective synthesis of axially chiral 2-alkenylindoles,but also provided an efficient strategy for catalytic asymmetric diastereodivergent construction of indole-based scaffolds bearing both axial and central chirality.

关键词： 2-Alkenylindole Axial chirality Central chirality Diastereodivergent synthesis Chiral phosphoric acid

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考虑相含量的TC17钛合金线性摩擦焊中的残余应力

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Transactions of Nonferrous Metals Society of China 2024年第1期34卷 184-193页

作者：何鹏吴运新张涛陈送义张晨中南大学轻合金研究院长沙410083 中南大学极端服役性能精准制造国家重点实验室长沙410083

为了获得准确的TC17钛合金线性摩擦焊中的残余应力,建立TC17钛合金弹性常数与相分数之间的数值关系。结合焊接区域的相分数,获得呈梯度分布的弹性常数,并将其引入轮廓法进行计算。结果表明,TC17钛合金的弹性常数与α相分数呈正相关,在... 详细信息

为了获得准确的TC17钛合金线性摩擦焊中的残余应力,建立TC17钛合金弹性常数与相分数之间的数值关系。结合焊接区域的相分数,获得呈梯度分布的弹性常数,并将其引入轮廓法进行计算。结果表明,TC17钛合金的弹性常数与α相分数呈正相关,在宽度约4 mm的焊接区域呈现明显的梯度分布特征;若忽略相分数的梯度分布,计算残余应力时相对误差可达36.06%;修正后的残余应力呈双峰分布,在热影响区边缘处达到峰值,约为442 MPa。这说明考虑相分数的梯度分布是必要的。

关键词：线性摩擦焊 TC17钛合金残余应力相分数梯度分布

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Dual-species biofilms of Escherichia coli and Pseudomonas promote temperature-dependent cross-contamination on meat surfaces

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Food Science and Human Wellness 2024年

作者： Yangyang Yuan Junke Ji chen zhang Yu cheng Wenzheng Liu Yun Jiang School of Food Science and Pharmaceutical Engineering， Nanjing Normal University

Temperature and contact surfaces are critical factors influencing biofilm formation of microbial communities derived from both lab and natural environments. However， there is limited understanding regarding how different temperatures impact transfer dynamics of individual microbial species between meat surfaces in dual-species biofilms. In this study， we evaluated the biofilm-forming capabilities of various meat-derived Escherichia coli and Pseudomonas strains on pork surfaces at 15 ℃ and 25 ℃. The results revealed that lower temperature had a significantly negative effect on the growth fitness of E. coli compared to Pseudomonas. Two robust biofilm-forming strains， E. coli C-13 and P. fluorescens S1-23， were selected under both temperature conditions to further explore their interactions in dual-species biofilms on meat surfaces. Outcome showed that E. coli exhibited a competitive growth advantage at 25 ℃， while Pseudomonas displayed enhanced growth at 15 ℃， indicating temperature-dependent competition patterns. Additionally， three established mathematical models were utilized to simulate the transfer dynamics of the two strains within mono- and dual-species biofilms. As anticipated， the numbers of transferred cells progressively declined with increased imprinting reactions between the meat surfaces. Interestingly， the transfer rates of both strains markedly improved in dual-species versus mono-species biofilms at 15 ℃， highlighting the influential role of inter-species interactions on transfer dynamics of microbes that may cross-contaminate meats. Our findings advance current understanding of mono- and dual-species biofilm development on meat surfaces under different temperature conditions. They also offer scientific evidence to support strategies for controlling microbial cross-contamination during meat processing to ensure product safety.

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融合粗糙数据推理的离散麻雀搜索算法求解HFSP问题

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北京航空航天大学学报 2024年第2期50卷 398-408页

作者：周宁张嵩霖张晨兰州交通大学电子与信息工程学院兰州730070

针对麻雀搜索算法(SSA)易陷入局部最优、无法求解离散优化问题等不足,提出了一种改进离散麻雀搜索算法(IDSSA)。抽象原始麻雀搜索算法的位置更新公式,针对个体的不同身份设计新的离散化启发式位置更新策略,并针对混合流水车间调度问题(H... 详细信息

针对麻雀搜索算法(SSA)易陷入局部最优、无法求解离散优化问题等不足,提出了一种改进离散麻雀搜索算法(IDSSA)。抽象原始麻雀搜索算法的位置更新公式,针对个体的不同身份设计新的离散化启发式位置更新策略,并针对混合流水车间调度问题(HFSP)设计了编码与解码方式;引入粗糙数据推理理论,通过数学证明解释了引入理论的可行性与合理性,为算法提供理论支撑,提高可解释性;利用上近似的性质扩大搜索空间,提高种群多样性,避免算法早熟,结合划分及粗糙数据推理提出3种策略,促进种群间信息共享,调节种群的开发能力与探索能力,降低算法陷入局部最优的概率;使用改进离散麻雀搜索算法求解混合流水车间调度问题,对3个小规模实例与10个Liao经典测试集进行仿真实验,验证了改进离散麻雀搜索算法求解混合流水车间调度问题的可行性,通过与遗传算法、差分进化算法等经典算法的对比实验,证明了所提算法的优越性与改进策略的有效性。

关键词：麻雀搜索算法离散化算法粗糙集理论全局优化近似算法数据关联混合流水车间调度

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Modeling urban redevelopment:A novel approach using time-series remote sensing data and machine learning

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Geography and Sustainability 2024年第2期5卷 211-219页

作者： Li Lin Liping Di chen zhang Liying Guo Haoteng Zhao Didarul Islam Hui Li Ziao Liu Gavin Middleton Center for Spatial Information Science and Systems George Mason UniversityFairfaxVA22030USA Department of Geography and Geoinformation Science George Mason UniversityFairfaxVA22030USA

Accurate mapping and timely monitoring of urban redevelopment are pivotal for urban studies and decisionmakers to foster sustainable urban *** mapping methods heavily depend on field surveys and subjective questionnaires,yielding less objective,reliable,and timely *** advancements in Geographic Information Systems(GIS)and remote-sensing technologies have improved the identification and mapping of urban redevelopment through quantitative analysis using satellite-based ***,challenges persist,particularly concerning accuracy and significant temporal *** study introduces a novel approach to modeling urban redevelopment,leveraging machine learning algorithms and remote-sensing *** methodology can facilitate the accurate and timely identification of urban redevelopment *** study’s machine learning model can analyze time-series remote-sensing data to identify spatio-temporal and spectral patterns related to urban *** model is thoroughly evaluated,and the results indicate that it can accurately capture the time-series patterns of urban *** research’s findings are useful for evaluating urban demographic and economic changes,informing policymaking and urban planning,and contributing to sustainable urban *** model can also serve as a foundation for future research on early-stage urban redevelopment detection and evaluation of the causes and impacts of urban redevelopment.

关键词： Urban redevelopment Urban sustainability Remote sensing Time-series analysis Machine learning

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Aspirin suppresses hepatocellular carcinoma progression by inhibiting platelet activity

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World Journal of Gastrointestinal Oncology 2024年第6期16卷 2742-2756页

作者： Li-Jun Zhao Zhi-Yin Wang Wei-Ting Liu Li-Li Yu Hao-Nan Qi Jie Ren chen-Guang zhang Hematology Laboratory The First Affiliated Hospital of Xinxiang Medical UniversityXinxiang 453100Henan ProvinceChina Xinxiang Key Laboratory of Tumor Microenvironment and Immunotherapy School of Medical TechnologyXinxiang Medical UniversityXinxiang 453003Henan ProvinceChina School of Public Health Xinxiang Medical UniversityXinxiang 453003Henan ProvinceChina

BACKGROUND Hepatocellular carcinoma(HCC)is the most common malignant liver disease in the ***(PLTs)are known to play a key role in the maintenance of liver homeostasis and the pathophysiological processes of a variety of liver *** is the most classic antiplatelet ***,the molecular mechanism of platelet action and whether aspirin can affect HCC progression by inhibiting platelet activity need further *** To explore the impact of the antiplatelet effect of aspirin on the development of *** Platelet-rich plasma,platelet plasma,pure platelet,and platelet lysate were prepared,and a coculture model of PLTs and HCC cells was ***-8 analysis,apoptosis analysis,Transwell analysis,and real-time polymerase chain reaction(RT-PCR)were used to analyze the effects of PLTs on the growth,metastasis,and inflammatory microenvironment of ***-PCR and Western blot were used to detect the effects of platelet activation on tumor-related signaling *** was used to block the activation and aggregation of PLTs both in vitro and in vivo,and the effect of PLTs on the progression of HCC RESULTS PLTs significantly promoted the growth,invasion,epithelial-mesenchymal transition,and formation of an inflammatory microenvironment in HCC *** PLTs promoted HCC progression by activating the mitogenactivated protein kinase/protein kinase B/signal transducer and activator of transcription three(MAPK/AKT/STAT3)signaling ***,aspirin inhibited HCC progression in vitro and in vivo by inhibiting platelet *** PLTs play an important role in the pathogenesis of HCC,and aspirin can affect HCC progression by inhibiting platelet *** results suggest that antiplatelet therapy has promising application prospects in the treatment and combined treatment of HCC.

关键词： Platelets Antiplatelet therapy Hepatocellular carcinoma Aspirin Antitumor

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