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science china(Physics,Mechanics & Astronomy) 2010年第5期53卷 856-863页

作者： cai xin1,2.liu jinsong1 & wang shenglie1 1 wuhan national laboratory for optoelectronics,{2.,Huazhong University of science and Technology,wuhan 43.074,china 2.school of science,wuhan University of Technology,wuhan 430070,china 1. wuhan national {2. for optoelectronics School of Optoelectronic Science and Engineering Huazhong University of Science and Technology Wuhan 430074 China2. School of Science Wuhan University of Technology Wuhan 430070 China

The transverse effects of two Gauss waves mixing in a photovoltaic photorefractive crystal,i.e.,the dynamical evolutions of signal beam with different parameters,are traced numerically and *** the one-dimensional numerical simulations and two-dimensional experimental investigations show that the self-focusing effect of signal beam becomes more obvious as the intensity of pump beam and the angle between the signal and pump beams *** accordance with these results,the state of two Gaussian waves mixing is controllable.

关键词： numerical simulation experimental investigation two-wave mixing transverse effects Gaussian distribution

Performance enhancement and active sites identification of Cu-Cd bimetallic oxide derived catalysts for electrochemical CO_(2. reduction

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Journal of Energy Chemistry 2024年第4期91卷 50-58页

作者： cai wang {2. Hu Bairong Chen Houan Ren Xiaoyu wang Yilin Zhang {2.yu Chen Yuping liu Qing{2. Guan Wei Li State Key laboratory of Elemento-Organic Chemistry Key Laboratory of Adv.Energy Mater.Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China

The development of earth-abundant electrocatalysts with high performance for electrochemical CO_(2.reduction(ECR)is of great ***-based catalysts have been widely investigated for ECR due to their unique ability to generate various carbonaceous products,but directing selectivity toward one certain product and identifying the real active sites during ECR are still full of ***,after the incorporation of CdO into CuO,the Cu_(0.5)Cd_(0.5)-O catalyst achieves a 10.3-fold enhancement for CO selectivity in comparison with CuO,and a CO faradic efficiency nearly 90%with a current density around2. mA cm^(-2.could maintain at least 60 ***,a wide CO/H_(2.ratio(0.07-10)is reached on Cu_(x)Cd_(1-x)-O catalysts by varying the Cu/Cd ratio,demonstrating the potential of syngas production using such *** results of ex situ XRD,XPS,and in situ Raman reveal that the real active sites of Cu_(0.5)Cd_(0.5)-O catalysts for CO production during ECR reaction are the reconstructed mixed phases of CuCd alloy and CdCO_(3).In situ FTIR and theoretical calculations further implicate the presence of Cd related species promotes the CO desorption and inhibits the H_(2.evolution,thus leading to an enhanced CO generation.

关键词： CO_(2.reduction Cu-Cd bimetallic Real active sites CO production

Accelerating the evaluation of operational lifetimes of perovskite solar cells and modules

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Journal of Energy Chemistry 2024年第7期94卷 1-9页

作者： Fumeng Ren Qian Lu xin Meng Jing Zhou Rui Chen Jianan wang Haixin wang Sanwan liu Zonghao liu Wei Chen wuhan national {2. for optoelectronics Huazhong University of Science and TechnologyWuhan 430074HubeiChina china-EU Institute for Clean and Renewable Energy Huazhong University of Science and TechnologyWuhan 430073HubeiChina Powerchina Huadong engineering Corporation Limited Hangzhou 311122ZhejiangChina Optics Valley laboratory Wuhan 430074HubeiChina

Compared with the power conversion efficicency,the operational stability of perovskite solar cells(PsCs)remains a major challenge hampering its ***,conducting a light soaking test under 1 sun illumination to get a long lifetime is time-consuming and experimentally ***,we report an accelerated stability test protocol by aging PsCs under high-intensity light illumination to accelerate the evaluation of their operation *** is found that the efficiency degradation rate of a typical inverted PsC is almost linearly dependent on the light intensity within the range of 1 to 4 suns regardless of the *** results prove that it can save the light-soaking time by at least 4 times to predict the operation lifetime on the basis of the equivalent light irradiation dose.

关键词： Perovskite Light-soaking Stability

A widely used nonionic surfactant with desired functional groups as aqueous electrolyte additives for stabilizing Zn anode

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Rare Metals 2024年第8期43卷 3692-3701页

作者： Yue-Xian Song Xiao-Feng wang cai-Bin {2. Kai-Xuan Guo Xu-Huan Guo Xiao-Bin Zhong Yao-Hui Zhang Kai wang Hui-Juan Guo Li-xin Zhang Jun-Fei Liang school of Energy and Power engineering North University of ChinaTaiyuan 030051China Key laboratory of Green Chemical Process of Ministry of Education Hubei Key Laboratory of Novel Chemical Reactor and Green Chemical TechnologySchool of Chemical Engineering and PharmacyWuhan Institute of TechnologyWuhan 430073China Shanxi Provincial Key laboratory for High Performance Battery Materials and Devices Taiyuan 030051China

Aqueous Zn-ion batteries(AZIBs) have emerged as potential candidates for Li-ion batteries due to their intrinsic safety and high ***,metallic Zn anodes encounter dendrite growth and water-induced corrosion,rendering poor stability and severe irreversibility at the electrode/electrolyte interface during *** stabilize the Zn anode,we report a low-cost and effective nonionic surfactant,Tween-2. polymer,as an electrolyte additive for *** Tween-2.,sequential oxyethylene groups tended to be preferentially adsorbed on the Zn electrode to form a shielding layer for regulating uniform Zn ***,the hydrophobic hendecyl chains prevented H_(2.O-induced corrosion on the Zn anode *** from the desired functional groups,when only trace amounts of Tween-2.(0.050 g·L^(-1)) were used,the Zn anode displayed good cycling stability over 2.70 h at10 mA·cm^(-2. and a high average Coulombic efficiency of98.94% over 1000 *** Tween-2. polymer can also be effectively employed in MnO_(2./Zn full *** their toxicity,price and amount of usage,these surfactant additives provide a promising strategy for realizing the stability and reversibility of high-performance Zn anodes.

关键词： Zn anode Dendrite growth Tween-2. polymer Surfactant additive Aqueous electrolyte

Naoxueshu Oral Liquid Accelerates Post-Craniotomy Hematoma Absorption in Patients:An Open-Label,Multicenter,and Randomized Controlled Trial

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Chinese Journal of Integrative Medicine 2024年第8期30卷 675-683页

作者： HE Qiu LIN Fu-xin SU Jin-ye ZHUO Ling-yun ZHU Qing SUN Xiao-chuan JIANG Rong-cai YAO Zhi-gang {2. Lei DANG Yan-wei liu De-zhong liu Yang FANG Wen-hua {2. Fang-yu LIN Yuan-xiang {2. An-xin {2. Deng-liang KANG De-zhi Department of Neurosurgery Neurosurgery Research InstituteThe First Affiliated Hospital of Fujian Medical UniversityFuzhou350004China Department of Neurosurgery Binhai Branch of National Regional Medical CenterThe First Affiliated HospitalFujian Medical UniversityFuzhou350209China Clinical Research and Translation Center The First Affiliated Hospital of Fujian Medical UniversityFuzhou350004China Fujian Clinical Research Center for Neurological Diseases The First Affiliated Hospital of Fujian Medical UniversityFuzhou350004China Fujian Provincial Institutes of Brain Disorders and Brain sciences The First Affiliated Hospital of Fujian Medical UniversityFuzhou350004China Department of Neurosurgery The Second Affiliated Hospital of Soochow UniversitySuzhouJiangsu Province215000China Department of Neurosurgery The First Affiliated Hospital of Chongqing Medical UniversityChongqing400000China Department of Neurosurgery Tianjin Medical University General HospitalTianjin300000China Department of Neurosurgery The Third Hospital of ShijiazhuangShijiazhuang050000China Department of Neurosurgery The First College of Clinical Medical ScienceChina Three Gorges UniversityYichangHubei Province443000China Department of Neurosurgery Yichang Central People’s HospitalYichangHubei Province443000China Department of Neurosurgery Xiangyang No.1 People’s Hospital Affiliated to Hubei University of MedicineXiangfanHubei Province441100China Department of Neurosurgery Zhoukou Central HospitalZhoukouHenan Province466000China Department of Neurosurgery The Third Hospital of MianyangMianyangSichuan Province621000China Department of Neurology Beijing Tiantan HospitalCapital Medical UniversityBeijing100000China china national Clinical Research Center for Neurological Diseases Beijing Tiantan HospitalCapital Medical UniversityBeijing100000China Department of Clinical Epidemiology and Clinical Trial Capital Medical UniversityBeijing100000China Beijing Municipal Key laboratory of Clinical

Objective: To investigate whether Naoxueshu Oral Liquid(NXS) could promote hematoma absorption in post-craniotomy hematoma(PCH) patients. Methods: This is an open-label, multicenter, and randomized controlled trial conducted at 9 hospitals in china. Patients aged 18–80 years with post-craniotomy supratentorial hematoma volume ranging from 10 to 30 mL or post-craniotomy infratentorial hematoma volume less than 10 mL, or intraventricular hemorrhage following cranial surgery were enrolled. They were randomly assigned at a 1:1 ratio to the NXS(10 m L thrice daily for 15 days) or control groups using a randomization code table. Standard medical care was administered in both groups. The primary outcome was the percentage reduction in hematoma volume from day 1 to day 15. The secondary outcomes included the percentage reduction in hematoma volume from day 1 to day 7, the absolute reduction in hematoma volume from day 1 to day 7 and 15, and the change in neurological function from day 1 to day 7 and 15. The safety was closely monitored throughout the study. Moreover, subgroup analysis was performed based on age, gender, history of diabetes, and etiology of intracerebral hemorrhage(ICH). Results: A total of 12. patients were enrolled and randomly assigned between March 30, 2.18 and April 15, 2.2.. One patient was lost to follow-up in the control group. Finally, there were 119 patients(60 in the NXS group and 59 in the control group) included in the analysis. In the full analysis set(FAS) analysis, the NXS group had a greater percentage reduction in hematoma volume from day 1 to day 15 than the control group [median(Q1, Q3): 85%(71%, 97%) vs. 76%(53%, 93%), P0.05). Furthermore, no adverse events were reported during the study. In the FAS analysis, the NXS group exhibited a higher percentage reduction in hematoma volume on day 15 in the following subgroups:

关键词： post-craniotomy hematoma Naoxueshu Oral Liquid hematoma absorption randomized controlled trial Chinese medicine

Organic ligand nanoarchitectonics for BiVO_(4) photoanodes surface passivation and cocatalyst grafting

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Nano Research 2024年第5期17卷 3667-3674页

作者： Jingyi Lin xin Li Zhiliang wang Runlu {2. Hui Pan Yixin Zhao Lingti Kong Yao Li Shenmin Zhu Lianzhou wang State Key laboratory of Metal Matrix Composites School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Nanomaterials Centre School of Chemical Engineering and Australian Institute for Bioengineering and Nanotechnologythe University of QueenslandQLD 4072Australia school of Environmental science and {2. Shanghai Jiao Tong UniversityShanghai 200240China Hubei Key laboratory of Plasma Chemistry and Advanced Materials Wuhan Institute of TechnologyWuhan 430205China

Bismuth vanadate(BiVO_(4))is a promising photoanode material for efficient photoelectrochemical(PEC)water splitting,whereas its performance is inhibited by detrimental surface *** solve the problem,herein,a low-cost organic molecule 1,3,5-benzenetricarboxylic acid(BTC)is selected for surface passivation of BiVO_(4) photoanodes(BVOs),which also provides bonding sites for Co^(2.)to anchor,resulting in a Co-BTC-BVO *** to its strong coordination with metal ions,BTC not only passivates surface states of BVO,but also provides bonding between BVO and catalytic active sites(Co^(2.))to form a molecular *** study and interfacial charge kinetic investigation reveal that chemical bonding formed at the interface greatly suppresses charge recombination and accelerates charge *** obtained Co-BTC-BVO photoanode exhibits a photocurrent density of 4.82.mA/cm^(2. at 1.2. V *** hydrogen electrode(RHE)and a low onset potential of 0.2. VRHE under AM 1.5 G illumination,which ranks among the best photoanodes coupled with Co-based *** work presents a novel selection of passivation layers and emphasizes the significance of interfacial chemical bonding for the construction of efficient photoanodes.

关键词： bismuth vanadate photoanode water splitting surface passivation bridging ligands

Cooperative structure of Li/Ni mixing and stacking faults for achieving high-capacity Co-free Li-rich oxides

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Journal of Energy Chemistry 2024年第8期95卷 315-324,I0007页

作者： Zhen Wu Yu-Han Zhang Hao wang Zewen liu Xudong Zhang {2. Dai Kunyang Zou Xiaoming Lou Xuechen Hu Lijing Ma Yan liu Yongning liu State Key laboratory for Mechanical Behavior of Materials Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina Qingdao Industrial Energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101ShandongChina Hefei Advanced Computing Center Operation Management Corp Ltd Hefei 230088AnhuiChina Center for High Performance Computing Network Information CenterXi’an Jiaotong UniversityXi’an 710049ShaanxiChina wuhan Dongfeng Motor Corporation Ltd Wuhan 430056HubeiChina school of Materials science and Intelligent {2. Nanjing UniversitySuzhou 215163JiangsuChina Key laboratory of MEMS of the Ministry of Education Southeast UniversityNanjing 210096JiangsuChina International Research Center for Renewable Energy State Key laboratory of Multiphase Flow in Power {2. Xi’an Jiaotong UniversityXi’an 710049ShaanxiChina

Co-free Li-rich layered oxides(LLOs)are emerging as promising cathode materials for Li-ion batteries due to their low cost and high ***,they commonly face severe structural instability and poor electrochemical activity,leading to diminished capacity and voltage ***,we introduce a Co-free LLO,Li_(1.167)Ni_(0.2.2.Mn_(0.611)O_(2.(Cf-L1),which features a cooperative structure of Li/Ni mixing and stacking *** structure regulates the crystal and electronic structures,resulting in a higher discharge capacity of 300.6 mA h g^(-1)and enhanced rate capability compared to the typical Co-free LLO,Li_(1.2.Ni_(0.2.Mn_(0.6)O_(2.(Cf-Ls).Density functional theory(DFT)indicates that Li/Ni mixing in LLOs leads to increased Li-O-Li configurations and higher anionic redox activities,while stacking faults further optimize the electronic interactions of transition metal(TM)3d and non-bonding O 2. ***,stacking faults accommodate lattice strain,improving electrochemical reversibility during charge/discharge cycles,as demonstrated by the in situ XRD of Cf-L1 showing less lattice evolution than *** study offers a structured approach to developing Co-free LLOs with enhanced capacity,voltage,rate capability,and cyclability,significantly impacting the advancement of the next-generation Li-ion batteries.

关键词： Co-free Li-rich oxides Li/Ni mixing Stacking faults Electronic structure

A flame-retardant binder with high polysulfide affinity for safe and stable lithium–sulfur batteries

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science china Chemistry 2024年第3期67卷 1028-1036页

作者： Guowei Yu Guofeng Ye Cheng wang Chenyang wang Zhaoyun wang Pu Hu Yu Li Xi-Xi Feng Shuang-Jie Tan Min Yan Sen xin Zhitian liu Hubei Key laboratory of Plasma Chemistry and Advanced Materials Hubei Engineering Technology Research Center of Optoelectronic and New Energy MaterialsSchool of Materials Science and EngineeringWuhan Institute of TechnologyWuhan 430205China State Key laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China CAS Key laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of sciences Beijing 100049China

Lithium-sulfur(Li-S) batteries have shown promises for the next-generation, high-energy electrochemical storage, yet are hindered by rapid performance decay due to the polysulfide shuttle in the cathode and safety concerns about potential thermal runaway. To address the above challenges, herein, we show a flame-retardant cathode binder that simultaneously improves the electrochemical stability and safety of batteries. The combination of soft and hard segments in the polymer framework of binders allows high flexibility and mechanical strength for adapting to the drastic volume change during the Li(de)intercalation of the S cathode. The binder contains a large number of polar groups, which show the high affinity to polysulfides so that they help to anchor active S species at the cathode. These polar groups also help to regulate and facilitate the Li-ion transport, promoting the kinetics of polysulfide conversion reaction. The binder contains abundant phosphine oxide groups, which, in the case of battery's thermal runaway, decompose and release PO· radicals to quench the combustion reactions and stop the fire. Consequently, Li-S batteries using the new cathode binder show the improved electrochemical performance, including a low-capacity decay of 0.046% per cycle for 800 cycles at 1 C and favorable rate capabilities of up to 3 C. This work offers new insights on the practical realization of high-energy rechargeable batteries with stable storage electrochemistry and high safety.

关键词： lithium–sulfur battery polymer binder polysulfide affinity flame retardancy

Multi-omics analysis of attenuated variant reveals potential evaluation marker of host damaging for SARS-CoV-2.variants

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science china(Life sciences) 2024年第1期67卷 83-95页

作者： Guangshan Xie Lin Zhu Siwen liu Cun Li xin Diao Yanhao Zhang Xiuli Su Yuanyuan Song Guodong Cao Li Zhong Pui {2. Xiaojuan liu Bobo Wing-Yee Mok Shusheng Zhang Dong-Yan Jin Jie Zhou Honglin Chen Zongwei cai State Key laboratory of Environmental and Biological Analysis Hong Kong Baptist UniversityHong Kong SARChina State Key laboratory for Emerging Infectious Diseases and Department of MicrobiologyLi Ka Shing Faculty of MedicineThe University of Hong KongHong Kong SARChina College of Chemistry Zhengzhou UniversityZhengzhou 450001China school of Biomedical sciences The University of Hong KongHong Kong SARChina HKBU Shenzhen Institute of Research and Continuing Education Shenzhen 518000China

SARS-CoV-2.continues to threaten human society by generating novel variants via mutation and *** high number of mutations that appeared in emerging variants not only enhanced their immune-escaping ability but also made it difficult to predict the pathogenicity and virulence based on viral nucleotide *** markers for evaluating the pathogenicity of new variants are therefore *** comparing host responses to wild-type and variants with attenuated pathogenicity at proteome and metabolome levels,six key molecules on the polyamine biosynthesis pathway including putrescine,SAM,dc-SAM,ODC1,SAMS,and SAMDC were found to be differentially upregulated and associated with pathogenicity of *** validate our discovery,human airway organoids were subsequently used which recapitulates SARS-CoV-2.replication in the airway epithelial cells of COVID-19 *** ODC1 as a proof-ofconcept,differential activation of polyamine biosynthesis was found to be modulated by the renin-angiotensin system(RAS)and positively associated with ACE2.*** experiments demonstrated that ODC1 expression could be differentially activated upon a panel of SARS-CoV-2.variants of concern(VOCs)and was found to be correlated with each VOCs’pathogenic ***,the presented study revealed the discriminative ability of key molecules on polyamine biosynthesis as a predictive marker for virulence evaluation and assessment of SARS-CoV-2.variants in cell or organoid *** work,therefore,presented a practical strategy that could be potentially applied as an evaluation tool for the pathogenicity of current and emerging SARS-CoV-2.variants.

关键词： SARS-CoV-2 multi-omics attenuated variant predictive pathogenic marker polyamine biosynthesis

Critical Solvation Structures Arrested Active Molecules for Reversible Zn Electrochemistry

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Nano-Micro Letters 2024年第8期16卷 64-78页

作者： Junjie Zheng Bao Zhang xin Chen Wenyu Hao Jia Yao Jingying Li Yi Gan Xiaofang wang xingtai liu Ziang Wu Youwei liu Lin Lv Li Tao Pei Liang Xiao Ji Hao wang Houzhao Wan Hubei Yangtze Memory Laboratories Wuhan 430205People’s Republic of China Hubei Key laboratory of Micro‑Nanoelectronic Materials and Devices School of MicroelectronicsHubei UniversityWuhan 430062People’s Republic of China school of Physical and Mathematical sciences Nanyang Technological UniversitySingapore 637371Singapore school of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China Institute of optoelectronics Technology China Jiliang UniversityHangzhou 310018People’s Republic of China

Aqueous Zn-ion batteries(AZIBs)have attracted increasing attention in next-generation energy storage systems due to their high safety and ***,the side reactions,dendrites and hydrogen evolution effects at the zinc anode interface in aqueous electrolytes seriously hinder the application of aqueous zinc-ion ***,we report a critical solvation strategy to achieve reversible zinc electrochemistry by introducing a small polar molecule acetonitrile to form a“catcher”to arrest active molecules(bound water molecules).The stable solvation structure of[Zn(H_(2.O)_(6)]^(2.)is capable of maintaining and completely inhibiting free water ***[Zn(H_(2.O)_(6)]^(2.)is partially desolvated in the Helmholtz outer layer,the separated active molecules will be arrested by the“catcher”formed by the strong hydrogen bond N-H bond,ensuring the stable desolvation of Zn^(2.).The Zn||Zn symmetric battery can stably cycle for 2.50 h at 1 mAh cm^(-2.,Zn||V_(6)O_(13) full battery achieved a capacity retention rate of 99.2.after 10,000 cycles at 10 A g^(-1).This paper proposes a novel critical solvation strategy that paves the route for the construction of high-performance AZIBs.

关键词： Zinc-ion battery Critical solvation Helmholtz layer Arrest active molecule Reversible zinc anode