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Synergistic integration of self-supported 1T/2H-WS_(2) and nitrogendoped rGO on carbon cloth for pH-universal electrocatalytic hydrogen evolution

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Nano Research 2024年第3期17卷 1267-1280页

作者： Feng Ming Yap Jian Yiing Loh Wee-Jun ong School of Energy and chemical Engineering Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia center of Excellence for NaNo Energy&catalysis Technology(cONNEcT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia State Key Laboratory of Physical chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China Gulei Innovation Institute Xiamen UniversityZhangzhou 363200China Shenzhen Research Institute of Xiamen University Shenzhen 518057China

Hydrogen economy based on electrochemical water splitting exemplified one of the most promising means for overcoming the rapid consumption of fossil fuels and the serious deterioration of global *** development of earth-abundant,efficient,and durable electrocatalysts for hydrogen evolution reaction(HER)plays a vital role in the commercialization of water ***,the self-supported electrode with unique nitrogen-doped reduced graphene oxide(N-rGO)nanoflakes and WS_(2) hierarchical nanoflower that were grown directly on carbon cloth(cc)substrate(WS_(2)/N-rGO/cc)was successfully synthesized using a facile dual-step hydrothermal *** as-synthesized 50%1T/2H-WS_(2)/N-rGO/cc(WGc),which possessed high metallic 1T phase of 57%not only efficiently exposed more active sites and accelerated mass/charge diffusion,but also endowed excellent structural lustiness,robust stability,and durability at a high current *** a result,the 50%WGc exhibited lower overpotentials and Tafel slopes of 21.13 mV(29.55 mV∙dec^(-1))and 80.35 mV(137.02 mV∙dec^(-1))as compared to 20%Pt-c/cc,respectively for catalyzing acidic and alkaline hydrogen evolution ***,the as-synthesized 50%WGc also depicted long-term stability for more than 8 h in the high-current-density regions(100 and 220 mA∙cm^(-2)).In brief,this work reveals a self-supported electrode as an extraordinary alternative to Pt-based catalysts for HER in a wide pH range,while paving a facile strategy to develop advanced electrocatalysts with abundant heterointerfaces for practical applications in energy-saving hydrogen production.

关键词： self-supported electrocatalyst carbon-based substrate phase engineering pH-universal water splitting

Enhancing MXene-based supercapacitors:Role of synthesis and 3d architectures

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Journal of Energy chemistry 2024年第4期91卷 1-26页

作者： Wen Siong Poh Wen Jie Yiang Wee-Jun ong Pau Loke Show chuan Yi Foo School of Energy and chemical Engineering Xiamen University MalaysiaSelangor Darul EhsanMalaysia&College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005FujianChina Kelip-kelip!center of Excellence for Light Enabling Technologies Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia center of Excellence for NaNo Energy&catalysis Technology(cONNEcT) Xiamen University MalaysiaSelangor Darul Ehsan 43900Malaysia department of chemical Engineering Khalifa UniversityShakhbout Bin Sultan St-Zone 1Abu DhabiUnited Arab Emirates Zhejiang Provincial Key Laboratory for Subtropical Water Environment and Marine Biological Resources Protection Wenzhou UniversityWenzhou 325035ZhejiangChina department of chemical and Environmental Engineering Faculty of Science and EngineeringUniversity of Nottingham MalaysiaJalan Broga43500 SemenyihSelangor Darul EhsanMalaysia department of Sustainable Engineering Saveetha School of EngineeringSIMATSChennai 602105India

MXene has been the limelight for studies on electrode active materials,aiming at developing supercapacitors with boosted energy density to meet the emerging influx of wearable and portable electronic *** its various desirable properties including intrinsic flexibility,high specific surface area,excellent metallic conductivity and unique abundance of surface functionalities,its full potential for electrochemical performance is hindered by the notorious restacking phenomenon of MXene *** to its two-dimensional(2d)nature and surface functional groups,inevitable Van der Waals interactions drive the agglomeration of nanosheets,ultimately reducing the exposure of electrochemically active sites to the electrolyte,as well as severely lengthening electrolyte ion transport *** a result,energy and power density deteriorate,limiting the application versatility of MXene-based *** 3d architectures using 2d nanosheets presents as a straightforward yet ingenious approach to mitigate the fatal flaws of ***,the sheer number of distinct methodologies reported,thus far,calls for a systematic review that unravels the rationale behind such 3d MXene structural ***,this review aims to serve this purpose while also scrutinizing the structure–property relationship to correlate such structural modifications to their ensuing electrochemical performance ***,the physicochemical properties of MXene play fundamental roles in determining the effective charge storage capabilities of 3d MXene-based *** largely depends on different MXene synthesis techniques and synthesis condition variations,hence,elucidated in this review as ***,the challenges and perspectives for achieving viable commercialization of MXene-based supercapacitor electrodes are highlighted.

关键词： MXene 3d architectures Synthesis design Supercapacitor Energy storage

Apolipoprotein E elicits targetdirected miRNA degradation to maintain neuronal integrity

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Neural Regeneration Research 2025年第9期20卷 2577-2578页

作者： Jiazi Tan chin-Tong ong Temasek Life Sciences Laboratory National University of SingaporeSingapore department of Biological Sciences National University of SingaporeSingapore

Apolipoprotein E has diverse functions in neurons:Apolipoprotein E(ApoE)is a glycoprotein that primarily regulates lipid metabolism and transport in the central nervous *** are three predominant human ApoE protein isoforms with cysteine and arginine substitutions at amino acid positions 112 and 158 that impact their lipidation and related functions(Flowers and Rebeck,2020).ApoE2 is characterized by cys112 and cys158,ApoE3 by cys112 and Arg158,whereas ApoE4 contains Arg112 and Arg158.

关键词： metabolism glycoprotein maintain

Synergistic redox reactions toward co-production of H_(2)O_(2)and value-added chemicals:dual-functional photocatalysis to achieving sustainability

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SusMat 2024年第3期4卷 36-72页

作者： Brenden Jing Su Joel Jie Foo Grayson Zhi Sheng Ling Wee-Jun ong School of Energy and chemical Engineering Xiamen University MalaysiaSelangor Darul EhsanMalaysia center of Excellence for NaNo Energy&catalysis Technology Xiamen University MalaysiaSelangor Darul EhsanMalaysia State Key Laboratory of Physical chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamenChina Gulei Innovation Institute Xiamen UniversityZhangzhouChina Shenzhen Research Institute Xiamen UniversityShenzhenChina

IntegratingH_(2)O_(2)evolution with oxidative organic synthesis in a semiconductordriven photoredox reaction is highly attractive since H_(2)O_(2)and high-value chemicals can be concurrently produced using solar light as the only energy *** dual-functional photocatalytic approach,free from sacrificial agents,enables simultaneous production of H_(2)O_(2)and high-value organic *** strategy promises a green and sustainable organic synthesis with minimal greenhouse gas *** this review,we first elucidate the fundamental principles of cooperative photoredox integration of H_(2)O_(2)synthesis and selective organic oxidation with simultaneous utilization of photoexcited electrons and holes over semiconductor-based ***,a thorough review on the recent advancements of cooperative photoredox synthesis of H_(2)O_(2)and value-added chemicals is ***,in-depth discussions and insights into the techniques for unravelling the photoredox reaction mechanisms are ***,critical challenges and prospects in this thriving field are comprehensively *** is envisioned that this review will serve as a pivotal guidance on the rational design of such dual-functional photocatalytic system,thereby further stimulating the development of economical and environmentally benignH_(2)O_(2)and high-value chemicals production.

关键词： cooperative photoredox synthesis dual-functional photocatalysts H_(2)O_(2) photocatalysis selective organic oxidation

Extreme Responses of An Integrated System with A Semi-Submersible Wind Turbine and Four Torus-Shaped Wave Energy converters in different Survival Modes

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china Ocean Engineering 2024年第5期38卷 877-892页

作者： WANG Kai LI Yu-meng ong Muk chen WAN Ling LI Liang-bi cHENG Zheng-shun School of Ocean Engineering and Technology Sun Yat-sen University & Southern Marine Science and Engineering Guangdong Laboratory (Zhuhai) School of Naval Architecture and Ocean Engineering Jiangsu University of Science and Technology department of Mechanical and Structural Engineering and Materials Science University of Stavanger Faculty of Maritime and Transportation Ningbo University State Key Laboratory of Ocean Engineering Shanghai Jiao Tong University SJTU Yazhou Bay Institute of deepsea Science and Technology

Offshore wind power is a kind of important clean renewable energy and has attracted increasing attention due to the rapid consumption of non-renewable energy. To reduce the high cost of energy, a possible try is to utilize the combination of wind and wave energy considering their natural correlation. A combined concept consisting of a semi-submersible wind turbine and four torus-shaped wave energy converters was proposed and numerically studied under normal operating conditions. However, the dynamic behavior of the integrated system under extreme sea conditions has not been studied yet. In the present work, extreme responses of the integrated system under two different survival modes are evaluated. Fully coupled time-domain simulations with consideration of interactions between the semi-submersible wind turbine and the torus-shaped wave energy converters are performed to investigate dynamic responses of the integrated system, including mooring tensions, tower bending moments, end stop forces, and contact forces at the column-Torus interface. It is found that the addition of four tori will reduce the mean motions of the yaw, pitch and surge. When the tori are locked at the still water line, the whole integrated system is more suitable for the survival modes.

关键词： combined wind and wave energy concept extreme response survival mode wave energy converter

Near resonance vibration isolation on a levered-dual response(LEdAR)coulomb-damped system by differential preloads/offsets in linear springs

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Applied Mathematics and Mechanics(English Edition) 2024年第6期45卷 1033-1050页

作者： T.I.TOLUWALOJU c.K.THEIN d.HALIM department of Mechanical Materials and Manufacturing EngineeringUniversity of Nottingham Ningbo ChinaNingbo 315100Zhejiang ProvinceChina Nottingham Ningbo china Beacons of Excellence Research and Innovation Institute University of Nottingham Ningbo ChinaNingbo 315048Zhejiang ProvinceChina

The levered-dual response(LEdAR)coulomb-damped system attains near resonant vibration isolation by differential preloads/offsets in linear *** takes the advantages of both the preloads/offsets in linear springs and the guiderail friction for realizing different levels of vibration *** isolation capacities are investigated on the strategies with both the horizontal and vertical guiderails,with the horizontal rail only,and without *** compressive preloads generally result in the consumption of most of the initial excitation energy so as to overcome the potential *** isolation onsets at the frequency ratio of 1∓0.095 on the left-hand side(LHS)and the right-hand side(RHS)of the lever are relative to the load plate *** observed near resonant isolation thus makes the LEdAR system a candidate for the isolation of the mechanical systems about resonance while opening a path for simultaneous harvesterisolation functions and passive functions at extreme frequencies.

关键词： lever ratio coulomb damping preload tension/compression isolation band/depth offset potential

Guest Editorial:Special issue on advances in representation learning for computer vision

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cAAI Transactions on Intelligence Technology 2024年第1期9卷 1-3页

作者： Andrew Beng Jin Teoh Thian Song ong Kian Ming Lim chin Poo Lee Electrical and Electronic Engineering department Yonsei UniversitySeoulSouth Korea Faculty of Information Science and Technology Multimedia UniversityMelakaMalaysia

deep learning has been a catalyst for a transformative revo-lution in machine learning and computer vision in the past *** these research domains,methods grounded in deep learning have exhibited exceptional performance across a spectrum of *** success of deep learning methods can be attributed to their capability to derive potent representations from data,integral for a myriad of downstream *** representations encapsulate the intrinsic structure,fea-tures,or latent variables characterising the underlying statistics of visual *** these achievements,the challenge per-sists in effectively conducting representation learning of visual data with deep models,particularly when confronted with vast and noisy *** special issue is a dedicated platform for researchers worldwide to disseminate their latest,high-quality articles,aiming to enhance readers'comprehension of the principles,limitations,and diverse applications of repre-sentation learning in computer vision.

关键词： spite computer representation

Prescribed-Time Nash Equilibrium Seeking for Pursuit-Evasion Game

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IEEE/cAA Journal of Automatica Sinica 2024年第6期11卷 1518-1520页

作者： Lei Xue Jianfeng Ye Yongbao Wu Jian Liu d.c.Wunsch Key Laboratory of Measurement and control of complex Systems of Engineering Ministry of EducationNanjing 210096 School of Automation Southeast UniversityNanjing 210096China department of Electrical and computer Engineering Missouri University of Science and TechnologyRollaMO 65409 USA IEEE

dear Editor,This letter is concerned with prescribed-time Nash equilibrium(PTNE)seeking problem in a pursuit-evasion game(PEG)involving agents with second-order *** order to achieve the prior-given and user-defined convergence time for the PEG,a PTNE seeking algorithm has been developed to facilitate collaboration among multiple pursuers for capturing the evader without the need for any global ***,it is theoretically proved that the prescribedtime convergence of the designed algorithm for achieving Nash equilibrium of ***,the effectiveness of the PTNE method was validated by numerical simulation results.A PEG consists of two groups of agents:evaders and *** pursuers aim to capture the evaders through cooperative efforts,while the evaders strive to evade *** is a classic noncooperative *** has attracted plenty of attention due to its wide application scenarios,such as smart grids[1],formation control[2],[3],and spacecraft rendezvous[4].It is noteworthy that most previous research on seeking the Nash equilibrium of the game,where no agent has an incentive to change its actions,has focused on asymptotic and exponential convergence[5]-[7].

关键词： seeking prescribed convergence

Recent advances in graphene-based phase change composites for thermal energy storage and management

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Nano Materials Science 2024年第2期6卷 115-138页

作者： Qiang Zhu Pin Jin ong Si Hui Angela Goh Reuben J.Yeo Suxi Wang Zhiyuan Liu Xian Jun Loh Institute of Materials Research and Engineering A*STAR(Agency for ScienceTechnology and Research)2 Fusionopolis WayInnovis#08-03138634Singapore Institute of Sustainability for chemicals Energy and EnvironmentA*STAR(Agency for ScienceTechnology and Research)1 Pesek RoadJurong Island627833Singapore School of chemistry Chemical Engineering and BiotechnologyNanyang Technological University21 Nanyang Link637371Singapore Shenzhen Institutes of Advanced Technology(SIAT) Chinese Academy of Sciences(CAS)1068 Xueyuan AvenueShenzhen518055China department of Material Science and Engineering National University of Singapore9 Engineering Drive 1#03-09 EA117575Singapore

Energy storage and conservation are receiving increased attention due to rising global energy ***,the development of energy storage materials is *** energy storage(TES)systems based on phase change materials(PcMs)have increased in prominence over the past two decades,not only because of their outstanding heat storage capacities but also their superior thermal energy regulation ***,issues such as leakage and low thermal conductivity limit their applicability in a variety of ***-based materials such as graphene and its derivatives can be utilized to surmount these *** study examines the recent advancements in graphene-based phase change composites(Pccs),where graphene-based nanostructures such as graphene,graphene oxide(GO),functionalized graphene/GO,and graphene aerogel(GA)are incorporated into PcMs to substantially enhance their shape stability and thermal conductivity that could be translated to better storage capacity,durability,and temperature response,thus boosting their attractiveness for TES *** addition,the applications of these graphene-based Pccs in various TES disciplines,such as energy conservation in buildings,solar utilization,and battery thermal management,are discussed and summarized.

关键词： Phase change material Nanocomposites Solar energy Sustainable energy Thermo-regulation