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Organic additives in all-inorganic perovskite solar cells and modules:from moisture endurance to enhanced efficiency and operational stability

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Journal of Energy Chemistry 2022年第4期31卷 361-390页

作者： Yameen Ahmed bilawal khan MBilal Faheem Keqing Huang Yuanji Gao Junliang Yang State Key Laboratory of Powder Metallurgy School of Physics and ElectronicsCentral South UniversityChangsha 410083HunanChina Department of Materials Science and Engineering City University of HongkongHongkong SAR 999077China Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054SichuanChina

Power conversion efficiency(PCE) of perovskite solar cells(PSC) has been skyrocketed to certified 25.5% owing to their improved and tunable optoelectronic properties. Although, various strategies have been adopted to date regarding PCE and stability enhancement within PSC technology, certain instability factors(moisture, heat, light) are hindering their commercial placement. Recently, all-inorganic PSCs got hype in the photovoltaic research community after they attained PCE > 20% and due to their significant endurance against heat and light mishmashes, but there only left moisture sensitivity as the only roadblock for their industrial integration. Here, we review the recent progress of additive inclusion into allinorganic(CsPbX_(3)) PSCs to stabilize their intrinsic structure and to withstand the performance limiting factors. We start with the detailed description of chemical instability of different perovskite compositions, phase segregation, and how organic molecules and dyes help to repair the structural defects to improve the overall PCE and stability of PSCs. Moisture endurance as a result of chemical passivation through organic additives, low-dimensional inorganic PSCs to enhance device stability and scalable fabrication of CsPbX_(3) PSCs are also reviewed. The challenges of module degradation and design implications with proposed strategies and outlook are interpreted in the ending phrases of this review.

关键词： Perovskite solar cells Organic additives Chemical instability Phase segregation Modules

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