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The effect of long-term application of nitrogen-rich fertilizers on soil resistome:A study of conventional and organic cropping systems

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soil Ecology Letters 2024年第3期6卷 135-150页

作者： alexey s.vasilchenko Evgenii O.Burlakov Darya V.Poshvina Denis s.Gruzdev sergey V.Kravchenko Aleksandr V.Iashnikov Ning Ling Anastasia V.vasilchenko Laboratory of Antimicrobial Resistance Institute of Environmental and Agricultural Biology(X-BIO)Tyumen State UniversityTyumenRussia Research Institute of Mathematics Physics and Computer ScienceDerzhavin Tambov State UniversityTambovRussia International Integrated Research Laboratory for Climate Change Land Use and BiodiversityInstitute of Environmental and Agricultural Biology(X-BIO)Tyumen State UniversityTyumenRussia sciBear OU Tartu Mnt 67/1-13bKesklinna Linnaosa10115 TallinnEstonia Center for Grassland Microbiome State Key Laboratory of Grassland Agro-EcosystemsCollege of Pastoral Agriculture Science and TechnologyLanzhou UniversityLanzhou 730000China

Metagenomic studies of various soil environments have previously revealed the widespread distribution of antibiotic resistance genes(ARGs)around the *** this study,we applied shotgun metagenomics to investigate differences in microbial communities and resistomes in Chernozem soils that have been under long-term organic and conventional cropping *** organic cropping system was seeded with Triticum spelta without any *** conventional cropping system was seeded with Tríticum durum Desf and used mineral fertilizer(NPK),that resulted in an increased amount of total and available carbon and nitrogen in *** all samples,we identified a total of 21 ARG classes,among which the dominant were vancomycin,tetracycline and *** of soil microbial communities revealed differences between the studied fields in the relative abundances of 14 and 53 genera in topsoil and subsoil,*** analysis showed significant correlations(positive and negative)among 18 genera and 6 ARGs,as well as between these ARGs and some chemical properties of *** analysis of metagenome-assembled genomes revealed that Nitrospirota,Thermoproteota,Actinobacteriota and Binatota phyla of archaea and bacteria serve as hosts for glycopeptide and fluoroquinolone/tetracycline ***,the data obtained enrich knowledge about the consequences of human agricultural activities in terms of soil microbiome modification and highlight the role of nitrogen cycling taxa,including uncultivated genera,in the formation of soil resistome.

关键词： soil microbiome inorganic fertilizer nitrogen cycle uncultured bacteria chemolithotrophs Binatia

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Effect of sodium nitroprusside on the microrheological properties of red blood cells in di®erent media

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Journal of Innovative Optical Health sciences 2024年第5期17卷 23-31页

作者： Petr Ermolinskiy Matvey Maksimov Andrei Lugovtsov alexey Muravyov Irina Tikhomirova Alexander Priezzhev Faculty of Physics M.V.Lomonosov Moscow State University Moscow 119991Russia Faculty of Physical Education K.D.Ushinsky Yaroslavl state Pedagogical University Yaroslavl 150000 Russia Faculty of Natural sciences K.D.Ushinsky Yaroslavl state Pedagogical University Yaroslavl 150000 Russia

Red blood cell(RBC)aggregation as well as their deformation signi¯cantly affects blood *** processes depend on various factors,one of which is concentration of the nitric oxide,one of the main signaling molecule in the *** purpose of this study was to investigate the effect of nitric oxide on the microrheological properties of red blood cells(RBCs)in RBC samples of various media after the addition of nitric oxide donor sodium nitroprusside in *** properties were measured using laser aggregometer and ektacytometer based on diffuse light scattering and diffraction of laser light on a suspension of RBCs,*** study found that heparin-stabilized blood showed increased RBC aggregation and deformation with sodium nitroprusside concentrations of 100,and 200M,while EDTA-stabilized blood showed slightly decreased aggregation and unchanged *** washed RBCs in dextran solution,the addition of sodium nitroprusside(in the concentrations of 100,and 200M)resulted in decreased aggregation and increased ***-ndings aid in our understanding of nitric oxide's effect on RBC microrheological properties.

关键词： sodium nitroprusside nitric oxide red blood cells RBC aggregation diffuse light scattering laser diffractometer

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Irisin/BDNF signaling in the muscle-brain axis and circadian system: A review

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The Journal of Biomedical Research 2024年第1期38卷 1-16页

作者： alexey N.Inyushkin Vitalii s.Poletaev Elena M.Inyushkina Igor s.Kalberdin Andrey A.Inyushkin Department of Human&Animal Physiology Samara National Research UniversitySamara 443011Russia.

In mammals,the timing of physiological,biochemical and behavioral processes over a 24-h period is controlled by circadian *** entrain the master clock located in the suprachiasmatic nucleus of the hypothalamus to a precise 24-h rhythm,environmental zeitgebers are used by the circadian *** is done primarily by signals from the retina via the retinohypothalamic tract,but other cues like exercise,feeding,temperature,anxiety,and social events have also been shown to act as non-photic *** recently identified myokine irisin is proposed to serve as an entraining non-photic signal of *** is a product of cleavage and modification from its precursor membrane fibronectin typeⅢdomain-containing protein 5(FNDC5)in response to *** from well-known peripheral effects,such as inducing the"browning"of white adipocytes,irisin can penetrate the blood-brain barrier and display the effects on the *** data suggest that FNDC5/irisin mediates the positive effects of physical activity on brain *** several brain areas,irisin induces the production of brain-derived neurotrophic factor(BDNF).In the master clock,a significant role in gating photic stimuli in the retinohypothalamic synapse for BDNF is ***,the brain receptor for irisin remains *** the current review,the interactions of physical activity and the irisin/BDNF axis with the circadian system are reconceptualized.

关键词： irisin brain-derived neurotrophic factor peroxisome proliferator-activated receptorγcoactivator 1α circadian rhythm circadian system muscle-brain axis

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Gradient-induced long-range optical pulling force based on photonic band gap

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Light(science & Applications) 2024年第5期13卷 865-874页

作者： Wenlong Lu alexey V.Krasavin sheng Lan Anatoly V.Zayats Qiaofeng Dai Guangdong Basic Research Center of Excellence for structure and Fundamental Interactions of Matter Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and DevicesSchool of Information and Optoelectronic Science and EngineeringSouth China Normal UniversityGuangzhou 510006China Department of Physics and London Centre for Nanotechnology King’s College LondonLondon WC2R 2LSUK

Optical pulling provides a new degree of freedom in optical *** is generally believed that long-range optical pulling forces cannot be generated by the gradient of the incident ***,we theoretically propose and numerically demonstrate the realization of a long-range optical pulling force stemming from a self-induced gradient field in the manipulated *** analogy to potential barriers in quantum tunnelling,we use a photonic band gap design in order to obtain the intensity gradients inside a manipulated object placed in a photonic crystal waveguide,thereby achieving a pulling *** the usual scattering-type optical pulling forces,the proposed gradient-field approach does not require precise elimination of the reflection from the manipulated *** particular,the Einstein-Laub formalism is applied to design this unconventional gradient *** magnitude of the force can be enhanced by a factor of up to 50 at the optical resonance of the manipulated object in the waveguide,making it insensitive to *** developed approach helps to break the limitation of scattering forces to obtain longrange optical pulling for manipulation and sorting of nanoparticles and other *** developed principle of using the band gap to obtain a pulling force may also be applied to other types of waves,such as acoustic or water waves,which are important for numerous applications.

关键词： optical waveguide scattering

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Electric tuning of plasmonic resonances in ultrathin gold nanoribbon arrays

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Photonics Research 2024年第8期12卷 1750-1759页

作者： ZHENXIN WANG alexey VKRAsAVIN CHENXINYU PAN JUNsHENG ZHENG ZHIYONG LI XIN GUO ANATOLY VZAYATs LIMIN TONG PAN WANG state Key Laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringZhejiang UniversityHangzhou 310027China Department of Physics and London Centre for Nanotechnology King’s College LondonStrandLondon WC2R 2LSUK Jiaxing Key Laboratory of Photonic sensing&Intelligent Imaging Intelligent Optics&Photonics Research CenterJiaxing Research Institute Zhejiang UniversityJiaxing 314000China

Ultrathin plasmonic nanostructures offer an unparalleled opportunity for the study of light–matter interactions at the nanoscale and realization of compact nanophotonic *** this study,we introduce an ultrathin gold nanoribbon array and demonstrate an electric approach to actively tuning its plasmonic resonance,which leveraging the extreme light confinement capability in the ultrathin plasmonic nanostructure and a robust nanoscale electro-optical effect in indium tin *** the design(to a total thickness as small as 12 nm for a 2-nmthick gold nanoribbon array),we numerically demonstrate a spectral shift in the plasmonic resonance up to 36 nm along with an approximately 16%change in the transmission at a gate voltage below 1.7 V at the wavelength of1.47μ*** work presents progress towards electric tuning of plasmonic resonances in ultrathin metallic nanostructures for various applications including surface-enhanced spectroscopy,spontaneous emission enhancement,and optical modulation.

关键词： plasmon tuning realization

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Insights into the hydrogen evolution reaction in vanadium redox flow batteries:A synchrotron radiation based X-ray imaging study

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Journal of Energy Chemistry 2024年第4期91卷 132-144页

作者： Kerstin Köble alexey Ershov Kangjun Duan Monja schilling Alexander Rampf Angelica Cecilia TomášFaragó Marcus Zuber Tilo Baumbach Roswitha Zeis Helmholtz Institute Ulm Karlsruhe Institute of Technology89081 UlmGermany Laboratory for Applications of synchrotron Radiation Karlsruhe Institute of Technology76131 KarlsruheGermany Institute for Photon science and synchrotron Radiation Karlsruhe Institute of Technology76344 Eggenstein-LeopoldshafenGermany Department of Electrical Electronicsand Communication EngineeringFaculty of EngineeringFriedrich-Alexander-Universität Erlangen-Nürnberg(FAU)91058 ErlangenGermany Department of Mechanical and Industrial Engineering University of TorontoToronto M5S 3G8OntarioCanada

The parasitic hydrogen evolution reaction(HER)in the negative half-cell of vanadium redox flow batteries(VRFBs)causes severe efficiency ***,a deeper understanding of this process and the accompanying bubble formation is *** benchmarking study locally analyzes the bubble distribution in thick,porous electrodes for the first time using deep learning-based image segmentation of synchrotron X-ray *** large three-dimensional data set was processed precisely in less than one minute while minimizing human errors and pointing out areas of increased HER activity in *** study systematically varies the electrode potential and material,concluding that more negative electrode potentials of-200 m V *** hydrogen electrode(RHE)and lower cause more substantial bubble formation,resulting in bubble fractions of around 15%–20%in carbon felt ***,the bubble fractions stay only around 2%in an electrode combining carbon felt and carbon *** detected areas with high HER activity,such as the border subregion with more than 30%bubble fraction in carbon felt electrodes,the cutting edges,and preferential spots in the electrode bulk,are potential-independent and suggest that larger electrodes with a higher bulk-to-border ratio might reduce HER-related performance *** described combination of electrochemical measurements,local X-ray microtomography,AI-based segmentation,and 3D morphometric analysis is a powerful and novel approach for local bubble analysis in three-dimensional porous electrodes,providing an essential toolkit for a broad community working on bubble-generating electrochemical systems.

关键词： Vanadium redox flow battery synchrotron X-ray imaging Tomography Hydrogen evolution reaction Gas bubbles Deep learning

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Elucidating elusive quaternary selenide EuCeCuse3:synthesis,crystal structure,properties and theoretical studies

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Journal of Rare Earths 2024年第1期42卷 163-171,I0006页

作者： Maxim V.Grigoriev Anna V.Ruseikina Maxim s.Molokeev Vladimir A.Chernyshev Aleksandr s.Aleksandrovsky Alexander s.Krylov svetlana N.Krylova Nikolai P.shestakov Dmitriy A.Velikanov Alexander A.Garmonov alexey V.Matigorov Evgeny A.Ostapchuk Thomas schleid Damir A.safin Laboratory of Theory and Optimization of Chemical and Technological Processes University of TyumenVolodarskogo Str.6625003TyumenRussian Federation Kirensky Institute of Physics Federal Research Center KSC SB RASAkademgorodok 50 Bld.38660036KrasnoyarskRussian Federation Department of Physics Far Eastern State Transport UniversitySerysheva Str.47680021KrasnoyarskRussian Federation Institute of Natural sciences and Mathematics Ural Federal University Named After the First President of Russia B.N.YeltsinMira Str.19620002EkaterinburgRussian Federation Department of Photonics and Laser Technology Siberian Federal UniversitySvobodnii Ave.79660079KrasnoyarskRussian Federation Institute of Physics and Technology University of TyumenVolodarskogo Str.6625003 TyumenRussian Federation Institute for Inorganic Chemistry University of StuttgartPfaffenwaldring 55D-70569StuttgartGermany scientific and Educational and Innovation Center for Chemical and Pharmaceutical Technologies Ural Federal University named after the First President of Russia B.N.YeltsinMira Str.19620002 EkaterinburgRussian Federation University of Tyumen Volodarskogo Str.6625003TyumenRussian Federation

We report on the novel heterometallic quaternary selenide EuCeCuse3,the fabrication of which has been a challenge until this *** structure of the reported selenide was elucidated from the powder X-ray diffraction data,which revealed the formation of EuCeCuse3with excellent yield(96.7%)accompanied with a minor fraction of Cese2(3.3%),and was best solved in orthorhombic space group Pnma with the BaLaCus3structural ***,the crystal structure of the title compound completes the row of the heterometallic quaternary selenides EuRECuse3(RE=La,Pr,Nd,sm,Eu,Gd,Tb,Dy,Ho,Er,Tm,Yb,Lu,Y),of which the cerium-based derivative exclusively belongs to the BaLaCus3structural *** distortion of the Cuse4polyhedron was compared for the whole series of EuRECuse3compounds using theτ4-descriptor for four coordinated ions,which revealed the highest degree of distortion for the Ce3+-containing selenide,followed by the La3+-based ***,the crystallographic and geometrical parameters of the reported selenide were discussed in comparison to the Ce3+-based sulfides srCeCus3and *** initio calculations of the crystal structure,a phonon spectrum and elastic constants for the crystal of EuCeCuse3were also *** types and wavenumbers of fundame ntal modes were determined and the involvement of ions participating in the phonon modes was *** experimental IR spectrum of the reported selenide was interpreted and found to be in agreement with the calculated *** experimental direct band gap of EuCeCuse3was measured to be 1.36 eV that is consistent with the concept of its origin due to interband transitions between orbitals emerging mainly from 4f(valence band)and 5d(conduction band)levels of the Eu2+*** dependence of the Young’s modulus on the direction demonstrates the anisotropy of the elastic properties,while the Vickers hardness for EuCeCuse3was calculated to be 5.2 ***,the title compound is paramagnetic above 4 K.

关键词： Quaternary selenide synthesis Crystal structure Ab initio calculations Magnetic measurements spectroscopy

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A high-power electromagnetic source for disabling improvised explosive devices

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High Voltage 2024年第2期9卷 403-409页

作者： Laurent Ariztia Njomza Ibrahimi alexey Zhabin Antoine silvestre de Ferron Marc Rivaletto Edson Martinod Valérie Bertrand Bucur Novac Laurent Pécastaing Universite de Pau et des Pays de l’Adour E2S UPPASIAMEPauFrance XLIM UMR CNRS BriveLimogesFrance CIsTEME LimogesFrance Wolfson school of Mechanical Electrical and Manufacturing EngineeringLoughborough UniversityLoughboroughLeicestershireUK

Ultra-wideband(UWB)microwave sources driven by specialised pulsed power generators have experienced a considerable development in the last decade due to their wide domain of new applications such as defence or counter-terrorism *** authors present the main findings of a research dedicated to the development of a pulsed power-driven electromagnetic field source for disabling improvised explosive devices(IED).The pulsed power generator driving the source is a 13-stage compact Marx producing voltage pulses reaching an amplitude of 0.5 MV,with a pulse repetition frequency(PRF)of up to 100 *** generator is coupled to a bipolar pulse forming line,providing bipolar pulses with a dV/dt of around 1.6 MV/*** pulsed power system feeds an array composed of 16 Koshelev-type UWB antennas through an impedance matching *** resulting electromagnetic source is capable to produce pulsed electric fields(PEFs)having a figure-of-merit(FOM)of 1 ***,practical experiments were carried out to study the effects of the PEFs on *** targets used in the present study are M2B type flashbulbs,known to have the same susceptibility as the Us army M6 *** configurations of wires(shielded,twisted,etc)with different lengths were used in connecting items inside these *** tests were performed by placing the flashbulbs at different distances to determine the essential parameters(i.e.,amplitude,duration,and frequency range)of the PEFs required to trigger *** overview of the experimental campaign and the main findings are also presented followed by conclusions.

关键词： power bipolar source

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Expanded Porphyrin Exhibiting Off-Centered Out-of-Plane Coordination to Dysprosium

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CCs Chemistry 2024年第7期6卷 1731-1738页

作者： Dmitry I.Nazarov Jorge Labella alexey V.Kuzmin Maxim A.Faraonov Evgenii N.Ivanov salavat s.Khasanov Tomas Torres Mikhail K.Islyaikin Dmitri V.Konarev Federal Research Center of Problems of Chemical Physics and Medicinal Chemistry RAs 142432 Chernogolovka Department of Organic Chemistry Universidad Autonoma de Madrid28049 Madrid Institute of solid-state Physics RAs 142432 Chernogolovka Research Institute of Macroheterocycles Ivanovo State University of Chemistry and Technology15300 Ivanovo G.A.Krestov Institute of solution Chemistry of the Russian Academy of sciences 153045 Ivanovo Institute for Advanced Research in Chemical sciences Universidad Autonoma de Madrid28049 Madrid IMDEA-Nanociencia 28049 Madrid

The complexation of high-spin lanthanides to porphyrinoids is a powerful strategy for the development of advanced molecular *** this context,the use of expanded porphyrinoids remains elusive since their coordination chemistry is challenging to ***,taking inspiration from on-surface chemistry,we explored the coordination of Dy^(3+)to a six-membered porphyrinoid,namely,the hemihexaphyrazine ***,we observed the selective formation of a mono-nuclear off-centered,out-of-plane H_(2)Hhp-Dy^(3+)complex when performing the complexation under reductive *** this reaction,the oxidation state of the macrocycle did not *** X-ray diffraction analysis,we found that the coordination number of Dy in this complex was *** macrocycle cocrystallized with decamethylcobaltocene(Cp_(2)^(*)Co)molecules,giving rise to a wellordered solid-state packing,governed byπ-π*** a result of this organization,a small magnetic coupling between the neighboring molecules was *** in all,this work provides key insights into the coordination of magnetically active metals with expanded porphyrinoids,thus motivating the development of advanced spintronic devices.

关键词： porphyrins dysprosium macrocycle coordination chemistry magnetism

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基于人地关系的东北农村空心化测度及其整治路径研究——以黑龙江省拜泉县为例

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地理科学进展 2024年第3期43卷 488-503页

作者：张茹杜国明李玉恒王玲 Monika stanny alexey Naumov 东北农业大学公共管理与法学院哈尔滨150030 中国科学院地理科学与资源研究所区域可持续发展分析与模拟重点实验室北京100101 中国科学院大学资源与环境学院北京100049 黑龙江省自然资源权益调查监测院哈尔滨150030 波兰科学院农村与农业发展研究所波兰华沙00-3306 罗蒙诺索夫莫斯科国立大学俄罗斯莫斯科119991

快速城镇化进程中,人口大规模流失引发乡村人地关系失衡,加剧了村庄空心化问题。科学测度乡村空心化、提出以乡村振兴为导向的空心村整治策略,具有重要的现实意义。论文以黑龙江省拜泉县为例,基于人口转移率测度了乡村空心化水平,运用熵... 详细信息

快速城镇化进程中,人口大规模流失引发乡村人地关系失衡,加剧了村庄空心化问题。科学测度乡村空心化、提出以乡村振兴为导向的空心村整治策略,具有重要的现实意义。论文以黑龙江省拜泉县为例,基于人口转移率测度了乡村空心化水平,运用熵权TOPsIs法评价了村庄发展潜力水平,将二者结合识别了村庄发展类型,提出差异化的空心村整治策略。研究结果显示:(1)拜泉县乡村空心化水平均值为0.6529,空心化程度明显。乡镇层面的空心化处于中度和高度水平,村庄以高度和重度空心化为主。农村人口流失主要归因于城乡建设不均衡、农村就业机会少、农村社会保障水平偏低等。(2)村庄发展潜力均值为0.2279,整体水平偏低且空间分布差异明显,县城周边、沿主要交通干线以及主要河流的村庄发展潜力水平普遍高于偏远地区的村庄。产业兴旺(0.5026)水平显著高于乡风文明(0.2703)、生态宜居(0.1472),治理有效(0.0317)、生活富裕(0.0482)水平较低,成为村庄发展潜力的短板。(3)拜泉县村庄类型划分为Ⅰ类——高潜力低空心化、Ⅱ类——高潜力高空心化、Ⅲ类——低潜力低空心化、Ⅳ类——低潜力高空心化4类,整体以Ⅱ类——高潜力高空心化为主,且县域南部村庄发展状态好于北部地区。未来村庄发展应以乡村振兴战略为指引,重心向Ⅰ类、Ⅱ类以及南部村镇转移,并完善宅基地、生态用地、耕地等相关制度体系,促进村庄内部结构调整;培育合作社、家庭农场等新型经营主体,探索特色产业规划与升级道路;构建“中心镇—中心村—农民社区—村庄”的新型村镇体系,加强城乡互动,促进要素聚集、资源共享;同时加大环境整治,增强社会保障,吸引人才回归,实现空心化治理与县域乡村振兴。

关键词：乡村振兴人地关系村庄空心化潜力评价村庄发展黑龙江省拜泉县

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