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Remarkable enhancement of gas selectivity on organosilica hybrid membranes using urea-modulated metal-organic framework nanoparticles

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 83-92页

作者： Yayun zhao Dechuan zhao chunlong Kong Yichao Lin Xuezhen Wang Liang Chen Key Laboratory of Advanced Fuel Cells and Electrolyzers Technology of Zhejiang Province Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201China University of Chinese Academy of Sciences Beijing 100049China Collaboration Innovation Center for Tissue Repair Material Engineering Technology China West Normal UniversityNanchong 637009China

Metal-organic framework/organosilica hybrid membranes on tubular ceramic substrates have shown great potential for the implementation of membrane technology in practical gas separation projects due to their higher permeance compared to commercial ***,the selectivities of the reported membranes are ***,we have incorporated urea-modulated metal-organic frameworks into organosilica membranes to greatly enhance its separation *** urea-modulated metal-organic frameworks exhibit less-defined edges of crystallographic facets and high defect *** can be well-dispersed in the organosilica layer,which substantially suppresses the interfacial defects between metal-organic frameworks and organosilica,which is beneficial for improving the selectivity of membranes for gas *** results have shown that the enhanced ideal selectivity of H_(2)/CH_(4) was 165 and that of CO_(2)/CH_(4) was 43,with H_(2) permeance of about 1.25×10^(−6) mol·m^(−2)·s^(−1)·Pa^(−1) and CO_(2) permeance of 3.27×10^(−7) mol·m^(−2)·s^(−1)·Pa^(−1) at 0.2 MPa and 25℃.In conclusion,the high level of hybrid membranes can be used to separate H_(2)(or CO_(2))from the binary gas mixture H_(2)/CH_(4)(or CO_(2)/CH_(4)),which is important for gas separation in practical ***,the simple and feasible modulation of metal-organic framework is a promising strategy to tune different metal-organic frameworks for membranes according to the actual demands.

关键词： ZIF-8 nanocrystals urea organosilica hybrid membrane enhanced separation performance

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Singularity analysis and avoidance for an SSRMS-type reconfigurable space manipulator with a non-spherical wrist and two lockable passive telescopic links

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Chinese Journal of Aeronautics 2024年第8期37卷 435-459页

作者： Zhiyuan zhao Xiaohang YANG Yuntao LI Zichun XU Jingdong zhao Hong LIU State Key Laboratory of Robotics and System Harbin Institute of TechnologyHarbin 150001China

This study focuses on addressing kinematic singularity analysis and avoidance issues for a space station remote manipulator system(SSRMS)-type reconfigurable space *** manipulator is equipped with a non-spherical wrist and two lockable passive telescopic links(LPTLs),which enable it to have both active revolute and passive prismatic joints and operate in two distinct *** begin with the kinematic singularity analysis,the study derives the differential kinematic equations for the manipulator and identifies the dominant Jacobian matrix that causes ***,an in-depth analysis of singularities from multiple perspectives is ***,a kinematic singularity map method is proposed to capture the distribution of singularities within the reachable ***,the influence of the two LPTLs on singularities is thoroughly ***,a new method based on the matrix rank equivalence principle is introduced to determine singularity conditions,enabling the identification of all the singular configurations for the SSRMS-type reconfigurable ***,this method significantly reduces computational complexity,and the singularity conditions obtained have more concise *** the singularity avoidance problem,a novel method is developed,which simultaneously addresses the requirements of real-time performance,high precision,and the avoidance of both kinematic singularities and joint limit *** from these excellent properties,the proposed method can effectively resolve the singularity issues encountered separately by the SSRMS-type reconfigurable manipulator in its two operational *** typical simulations validate the utility of all the proposed methods.

关键词： Reconfigurable space manipulator Redundant manipulator Kinematics Singularity analysis Singularity avoidance

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Tribological properties of low-temperature time-dependent pretreated graphite for mechanical seal pairs in high-speed turbopump

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Friction 2024年第2期12卷 305-318页

作者： Yangyang zhao Guoyuan ZHANG Junqian WANG He WANG Weigang zhao Qunfeng ZENG School of Mechano-Electronic Engineering Xidian UniversityXi’an 710071China Xi’an Aerospace Propulsion Institute Xi’an 710071China Key Laboratory of Education Ministry for Modern Design and Rotor-Bearing System Xi’an Jiaotong UniversityXi’an 710049China

The friction coefficient and wear rate of pretreated graphite with liquid nitrogen were obtained by using a ball-on-disk tester,and the wear of GCr15–graphite seal pairs with the low-temperature time-dependent pretreatment was discussed by comparing the wear *** results show that liquid nitrogen pretreatment can affect the hardness and interlayer spacing of *** range of the friction coefficients of pretreated graphite changes from 0.17 to *** the increase of liquid nitrogen pretreatment time,the wear mechanism of graphite would change from dominated three-body wear to adhesion *** experimental results of the mechanical seal with liquid nitrogen pretreatment show that the wear rate of stator is less than 0.00165 mm^(3)·N^(−1)·m^(−1),and the graphite shows a good low-temperature compatibility.

关键词： graphite low-temperature pretreatment mechanical seal friction and wear

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An Environment‑Tolerant Ion‑Conducting Double‑Network Composite Hydrogel for High‑Performance Flexible Electronic Devices

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Nano-Micro Letters 2024年第5期16卷 352-369页

作者： Wenchao zhao Haifeng Zhou Wenkang Li Manlin Chen Min Zhou Long zhao State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074People’s Republic of China

High-performance ion-conducting hydrogels(ICHs)are vital for developing flexible electronic ***,the robustness and ion-conducting behavior of ICHs deteriorate at extreme tempera-tures,hampering their use in soft *** resolve these issues,a method involving freeze–thawing and ionizing radiation technology is reported herein for synthesizing a novel double-network(DN)ICH based on a poly(ionic liquid)/MXene/poly(vinyl alcohol)(PMP DN ICH)*** well-designed ICH exhibits outstanding ionic conductivity(63.89 mS cm^(-1) at 25℃),excellent temperature resistance(-60–80℃),prolonged stability(30 d at ambient temperature),high oxidation resist-ance,remarkable antibacterial activity,decent mechanical performance,and ***,the ICH performs effectively in a flexible wireless strain sensor,thermal sensor,all-solid-state supercapacitor,and single-electrode triboelectric nanogenerator,thereby highlighting its viability in constructing soft electronic *** highly integrated gel structure endows these flexible electronic devices with stable,reliable signal output *** particular,the all-solid-state supercapacitor containing the PMP DN ICH electrolyte exhibits a high areal specific capacitance of 253.38 mF cm^(-2)(current density,1 mA cm^(-2))and excellent environmental *** study paves the way for the design and fabrication of high-performance mul-tifunctional/flexible ICHs for wearable sensing,energy-storage,and energy-harvesting applications.

关键词： Ionic liquids Double-network hydrogels Temperature tolerance Multifunctionality Flexible electronic devices

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面向全量测点耦合结构分析与估计的工业过程监测方法

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自动化学报 2024年第8期50卷 1517-1538页

作者：赵健程赵春晖浙江大学控制科学与工程学院杭州310027

实际工业场景中,需要在生产过程中收集大量测点的数据,从而掌握生产过程运行状态.传统的过程监测方法通常仅评估运行状态整体的异常与否,或对运行状态进行分级评估,这种方式并不会直接定位故障部位,不利于故障的高效检修.为此,提出一种... 详细信息

实际工业场景中,需要在生产过程中收集大量测点的数据,从而掌握生产过程运行状态.传统的过程监测方法通常仅评估运行状态整体的异常与否,或对运行状态进行分级评估,这种方式并不会直接定位故障部位,不利于故障的高效检修.为此,提出一种基于全量测点估计的监测模型,根据全量测点估计值与实际值的偏差定义监测指标,从而实现全量测点的分别精准监测.为克服原有的基于工况估计的监测方法监测不全面且对测点间耦合关系建模不充分的问题,提出多核图卷积网络(Multi-kernel graph convolutional network,MKGCN),通过将全量传感器测点视为一张全量测点图,显式地对测点间耦合关系进行建模,从而实现全量传感器测点的同步工况估计.此外,面向在线监测场景,设计基于特征逼近的自迭代方法,从而克服在异常情况下由于测点间强耦合导致的部分测点估计值异常的问题.所提出的方法在电厂百万千瓦超超临界机组中引风机的实际数据上进行验证,结果显示,与其他典型方法相比,所提出的监测方法能够更精准地检测出发生故障的测点.

关键词：自迭代特征替换多核图卷积网络全量测点估计故障检测

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A new gravitational theory and dark matter problem

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Communications in Theoretical Physics 2024年第6期76卷 129-136页

作者： Xiong zhao Yongge Ma Department of Physics Beijing Normal UniversityBeijing 100875China

We propose a new gravitational theory with torsion based on Riemann-Cartan geometry,in which all physical quantities are *** addition to the spacetime metric,the gravitational degrees of freedom in this theory also include the torsion and two scalar *** energy-momentum tensor of the matter fields in this theory is also proposed.A spherically symmetric static vacuum solution of the theory is *** turns out that this solution can fit the observational data of the rotation curve outside the stellar disk in the Milky ***,the galactic dark matter may just be the gravitational effect of the theory with torsion.

关键词： gravity torsion dark matter

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New pimarane diterpenoids with antibacterial activity from fungus Arthrinium ***03

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Chinese Journal of Natural Medicines 2024年第4期22卷 356-364页

作者： zhao Songfeng JING Ziwei Department of Pharmacy the First Affiliated Hospital of Zhengzhou UniversityZhengzhou 450052China

A comprehensive chemical study of the endophytic fungus Arthrinium sp. ZS03, associated with Acorus tatarinowii Schott, yielded eleven pimarane diterpenoids (compounds 1–11), including seven novel compounds designated arthrinoids A–G (1–7). The determination of their structures and absolute configurations was achieved through extensive spectroscopic techniques, quantum chemical calculations of electronic circular dichroism (ECD), and single-crystal X-ray diffraction analysis. Furthermore, 7 demonstrated inhibitory activity against Klebsiella pneumoniae, comparable to the reference antibiotic amikacin, with a minimum inhibitory concentration (MIC) of 8 μg·mL^(−1).

关键词： Arthrinium sp.ZS03 Pimarane diterpenoids Structural elucidation Antibacterial activity

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New lump solutions and several interaction solutions and their dynamics of a generalized(3+1)-dimensional nonlinear differential equation

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Communications in Theoretical Physics 2024年第2期76卷 1-13页

作者： Yexuan Feng Zhonglong zhao School of Mathematics North University of ChinaTaiyuanShanxi 030051China

In this paper,we mainly focus on proving the existence of lump solutions to a generalized(3+1)-dimensional nonlinear differential ***’s bilinear method and a quadratic function method are employed to derive the lump solutions localized in the whole plane for a(3+1)-dimensional nonlinear differential *** examples of such a nonlinear equation are presented to investigate the exact expressions of the lump ***,the 3d plots and corresponding density plots of the solutions are given to show the space structures of the lump *** addition,the breath-wave solutions and several interaction solutions of the(3+1)-dimensional nonlinear differential equation are obtained and their dynamics are analyzed.

关键词： lump solutions generalized(3+1)-dimensional nonlinear differential equation Hirota's bilinear method quadratic function method interaction solutions

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Towards catalytic reactions of Cu single-atom catalysts:Recent progress and future perspective

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Chinese Chemical Letters 2024年第2期35卷 197-207页

作者： Yitao zhao Lei Tao Jiangsu Province Engineering Research Center of Special Functional Textile Materials Changzhou Vocational Institute of Textile and GarmentChangzhou 213164China Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology Advanced Catalysis and Green Manufacturing Collaborative Innovation CenterSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China

One of the urgent and challenging topics in diversified sustainable energy conversion is the development of high-performance,low-cost,and well durable *** single-atom catalysts(SACs)have become promising catalysts for diversified sustainable energy conversion due to their capability to maximize the utilization efficiency,acquire modulated electronic structure and optimized binding strength with *** this review,we have provided an interview of the recent progress achieved in the field of electrocatalysis,photocatalysis,and heterogeneous reaction based on Cu *** by this review,we have summarized some advanced synthetic strategies for the construction of Cu ***,the performance-improving strategies are discussed in terms of the coordination environments of the reaction center,reaction mechanism and selectivity,based on free energy diagram and electron structure ***,the remaining issues,challenges,and opportunities of Cu SACs are also provided,affording a perspective for future *** review not only offers us a deep understanding on the catalytic mechanism of Cu SACs for energy conversion,but also encourages more endeavors in prompting their practical application.

关键词： Cu SACs Energy conversion Catalysis Coordination environment

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Universal method for designing periodic orbits by homotopy classes in the elliptic restricted three-body problem

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Astrodynamics 2024年第1期8卷 175-188页

作者： Yue Zheng Min zhao School of Electronic Engineering Xi’an Aeronautical InstituteXi’an710077China School of aircraft Engineering Xi’an Aeronautical InstituteXi’an710077China School of Astronautics Northwestern Polytechnical UniversityXi’an710072China

The current methods for designing periodic orbits in the elliptic restricted three-body problem(ERTBP)have the disadvantages of targeting limited orbits and ergodic searches and considering only symmetric orbits.A universal method for designing periodic orbits is proposed in this ***,the homotopy classes of orbits are structured based on their topological ***,a dynamic model based on homotopy classes,ranging from the circular restricted three-body problem(CRTBP)to the ERTBP,can be built using the homotopy ***,a multi-and a single-period orbit were selected based on the resonance ***,the corresponding orbit in the ERTBP was computed by modifying the initial condition of the orbit in the *** method,without an ergodic search,can extend to any orbit,including an asymmetric orbit in the CRTBP,to the ERTBP model,and the two orbits are of the same homotopy *** of the Earth–Moon ERTBP are presented to verify the efficiency of this method.

关键词： periodic orbit elliptic restricted three-body problem(ERTBP) topology homotopy circular restricted three-body problem(CRTBP)

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