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Bio-regeneration of p-complexation desulfurization adsorbents

Science China Chemistry 2005年第6期48卷 538-544页

作者： LI Wangliang1,2. XING Jianmin1, XIONG Xiaochao1,2. SHAN Guobin1,2.& LIU Huizhou1 1. Laboratory of Separation Science and Engineering, Institute of Process Engineering, chinese academy of {2., Beijing 100080, China 2. graduate School of the chinese academy of {2.,Beijing 100039, China 1. Laboratory of Separation Science and Engineering Institute of Process Engineering Chinese Academy of Sciences 100080 Beijing China 2. graduate School of the chinese {2. of sciences 100039 Beijing China

The coupling of adsorption desulfurization and biodesulfurization is a new approach to produce clean fuels. Sulfur compounds are firstly adsorbed on adsorbents, and then the ad-sorbents are regenerated by microbial conversion. p-Complexation adsorbent, Cu(I)-Y, was ob-tained by ion exchanging Y-type zeolite with Cu2. and then by auto-reduction in helium at 45.℃ for 3 h. Dibenzothiophene (DBT) was used as a model compound. The effects of cell concentra-tion, volume of oil phase, the ratio of aqueous phase to adsorbent on DBT desorption by a bac-terium were studied. The amounts of DBT desorbed and 2.HBP produced can be apparently increased with addition of n-octane. BDS activity can be improved by increasing cell concentra-tion and the ratio of water-to-adsorbent. 89% of DBT desorbed from the adsorbents can be converted to 2.HBP within 6 h and almost 100% within 2. h, when the volume ratio of oil-to-water was 1/5.mL/mL, the cell concentration was 60 g·L?1, and the ratio of adsorbent-to-oil was 0.03 g·mL?1. The amount of 2.HBP produced was strongly dependent on the volume ratio of oil-to- water, cell concentration and amount of adsorbent. Adsorption capacity of the regenerated ad-sorbent is 95. that of the fresh one after being desorbed with Pseudomonas delafieldii R-8, washed with n-octane, dried at 100℃ for 2. h and auto-reduced in He.

关键词： adsorption desulfurization p-complexation adsorbents bio-regeneration Pseudomonas delafieldii desorption.

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Cloning and characterization of interferon stimulated genes Viperin and ISG15.and their promoters from snakehead Channa argus

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Progress in Natural Science:Materials International 2007年第12期17卷 1425-1435页

作者： Jia Weizhang1,2. Zhou Xiuxia1,2. Huang Rong1,2.and Guo Qionglin1(1. Institute of Hydrobiololgy, chinese academy of {2., Wuhan 430072. China 2. graduate university of chinese academy of sciences, Beijing 100039, China) Institute of Hydrobiololgy Chinese Academy of Sciences Wuhan 430072 China graduate university of {2. academy of sciences Beijing 100039 China

By suppression subtractive hybridization, rapid amplification of cDNA ends and gene walking methods, interferon stimulated genes (ISGs), Viperin and ISG15. and their promoters have been cloned and characterized from snakehead Channa argus. The Viperin cDNA was found to be 1474 nt and contain an open reading frame (ORF) of 105. nt that translates into a putative peptide of 35.0}amino acid (aa). The putative peptide of Viperin shows high identity to that in teleosts and mammals except for the N-terminal 70 aa. The ISG15.cDNA was found to be 75. nt and contain an ORF of 468 nt that translates into a putative peptide of 15. aa. The putative peptide of ISG15.is composed of two tandem repeats of ubiquitin-like (UBL) domains, and a canonical conjugation motif (LRGG) at C-terminal. Viperin and ISG15.promoter regions were characterized by the presence of interferon stimulating response elements (ISRE) and γ-IFN activation sites (GAS). ISRE is a feature of IFN-induced gene promoter and partially overlaps interferon regulatory factor (IRF) 1 and IRF2.recognition sites. GAS is responsible for the γ-IFN mediated transcription. One conserved site for NF-κB was found in the promoter region of Viperin. This is the first report of conservative binding motif for NF-κB in accordance with the consensus sequence (GGGRNNYYCC) among teleost ISG promoters. Moreover, there were also TATA, CAAT and Sp1 transcription factor sites in Viperin and ISG15.promoters. In 5. untranslated region (UTR), snakehead ISG15.gene contains a single intron, which differs from Viperin gene. The transcripts of Vipeirn and ISG15.mRNA were mainly expressed in head kidney, posterior kidney, spleen and gill. The expression levels in liver were found to increase obviously in response to induction by IFN-inducer poly I∶C.

关键词： interferon interferon stimulated gene (ISG) Viperin ISG15 snakehead (Channa argus).

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The deep thermal characteristic of continental margin of the northern South China Sea

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chinese Science Bulletin 2000年第18期45卷 1717-1722页

作者： ZHANG Jian & WANG Jiyang1. graduate School, university of Science and Technology of China, {2. academy of sciences, Beijing {5., China 2. Institute of Geology, {2. academy of sciences, Beijing 10002., China graduate School University of Science and Technology of China Chinese Academy of Sciences Beijing China Institute of Geology Chinese Academy of Sciences Beijing China

Heat flow plays an important role in the study ot thermal structure and thermal evolutionof continental margin of the northern South China Sea. The analysis of heat flow value shows that margin heat flow in the northern South China Sea is relatively high setting, but the percentage of crustal heat flow is lower than 35. in terrestrial heat flow. The terrestrial heat flow exhibited a current of rise from the Northern Continental Margin to the Southern Central Basin. However, the proportion of crustal heat flow in terrestrial heat flow slowly dropped down in the same direction. It is suggested that the main factor causing high heat flow setting is the moving up of hot material from asthenosphere.

关键词： margin of northern South China Sea terrestrial heat flow thermal structures.

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Wet-chemical synthesis and characteristics of Au nanoshell

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Science China Chemistry 2005年第5期48卷 431-435页

作者： LIU Zhongxin1,2. SONG Hongwei1, YU Lixin1,2. YANG Linmei1,2.& PAN Guohui1,2.1. Key Laboratory of Excited State Physics, Changchun Institute of Optics, Fine Mechanics and Physics, chinese {5. of {2., Changchun 130033, China 2. graduate School of the chinese {5. of {2., Beijing 100039, China 1. Key Laboratory of Excited State Physics Changchun Institute of Optics Fine Mechanics and Physics Chinese Academy of Sciences 130033 Changchun China 2. graduate School of the chinese {2. of sciences 100039 Beijing China

Gold nanoshells were prepared by an easy wet-chemical method, with Ag nanoparticles used as the templates. Transmission electron microscopy (TEM) indicated that the shells were sphere in shape, the size was homogenous, being about 2. nm, and no hard ag-glomerates were observed. The plasma resonance absorption of gold was tuned from visible to near-infrared (NIR) with the increased volume of HAuCl4. The temperature grads (?T) of the gold nanoshell hydrosol under the exposure of an 808-nm optical fiber laser with different power den-sities were measured. The highest ?T was 30℃ (5.W/cm2. irradiation area was 2.cm2.. This kind of gold nanoshell hydrosol is a promising material to be used in biomedicine such as photo-thermal cancer therapy, and its special photothermal convert property will photothermally trigger drug release.

关键词： wet-chemical synthesis, Au, nanoshell, NIR absorption, photothermal conversion.

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Gasdynamic characteristics of toroidal shock and detonation wave converging

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Science China(Physics,Mechanics & Astronomy) 2005年第6期48卷 739-749页

作者： TENG Honghui1,2.& JIANG Zonglin2.1. Key Laboratory of High Temperature Gas Dynamics, Institute of Mechanics, chinese academy of Sci- ences, Beijing 100080, China {2., Beijing {5., China 1. Key Laboratory of High Temperature Gas Dynamics Institute of Mechanics Chinese Academy of Sciences 100080 Beijing China 2. graduate university of chinese academy of sciences 100039 Beijing China

The modified CCW relation is applied to analyzing the shock, detonation wave converging and the role of chemical reactions in the process. Results indicate that the shock wave is strengthened faster than the detonation wave in the converging at the same initial Mach number. Euler equations implemented with a detailed chemical reaction model are solved to simulate toroidal shock and detonation wave converging. Gasdynamic characteristics of the converging are investigated, including wave interaction patterns, observable discrepancies and physical phenomena behind them. By comparing wave diffractions, converging processes and pressure evolutions in the focusing area, the different effects of chemical reactions on diffracting and converging processes are discussed and the analytic conclusion is demonstrated through the observation of numerical simulations.

关键词： converging, CCW relation, shock wave, detonation wave.

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Nonlinear interactions between gravity waves and background winds

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Progress in Natural Science:Materials International 2007年第6期17卷 639-644页

作者： Liu Xiao1,2.and Xu Jiyao1(1. State Key Laboratory for Space Weather, Center for Space Science and Applied Research, chinese academy of {2., Beijing 100080, China 2. graduate university of chinese academy of sciences, Beijing {5., China) [a]State Key Laboratory for Space Weather Center for Space Science and Applied Research Chinese Academy of Sciences Beijing China [b]graduate university of {2. academy of sciences Beijing China

Using the nonlinear propagating gravity waves (GW) model in the two-dimensional compressible atmosphere and the linear GW theory, the process of GW propagation in different background winds, e.g. the direction of the background wind is opposite to (dead wind) or the same as (tail wind) the direction of the horizontal phase velocity of GW, is studied. The results show that the dead wind prolongs the vertical wavelength and accelerates GW propagation. Therefore, GW propagates up to a higher height becomes instable in a short time and eventually induces an inverse jet flow. Then, the vertical wavelength is becoming short due to the nonlinear interactions between GW and the inverse jet flow. The vertical wavelength and group velocity decrease after GW propagates into the tail wind. The initial instable time is delayed. Although most of GW is trapped in the instable region, some of GW propagates above the instable region. Compared with GW propagation in the tail wind, the nonlinear interactions between GW and the dead wind are also strong. In contrast, the linear GW theory predicts that GW can propagate freely in the dead wind. The vertical wavelength simulated by the nonlinear numerical model is different from that predicted by the linear theory greatly after GW propagates into the dead wind.

关键词： gravity waves background winds vertical group velocity vertical wavelength nonlinear interactions.

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Statistical distribution of nonlinear random wave height

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Science China Earth sciences 2006年第4期49卷 443-448页

作者： HOU Yijun1, GUO Peifang1,2. SONG Guiting1,2. SONG Jinbao1, YIN Baoshu1 & ZHAO Xixi1,2.1. Institute of Oceanology, chinese academy of {2., Qingdao 2.6071, China 2. graduate university of the chinese academy of {2., Beijing 100039, China 1. Institute of Oceanology Chinese Academy of Sciences Qingdao 266071 China 2. graduate university of the {2. academy of {5. Beijing 100039 China

A statistical model of random wave is developed using Stokes wave theory of water wave dynamics. A new nonlinear probability distribution function of wave height is presented. The results indicate that wave steepness not only could be a parameter of the distribution function of wave height but also could reflect the degree of wave height distribution deviation from the Rayleigh distribution. The new wave height distribution overcomes the problem of Rayleigh distribution that the prediction of big wave is overestimated and the general wave is underestimated. The prediction of small probability wave height value of new distribution is also smaller than that of Rayleigh distribution. Wave height data taken from East China Normal university are used to verify the new distribution. The results in- dicate that the new distribution fits the measurements much better than the Rayleigh distribution.

关键词： Random ocean wave, nonlinearity, wave height distribution.

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Environmental characteristics of Mid-Holocene recorded by lacustrine sediments from Lake Daihai, north environment sensitive zone, China

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Science China Earth sciences 2006年第9期49卷 968-981页

作者： SUN Qianli1,2. ZHOU Jie1, SHEN Ji3, CHEN Peng1,2. WU Feng1,2.& XIE Xiuping1,2.1. State Key Lab of Loess and Quaternary Geology, Institute of Earth Environment, chinese {5. of {2., Xi’an 710075. China 2. graduate university of chinese academy of sciences, Beijing 100039, China 3. Nanjing Institute of Geography and Limnology, chinese {5. of {2., Nanjing 2.0008, China 1. State Key Lab of Loess and Quaternary Geology Institute of Earth Environment Chinese Academy of Sciences Xi’an 710075 China 2. graduate university of chinese academy of sciences Beijing 100039 China 3. Nanjing Institute of Geography and Limnology Chinese Academy of Sciences Nanjing 210008 China

Climate proxies, such as total organic carbon and nitrogen (TOC, TN), carbonate content (CaCO3), grain-size and pollen of the sediment core retrieved from enclosed Lake Daihai which lies in the north China environment sensitive zone are analyzed to reconstruct the environment evolution of the area based on high-resolution radiocarbon chronology. The results reveal that the TOC and TN contents of the sediments correlate well with pollen percentage and pollen flux variations during the Holocene, and both reach their peak values simultaneously at 6.7―3.5.ka BP (calendar age, 7.6―3.6 ka BP). Since 6.7 ka BP, both the CaCO3 and organic matter contents of the core have simultaneous variations, and their high values also occur during 6.7―3.5.ka BP. While during 9.0―6.7 ka BP (calendar age, 10―7.6 ka BP) relatively lower level of organic matter content and pollen flux corre- spond to the higher level of carbonate content. The above relations suggest that during 6.7―3.5.ka BP, the productivity and effective precipitation were greatly improved in the lake drainage area, and this would probably strengthen the hydrodynamic conditions, enhancing organic matter, pollen and carbonate inputs from terrestrial sources. Such processes would account for the enrichment of both organic matter and carbonate in the sediments. While during 9.0―6.7 ka BP, the lower level of or- ganic matter, pollen flux but high carbonate content show depressed productivity and declined vege- tation coverage. The higher carbonate content at this stage would have probably resulted from the higher evaporation ratio of the lake water under relatively drier climate conditions. Therefore, it is in- ferred that during 6.7―3.5.ka BP, the climate was more humid with abundant rainfalls and vegetation was more flourishing in the Lake Daihai area. This can be seen as Holocene Climate Optimum (HCO). As a result, this has evident discrepancies with the traditional notion that the HCO occurs at Early Holocene or early Mid

关键词： Lake Daihai, Mid-Holocene, lacustrine sediments, environmental characteristics.

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A new class of symmetric periodic solutions of the spatial elliptic restricted three-body problem

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Science China(Physics,Mechanics & Astronomy) 2009年第9期52卷 1404-1413页

作者： XU XingBo1,2.& FU YanNing1 1 Purple Mountain Observatory, chinese academy of {2., Nanjing 2.0008, China 2.graduate university of chinese academy of {2., Beijing 100039, China 1. Purple Mountain Observatory Chinese Academy of Sciences Nanjing 210008 China 2. graduate university of chinese academy of sciences Beijing 100039 China

We show that there exists a new class of symmetric periodic solutions of the spatial elliptic restricted three-body problem. In such a solution, the infinitesimal body is confined to the vicinity of a primary and moves on a nearly circular orbit. This orbit is almost perpendicular to the orbital plane of the primaries, where the line of symmetry of the orbit lies. The existence is shown by applying a corollary of Arenstorf's fixed point theorem to a periodicity equation system of the problem. And this existence doesn't require any restriction on the mass ratio of the primaries, nor on the eccentricity of their relative elliptic orbit. Potential relevance of this new class of periodic solutions to real celestial body systems and the follow-up studies in this respect are also discussed.

关键词： periodic orbits spatial restricted three-body problem symmetric orbits averaging

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Research on the method for retrieving soil moisture using thermal inertia model

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Science China Earth sciences 2006年第5期49卷 539-545页

作者： LIU Zhenhua1 & ZHAO Yingshi2.1. Information College, South China Agricultural university, Guangzhou 5.0642. China 2. graduate university of chinese academy of sciences, Beijing 100049, China 1. Information College South China Agricultural University Guangzhou 510642 China 2. graduate university of chinese academy of sciences Beijing 100049 China

In order to improve accuracy of soil moisture inversion using remote sensing, a new thermal inertia model is proposed in this paper. The improved model needs only surface maximum temperature as the temperature parameter input instead of input of the surface temperature difference, as well as the surface sensible and latent fluxes are introduced into boundary conditions of thermal conductivity equation. Furthermore, surface soil conductive heat transfer equation of two-layer model is used to solve the soil thermal inertia so that the remote sensing thermal inertia method can be ap- plied to regions with better-covered vegetation, but usually only for the bare areas or worse vegetation covered areas. The model has been tested at several locations in the area of west Inner Mongolia. Comparing the simulation of the new model with the measurements obtained by apparent thermal inertia and by field test, the result shows that the inertia thermal model can be used to estimate soil moisture in more reasonable accuracy.

关键词： thermal model, thermal conductivity equation, soil initial, sensible flux, latent flux, two-layer model.

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