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STUDY ON THE CONCENTRATION DEPENDENCE OF ORIENTATION OF POLYSTYRENE ON SILVER BY THE SERS TECHNIQUE

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chinese Journal of Polymer Science 2000年第2期18卷 177-180页

作者： Dong-hui Zhang Jin-gui Qin Jing-shu Shen You Wang Wan-jun Liu Department of Chemistry, Wuhan University, Wuhan 430072, china Polymer physics laboratory, institute of Chemistry, chinese academy of sciences beijing 100080, china Wuhan Univ Dept Chem Wuhan 430072 Peoples R China chinese Acad Sci Inst Chem Polymer Phys Lab Beijing 100080 Peoples R China

Polystyrene films were adsorbed onto a silver surface from dichloromethane solutions with concentrations of 0.1 to 12 wt%, and then studied by the surface enhanced Raman technique. A critical concentration for coil in... 详细信息

关键词： surface enhanced Raman scattering (SERS) polystyrene concentration dependence

Systematic study of survival probability of excited superheavy nuclei

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Science china(physics,Mechanics & Astronomy) 2011年第S1期54卷 109-113页

作者： XIA ChengJun1, SUN BaoXi1, ZHAO EnGuang2,3 & ZHOU ShanGui2,3 1College of Applied sciences, beijing University of Technology, beijing 100124, china 2institute of Theoretical physics, chinese academy of sciences, beijing 100190, china 3Center of Theoretical Nuclear physics, national laboratory of Heavy Ion Accelerator, Lanzhou 730000, china chinese Acad Sci Inst Theoret Phys Beijing 100190 Peoples R China beijing Univ Technol Coll Appl Sci Beijing 100124 Peoples R China Ctr Theoret Nucl Phys Natl Lab Heavy Ion Accelerator Lanzhou 730000 Peoples R China

The stability of excited superheavy nuclei (SHN) with 100 Z 134 against neutron emission and fission is investigated by using a statistical model. In particular, a systematic study of the survival probability against fission in the 1n-channel of these SHN is made. The present calculations consistently take the neutron separation energies and shell correction energies from the calculated results of the finite range droplet model which predicts an island of stability of SHN around Z = 115 and N = 179. It turns out that this island of stability persists for excited SHN in the sense that the calculated survival probabilities in the 1n-channel of excited SHN at the optimal excitation energy are maximized around Z = 115 and N = 179. This indicates that the survival probability in the 1n-channel is mainly determined by the nuclear shell effects.

关键词： survival probability superheavy elements island of stability neutron emission fission

Bio-regeneration of p-complexation desulfurization adsorbents

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Science china Chemistry 2005年第6期48卷 538-544页

作者： LI Wangliang1,2, XING Jianmin1, XIONG Xiaochao1,2, SHAN Guobin1,2 & LIU Huizhou1 1. laboratory of Separation Science and Engineering, institute of Process Engineering, chinese academy of sciences, beijing 100080, china 2. Graduate School of the chinese academy of sciences,beijing 100039, china 1. laboratory of Separation Science and Engineering Institute of Process Engineering Chinese Academy of Sciences 100080 Beijing China 2. Graduate School of the chinese academy of sciences 100039 Beijing China

The coupling of adsorption desulfurization and biodesulfurization is a new approach to produce clean fuels. Sulfur compounds are firstly adsorbed on adsorbents, and then the ad-sorbents are regenerated by microbial conversion. p-Complexation adsorbent, Cu(I)-Y, was ob-tained by ion exchanging Y-type zeolite with Cu2+ and then by auto-reduction in helium at 450℃ for 3 h. Dibenzothiophene (DBT) was used as a model compound. The effects of cell concentra-tion, volume of oil phase, the ratio of aqueous phase to adsorbent on DBT desorption by a bac-terium were studied. The amounts of DBT desorbed and 2-HBP produced can be apparently increased with addition of n-octane. BDS activity can be improved by increasing cell concentra-tion and the ratio of water-to-adsorbent. 89% of DBT desorbed from the adsorbents can be converted to 2-HBP within 6 h and almost 100% within 24 h, when the volume ratio of oil-to-water was 1/5 mL/mL, the cell concentration was 60 g·L?1, and the ratio of adsorbent-to-oil was 0.03 g·mL?1. The amount of 2-HBP produced was strongly dependent on the volume ratio of oil-to- water, cell concentration and amount of adsorbent. Adsorption capacity of the regenerated ad-sorbent is 95% that of the fresh one after being desorbed with Pseudomonas delafieldii R-8, washed with n-octane, dried at 100℃ for 24 h and auto-reduced in He.

关键词： adsorption desulfurization p-complexation adsorbents bio-regeneration Pseudomonas delafieldii desorption.

Electron dynamics in collisionless magnetic reconnection with a PIC simulation

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chinese Science Bulletin 2009年第3期54卷 456-460页

作者： GUO Jun1,2 1 School of Mathematics and physics, Qingdao University of Science and Technology, Qingdao 266042, china 2 State Key laboratory of Space Weather, chinese academy of sciences, beijing 100080, china School of Mathematics and physics Qingdao University of Science and Technology Qingdao China State Key laboratory of Space Weather Chinese Academy of Sciences Beijing China

Two-dimensional particle-in-cell (PIC) simulation is used to investigate electron dynamics in colli- sionless magnetic reconnection, and the proton/electron mass ratio is taken to be mi /me = 256. The results show that the presence of a strong initial guide field will change the direction of the electron flow. The electron density cavities and the parallel electric field can be found in the electron inflow re- gion along the separatrix, and the electron inflow and density cavities only appear in the second and fourth quadrants. What is different from the results with a smaller mass ratio is that new structures appear in the diffusion region near the X line: (1) Narrow regions of density enhancement and density cavities can be found synchronously in this region; and (2) corresponding to the electron density changes near the X line, the strong parallel electric fields are found to occur in the first and third quadrants. These electric fields perhaps play a more important role in acceleration and heating electrons than those fields located in the density cavities.

关键词： PIC模仿磁链接导向场电子动力学

Discovery of immune related factors in Fenneropenaeus chinensis by annotation of ESTs

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Progress in Natural Science:Materials International 2004年第1期14卷 48-55页

作者： SHEN Yaoqing 1,2 , XIANG Jianhai 1*, WANG Bing 1,2 , LI Fuhua 1 and TONG Wei 3(1. Experimental Marine Biology laboratory, institute of Oceanology, chinese academy of sciences, Qingdao 266071,china 2. Graduate School of the chinese academy of sciences, beijing 100039, china 3. Genomics & Bioinformatics institute, chinese academy of sciences, beijing 101300, china) chinese Acad Sci Inst Oceanol Expt Marine Biol Lab Qingdao 266071 Peoples R China chinese Acad Sci Grad Sch Beijing 100039 Peoples R China chinese Acad Sci Geonom & Bioinformat Inst Beijing 101300 Peoples R China

A total of 10446 expressed sequence tags (ESTs) are obtained by a large scale sequencing of a cDNA library from cephalothorax of adult Fenneropenaeus chinensis . An EST analysis platform was built up based on local computers and bioinformatic techniques were used to annotate these ESTs in order to promptly find possible functional genes, especially for immune related factors. About 4% of the ESTs show similarity to the coding sequences of such factors, including lectin, serine protease, serpin, lysozyme, etc. These ESTs provide a partial profile of the immune system in F. chinensis and useful information for further study on these genes.

关键词： Fenneropenaeus chinensis bioinformatics ESTs immune factors

Nonlinear interactions between gravity waves and background winds

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Progress in Natural Science:Materials International 2007年第6期17卷 639-644页

作者： Liu Xiao1,2 and Xu Jiyao1(1. State Key laboratory for Space Weather, Center for Space Science and Applied Research, chinese academy of sciences, beijing 100080, china 2. Graduate University of chinese academy of sciences, beijing 100039, china) [a]State Key laboratory for Space Weather Center for Space Science and Applied Research Chinese Academy of Sciences Beijing China [b]Graduate University of chinese academy of sciences Beijing China

Using the nonlinear propagating gravity waves (GW) model in the two-dimensional compressible atmosphere and the linear GW theory, the process of GW propagation in different background winds, e.g. the direction of the background wind is opposite to (dead wind) or the same as (tail wind) the direction of the horizontal phase velocity of GW, is studied. The results show that the dead wind prolongs the vertical wavelength and accelerates GW propagation. Therefore, GW propagates up to a higher height becomes instable in a short time and eventually induces an inverse jet flow. Then, the vertical wavelength is becoming short due to the nonlinear interactions between GW and the inverse jet flow. The vertical wavelength and group velocity decrease after GW propagates into the tail wind. The initial instable time is delayed. Although most of GW is trapped in the instable region, some of GW propagates above the instable region. Compared with GW propagation in the tail wind, the nonlinear interactions between GW and the dead wind are also strong. In contrast, the linear GW theory predicts that GW can propagate freely in the dead wind. The vertical wavelength simulated by the nonlinear numerical model is different from that predicted by the linear theory greatly after GW propagates into the dead wind.

关键词： gravity waves background winds vertical group velocity vertical wavelength nonlinear interactions.

Growth of Pb S nanoclusters on specific sites of programmed oligodeoxynucleotides

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chinese physics B 2015年第1期24卷 398-403页

作者：陆颖滕翠娟李颖王惠徐春华胡书新李明 beijing national laboratory for condensed matter physics and Key laboratory of Soft matter physics Institute of PhysicsChinese Academy of Sciences

We develope a method to synthesize Pb S nanoclusters（NCs） using guanine-containing oligodeoxynucleotides（ODNs）as templates. The NCs on the ODNs are ultra small（ranging from ～ 0.5 nm to 2.1 nm） and luminescent in the visible region. They are characterized by photoluminescence（PL） spectra, transmission electron microscopy（TEM）, and X-ray powder diffraction（XRD）. The ODN–NC complexes can be used as customer-designed fluorophores which do not have the problem of multiple conjugations. The same method enables us to fabricate Pb S quantum dot molecules and connect them into nanowires, expanding their potential applications in molecule electronics and quantum computing.

关键词： Pb S nanoclusters quantum dot molecules oligodeoxynucleotides photoluminescence

Application of the moist vorticity vector in the analysis of a heavy rainfall event in North china

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Progress in Natural Science:Materials International 2007年第12期17卷 1457-1465页

作者： Zhao Yu1,2,3, Wang Jianguo4 and Xue Deqiang2(1. laboratory of Cloud-Precipitation physics and Severe Storms, institute of Atmospheric physics, chinese academy of sciences, beijing 100029, china 2. Shandong Provincial Meteorological Observatory, Jinan 250031, china 3. Graduate University of chinese academy of sciences, beijing 100039, china 4. Shandong Provincial Meteorological Bureau, Jinan 250031, china) laboratory of Cloud-Precipitation physics and Severe Storms Institute of Atmospheric Physics Chinese Academy of Sciences Beijing 100029 China Shandong Provincial Meteorological Observatory Jinan 250031 China Graduate University of chinese academy of sciences Beijing 100039 China Shandong Provincial Meteorological Bureau Jinan 250031 China

The moist vorticity vector (MVV), defined as (ζa×▽qv)/ρ introduced by Gao et al. is used to study a heavy rainfall event in North china. The MVV has zonal, meridional and vertical components in a three-dimensional framework. Analysis of domain-mean and mass-integrated quantities shows that the variation of the vertical component of the MVV closely follows the variation of the cloud hydrometeors, with a linear correlation coefficient of 0.95, indicating that the vertical component of the MVV is strongly associated with midlatitude convection. Further analysis shows that the vertical component of the MVV reflects the interaction between the horizontal vorticity and the horizontal specific humidity gradient, which can associate dynamic and thermodynamic processes with cloud microphysical processes. Thus, this study can help to understand how the interaction between circulations and clouds aids the development of convection, and the MVV can be used to trace the development and evolution of heavy rainfall.

关键词： moist vorticity vector heavy rainfall modeling study.

SHRIMP zircon U-Pb geochronology of early Mesozoic felsic igneous rocks from the southern Lancangjiang and its tectonic implications

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Science china Earth sciences 2006年第10期49卷 1032-1042页

作者： PENG Touping1,2, WANG Yuejun1, FAN Weiming1, LIU Dunyi3, SHI Yuruo3 & MIAO Laicheng4 1. Key laboratory of Isotope Geochronology and Geochemistry, Guangzhou institute of Geochemistry, chinese academy of sciences, Guangzhou 510640, china 2. Graduate University of chinese academy of sciences, beijing 100039, china 3. SHRIMP isotope laboratory, chinese academy of Geological sciences, beijing 100037, china 4. institute of Geology and Geophysics, chinese academy of sciences, beijing 100029, china Key laboratory of Isotope Geochronology and Geochemistry Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou China Graduate University of chinese academy of sciences Beijing China SHRIMP isotope laboratory Chinese Academy of Geological Sciences Beijing China institute of Geology and Geophysics Chinese Academy of Sciences Beijing China

The SHRIMP zircon U-Pb geochronology of three typical samples, including two monzo nitic granites from the Lincang batholith and a rhyolite from the Manghuai Formation are presented in the southern Lancangjiang, western Yunnan Province. The analyses of zircons for the biotite monzonitic granites from the northern (02DX-137) and southern (20JH-10) Lincang batholith show the single and tight clusters on the concordia, and yield the weighted mean 206Pb/238U ages of 229.4 ± 3.0 Ma and 230.4 ± 3.6 Ma, respectively, representing the crystallized ages of these granites. The zircons for the rhyolitic sample (02DX-95) from the Manghuai Formation give a weighted mean 206Pb/238U age of 231.0 ± 5.0 Ma. These data suggest that the igneous rocks from the Lincang granitic batholith and Manghuai Formation have a similar crystallized age. In combination with other data, it is inferred that both were generated at a narrow age span (~230 Ma) and were originated from the postcollisional tectonic regime. An early Proterozoic 206Pb/238U apparent age of 1977±44 Ma is additionally obtained from one zircon from the biotite monzonitic granite (southern Lincang batholith), indicative of devel- opment of the early Proterozoic Yangtze basement in the region. These precisely geochronological data provide important constraints on better understanding the Paleozoic tectonic evolution of the Tethys, western Yunnan Province.

关键词： SHRIMP zircon U-Pb dating, Middle Triassic, Lincang granitic batholith, Manghuai Formation rhyolite, southern Lancangjiang.