The synthetic strategies of hierarchical TS-1 zeolites for the oxidative desulfurization reactions

作     者：Guoju Yang Ji Han Yue Liu Ziyi Qiu Xiaoxin Chen Guoju Yang;Ji Han;Yue Liu;Ziyi Qiu;Xiaoxin Chen

作者机构：State Key Laboratory of Inorganic Synthesis and Preparative ChemistryCollege of ChemistryJilin UniversityChangchun 130012China International Center of Future ScienceJilm UniversityChangchun 130012China Department of Chemistry and Catalysis Research CenterTechnische Universitat MunchenLichtenbergstrasse 485747 GarchingGermany 

出 版 物：《Chinese Journal of Chemical Engineering》 (中国化学工程学报（英文版）)

年 卷 期：2020年第28卷第9期

页      面：2227-2234页

核心收录：

学科分类：081702[工学-化学工艺] 081705[工学-工业催化] 08[工学] 0817[工学-化学工程与技术] 080502[工学-材料学] 0805[工学-材料科学与工程（可授工学、理学学位）] 

基　　金：supported by the National Natural Science Foundation of China(21971082) the Jilin Province Science and Technology Development Plan(20200201096JC and 20190201229JC) the China Postdoctoral Science Foundation(2019T120235 and 2018M640280)for supporting this work the 111 Project(B17020) 

主　　题：Zeolites TS-1 Synthesis Hierarchical ODS 

摘      要：With the increasingly stringent standards for limiting sulfide content in liquid fuels,oxidative desulfurization(ODS)has become a promising ultra-deep desulfurization process in fuel ***-1 zeolites show great potential as catalysts for ODS reactions,due to its remarkable oxidation activity at low temperatures and ***,the inherent microporous structure of conventional TS-1 zeolites restricts the mass transportation and renders the active sites in the microporous space of TS-1 zeolites inaccessible for bulky aromatic organosulfur *** of hierarchical TS-1 zeolites by incorporating meso-/macropores into microporous TS-1 zeolites is an effective strategy to improve mass *** recent years,abundant efforts have been dedicated to developing synthetic strategies of hierarchical TS-1 zeolite,thereby improving its catalytic performance in the ODS *** mini-review addresses the synthetic methods of hierarchical TS-1 catalysts and their catalytic performance in the ODS *** addition,some current problems and prospects of synthesis routes for constructing hierarchical TS-1 catalysts have also been *** expect this mini-review to shed light on the more efficient preparation strategies of hierarchical TS-1 zeolites for the ODS process.