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DNA origami mediated electrically connected metal–semiconductor junctions

DNA origami 电子上调停了连接 metalsemiconductor 连接

作     者:Basu R.Aryal Dulashani R.Ranasinghe Tyler R.Westover Diana G.Calvopia Robert C.Davis John N.Harb Adam T.Woolley Basu R.Aryal;Dulashani R.Ranasinghe;Tyler R.Westover;Diana G.Calvopi(n)a;Robert C.Davis;John N.Harb;Adam T.Woolley

作者机构:Department of Chemistry and BiochemistryBrigham Young UniversityProvoUT 84602USA Department of Chemical EngineeringBrigham Young UniversityProvoUT 84602USA Department of Physics and AstronomyBrigham Young UniversityProvoUT 84602USA 

出 版 物:《Nano Research》 (纳米研究(英文版))

年 卷 期:2020年第13卷第5期

页      面:1419-1426页

核心收录:

学科分类:08[工学] 0805[工学-材料科学与工程(可授工学、理学学位)] 080502[工学-材料学] 

基  金:We thank the National Science Foundation(No.1562729)and BYUs Simmons Research Endowment for support of this work.B.R.A.acknowledges the BYU Department of Chemistry and Biochemistry for a Roland K.Robins Graduate Research Fellowship 

主  题:current-voltage measurement DNA nanofabrication electroless plating gold nanorods nanoelectronics tellurium nanorods 

摘      要:DNA-based nanofabrication of inorganic nanostructures has potential application in electronics,catalysis,and *** DNA metallization has generated conductive DNA-assembled nanostructures;however,the use of semiconductors and the development of well-connected nanoscale metal-semiconductor junctions on DNA nanostructures are still at an early ***,we report the first fabrication of multiple electrically connected metal-semiconductor junctions on individual DNA origami by location-specific binding of gold and tellurium *** attachment to DNA origami was via DNA hybridization for Au and by electrostatic interaction for *** gold plating was used to create nanoscale metal-semiconductor interfaces by filling the gaps between Au and Te ***-point electrical characterization indicated that the Au-Te-Au junctions were electrically connected,with current-voltage properties consistent with a Schottky ***-based nanofabrication of metal-semiconductor junctions opens up potential opportunities in nanoelectronics,demonstrating the power of this bottom-up approach.

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