Composition and source apportionment of dust fall around a natural lake

作     者：Mohd Talib Latif Sofia Aida Ngah Doreena Dominick Intan Suraya Razak Xinxin Guo Thunwadee Srithawirat Idris Mushrifah 

作者机构：School of Environmental and Natural Resource Sciences Faculty of Science and Technology Universiti Kebangsaan Malaysia Institute for Environment and Development (LESTARI) Universiti Kebangsaan Malaysia Centre for Atmospheric Chemistry University of Wollongong Department of Environmental Engineering Faculty of Engineering and Green Technology Universiti Tunku Abdul Rahman Department of Environmental Science Faculty of Science and Technology Pibulsongkram Rajabhat University Pusat Penyelidikan Tasik Chini (PPTC) Faculty of Science and Technology Universiti Kebangsaan Malaysia 

出 版 物：《Journal of Environmental Sciences》 (环境科学学报（英文版）)

年 卷 期：2015年第27卷第7期

页      面：143-155页

核心收录：

学科分类：081704[工学-应用化学] 07[理学] 08[工学] 0817[工学-化学工程与技术] 070602[理学-大气物理学与大气环境] 070302[理学-分析化学] 0706[理学-大气科学] 0703[理学-化学] 

基　　金：the Malaysian Ministry of Higher Education for funding via Fundamental Research Grants (UKMTOPDOWN-ST-08-FRGS0003-2010 and FRGS/1/ 2013/SPWN01/UKM/02/) 

主　　题：Trace metal Major element Anion Source apportionment Lake Ghini Malaysia 

摘      要：The aim of this study was to determine the source apportionment of dust fall around Lake Chini, Malaysia. Samples were collected monthly between December 2012 and March2013 at seven sampling stations located around Lake Chini. The samples were filtered to separate the dissolved and undissolved solids. The ionic compositions（NO-3, SO2-4, Cl-and NH＋4） were determined using ion chromatography（IC） while major elements（K, Na, Ca and Mg） and trace metals（Zn, Fe, Al, Ni, Mn, Cr, Pb and Cd） were determined using inductively coupled plasma mass spectrometry（ICP-MS）. The results showed that the average concentration of total solids around Lake Chini was 93.49 ± 16.16 mg/（m2·day）. SO2-4, Na and Zn dominated the dissolved portion of the dust fall. The enrichment factors（EF） revealed that the source of the trace metals and major elements in the rain water was anthropogenic, except for Fe. Hierarchical agglomerative cluster analysis（HACA） classified the seven monitoring stations and 16 variables into five groups and three groups respectively. A coupled receptor model, principal component analysis multiple linear regression（PCA-MLR）, revealed that the sources of dust fall in Lake Chini were dominated by agricultural and biomass burning（42%）,followed by the earth＇s crust（28%）, sea spray（16%） and a mixture of soil dust and vehicle emissions（14%）.