Two-Dimensional Materials for Highly Efficient and Stable Perovskite Solar Cells

作     者：Xiangqian Shen Xuesong Lin Yong Peng Yiqiang Zhang Fei Long Qifeng Han Yanbo Wang Liyuan Han Xiangqian Shen;Xuesong Lin;Yong Peng;Yiqiang Zhang;Fei Long;Qifeng Han;Yanbo Wang;Liyuan Han

作者机构：State Key Laboratory of Metal Matrix CompositesShanghai Jiao Tong UniversityShanghai 200240People's Republic of China Xinjiang Key Laboratory of Solid State Physics and DevicesSchool of Physical Science and TechnologyXinjiang UniversityUrumqi 830046People's Republic of China Special Division of Environmental and Energy ScienceCollege of Arts and SciencesKomaba Organization for Educational ExcellenceUniversity of TokyoTokyo 153-8902Japan State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070People's Republic of China College of ChemistryHenan Institute of Advanced TechnologyZhengzhou UniversityZhengzhou 450001People's Republic of China Guangxi Key Laboratory of Optical and Electronic Materials and DevicesCollaborative Innovation Center for Exploration of Nonferrous Metal Deposits and Efficient Utilization of ResourcesSchool of Materials Science and EngineeringGuilin University of TechnologyGuilin 541004People's Republic of China 

出 版 物：《Nano-Micro Letters》 (纳微快报（英文版）)

年 卷 期：2024年第16卷第10期

页      面：176-212页

核心收录：

学科分类：08[工学] 0805[工学-材料科学与工程（可授工学、理学学位）] 080502[工学-材料学] 0702[理学-物理学] 

基　　金：the financial support of the National Natural Science Foundation of China(Nos.U21A20171,12074245,and 52102281) National Key R&D Program of China(Nos.2021YFB3800068 and 2020YFB1506400) Shanghai Sailing Program(No.21YF1421600) Young Elite Scientists Sponsorship Program by China Association for Science and Technology(No.2021QNRC001) 

主　　题：Perovskite solar cells Two-dimensional materials Interface engineering Van der Waals heterojunction Electrodes 

摘      要：Perovskite solar cells(PSCs)offer low costs and high power conversion ***,the lack of long-term stability,primarily stemming from the interfacial defects and the sus-ceptible metal electrodes,hinders their practical *** the past few years,two-dimensional(2D)materials(e.g.,graphene and its derivatives,transitional metal dichalcogenides,MXenes,and black phosphorus)have been identified as a promising solution to solving these problems because of their dangling bond-free surfaces,layer-dependent electronic band structures,tunable functional groups,and inherent ***,recent progress of 2D material toward efficient and stable PSCs is summarized,including its role as both interface materials and *** discuss their beneficial effects on perovskite growth,energy level alignment,defect passivation,as well as blocking external *** particular,the unique properties of 2D materials to form van der Waals heterojunction at the bottom interface are ***,perspectives on the further development of PSCs using 2D materials are provided,such as designing high-quality van der Waals heterojunction,enhancing the uniformity and coverage of 2D nanosheets,and developing new 2D materials-based electrodes.