A novel“Snowflake”--rGO-CuO for ultrasonic degradation of rhodamine and methyl orange
作者机构:Hubei Province Key Laboratory of Science in Metallurgical ProcessWuhan University of Science and TechnologyWuhan430081China Department of Engineering and TechnologyWuhan College of Foreign Languages&Foreign AffairsWuhan430070China Key Laboratory of Advanced Batteries Materials for Electric Vehicles of China Petroleum and Chemical Industry FederationSchool of Materials Science and EngineeringXi'an University of TechnologyXi'an710048China
出 版 物:《Nano Materials Science》 (纳米材料科学(英文版))
年 卷 期:2024年第6卷第3期
页 面:365-373页
核心收录:
学科分类:081705[工学-工业催化] 07[理学] 08[工学] 070206[理学-声学] 083002[工学-环境工程] 0830[工学-环境科学与工程(可授工学、理学、农学学位)] 0817[工学-化学工程与技术] 0805[工学-材料科学与工程(可授工学、理学学位)] 080502[工学-材料学] 0901[农学-作物学] 0703[理学-化学] 0802[工学-机械工程] 0702[理学-物理学]
基 金:supported by the National Natural Science Foundation of China (No.11375136)
主 题:rGO-CuO Nanocomposites Characterization Nanomaterial catalyst First principle
摘 要:Graphene-doped CuO(rGO-CuO)nanocomposites with flower shapes were prepared by an improved solvothermal *** samples were characterized by X-ray diffraction,X-ray photoelectron spectroscopy and UV–visible *** active species in the degradation reaction of rGO-CuO composites under ultrasonic irradiation were detected by electron paramagnetic *** the basis of comparative experiments,the photodegradation mechanisms of two typical dyes,Rhodamine B(Rh B)and methyl orange(MO),were *** results demonstrated that the doped CuO could improve the degradation *** catalytic degradation efficiency of rGO-CuO(2:1)to rhodamine B(RhB)and methyl orange(MO)reached 90%and 87%respectively,which were 2.1 times and 4.4 times of the reduced graphene *** the first-principles and other theories,we give the reasons for the enhanced catalytic performance of rGO-CuO:combined with internal and external factors,rGO-CuO under ultrasound could produce more hole and active sites that could interact with the OH·in pollutant molecules to achieve *** rGO-CuO nanocomposite has a simple preparation process and low price,and has a high efficiency of degrading water pollution products and no secondary pollution *** has a low-cost and high-efficiency application prospect in water pollution industrial production and life.